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At least 73 records · Page 4

A substandard candle: the low-$$\nu $$ method at few-GeV neutrino energies

Abstract As accelerator-based neutrino oscillation experiments improve oscillation parameter constraints with more data, control over systematic uncertainties on the incoming neutrino flux and interaction models is increasingly important. The intense beams offered by modern experiments permit a variety of options to constrain the flux using in situ “standard candle” measurements. These standard candles must use very well understood interaction processes to avoid introducing additional interaction model dependence. One option often discussed in this context is the “low- $$\nu $$ ν ” method, which is designed to isolate neutrino interactions where there is low energy-transfer to the nucleus, such that the interaction cross section is expected to be approximately constant as a function of neutrino energy. The shape of the low-energy transfer event sample can then be used to extract the flux shape. Applications of the method at high neutrino energies (many tens of GeV) are well understood. However, the applicability of the method at the lower energies of current and future few-GeV accelerator neutrino experiments remains unclear due to the presence of nuclear and form-factor effects inherent in the interaction models.In this analysis we examine the prospects for improving constraints on the accelerator neutrino fluxes in situ with the low- $$\nu $$ ν method in an experiment-independent way, using (anti)neutrino interactions on argon and hydrocarbon targets from the GENIE, NEUT, NuWro and GiBUU event generators. We begin by investigating the extent to which deviations from the constant cross-section assumption are dependent on poorly understood aspects of the neutrino interaction model. We then assess whether a low energy-transfer event sample can be confidently identified using experimentally accessible observables. We finally consider how the practicalities of reconstructing the energy spectrum of interacting neutrinos in realistic detectors might further limit the utility of low- $$\nu $$ ν flux constraints. The results show that flux constraints from the low- $$\nu $$ ν method would be severely dependent on the interaction model assumptions used in an analysis of neutrinos with energies below 5 GeV, and anti-neutrinos below at least 15 GeV. The spread of model predictions show that a low- $$\nu $$ ν analysis is unlikely to offer much improvement on typical neutrino flux uncertainties, even with a perfect detector. Notably—running counter to the assumption inherent to the low- $$\nu $$ ν method—the model-dependence increases with decreasing energy transfer for experiments in the few-GeV region.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Air-, N2-, and O2-broadening and shift coefficients in the nu(3) spectral region of (C-12)H4

Results are presented of an analysis of 29 room-temperature laboratory absorption spectra of a dilute CH4 sample in dry air, N2, and O2 at total pressures ranging from 60 to 550 torr, yielding values of pressure-broadening and pressure-induced-shift coefficients for more than 450 vibration-rotation transitions in the nu(3), nu(2) + nu(4), and 2nu(2)-super-2 bands of (C-12)H4. Comparisons of the present results for the nu(3) and nu(2) + nu(4) bands with previous measurements on other bands and isotopes of CH4 show that, for a given transition, broadening by air and N2 are nearly equal, and broadening by O2 is smaller by less than 10 percent. It is also found that the pressure shift coefficients are more vibrational dependent than the pressure broadening coefficients.

