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At least 73 records · Page 4

Preliminary Analysis of Advanced Reactors Storage, Transportation, and Disposal

Based on the higher interest in Advanced Reactor (AR) deployment (e.g., ARDP[1]) for potential new fuel cycles, the Spent Fuel & Waste Science and Technology (SFWST) Program has begun to evaluate the possible implications of long-term management and final disposition of potential Advance Reactor spent nuclear fuels (SNF) that would be generated in potential advanced reactors. Safely managing and dispositioning the potential future AR SNF, and any other associated radioactive wastes, is the primary focus of this initial preliminary assessment of those. This paper summarizes the efforts by the Spent Fuel & Waste Science and Technology (SFWST) in evaluating characteristics and packaging options for advanced reactor spent nuclear fuel forms. The fuel forms were categorized into three types: (1) tristructural isotropic (TRISO), (2) metallic, and (3) fuel salt. This work emphasized TRISO and metallic SNF and waste streams because of the near-term anticipated operation of the Xe-100 and the Natrium reactors as advanced-reactor demonstrations. Preliminary information for the spent-fuel salts discharged from molten-salt reactors (MSRs) is also examined to provide a baseline for future efforts. All calculations and assumptions used publicly available information. The following characteristics are calculated or estimated for use in the preliminary assessments: SNF volume and mass, radiation/activity levels through time, thermal conditions through time, potential radionuclide source terms, chemical interactions and evolutions, disposal inventories, and waste-form lifetime. Using those characteristics, calculations to determine the applicability of existing canister designs were performed. These evaluations included geometric (e.g., dimension, volume) and mass/weight considerations, known operational approaches and loading procedures, physical and chemical considerations/conditions for storage environments, as-loaded radiation, thermal, and criticality analyses to identify constraints for storage, transportation, and disposal. The paper also includes a literature review and analysis on the storage, transportation, and disposal evaluations and experiences from reactors with similar fuel forms. Advanced-reactor vendors cite past experiences with Fort St. Vrain for TRISO and the Experimental Breeder Reactor II (EBR-II) for metallics that have major influences on fuel design. Finally, the paper includes preliminary concepts of operation for advanced-reactor SNF. This encompasses storage, transportation, potential treatment, and disposal activities from both a per-canister and systems-integration perspective.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Lower bias, lower noise CMB lensing with foreground-hardened estimators

Extragalactic foregrounds in temperature maps of the cosmic microwave background (CMB) severely limit the ability of standard estimators to reconstruct the weak lensing potential. These foregrounds are not fully removable by multifrequency cleaning or masking and can lead to large biases if not properly accounted for. For foregrounds made of a number of unclustered point sources, an estimator for the source amplitude can be derived and deprojected, removing any bias to the lensing reconstruction. We show with simulations that all of the extragalactic foregrounds in temperature can be approximated by a collection of sources with identical profiles, and that a simple bias hardening technique is effective at reducing any bias to lensing, at a minimal noise cost. In this work, we compare the performance and bias to other methods such as "shear-only" reconstruction, and discuss how to jointly deproject any arbitrary number of foregrounds, each with an arbitrary profile. In particular, for a Simons Observatory-like experiment foreground-hardened estimators allow us to extend the maximum multipole used in the reconstruction, increasing the overall statistical power by ~50% over the standard quadratic estimator, both in auto and cross-correlation. We conclude that source hardening outperforms the standard lensing quadratic estimator both in auto- A nd cross-correlation, and in terms of lensing signal-to-noise and foreground bias.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Literature Review of Documented Persistent Secondary Uranium Sources at DOE LM Sites

