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At least 73 records · Page 4

Heterogeneous multiphase flow properties of volcanic rocks and implications for noble gas transport from underground nuclear explosions

Of interest to the Underground Nuclear Explosion Signatures Experiment are patterns and timing of explosion-generated noble gases that reach the land surface. The impact of potentially simultaneous flow of water and gas on noble gas transport in heterogeneous fractured rock is a current scientific knowledge gap. This article presents field and laboratory data to constrain and justify a triple continua conceptual model with multimodal multiphase fluid flow constitutive equations that represents host rock matrix, natural fractures, and induced fractures from past underground nuclear explosions (UNEs) at Aqueduct and Pahute Mesas, Nevada National Security Site, Nevada, USA. Capillary pressure from mercury intrusion and direct air–water measurements on volcanic tuff core samples exhibit extreme spatial heterogeneity (i.e., variation over multiple orders of magnitude). Petrographic observations indicate that heterogeneity derives from multimodal pore structures in ash-flow tuff components and post-depositional alteration processes. Comparisons of pre- and post-UNE samples reveal different pore size distributions that are due in part to microfractures. Capillary pressure relationships require a multimodal van Genuchten (VG) constitutive model to best fit the data. Relative permeability estimations based on unimodal VG fits to capillary pressure can be different from those based on bimodal VG fits, implying the choice of unimodal vs. bimodal fits may greatly affect flow and transport predictions of noble gas signatures. The range in measured capillary pressure and predicted relative permeability curves for a given lithology and between lithologies highlights the need for future modeling to consider spatially distributed properties.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

The degassing history of the Earth: Noble gas studies of Archaean cherts and zero age glassy submarine basalts

Recent noble gas studies suggests the Earth's atmosphere outgassed from the Earth's upper mantle synchronous with sea floor spreading, ocean ridge hydrothermal activity and the formation of continents by partial melting in subduction zones. The evidence for formation of the atmosphere by outgassing of the mantle is the presence of radionuclides H3.-4, Ar-040 and 136 Xe-136 in the atmosphere that were produced from K-40, U and Th in the mantle. How these radionuclides were formed is reviewed.

Hart, R.↗

A system for low field imaging of laser-polarized noble gas

We describe a device for performing MRI with laser-polarized noble gas at low magnetic fields (<50 G). The system is robust, portable, inexpensive, and provides gas-phase imaging resolution comparable to that of high field clinical instruments. At 20.6 G, we have imaged laser-polarized (3)He (Larmor frequency of 67 kHz) in both sealed glass cells and excised rat lungs, using approximately 0.1 G/cm gradients to achieve approximately 1 mm(2) resolution. In addition, we measured (3)He T(2)(*) times greater than 100 ms in excised rat lungs, which is roughly 20 times longer than typical values observed at high ( approximately 2 T) fields. We include a discussion of the practical considerations for working at low magnetic fields and conclude with evidence of radiation damping in this system. Copyright 1999 Academic Press.

NASA Program Biomedical Research and Countermeasur↗

Noble gas component organization in 14301

A study is conducted of the organization of noble gases in the Apollo 14 breccia 14301, giving particular attention to xenon from the extinct radionuclides I-129 and Pu-244. An essential ingredient of this work is the intercomparison between noble gases released in single-stage melts of grain size fractions and those released in stepwise extractions. This approach resolves 'functional' noble gas components, which are organized by siting, into the specific genetic contributions on the basis of the 'activation energies' for diffusive loss. The procedure makes it possible to resolve various genetic components on the basis of the chemical and structural differences in their specific locations. Consequently, distinctions can be made among components acquired by different processes and among components which have undergone different regolith histories.