Benner, D. C.↗

Analysis of Voyager spectra of the beta Cephei star nu Eridani

Voyager 500-1700 A spectrophotometric observations of the beta Cephei star nu Eri are presented and discussed. The Voyager observations were obtained in 1981 and cover six pulsation cycles of the star. These data are supplemented with a set of nine International Ultraviolet Explorer (IUE) SWP high-resolution observations covering one, earlier epoch, pulsation cycle. Light curves are derived from the Voyager data at 1055 and 1425 A. These light curves are found to be consistent in both shape and period with published optical curves. The 1055 A light curve also exhibits a phenomenon not seen in the optical curves: a small but highly significant systematic increase in the flux of the maximum light phases while maintaining a constant minimum light level over the interval of observation. Substantially larger errors in the longer wavelength data preclude discussion of this phenomenon in the 1425 A light curve. Examination of the far-UV continuum in nu Eri during this period shows that the color temperature is lower for the brighter maxima. Analysis of the far-UV continuum at maximum and minimum light yields an effective temperature difference between these two phases of 2200 + or - 750 K. Spectroscopically, three prominent features are seen in the Voyager data: a feature at 985 A mostly due to a blend of C III 977 A, H I Ly gamma 972 A, and N III 990 A; a feature at 1030 A due to H I Ly beta 1026 A and C II 1037 A; and the Si IV resonance doublet near 1400 A. A comparison of the 912-1700 A spectral region in nu Eri with a set of standard, i.e., nonpulsating stars, shows that nu Eri closely resembles the standard both in continuum shape and spectral line strengths with the possible exception of a slight flux excess between 912 and 975 A. The equivalent width of the 985 A feature is shown to vary in strength over the pulsation cycle in antiphase with the light curve and variations seen in the C IV 1548-1551 lines from the IUE data. This behavior of the 985 A feature is most likely caused by variations in the strength of the Ly gamma component of the blend. Comparisons are also made between nu Eri and the only other beta Cephei star studied in the far-UV, BW Vul, with the most notable differences between the two stars being the much larger delta(T(sub eff)) for BW Vul and the almost total absence of abnormalities in observed spectrum of nu Eri.

Porri, A.↗

Infrared laser spectroscopy of jet-cooled carbon clusters: the nu 5 band of linear C9

The nu 5 antisymmetric stretching vibration of 1 sigma+g C9 has been observed using direct infrared diode laser absorption spectroscopy of a pulsed supersonic cluster beam. Twenty-eight rovibrational transitions measured in the region of 2079-2081 cm-1 were assigned to this band. A combined least squares fit of these transitions with previously reported nu 6 transitions yielded the following molecular constants for the nu 5 band: nu 0 = 2 079.673 58(17) cm-1, B"= 0.014 321 4(10) cm-1, and B'=0.014 288 9(10) cm-1. The IR intensity of the nu 5 band relative to nu 6 was found to be 0.108 +/- 0.006. Theoretical predictions for the relative intensities vary widely depending upon the level of theory employed, and the experimental value reported here is in reasonable agreement only with the result obtained from the most sophisticated ab initio calculation considered (CCSD).

Non-NASA Center↗

Functionalized NU-1000 with an Iridium Organometallic Fragment: SO 2 Capture Enhancement

In this study, a new material, MOF-type [Ir]@NU-1000, was accessed from the incorporation of the iridium organometallic fragment [Ir{κ 3 (P,Si,Si)PhP(o-C 6 H 4 CH 2 Si i Pr 2 ) 2 }] into NU-1000. The new material incorporates less than 1 wt % of Ir(III) (molar ratio Ir to NU-1000, 1:11), but the heat of adsorption for SO 2 is significantly enhanced with respect to that of NU-1000. Being a highly promising adsorbent for SO 2 capture, [Ir]@NU-1000 combines exceptional SO 2 uptake at room temperature and outstanding cyclability. Additionally, it is stable and can be regenerated after SO 2 desorption at low temperature.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Final results on the $$0\nu \beta \beta $$ decay half-life limit of $$^{100}$$Mo from the CUPID-Mo experiment

