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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

MAPPING THE GAS TURBULENCE IN THE COMA CLUSTER: PREDICTIONS FOR ASTRO-H

Astro-H will be able for the first time to map gas velocities and detect turbulence in galaxy clusters. One of the best targets for turbulence studies is the Coma cluster, due to its proximity, absence of a cool core, and lack of a central active galactic nucleus. To determine what constraints Astro-H will be able to place on the Coma velocity field, we construct simulated maps of the projected gas velocity and compute the second-order structure function, an analog of the velocity power spectrum. We vary the injection scale, dissipation scale, slope, and normalization of the turbulent power spectrum, and apply measurement errors and finite sampling to the velocity field. We find that even with sparse coverage of the cluster, Astro-H will be able to measure the Mach number and the injection scale of the turbulent power spectrum—the quantities determining the energy flux down the turbulent cascade and the diffusion rate for everything that is advected by the gas (metals, cosmic rays, etc.). Astro-H will not be sensitive to the dissipation scale or the slope of the power spectrum in its inertial range, unless they are outside physically motivated intervals. We give the expected confidence intervals for the injection scale and the normalization of the power spectrum for a number of possible pointing configurations, combining the structure function and velocity dispersion data. Importantly, we also determine that measurement errors on the line shift will bias the velocity structure function upward, and show how to correct this bias.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2017

Attosecond transient absorption of a bound wave packet coupled to a smooth continuum

Here, we investigate the possibility of using transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In a recent work, we have shown that photoionization of such a coherent bound electron wave packet opens up for pulse characterization with unprecedented temporal accuracy—independent of the atomic structure—with maximal photoemission at all kinetic energies given a wave packet with zero relative phase. Here, we perform numerical propagation of the time-dependent Schrödinger equation and analytical calculations based on perturbation theory to show that the energy-resolved maximal absorption of photons from the attosecond pulse does not uniquely occur at a zero relative phase of the initial wave packet. Instead, maximal absorption occurs at different relative wave packet phases, distributed as a non-monotonous function with a smooth $-\pi /2$ shift across the central photon energy (given a Fourier-limited Gaussian pulse). Similar results are also found in helium. Our finding is surprising, because it implies that the energy-resolved photoelectrons are not mapped one-to-one with the energy-resolved absorbed photons of the attosecond pulse.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

In-Operando Characterization of P-I-N Perovskite Solar Cell Under Reverse Bias

A solar module is often exposed to a variety of intensity and uniformity illumination conditions throughout a day. In the field, objects or dirt can block light from hitting the module creating a partial shading event. When a partial shading event occurs the module power point tracking system will typically push the shaded cells into reverse bias in order to avoid the current loss from the other series connected illuminated cells. When perovskite solar cells are operated in reverse bias, electrochemical reactions can occur, leading to both reversible and irreversible performance losses. Excess holes generated by reverse bias cause and push the oxidation reaction of halide ions from the lattice to neutral halogen interstitial. Small interstitial halogen atoms can diffuse across the device and potentially move from the perovskite layer and into the transport layers, shifting the fermi levels in the devices. In this investigation we utilize cross-sectional kelvin probe atomic force microscopy to map the band energetics of perovskite solar cells during reverse bias. We observe a 150 meV decrease in the work function of the C 60 . This leads to a decrease of 150 mV and 4 mA/cm 2 in V oc and in J sc respectively. Finally, we discuss methods to prevent this irreversible degradation after a perovskite device is held under reverse bias.

fullerene↗
NASA NTRS1990

QPSK carrier-acquisition performance in the advanced receiver 2

The frequency-acquisition performance of the Costas cross-over loop which is used in the Advanced Receiver 2 (ARX 2) to perform Quadrature Phase Shift Keying (QPSK) carrier tracking is described. The performance of the Costas cross-over loop is compared to two other QPSK carrier tracking loops: the MAP estimation loop and the generalized Costas loop. Acquisition times and probabilities of acquisition as functions of both loop signal-to-noise ratio and frequency-offset to loop-bandwidth ratio are obtained using computer simulations for both type-2 and type-3 loops. It is shown that even though the MAP loop results in the smallest squaring loss for all signal-to-noise ratios, the MAP loop is sometimes outperformed by the other two loops in terms of acquisition time and probability.