Bernatowicz, T. J.↗

Effect of Zeolitization on Noble Gas Transport in Natural Materials [Poster]

The goal of this project is to quantify the effect of adsorption on noble gas transport though rocks that contain zeolite compared with rocks that don't. Success is defined by developing a coefficient called Retardation that describes the separation effect of zeolites. This coefficient can then be used by gas transport modelers to predict field-scale observations of noble gases released underground in a chemical explosion

36 MATERIALS SCIENCE↗

Noble gas patterns in the atmospheres of Mars and Earth: A comparison via the SNC meteorites

Noble gas and nitrogen compositions in the glassy phase of the EETA 79001 shergottite correspond closely with Viking measurements. This direct evidence for the origin of the SNC meteorites on Mars, and for trapping of an unfractionated sample of Martian atmospheric gases in the 79001 glass, provides a reasonable basis for comparing the Martian and terrestrial atmospheres with more precision than that afforded by the Viking data set. Results are that, with one exception, elemental and isotopic compositions of nonradiogenic Martian noble gases are similar to those in the Earth's atmosphere; relatively small isotopic discrepancies in Kr and perhaps Xe may be attributable to different degrees of mass fractionation of a common parent reservoir. The anomaly is in Ar composition, where Martian Ar-36/AR-38 approx. 4 is strikingly lower than the values near 5.3 that characterize both the Earth and major meteoritic gas carriers. Although a primordial Martian ratio of 5.3 could in principle be altered by some planet specific process (e.g., cosmic ray spallation of surface materials) operating over geologic time, one has not been found that works.

Pepin, R. O.↗

A search for noble-gas evidence for presolar oxide grains

Early results from an ongoing search for isotopically distinctive noble gases as evidence for presolar oxide grains are presented. With some qualifications, we do not see such evidence in spinel rich acid residue fractions from the Allende meteorite. We remain hopeful that less abundant mineral separates may yet be fruitful. Presolar grains, micro-diamonds, silicon carbide, and graphite, were found in primitive meteorites. While the abundances of these three refractory C rich grains are low, a few hundred ppm, a few ppm, & less than 1 ppm, respectively in primitive meteorites, they are tagged with high concentrations of isotopically anomalous noble gas components, Xe-HL, KR & Xe-s and Ne-E(H), and Ne-E(L). These tags have served as tracers and allowed the development of techniques for their purification and eventual identification. One might expect similar amounts of refractory presolar oxides to have survived, but so far only three cases exist for their identification. The first two cases are individual corundum oxide grains. Huss et al. found one such grain from an Orgueil residue with an Al-26/Al-27 ratio of 8.9 x 10(exp -5), about 18 times higher than the canonical initial solar system value. The second corundum grain, from Murchison, was found by Nittler et al. to have unusual oxygen in addition to a similar Al-26/Al-27 ratio of 8.7 x 10(exp -4). The oxygen was depleted in O-18 by 22 percent and enriched in O-17 by a factor of 2. The third case is a measurement by Zinner et al. on an aggregate of fine grained spinels from a Murray residue with an O-17 enrichment and a possible O-18 depletion similar to the second grain, but much subdued. This is consistent with a few such presolar grains diluted by a much larger population of isotopically normal corundum grains and an even larger number of normal spinel grains.

Lewis, Roy S.↗

Noble gas evidence for the depositional and irradiational history of 60010-60009 core soils

Isotopic abundances of the noble gases have been determined in grain size separates of eleven soils from different depths in the 60010-60009 double drive tube and in magnetic and plagioclase separates from a few of these soils. Data for the 60010 core are presented here. The entire core was deposited a maximum of approximately 125 m.y. ago as deduced from the Ar-38 cosmic ray exposure age of soil 60009,457. Soils in the topmost 12 cm of the core show loss of cosmogenic He-3 and Ne-21 and gain of trapped solar gases in proportion to the degree of surface reworking by micrometeorites as deduced from FMR data. A variety of compositional and irradiational evidence suggests that soils in the core were formed by mixing of three or more components during or immediately prior to core deposition less than about 125 m.y. ago. Based on cosmogenic noble gases and a variety of other data soils 60009,457 and 60010,3107 are similar (and possibly identical) to two of the end member soils which formed the mixture. More mature soils in the core, however, could not have matured in situ from these two soils because of significant differences in noble gas abundances and chemical composition.

Bogard, D. D.↗

Noble gas studies on regolith materials from Apollo 14 and 15.