Abstract The CUPID-Mo experiment to search for 0 $$\nu \beta \beta $$ ν β β decay in $$^{100}$$ 100 Mo has been recently completed after about 1.5 years of operation at Laboratoire Souterrain de Modane (France). It served as a demonstrator for CUPID, a next generation 0 $$\nu \beta \beta $$ ν β β decay experiment. CUPID-Mo was comprised of 20 enriched $$\hbox {Li}_{{2}}$$ Li 2 $$^{100}$$ 100 $$\hbox {MoO}_4$$ MoO 4 scintillating calorimeters, each with a mass of $$\sim 0.2$$ ∼ 0.2 kg, operated at $$\sim 20$$ ∼ 20 mK. We present here the final analysis with the full exposure of CUPID-Mo ( $$^{100}$$ 100 Mo exposure of 1.47 $$\hbox {kg} \times \hbox {year}$$ kg × year ) used to search for lepton number violation via 0 $$\nu \beta \beta $$ ν β β decay. We report on various analysis improvements since the previous result on a subset of data, reprocessing all data with these new techniques. We observe zero events in the region of interest and set a new limit on the $$^{100}$$ 100 Mo 0 $$\nu \beta \beta $$ ν β β decay half-life of $$T_{1/2}^{0\nu }$$ T 1 / 2 0 ν $$> {1.8}\times 10^{24}$$ > 1.8 × 10 24 year (stat. + syst.) at 90% CI. Under the light Majorana neutrino exchange mechanism this corresponds to an effective Majorana neutrino mass of $$\left $$ m β β $$<~{(0.28{-}0.49)} $$ < ( 0.28 - 0.49 ) eV, dependent upon the nuclear matrix element utilized.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for Heavy Neutral Leptons at the MINER$\nu$A detector

Heavy Neutral Leptons (HNL) are particles hypothesised to provide a mass generation mechanism for the active (observed) neutrino species, which are known to have nonzero mass from the definitive observation of neutrino oscillations. HNL are eigenstates of mass of the order $\mathcal{O}(0.1 − 1\,\,\mathrm{GeV}/c^{2})$, which mix into the active flavour eigenstates through the extended leptonic mixing matrix. Apart from neutrino mass, they could provide a natural dark matter candidate and a mechanism for matter-antimatter asymmetry in the early Universe, giving rise to today’s matter-dominated cosmos. Searches for HNL typically attempt to either confirm the existence of HNL through an excess in data that is most compatible with an HNL hypothesis, or by setting limits on the HNL parameter space $\left(M_{N4}, \left|U_{\alpha 4}\right|^{2}\right)$ in the case of statistically insignificant excess. Such searches are intensifying as part of a global research programme at both colliders and accelerator / atmospheric neutrino experiments. One such setting is the MINER$\nu$A experiment, located in the NuMI beamline at Fermilab. MINER$\nu$A has collected a large amount of data over seven years of operation to measure the cross-sections of neutrino-nucleus interactions necessary to drive systematic uncertainties down, in order for neutrino oscillation experiments to achieve sensitivity to CP violation in the neutrino sector. With the high-energy, high-intensity NuMI beam, and with good timing, position, and angular resolution leading to sensitivity to HNL decays, MINER$\nu$A is fertile ground for an HNL search, which is performed in this thesis. Specifically, a novel, experiment-agnostic and general simulation of HNL production and decay is presented and deployed; this simulation has been incorporated in the ubiquitous GENIE neutrino event generator for use with neutrino experiments in the future. The event selection and background characterisation is discussed in detail, including the primary background coming from charged-current coherent and diffractive pion production from neutrino-nucleus interactions, and constraints on the background using control regions from MINER$\nu$A data are derived. Finally, by means of a fake-data study given a background of $\mathcal{O}(500)$ events, the discovery potential and limit-setting capacity of MINER$\nu$A is demonstrated, and ways to improve this capacity are expounded upon.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effective CH4/N2 Separation using NU-1000 at High Pressures

Separation of methane (CH4) from other gases is of significant importance to reducing greenhouse gas emissions. In particular, the development and discovery of efficient adsorbents under pressure swing adsorption (PSA) conditions is a focus many research papers. We evaluated the potential of CH4/N2 separation performance using four adsorbents, including zirconium-based metal organic frameworks (NU-1000, UiO-66, and UiO-67) and a conventional adsorbent, zeolite-13X. Among them, NU-1000 presented high CH4/N2 selectivity (2.8) at 15 bar through ideal adsorbed solution theory because it has micro- and mesopores coupled with the large surface area, and a polar hydroxyl group along the pore surface. NU-1000 has a large CH4 working capacity (4.79) under PSA processes. These results demonstrated that NU-1000 is a sufficiently competitive adsorbent in PSA processes for CH4/N2 separation.