The U.S. Department of Energy Office of Legacy Management (LM) has the responsibility to protect human health and the environment at 101 legacy uranium sites across the nation by implementing long-term surveillance and maintenance requirements. Included in these responsibilities is to provide for the safe and environmentally sound disposal, long-term stabilization, and control of uranium mill tailings in a manner that minimizes or eliminates radiation health hazards to the public at 21 Uranium Mill Tailings Radiation Control Act (UMTRCA) Title I sites; 6 UMTRCA Title II sites; and 9 Comprehensive Environmental Response, Compensation, and Liability Act/Resource Conservation and Recovery Act sites. These sites are former uranium mills (processing sites), or sites with wastes from processing sites encapsulated in engineered disposal cells (disposal sites), or sites where components of atomic weapons were manufactured. During site characterization, groundwater contamination was often discovered and evaluated or modeled for future movement with the inclusion of uranium sorption in the groundwater plume. Much of this original work did identify uranium processing wastes as the original contaminant source. However, more recent work has identified the existence and influence of persistent secondary uranium sources that may prevent uranium in groundwater from attenuating as quickly as initial evaluations or modeling indicated. By understanding these processes, better decisions can be made to choose the appropriate remediation and closure strategies, identify long-term surveillance and maintenance activities, and more accurately estimate life-cycle costs. The purpose of this report is to summarize the literature available on documented persistence secondary uranium sources at LM sites as part of the Applied Studies and Technology Persistent Secondary Contaminant Sources Project.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

TRITON: A Multi-GPU open source 2D hydrodynamic flood model

A new open source multi-GPU 2D flood model called TRITON is presented in this work. The model solves the 2D shallow water equations with source terms using a time-explicit first order upwind scheme based on an Augmented Roe's solver that incorporates a careful estimation of bed strengths and a local implicit formulation of friction terms. Here, the scheme is demonstrated to be first order accurate, robust and able to solve for flows under various conditions. TRITON is implemented such that the model effectively utilizes heterogeneous architectures, from single to multiple CPUs and GPUs. Different test cases are shown to illustrate the capabilities and performance of the model, showing promising runtimes for large spatial and temporal scales when leveraging the computer power of GPUs. Under this hardware configuration, communication and input/output subroutines may impact the scalability. The code is developed under an open source license and can be freely downloaded in https://code.ornl.gov/hydro/triton.

2D flood model↗

Mechanistic Source Term Determination

Understand the function and performance of the different barriers to radionuclide release in HTGRs, how these are incorporated into reactor design and safety analyses, and approaches to estimate radionuclide release under specific reactor conditions.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Data for Responsiveness of Miscanthus and Switchgrass Yields to Stand Age and Nitrogen Fertilization: A Meta-regression Analysis

The compiled datasets include plot level observations of energy crops (miscanthus and switchgrass) from recent experimental field trials in the US including dry biomass yield, location, state, region, harvest year, growing season degree days (GDD), winter season heating degree days (HDD), growing season cumulative precipitation, annual nitrogen application rate, age of the pant when harvested, National Commodity Crop Productivity Index (NCCPI) values, and cultivar type (switchgrass) from various published and unpublished sources. The stata codes include estimation procedures for four different specifications, i.e., Model A includes deterministic effect without interaction terms; Model B includes deterministic effect with interaction terms (N2, age2, N × age, GDD2, precip2, N × NCCPI); Model C includes deterministic effect with interaction terms, study, and location random effect; Model D includes deterministic effect with interaction terms, harvest year augmented study, and location random effect.

Age↗

Source-Resolved Inversion of Elemental Carbon Emissions in California Using Log-Space Bayesian Inference

Elemental carbon (EC), operationally quantified by thermal-optical analysis, is widely used as a proxy for black carbon (BC) relevant to short-term climate forcing and public health. Current EC emission inventories remain highly uncertain, with persistent discrepancies between bottom-up and top-down estimates. In this study, we develop a source-resolved, log-space Bayesian inversion framework applied to estimate California’s statewide EC emissions in 2019. By integrating surface EC measurements from the EPA’s Air Quality System network with high-resolution source contributions simulated by a chemical transport model, we identify a one-third underestimation in the existing statewide EC inventory, requiring an increase of the total from a prior of 8.58 [5.49–13.75] Gg year–1 to a posterior estimate of 12.78 [10.71–15.37] Gg year–1. This discrepancy is primarily driven by substantial underestimations in the power and industrial and off-road mobile sectors. Furthermore, population-weighted exposure analysis reveals a marked sectoral divergence between emission mass and health burden: off-road mobile sources dominate both emissions and exposure, accounting for 31% of statewide exposure, while residential wood combustion contributes 26% of total exposure despite comprising only 19% of total emissions, due to its source proximity to population. These findings underscore the need to update sector-specific EC speciation profiles and demonstrate that mitigation strategies targeting off-road mobile sources and residential wood combustion are critical for reducing EC-related health impacts in California.