Hinedi, S.↗
NASA NTRS2016

ERRATUM: 'MAPPING THE GAS TURBULENCE IN THE COMA CLUSTER: PREDICTIONS FOR ASTRO-H'

The published version of this paper contained an error in Figure 5. This figure is intended to show the effect on the structure function of subtracting the bias induced by the statistical and systematic errors on the line shift. The filled circles show the bias-subtracted structure function. The positions of these points in the left panel of the original figure were calculated incorrectly. The figure is reproduced below (with the original caption) with the correct values for the bias-subtracted structure function. No other computations or figures in the original manuscript are affected.

galaxies: clusters: intracluster medium- methods: ↗
DOE OSTI2019

Shifts in dominant tree mycorrhizal associations in response to anthropogenic impacts

Plant-fungal symbioses play critical roles in vegetation dynamics and nutrient cycling, modulating the impacts of global changes on ecosystem functioning. Here, we used forest inventory data consisting of more than 3 million trees to develop a spatially resolved “mycorrhizal tree map” of the contiguous United States. We show that abundances of the two dominant mycorrhizal tree groups—arbuscular mycorrhizal (AM) and ectomycorrhizal trees—are associated primarily with climate. Further, we show that anthropogenic influences, primarily nitrogen (N) deposition and fire suppression, in concert with climate change, have increased AM tree dominance during the past three decades in the eastern United States. Given that most AM-dominated forests in this region are underlain by soils with high N availability, our results suggest that the increasing abundance of AM trees has the potential to induce nutrient acceleration, with critical consequences for forest productivity, ecosystem carbon and nutrient retention, and feedbacks to climate change.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Gating Single Molecules with Counterions

We report atomic-scale gating and visualization of local charge distribution within individual rare-earth-based molecular complexes on a metallic surface. The complexes are formed by a positively charged lanthanum ion coordinated to a (pcam)3 molecule and a negatively charged counterion trapped underneath via electrostatic interactions on a Au(111) surface. Local gating is performed by adding an additional negatively charged counterion to one side of the complex, which results in the redistribution of charges within the complex and a positive shift of the frontier orbitals. This is caused by the internal Stark effect induced by the added counterion. This effect is directly captured using tunneling spectroscopy and spectroscopic mapping at 5 K substrate temperature. The polarizability of the complex is corroborated by density functional theory and analytical calculations based on experimental findings. Furthermore, the influence of charge polarization on nearby complexes is investigated in a cluster purposely assembled using three complexes, which reveals maintaining the charge states as in single complexes. These findings will enable the design of robust charged rare-earth complexes to be tailored for potential solid-state applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Lithium's low-temperature phase transitions: Insights into quantum lattice dynamics and superconductivity

The large lattice dynamics of lithium, driven by its low atomic mass, results in energetically similar structures and significant isotope effects under pressure, posing challenges to current theoretical models. Above 20 GPa and at low temperatures, lithium's electronic properties deviate from simple metallic behavior, with superconductivity emerging in a complex, pressure-dependent manner, alongside an unusual isotope effect. The structural phases of 7 Li reported under these conditions are inconsistent across studies, and the structures of 6 Li remain unexamined. These gaps limit our understanding of the effects of pressure on lithium's electronic properties and the role of quantum lattice effects on its structural behavior under pressure. Here, we integrate experimental and theoretical approaches to investigate the low-temperature structural phase boundaries in lithium isotopes. We map the structural phase diagram of 7 Li from 5 to 55 GPa and 15–75 K, identifying the sequence fcc → ℎ⁡R⁢1 → cI16. A pronounced isotope effect is observed, with 6 Li shifting the fcc → ℎ⁡R⁢1 phase boundary to lower pressures at 15 K. Density functional theory calculations further clarify how these structural changes affect superconducting properties, particularly emphasizing the role of the fcc → ℎ⁡R⁢1 transition in lithium's superconductivity. Furthermore, our findings offer insights into the unique behavior of lithium isotopes under pressure.