Abundances and isotopic compositions of the five stable noble gases, He, Ne, Ar, Kr, and Xe in soils and breccia were determined. The samples investigated included material from a range of depths in a trench and a core tube. Noble gas determinations were performed in a 6-inch all-metal mass spectrometer of high sensitivity. The grain size separates and stepwise heating experimental methods used give results that supplement each other. Calculated concentrations of spallation Xe-126 in many of the fines and gas-rich breccia are presented in a table. Bulk soil samples obtained by Apollo 14 show an inverse correlation of spallation Xe-126 with grain size.

Bogard, D. D.↗

Production Rates for Noble-Gas Isotopes in Eucrites

To get cosmic-ray exposure ages of meteorites from measured concentrations of cosmic-ray-produced ("cosmogenic") noble-gas isotopes, production rates for those isotopes are needed. The best production rates take into consideration the composition of the meteorite and the "shielding" of the sample (the pre-atmospheric size and shape of the meteoroid and the sample s location in the meteoroid). For ordinary chondrites, there have been many sets of measurements to establish production systematics. The Ne-22/Ne-21 is often used to help to get shielding-dependent production rates. We report here numerical simulations for the production of isotopes of the light noble gases He, Ne, and Ar in both basaltic and cumulate eucrites for several sizes.

Reedy, R. C.↗

Element distribution and noble gas isotopic abundances in lunar meteorite Allan Hills A81005

Antarctic meteorite ALLAN HILLS A81005, an anorthositic breccia, is recognized to be of lunar origin. The noble gases in this meteorite were analyzed and found to be solar-wind implanted gases, whose absolute and relative concentrations are quite similar to those in lunar regolith samples. A sample of this meteorite was obtained for the analysis of the noble gas isotopes, including Kr(81), and for the determination of the elemental abundances. In order to better determine the volume derived from the surface correlated gases, grain size fractions were prepared. The results of the instrumental measurements of the gamma radiation are listed. From the amounts of cosmic ray produced noble gases and respective production rates, the lunar surface residence times were calculated. It was concluded that the lunar surface time is about half a billion years.

Kraehenbuehl, U.↗

Comparison of different noble gas injections by massive gas injection on plasma disruption mitigation on Experimental Advanced Superconducting Tokamak

Massive gas injection (MGI) is a traditional plasma disruption mitigation method. This method directly injected massive gas into the pre-disruption plasma and had been developed on the Experimental Advanced Superconducting Tokamak (EAST). Different noble gas injection experiments, including He, Ne, and Ar, were performed to compare the mitigation effect of plasma disruption by evaluating the key parameters such as flight time, pre-thermal quench (pre-TQ), and current quench (CQ). The flight time was shorter for low atomic number ( Z ) gas, and the decrease in flight time by increasing the amount of gas was insignificant. However, both pre-TQ and CQ durations decreased considerably with the increase in gas injection amount. The effect of atomic mass on pre-TQ and CQ durations showed the opposite trend. The observed trend could help in controlling CQ duration in a reasonable area. Moreover, the analysis of radiation distribution with different impurity injections indicated that low Z impurity could reduce the asymmetry of radiation, which is valuable in mitigating plasma disruption. These results provided essential data support for plasma disruption mitigation on EAST and future fusion devices.

Physics↗

The Origin of Noble Gas Isotopic Heterogeneity in Icelandic Basalts

Two models for generation of heterogeneous He, Ne and Ar isotopic ratios in Icelandic basalts are evaluated using a mixing model and the observed noble gas elemental ratios in Icelandic basalts,Ocean island Basalt (OIBs) and Mid-Ocean Ridge Basalt (MORBs). Additional information is contained in the original extended abstract.

Dixon, E. T.↗

Data supporting the article titled "Heterogeneous Multiphase Flow Properties of Volcanic Rocks and Implications for Noble Gas Transport from Underground Nuclear Explosions"

The submission is a Reproducible Research (RR) data archive that contains the supporting multiphase fluid flow and curve fitting results of the Vadose Zone Journal article titled: "Heterogeneous Multiphase Flow Properties of Volcanic Rocks and Implications for Noble Gas Transport from Underground Nuclear Explosions." The article's DOI number is the following: https://doi.org/10.1002/vzj2.20123. Please see the "Methods and Materials" section of the journal article and the ReadMe.txt in the RR_ARCHIVE folder for further details. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-NA0003525. SAND Number: SAND2021-3407 O.

mercury injection capillary pressure↗