Zhang, Jie↗

Radionuclide Screening Analysis and Transport Parameters for Pahute Mesa Detonations, Nevada National Security Site

A “screening analysis” is implemented at Pahute Mesa (PM), Nevada National Security Site (NNSS), to determine subsets of the 43 radionuclides listed in the radionuclide inventory of Finnegan et al. (2016) that are of relevance or potential relevance to the hydrologic source term (HST) for assessment of radionuclide transport in groundwater. Consideration is added to how levels of contamination are defined and whether any other radionuclides not in the inventory are relevant to the HST. A model is developed to estimate a range of possible source concentrations in groundwater that account for uncertainty in partitioning into melt glass and sorption into surrounding rock of the exchange zone for the 82 PM underground nuclear tests detonated in vertical shafts. The model also accounts for the varied hydrogeochemical settings. Transport parameters needed for the screening model calculations are developed from databases for hydrogeologic units, chemistry, mineralogy, fracture spacing, fracture aperture, fracture openness, matrix porosity, bulk density, saturation, and alteration. Of key importance is consideration of diagenetic zonation of the mineralogy related to hydrothermal alteration. The screening analysis compares model results with available groundwater radiochemistry data. Consistency between screening model results and available data helps validate the model for application to all 43 radionuclides, most of which have no measurements or only non-detect measurements of concentration in groundwater. The screening analysis determines that ten radionuclides – tritium, Sr-90, I-129, Cs-137, U-232, U-233, U-234, U-238, and the total of Pu-239 and Pu-240 are relevant to the HST. Determination of relevance is primarily based on data and/or model results indicating source concentration exceeding a maximum contaminant level (MCL) out to 100 years since the time of detonation. U-238 is relevant to assessment of contamination relative to MCLs for uranium and gross alpha particle activity. Five other radionuclides – C-14, Cl-36, Tc-99, Np-237, and Pu-238 – are determined potentially relevant to the HST based on a 0.1 MCL threshold. The screening analysis recommends additional attention to the natural daughter radionuclides of the uranium series (U-238) and thorium series (Th-232) decay chains, particularly Ra-226 and Ra-228, that were not included the inventory.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

A Comparison of RESRAD and GoldSim Models for Assessing Radiological Dose for a RCRA Landfill - 20418

US Ecology Idaho (USEI) operates a Resource Conservation and Recovery Act (RCRA) Subtitle C, Hazardous Waste Treatment, Storage, and Disposal (TSD) Facility on a 640-acre property in Owyhee County, Idaho. USEI accepts a wide variety of RCRA-exempt low activity radioactive wastes, including naturally occurring radioactive material (NORM) and technologically enhanced NORM (TENORM) (USEI 2009). The performance of the landfill with regard to radiological operating permit requirements was previously assessed using a model constructed with the residual radioactivity (RESRAD) computer program, developed by Argonne National Laboratory for the U.S. Department of Energy (DOE). RESRAD supports the evaluation of several environmental transport pathways related to a radionuclide-contaminated soil source term, but it was not conceived as a model for the evaluation of landfill radiological performance. A more comprehensive and realistic model is desired in order to better support submissions to both the State of Idaho's Department of Environmental Quality as well as the U.S. Nuclear Regulatory Commission. A Performance Assessment (PA) computer model was developed using GoldSim software for the USEI RCRA Subtitle C landfill. The RESRAD computer model was specifically developed for calculating soil cleanup criteria and radiological dose and cancer risk from residual radioactive material in soil. To evaluate site-specific conditions, users may select from among a number of available environmental transport and exposure pathways and modify 'default' parameter values. In GoldSim, a user must construct the model 'from scratch.' However, this modeling is facilitated by a number of specialized elements available in GoldSim to support a radiological mass transport model. These include elements for defining radiological decay and ingrowth, container failure and radiological release, advective and diffusive transport, and other processes. Advantages afforded by the use of RESRAD for modeling radiological dose for a RCRA Subtitle C landfill include ease of use and reasonable flexibility in specifying site-specific conditions. GoldSim allows for considerably more flexibility and site-specificity than RESRAD, including evaluation of potentially relevant environmental transport processes not supported in RESRAD. The probabilistic modeling capabilities of GoldSim also far exceed those of RESRAD. The pros and cons of RESRAD and GoldSim for this modeling problem are explored with a focus on identifying approaches and critical factors in identifying the appropriate platform. The capabilities of RESRAD and GoldSim for mathematically modeling the disposal system will be contrasted and compared. For example, the existing RESRAD radiological safety assessment evaluated potentially complete exposure pathways related to infiltration to groundwater and upwards diffusion of radon. Additional transport pathways identified in the USEI Idaho facility Conceptual Site Model include deposition of radon decay products in cover material, root uptake of radionuclides in disposed wastes by native plants, and mixing of cover material by burrowing animals. Results of the two models and how the different transport and dose pathways affect results will be discussed. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