36 MATERIALS SCIENCE↗
NASA NTRS2000

Remote Sensing of Wind Fields and Aerosol Distributions with Airborne Scanning Doppler Lidar

The coherent Doppler lidar, when operated from an airborne platform, offers a unique measurement capability for study of atmospheric and surface processes and feature. This is especially true for scientific objectives requiring measurements in optically-clear air, where other remote sensing technologies such as Doppler radar are at a disadvantage in terms of spatial resolution and coverage. The atmospheric lidar remote sensing groups of several US institutions, led by Marshall Space Flight Center, have developed an airborne coherent Doppler lidar capable of mapping the wind field and aerosol structure in three dimensions. The instrument consists of about a 1 Joule/pulse (eyesafe) lidar transceiver, telescope, scanner, inertial measurement unit, and operations control system to orchestrate all subsystem functions and tasks. The scanner is capable of directing the expanded lidar beam in a variety of ways, in order to extract vertically resolved wind fields. Horizontal resolution is about 1 km; vertical resolution is even finer. Winds are obtained by measuring backscattered, Doppler-shifted laser radiation from naturally-occurring aerosol particles (on an order of 1 micron in diameter). Measurement coverage depends on aerosol spatial distribution and concentration. Velocity accuracy has been verified to be about 1 m/s. A variety of applications has been demonstrated during the three flight campaigns conducted during 1995-1998. Examples will be shown during the presentation. In 1995, boundary layer winds over the ocean were mapped with unprecedented resolution. In 1996, unique measurements were made of flow over the complex terrain of the Aleutian Islands; interaction of the marine boundary layer jet with the California coastal mountain range; a weak dry line in Texas - New Mexico; an upper tropospheric jet stream; the angular dependence of sea surface scattering; and in-flight radiometric calibration using the surface of White Sands National Monument. In 1998, the first measurements of eyewall and boundary layer winds within a hurricane were made with the airborne Doppler lidar. Potential future applications, and plans for improvements, will also be identified.

Rothermel, Jeffry↗
DOE OSTI2018

Efficient design of random metasurfaces

Random media introduce large degrees of freedom in device design and can thus address challenges in manipulating optical waves. Wave shaping with metasurfaces has mainly utilized periodic or quasi-periodic grids, and the potential of random arrangement of particles for devices has only come under investigation recently. The main difficulty in pursuing random metasurfaces is the identification of the degrees of freedom that optimize their efficiencies and functions. They can also encode information using the statistics of particle distribution. We propose a phase-map that accounts for the statistical nature of random media. The method takes into account effects of random near-field couplings that introduce phase errors by affecting the phase shift of elements. The proposed approach increases the efficiency of our random metasurface devices by up to ~20%. Furthermore, this work paves the way toward the efficient design of random metasurfaces with potential applications in highly secure optical cryptography and information encoding.

Nasari, Hadiseh↗
DOE OSTI2018

Interface properties and built-in potential profile of a LaCr O 3 / SrTi O 3 superlattice determined by standing-wave excited photoemission spectroscopy

LaCrO 3 (LCO)/SrTiO 3 (STO) heterojunctions are intriguing due to a polar discontinuity along [001], exhibiting two distinct and controllable charged interface structures [(LaO) + /(TiO 2 ) 0 and (SrO) 0 /(CrO 2 ) - ] with induced polarization, and a resulting depth-dependent potential. In this study, we have used soft- and hard-x-ray standing-wave excited photoemission spectroscopy (SW-XPS) to quantitatively determine the elemental depth profile, interface properties, and depth distribution of the polarization-induced built-in potentials. We observe an alternating charged interface configuration: a positively charged (LaO) + /(TiO 2 ) 0 intermediate layer at the LCO top /STO bottom interface and a negatively charged (SrO) 0 /(CrO 2 ) - intermediate layer at the STO top /LCO bottom interface. Using core-level SW data, we have determined the depth distribution of species, including through the interfaces, and these results are in excellent agreement with scanning transmission electron microscopy and electron energy-loss spectroscopy mapping of local structure and composition. SW-XPS also enabled deconvolution of the LCO and STO contributions to the valence-band (VB) spectra. Using a two-step analytical approach involving first SW-induced core-level binding-energy shifts and then VB modeling, the variation in potential across the complete superlattice is determined in detail. As a result, this potential is in excellent agreement with density functional theory models, confirming this method as a generally useful tool for interface studies.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2023

