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There from the Beginning: The Women of Los Alamos National Laboratory Supporting National and International Nuclear Security

From the beginning of the Manhattan Project in the early 1940s, the women of what would become Los Alamos National Laboratory (LANL) worked in technical positions alongside their male counterparts, played a key role as computers, and worked in administrative jobs as secretaries, phone operators, bookkeepers, and on behalf of the U.S. Army in the Women’s Army Corps. Throughout the history of the Laboratory, women experts at LANL helped establish and lead important national and international security programs, with careers in science, technology, engineering, and mathematics. Over time, the women of Los Alamos have come together under various Employee Resource Groups, such as the Atomic Women, to help the next generation succeed in their technical fields. The Laboratory’s commitment to diversity and inclusion continues to this day, with current Laboratory Director Thom Mason leading LANL as the first national laboratory to join the Gender Champions in Nuclear Policy.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

High-Current Light-Ion Cyclotron for Applications in Nuclear Security and Radioisotope Production

In this article, we propose the conceptual design, with supporting beam dynamics results, of a normal conducting, separated-sector cyclotron with a strong-focusing field gradient designed to accelerate light ions with a charge-to-mass ratio of 1/2 up to 15–20 MeV/u. The design can support a host of applications for therapy, radiobiology, material science, and instrumentation development. The light-ion species, which can include a mixed ion beam, can be dynamically chosen to provide a range of characteristic signals appropriate for specific material identification such as special nuclear materials. A conservative baseline concept is presented which has been optimized for radioisotope production of alpha emitters and theranostic radiopharmaceuticals. The modular design is also demonstrated to be scalable in gross physical parameters by a factor of 2–3, thereby reducing the size, weight, and power requirements (SWaP) and enabling near-term security applications.

07 ISOTOPE AND RADIATION SOURCES↗

Nuclear Security Risks for HALEU Fuels

There is growing interest in high-assay low-enriched uranium (HALEU) for use in advanced nuclear reactors as a high-energy fuel source. The primary objectives of this report are to identify the security risks that directly result from HALEU and to identify the gaps and challenges it presents from a theft and sabotage perspective. This study focuses on HALEU security risks for the front end of the fuel cycle and includes a review of the supply chain, fuel fabrication, and transport for terrestrial reactors.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The Russian Invasion of Ukraine and Nuclear Security

You have in your hands a unique publication. Voices of Ukraine is a collection of testimonies from people working in the nuclear and radioactive source sector in Ukraine. The five texts in this extract are a preview of the full volume that will be published in early 2023. The accounts presented in this extract are very different from the newspaper articles or reports you may have read about the Russian invasion of Ukraine and the attack on and occupation of the Chornobyl Exclusion Zone and Zaporizhzhia NPP. Five people share their own stories of the personal and professional dilemmas they faced: How to endure an unending shift under enemy occupation when replacement workers weren’t permitted to relieve the staff; whether to remain in your childhood home or to flee abroad; how to support your community and country while maintaining the safe operation of nuclear sites in wartime conditions? The narratives of these individuals have far-reaching consequences for the nuclear sector in Ukraine but also far beyond it.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Precision γ-ray branching ratio measurements for long-lived fission products of importance to nuclear-security applications (TAMU Annual Report 2020)

Continuing with our effort of precisely measuring the branching ratios for long-lived fission products we have collected and measured two radiopure ¹⁵⁶Eu samples. The samples were collected on thin (40 μg/cm²) carbon-foil backings using a low-energy mass-separated beam of A = 156 fission products from CARIBU at Argonne National Laboratory. During collection, a HPGe detector was used to continuously monitor the implantation rate by detecting the characteristic γ rays emitted following the β decay of the shorter-lived fission products. The first sample had measured activity of 375 Bq while the second one had an activity of 700 Bq. The implanted samples were then shipped to Texas A&M University for measurement of the subsequent decay.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Development of Hopfield Artificial Neural Network for Anomaly Detection in Environmental Gamma Radiation Background: Consortium on Nuclear Security Technologies (CONNECT) (Q2 Report)