A Comparison of As-loaded Dose Calculations to Measured Dose Rates

Demonstrating that the radiation dose fields surrounding spent nuclear fuel (SNF) storage and transportation systems meet the applicable limits set forth in 10 CFR 72 for storage and 10 CFR 71 for transportation is essential for the safe handling of radioactive material. The Used Nuclear Fuel-Storage, Transportation, and Disposal Analysis Resource and Data System (UNF-ST&DARDS) [2] is used to provide realistic estimates of SNF-related safety margins. The UNF-ST&DARDS dose rate analysis approach differs from that used in typical licensing approaches, which use design-basis assemblies with bounding source term characteristics to demonstrate the packaging design complies with the regulations. These bounding licensing approaches can increase the time needed to qualify fuel for loading into dry storage and the time a loaded system must wait prior to transportation. UNF-ST&DARDS dose rate assessments allow quantification of realistic, uncredited safety margins associated with actual fuel loading compared with the regulatory limits. While realistic estimation of the dose field surrounding SNF systems may allow for additional flexibility in operations, it is essential to understand how these predictions compare to measured doses. The U.S. Department of Energy Office of Integrated Waste Management and the Prairie Island Indian Community conducted a transportation dose assessment to estimate the site-specific incident-free radiation doses from shipping SNF by rail from the Prairie Island Nuclear Generating Plant (PINGP) through the Prairie Island Indian Community Reservation and Trust Land [5,6]. For that effort, the dose rates were obtained for 50 TN-40 and TN-40HT systems in storage configurations. This work compares the predicted dose rates from UNF-ST&DARDS as-loaded calculations with dose rates measured from 50 SNF storage systems at PINGP. The remainder of this paper discusses the data obtained for the evaluation, the modeling methods, and the results of the calculations.

spent nuclear fuel (SNF), UNF-ST&DARDS, Validation↗

Test Plan for Investigation of Hydrogen Generation in SNF Canisters

This report presents a test plan to investigate radiolytic hydrogen generation in spent nuclear fuel (SNF) canisters containing Zr-based cladding materials. The initial primary contributor to the generation of radiolytic hydrogen is estimated to be the residual physisorbed water on the ZrO 2 film, post-dry out. Over the longer term the primary hydrogen source is associated with the aluminum hydroxides and water vapor. The proposed testing to be conducted in FY22 would consist of lab-scale testing on non-radioactive surrogates of oxidized ZIRLO tubing and unalloyed zirconium using a miniature steel canister (“mini-canister") designed to allow intermittent, in-situ sampling of the canister gas during irradiation. The mini-canister approach for irradiation with in-situ monitoring system was used in a recent and on-going study [McNamara and Verst, 2020a & 2020b; Verst et al., 2021] to measure radiolytic hydrogen generation from aluminum SNF cladding surrogate materials. This proposed testing will form part of the overall materials performance evaluation of the commercial SNF-in-canister system and is part of the technical bases for their continued safe dry storage

08 HYDROGEN↗

Variability and Spectral Characteristics of Three Flaring Gamma-Ray Quasars Observed by VERITAS and Fermi-LAT