Top‐Down Regulation by a Reindeer Herding System Limits Climate‐Driven Arctic Vegetation Change at a Regional Scale

Warming-driven growth of tall woody vegetation in the Arctic has the potential to accelerate climate change through multiple positive feedbacks. Local-scale evidence suggests that large herbivores limit this vegetation shift, but there is uncertainty at larger, regional scales whether current herbivory pressure is a major top-down control on ecosystem structure and functioning. Across a 67,000 km2 region of the Yamal Peninsula in West Siberia, we integrated satellite remote sensing with a novel data set mapping the migrations of herds comprising 151,000 domesticated reindeer. Where reindeer numbers varied over space, higher reindeer herbivory pressure was consistently linked with lower coverage of tall woody vegetation. Within areas dominated by this vegetation type, productivity and climate were increasingly decoupled where reindeer density was higher. Our spaceborne fingerprint detection suggests that large herbivores, at current population densities, counteract Arctic vegetation responses to climate change over large spatial scales.

Reindeer Herding System↗
NASA NTRS2001

Remote Sensing of Wind Fields and Aerosol Distribution with Airborne Scanning Doppler Lidar

The coherent Doppler laser radar (lidar), when operated from an airborne platform, is a unique tool for the study of atmospheric and surface processes and features. This is especially true for scientific objectives requiring measurements in optically-clear air, where other remote sensing technologies such as Doppler radar are typically at a disadvantage. The atmospheric lidar remote sensing groups of several US institutions, led by Marshall Space Flight Center, have developed an airborne coherent Doppler lidar capable of mapping the wind field and aerosol structure in three dimensions. The instrument consists of an eye-safe approx. 1 Joule/pulse lidar transceiver, telescope, scanner, inertial measurement unit, and flight computer system to orchestrate all subsystem functions and tasks. The scanner is capable of directing the expanded lidar beam in a variety of ways, in order to extract vertically-resolved wind fields. Horizontal resolution is approx. 1 km; vertical resolution is even finer. Winds are obtained by measuring backscattered, Doppler-shifted laser radiation from naturally-occurring aerosol particles (of order 1 micron diameter). Measurement coverage depends on aerosol spatial distribution and composition. Velocity accuracy has been verified to be approx. 1 meter per second. A variety of applications have been demonstrated during the three flight campaigns conducted during 1995-1998. Examples will be shown during the presentation. In 1995, boundary layer winds over the ocean were mapped with unprecedented resolution. In 1996, unique measurements were made of. flow over the complex terrain of the Aleutian Islands; interaction of the marine boundary layer jet with the California coastal mountain range; a weak dry line in Texas - New Mexico; the angular dependence of sea surface scattering; and in-flight radiometric calibration using the surface of White Sands National Monument. In 1998, the first measurements of eyewall and boundary layer winds within a hurricane were made with the airborne Doppler lidar. Potential applications and plans for improvement will also be described.

Rothermel, Jeffry↗
DOE OSTI2025

Success Path Method: Introduction to the Success Path Method Software Tool©

As part of its commitment to advancing safety and reliability assessment methodologies, Argonne National Laboratory pioneered the use of an evaluation method called the Success Path Method (SPM) to improve risk management for offshore oil and gas operations. The development of the SPM at Argonne has been driven by the need to improve existing risk assessment methodologies by focusing on the steps necessary for success rather than failure modes alone. This is particularly important for industrial environments like offshore facilities that perform multiple functions under a continuously evolving set of operational conditions – such as water depth and temperature, currents, and weather conditions. In these dynamic environments, the traditional Probabilistic Risk Assessment (PRA) approach is far too complex as it focuses on what can go wrong – which comprises an infinite failure space that must be fully explored and understood. By shifting the focus to a finite space of success paths, the SPM enables operators and decision makers to prioritize a manageable number of steps that must go right to ensure success. Building on its five decades of experience in safety assessments for the nuclear industry, Argonne made major adaptations to existing risk assessment methods utilizing features similar to fault trees that are traditionally used in PRA to map all pathways in which the system can malfunction. In contrast, SPM identifies the components and processes that must function correctly to achieve specific outcomes – such as preventing the uncontrolled release of hydrocarbons during drilling operations. The SPM framework integrates equipment, procedures, software, processes, and human actions to ensure that physical barriers meet critical safety functions in dynamic operational conditions. This approach helps identify failure modes and improve operational risk management by narrowing the focus to key success elements, which in turn reduces uncertainty and helps users understand, manage, and respond to failures.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2016