MOFs, NU-1000, separation↗

Computational and Experimental Characterization of the Ligand Environment of a Ni-Oxo Catalyst Supported in the Metal–Organic Framework NU-1000

Heterogeneous catalysts exhibit significant changes in composition due to the influence of operating conditions, and these compositional changes can have dramatic effects on catalytic performance. For traditional bulk metal heterogeneous catalysts, relationships between composition and catalytic operating conditions are well documented. However, the influence of operating conditions on the compositions of single-site heterogeneous catalysts remains largely unresolved. To address this, we report a combined computational and experimental characterization of a Ni oxo catalyst under catalytic hydrogenation conditions. Specifically, pair distribution function (PDF) analysis is combined with ab initio thermodynamic modeling to investigate ligand environments present on a Ni oxo cluster supported in the metal–organic framework NU-1000. Comparisons of the experimentally observed and simulated Ni–O coordination numbers and Ni–O, Ni···Ni, and Ni···Zr distances provide insight into the Ni ligand environment under H 2 (g). These comparisons suggest significant OH and H 2 O content and, further, that different Ni ions within the cluster and/or NU-1000 structure may comprise subtly different numbers of these ligands. Further, the observation of significant H 2 O content under H 2 (g) suggests that the NU-1000 support supplies H 2 O to the cluster. Examples of ligand environments that could lead to the observed PDFs are provided. Furthermore, the combination of simulations and experiments provides new insights into the ligand environment for Ni-NU-1000 catalysts that will be useful for understanding the ligand environments of other single-site Ni catalysts as well.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

The Covariance of PFNS Results from the Chi-Nu Experiment

The prompt fission neutron spectrum (PFNS) from neutron-induced fission is a fundamental quantity for the behavior of nuclear reactors, and has been measured many times on a wide variety of nuclei and covering different ranges of incident and emitted neutron energies. However, results from past measurements are frequently called into question in modern nuclear data evaluations because of a lack of thorough experimental documentation and incomplete uncertainty analyses. The Chi-Nu experiment at Los Alamos National Laboratory was designed to produce high-precision measurements of the PFNS of major actinides over a wide range of incident and emitted neutron energies, and with the documentation and covariance analysis required to ensure that the results of this experiment maintain their impact long into the future, thereby avoiding this pitfall of past measurements. In this work we describe the Chi-Nu experiment along with summaries of the treatment of and methods developed to address two important components of the analysis of Chi-Nu data: random-coincidence backgrounds and MCNP simulations. Furthermore, we describe the first results for correlations not just between all data points collected on a single target nucleus, but also between all data points from separate Chi-Nu measurements on 235 U and 239 Pu. These correlations are important for accurately calculating ratios of the PFNS from one actinide to another, which are rare and can be informative for nuclear data evaluation efforts.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Experimental and theoretical studies on collision-broadened lines in the nu-4 fundamental of methane.

High-resolution experimental and theoretical studies performed earlier by us on the collision-broadened rotational lines in the nu-3 and 2nu-3 bands of methane have been repeated on the lines in the nu-4 fundamental of the molecule. Line-width measurements and computations, as well as line-shape measurements, indicate that the significant differences which exist between the rotational term values of the nu-3 and nu-4 vibrational levels have no observable effect on the collision-broadening mechanism. Using the predictions of line-widths, based on the Anderson-Tsao-Curnutte theory in the extended version of Tejwani for octopolar molecules, the theoretical dependence of line-widths on temperature has been calculated for CH4-CH4, CH4-H2 and CH4-He collisions.