Flat-spectrum radio quasars (FSRQs) are the most luminous blazars at GeV energies but only rarely emit detectable fluxes of TeV gamma rays, typically during bright GeV flares. We explore the gamma-ray variability and spectral characteristics of three FSRQs that have been observed at GeV and TeV energies by Fermi-LAT and VERITAS, making use of almost 100 hr of VERITAS observations spread over 10 yr: 3C 279, PKS 1222+216, and Ton 599. We explain the GeV flux distributions of the sources in terms of a model derived from a stochastic differential equation describing fluctuations in the magnetic field in the accretion disk and estimate the timescales of magnetic flux accumulation and stochastic instabilities in their accretion disks. We identify distinct flares using a procedure based on Bayesian blocks and analyze their daily and subdaily variability and gamma-ray energy spectra. Using observations from VERITAS, as well as Fermi, Swift, and the Steward Observatory, we model the broadband spectral energy distributions of PKS 1222+216 and Ton 599 during very high energy (VHE)–detected flares in 2014 and 2017, respectively, strongly constraining the jet Doppler factors and gamma-ray emission region locations during these events. Finally, we place theoretical constraints on the potential production of PeV-scale neutrinos during these VHE flares.

79 ASTRONOMY AND ASTROPHYSICS↗

Angular-momentum Transport in Proto-neutron Stars and the Fate of Neutron Star Merger Remnants

Both the core collapse of rotating massive stars, and the coalescence of neutron star (NS) binaries result in the formation of a hot, differentially rotating NS remnant. The timescales over which differential rotation is removed by internal angular-momentum transport processes (viscosity) have key implications for the remnant’s long-term stability and the NS equation of state (EOS). Guided by a nonrotating model of a cooling proto-NS, we estimate the dominant sources of viscosity using an externally imposed angular-velocity profile Ω(r). Although the magneto-rotational instability provides the dominant source of effective viscosity at large radii, convection and/or the Tayler–Spruit dynamo dominate in the core of merger remnants where dΩ/dr ≥ 0. Furthermore, the viscous timescale in the remnant core is sufficiently short that solid-body rotation will be enforced faster than matter is accreted from rotationally supported outer layers. Guided by these results, we develop a toy model for how the merger remnant core grows in mass and angular momentum due to accretion. We find that merger remnants with sufficiently massive and slowly rotating initial cores may collapse to black holes via envelope accretion, even when the total remnant mass is less than the usually considered threshold ≈1.2 M TOV for forming a stable solid-body rotating NS remnant (where M TOV is the maximum nonrotating NS mass supported by the EOS). This qualitatively new picture of the post-merger remnant evolution and stability criterion has important implications for the expected electromagnetic counterparts from binary NS mergers and for multimessenger constraints on the NS EOS

79 ASTRONOMY AND ASTROPHYSICS↗

Silicon-Equivalent Neutron Dose Estimations

Radiation transport calculations are often used to estimate dose or exposure to components and personnel surrounding a radiation source. The sources for these calculations are decaying radionuclides within the various nuclear materials. Under long-term radiation exposure, some components may show signs of material damage such as hardening, cracking, discoloration, etc. resulting from the dose received from nearby radioactive sources. Radiation dose quantities are a useful means to correlate material damage or degradation to radiation interactions. The degradation is often dependent on how incident radiation interacts and deposits energy into the material. This dependence implies that radiation dose should be properly defined for the material effect of interest. Generic dose quantities, such as total energy deposited, may not necessarily correlate well for degradation of any given material.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Graphite waste classification and disposal cost estimation for high temperature gas and salt reactors

As high-temperature reactor designs progress to demonstration, managing the radioactive wastes from these systems presents unique challenges. This work explores the irradiated graphite source term produced by three reactor designs: The Modular High Temperature Gas reactor (MHTGR), a pebble-bed High Temperature Gas Reactor (pb-HTGR), and a Fluoride-cooled High-temperature Reactor (FHR). We predicted a C-14 concentration of 4.3 Ci/m 3 for the MHTGR, 1.2 Ci/m 3 for the pebble bed HTGR, and 2.5 Ci/m 3 for the gFHR after 20 years of operation. The final C-14 concentration highly depended on the graphite nitrogen impurity, a major precursor for C-14. The C-14 concentration in all reactor types exceeded the 0.8 Ci/m3 threshold, resulting in a Class C waste classification. The costs associated with accepting the graphite after 20 years in a low-level waste disposal facility were projected to be 255 dollars per kWe for the MHTGR, 248 dollars per kWe for the pb-HTGR, and 56.8 dollars per kWe for the FHR.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Life Cycle Emissions and Health Cost Impacts of Producing Ethanol and Electricity from Willow and Switchgrass in the Riparian Buffers of Mid-Atlantic United States