Environmental screening of gamma radiation consists of detecting weak nuisance and anomaly signal in the presence of strong and highly varying background. In a typical scenario, a mobile detector-spectrometer continuously measures gamma radiation spectra in short, e.g., one-second, signal acquisition intervals. The measurement data is a 2D matrix, where one dimension is gamma ray energy, and the other dimension is the number of measurements or total time. In principle, gamma radiation sources can be detected and identified from the measured data by their unique spectral lines. Detecting sources from data measured in a search scenario is difficult due to the highly varying background because of naturally occurring radioactive material (NORM), and low signal-to-noise ratio (S/N) of spectral signal measured during one-second acquisition intervals. The objective of this work is to explore supervised machine learning (ML) algorithms for development of a Hopfield Neural Network (HNN) in conjunction with an image processing algorithm for detection and identification of weak nuisances and anomalies events in the presence of a highly fluctuating background.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Detection of Anomalies in Environmental Gamma Radiation Background with Hopfield Artificial Neural Network - Consortium on Nuclear Security Technologies (CONNECT) Q3 Report

Environmental screening of gamma radiation consists of detecting weak nuisance and anomaly signal in the presence of strong and highly varying background. In a typical scenario, a mobile detector-spectrometer continuously measures gamma radiation spectra in short, e.g., one-second, signal acquisition intervals. The measurement data is a 2D matrix, where one dimension is gamma ray energy, and the other dimension is the number of measurements or total time. In principle, gamma radiation sources can be detected and identified from the measured data by their unique spectral lines. Detecting sources from data measured in a search scenario is difficult due to the highly varying background because of naturally occurring radioactive material (NORM), and low signal-to-noise ratio (S/N) of spectral signal measured during one-second acquisition intervals. The objective of this work is to investigate performance of a Hopfield Neural Network (HNN) in in detection and identification of weak nuisances and anomalies events in the presence of a highly fluctuating background. Performance of HNN algorithm is benchmarked using search data from an environmental screening campaign. One data set contained a 137 Cs source, and another dataset contained a 131 I source.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Detection of Anomalies in Gamma Background Radiation Data with K-Means and Self-Organizing Map Clustering Algorithms (Consortium on Nuclear Security Technologies (CONNECT) Q1 Report)

Environmental screening of gamma radiation consists of detecting weak nuisance and anomaly signal in the presence of strong and highly varying background. In a typical scenario, a mobile detector-spectrometer continuously measures gamma radiation spectra in short, e.g., one-second, signal acquisition intervals. The measurement data is a 2D matrix, where one dimension is gamma ray energy, and the other dimension is the number of measurements or total time. In principle, gamma radiation sources can be detected and identified from the measured data by their unique spectral lines. Detecting sources from data measured in a search scenario is difficult due to the highly varying background because of naturally occurring radioactive material (NORM), and low signal-to-noise ratio (S/N) of spectral signal measured during one-second acquisition intervals. The objective of this work is to explore unsupervised machine learning (ML) algorithms for detection and identification of weak nuisances and anomalies events in the presence of highly fluctuating background. The challenge is that spectral lines of isotopes are difficult to observe in one-second measurements. Averaging over the entire measurement campaign data set reveals spectral lines of most common background isotopes. Spectral lines of orphan sources, which might appear only in a few measurements during the campaign, will be washed out if averaging is performed over the entire measurement data set. The approach we have explored consists of extracting one-second measurements containing weak spectral features through data clustering. Averaging one-second spectra in a cluster should reveal the presence of anomaly sources. We created two ML models using K-means clustering and Neural Network Self-organizing Map (SOM). Performance of these ML models was benchmarked using search data. One data set contained 137 Cs source, and another dataset contained 131 I source.

61 RADIATION PROTECTION AND DOSIMETRY↗