Varanasi, P.↗

Analysis of the upper atmosphere CO2(nu-2) vibrational temperatures retrieved from ATMOS/Spacelab 3 observations

An analysis of the upper atmospheric (80-116 km) CO2(nu-2) vibrational temperatures retrieved from atmospheric trace molecule spectroscopy (ATMOS) experiment Spacelab 3 spectra by using a nonlocal thermodynamic equilibrium (non-LTE) radiative transfer model is presented. Thermal collisions with atmospheric atomic oxygen keep this vibrational state very close to LTE up to around 100 km. Above this height, the different deviations from LTE retrieved from ATMOS/Spacelab 3 spectra for the Northern and the Southern Hemispheres are explained in terms of this collisional process and in terms of the different kinetic temperature profiles measured at those locations. From these simultaneous observations of the kinetic and CO2(nu-2) vibrational temperatures, a deactivation rate of CO2(nu-2) by O(3P) has been derived which leads to a rate coefficient value between 3 and 6 x 10 exp -12 cu cm/s and favors an independent or negative temperature dependence rate constant for the atmospheric temperature range. Cooling rates induced by the CO2 15-micron fundamental band in the upper mesosphere and lower thermosphere were derived from the simultaneous kinetic temperature, CO2(nu-2) vibrational temperature, and CO2 concentration, as measured by ATMOS/Spacelab 3, and found to be a factor of between 5 and 10 times larger than those generally accepted until very recently.

Lopez-Puertas, M.↗

Spectral intensities in the nu(sub 1) band of NH3

Intensities have been measured for individual transitions in the Q and R branches of the nu(sub 1) band of NH3 using a difference-frequency laser spectrometer. The data yield an integrated band strength of S(sup 0 sub v) = 219.36 +/- 1.03/sq cm/MPa at 297 K, corresponding to a transition moment of absolute value of mu(sub v) = 8.535(20) x 10(exp -32) C x m, and a Herman-Wallis correction factor,(1 + alpha(sub J)m), where alpha(sub J) = 0.0209(20). The intensities of a few lines for K greater than or equal to 7 were noticeably perturbed by a perpendicular Coriolis interaction with 2nu(sub 4)(E, l = 2), so were excluded from the fit. A small sample of nu(sub 3) band lines occurring in the nu(sub 1) band scans also yields a rough estimate of the nu(sub 3) band intensity with evident irregular perturbations.

Pine, A. S.↗

Model-Independent Description of $B\rightarrow D \pi \ell \nu$ Decays

In this contribution we present a novel, model-independent description of semileptonic $B\rightarrow D \pi \ell \nu$ decays. In addition, we discuss recent developments in the understanding of coupled-channel $D \pi$-$D \eta$-$D_s K$ S-wave scattering and, for the first time, apply them to semileptonic decays. We not only obtain model-independent predictions for kinematic distributions in $B\rightarrow D \pi \ell \nu$ decays, but also rule out the hypothesis that the gap between the inclusive $B\rightarrow X\ell\nu$ branching fraction and the sum over exclusive channels is made up predominantly by $B\rightarrow D^{(\ast)} \eta \ell \nu$ decays.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

RF Metrology of Lunar Highlands Regolith Simulant NU-LHT-2M

Understanding the electrical properties of lunar regolith is vital to modeling radiofrequency(RF) propagation on the lunar surface a fundamental step in planning lunar surface missions. Near the lunar south pole, the regolith has yet to be directly sampled and thus there remains uncertainty in the electrical properties of the regolith. The regolith simulant NU-LHT-2M is a highlands simulant that is representative of the expected chemical composition of the regolith near the lunar south pole. Previous studies have investigated properties of NU-LHT at UHF and S-band[1]. Future missions to the lunar south pole are expected to utilize X and Ka-band for direct-to-Earth links and UHF, S-band, C-band, and Ka-band for lunar surface communication[2]. As a result, it is necessary to electrically characterize the lunar regolith at these frequencies. In this paper, coaxial impedance dielectric reflectometry is performed on the NU-LHT-2M simulant using a commercially available soil permittivity measurement device. This study serves as a preliminary measurement of the simulant and may lead to enhanced efficacy of the measurement hardware for future applications.