The United States (US Mid-Atlantic Region (MAR) has the potential to grow a variety of perennial feedstocks such as switchgrass and shrub willow to increase domestic energy production. These cellulosic feedstocks have also shown improved ecosystem services, such as soil carbon sequestration, nitrate leaching reduction, and flood mitigation along rivers and streams as partially harvested riparian buffers. To examine the effects on greenhouse gases (GHGs) and criteria air pollutants (CAPs) from using these feedstocks to produce ethanol or electricity, we conducted a comprehensive life cycle assessment (LCA) and estimated the impact on human health costs when land use is changed from corn production for ethanol. Results indicate up to 54% reduced GHG per hectare from using willow and switchgrass feedstock sources to produce ethanol instead of corn. However, there was a trade-off in terms of CAP emission, as grass-based energy emitted more NO x and SO x compared to the corn ethanol pathway, except for SO X emissions from willow-based electricity. Electricity from cellulosic biomass had higher particulate matter (PM) emission compared to that from corn ethanol. Estimates for health cost to society ranged from $2498 ha –1 for electricity from switchgrass to a net benefit of $448 ha –1 for ethanol production from willow, depending on varying biomass yield under different market scenarios. Although using cellulosic feedstocks to produce bioenergy has great potential to reduce GHG emissions, CAP control measures are needed to manage CAP-induced health costs.

Bioenergy↗

A selection function toolbox for subsets of astronomical catalogues

ABSTRACT Large catalogues are ubiquitous throughout astronomy, but most scientific analyses are carried out on smaller samples selected from these catalogues by chosen cuts on catalogued quantities. The selection function of that scientific sample – the probability that a star in the catalogue will satisfy these cuts and so make it into the sample – is thus unique to each scientific analysis. We have created a general framework that can flexibly estimate the selection function of a sample drawn from a catalogue in terms of position, magnitude and colour. Our method is unique in using the binomial likelihood and accounting for correlations in the selection function across position, magnitude, and colour using Gaussian processes and spherical harmonics. We have created a new open-source python package selectionfunctiontoolbox that implements this framework and used it to make three different estimates of the APOGEE DR16 red giant sample selection function, as a subset of 2MASS, with each estimate using an increasing amount of technical knowledge of the APOGEE targeting. In a companion paper, we applied our methodology to derive estimates of the astrometric and spectroscopic selection functions of Gaia EDR3. Our framework will make it trivial for astrophysicists to estimate the selection function that they should be using with the custom sample of stars that they have chosen to answer their scientific question.

79 ASTRONOMY AND ASTROPHYSICS↗

MADWEC Techno-Economic Analysis: Cooperative Research and Development Final Report

The objective of this project was for the facility to conduct a techno-economic assessment of the Maximal Asymmetric Drag Wave Energy Converter (MADWEC), developed by the University of Massachusetts Dartmouth (UMass Dartmouth), used for powering remote monitoring and AUV charging systems compared to other existing power supply options. The assessment estimates capital expenditures (CapEx), operational expenditures (OpEx), and power performance for 18 scenarios with the purpose of identifying key cost drivers, comparing total system cost, and comparing the power performance of the power supply options in terms of required installed capacity and estimated theoretical annual energy performance. The scenarios include two end-uses: (1) AUV charging and (2) offshore remote monitoring); three power sources: (1) MADWEC), (2) photovoltaic (PV) solar buoy, (3) and traditional battery swapping); and three locations; (1) nearshore, (2) far-offshore, and (3) high-latitude). In addition, other project goals included developing high level installation, operation, and maintenance plans for each scenario.

16 TIDAL AND WAVE POWER↗