simulant↗

RF Metrology of Lunar Highlands Regolith Simulant NU-LHT-2M

*Presentation for the publication* Understanding the electrical properties of lunar regolith is vital to modeling radiofrequency (RF) propagation on the lunar surface, a fundamental step in planning lunar surface missions. Near the lunar south pole, the regolith has yet to be directly sampled and thus there remains uncertainty in the electrical properties of the regolith. The regolith simulant NU-LHT-2M is a highlands simulant that is representative of the expected chemical composition of the regolith near the lunar south pole. Previous studies have investigated properties of NU-LHT at UHF and S-band[1]. Future missions to the lunar south pole are expected to utilize X and Ka-band for direct-to-Earth links and UHF, S-band, C-band, and Ka-band for lunar surface communication [2]. As a result, it is necessary to electrically characterize the lunar regolith at these frequencies. In this paper, coaxial impedance dielectric reflectometry is performed on the NU-LHT-2M simulant using a commercially available soil permittivity measurement device. This study serves as a preliminary measurement of the simulant and may lead to enhanced efficacy of the measurement hardware for future applications.

simulant↗

Structural reversibility of Cu doped NU-1000 MOFs under hydrogenation conditions

The metal-organic framework (MOF), NU-1000, and its metalated counterparts have found proof-of-concept application in heterogeneous catalysis and hydrogen storage amongst others. A vapor-phase technique, akin to atomic layer deposition (ALD), is used to selectively deposit divalent Cu ions on oxo, hydroxo-bridged hexa-zirconium(IV) nodes capped with terminal –OH and -OH 2 ligands. Subsequent reaction with steam yields node-anchored, CuII-oxo,hydroxo clusters. We find that cluster installation via AIM (= ALD In MOFs) is accompanied by an expansion of MOF mesopore (channel) diameter . We investigated the behavior of the cluster-modified material, termed Cu-AIM-NU-1000, to heat treatment up to 325 °C, at atmospheric pressure with a low flow of H2 into the reaction cell. The response under these conditions revealed two important results: (1) Above 200 °C, the initially installed few-metal-ion clusters reduce to neutral Cu atoms. The neutral atoms migrate from the nodes and aggregate into Cu nanoparticles. While the size of particles formed in the MOF interior is constrained by the width of mesopores (ca. 3 nm), those formed on the exterior surface of the MOF can grow as large as ca. 8 nm. (2) Reduction and release of Cu atoms from the MOFs nodes is accompanied NU-1000 undergoes dynamic structural transformation as it reverts back to its original dimension following the release. These results show while the MOF framework itself remains intact at 325 °C in an H 2 atmosphere, the small, AIM-installed Cu II -oxo,hydroxo clusters are stable with respect to reduction and conversion to metallic nanoparticles only up to ~200 °C.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Including Chi-Nu 235 U PFNS Experimental Data into an ENDF/B-VIII.1 Release Candidate Evaluation

This report documents an evaluation of 235 U prompt fission neutron spectra (PFNS) that is a release candidate for the upcoming U.S. nuclear data library, ENDF/B-VIII.1. This evaluation differs from its predecessor, ENDF/B-VIII.0, mainly by the inclusion of 235 U PFNS measured by the Chi-Nu team of LANL and LLNL. This data set is the first one that covers the 235 U PFNS for continuous incident-neutron energies of 1⁻20 MeV and outgoing-neutron energies from 10 keV⁻10 MeV with high precision. Previous data sets were either measured in a limited energy range or with less precision. Hence, these new Chi-Nu data provide decisive information for the evaluation. The resulting evaluated data correspond well to the new experimental PFNS. The evaluated PFNS also produce average mean energies and 239 Pu/ 235 U PFNS in agreement with associated Chi-Nu data. If one uses the new evaluated data to predict the neutron multiplication factor, k eff , of selected ICSBEP critical assemblies, the differences of simulated values compared to those using ENDF/B-VIII.0 is modest (less than 55 pcm). This difference in k eff can be easily accommodated by changes in the 235 U average prompt fission neutron multiplicity that is currently being re-evaluated. In addition to that, the new PFNS predict on average 235 U LLNL pulsed-sphere neutron-leakage spectra better than ENDF/B-VIIII.0 PFNS.

235U↗