Vortex flux dynamics and harmonic ac magnetic response of Ba(Fe 0.94 Ni 0.06 ) 2 As 2 bulk superconductor

Vortex dynamics and nonlinear ac response are studied in a Ba(Fe 0.94 Ni 0.06 ) 2 As 2 ( T c = 18.5 K) bulk superconductor in magnetic fields up to 12 T via ac susceptibility measurements of the first ten harmonics. A comprehensive study of the ac magnetic susceptibility and its first ten harmonics finds shifts to higher temperatures with increasing ac measurement frequencies (10 to 10,000 Hz) for a wide range of ac (1, 5, and 10 Oe) and dc fields (0 to 12 T). The characteristic measurement time constant t1 is extracted from the exponential fit of the data and linked to vortex relaxation. The Anderson-Kim Arrhenius law is applied to determine flux activation energy E a /k as a function dc magnetic field. The de-pinning, or irreversibility lines, were determined by a variety of methods and extensively mapped. The ac response shows surprisingly weak higher harmonic components, suggesting weak nonlinear behavior. Lastly, our data does not support the Fisher model; we do not see an abrupt vortex glass to vortex liquid transition and the resistivity does not drop to zero, although it appears to approach zero exponentially.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2012

Wavespace-Based Coherent Deconvolution

Array deconvolution is commonly used in aeroacoustic analysis to remove the influence of a microphone array's point spread function from a conventional beamforming map. Unfortunately, the majority of deconvolution algorithms assume that the acoustic sources in a measurement are incoherent, which can be problematic for some aeroacoustic phenomena with coherent, spatially-distributed characteristics. While several algorithms have been proposed to handle coherent sources, some are computationally intractable for many problems while others require restrictive assumptions about the source field. Newer generalized inverse techniques hold promise, but are still under investigation for general use. An alternate coherent deconvolution method is proposed based on a wavespace transformation of the array data. Wavespace analysis offers advantages over curved-wave array processing, such as providing an explicit shift-invariance in the convolution of the array sampling function with the acoustic wave field. However, usage of the wavespace transformation assumes the acoustic wave field is accurately approximated as a superposition of plane wave fields, regardless of true wavefront curvature. The wavespace technique leverages Fourier transforms to quickly evaluate a shift-invariant convolution. The method is derived for and applied to ideal incoherent and coherent plane wave fields to demonstrate its ability to determine magnitude and relative phase of multiple coherent sources. Multi-scale processing is explored as a means of accelerating solution convergence. A case with a spherical wave front is evaluated. Finally, a trailing edge noise experiment case is considered. Results show the method successfully deconvolves incoherent, partially-coherent, and coherent plane wave fields to a degree necessary for quantitative evaluation. Curved wave front cases warrant further investigation. A potential extension to nearfield beamforming is proposed.

Bahr, Christopher J.↗
DOE OSTI2025

Seedless nonresonant gas-flow velocimetry with single-shot coherent Rayleigh-Brillouin scattering

We demonstrate neutral gas-flow velocimetry by exploiting the optical dipole forces exerted by precisely tailored high-intensity laser fields on polarizable particles, in the form of single-shot coherent Rayleigh-Brillouin scattering (CRBS). This enables mapping of the velocity distribution function of the particles in a single laser shot of approximately 200 ns duration, allowing us to perform spectroscopic measurements in the time, rather than the frequency, domain. Importantly, CRBS results in a coherent signal beam, which renders the technique ideal for measurements in optically noisy environments. By correlating the time shift of the resulting spectrum to the Doppler shift caused by the bulk motion of particles, we perform neutral gas-flow velocimetry without the need to seed the flow, nondestructively, for a variety of gases, atomic or molecular. We demonstrate gas-flow velocimetry at flow velocities as low as 1 m ⁢s −1 , with similar velocity resolution, while temperature and gas density can also be estimated from the same single-shot spectra. To prove the effectiveness of the measurement technique, we benchmark it against Pitot tube measurements, which show excellent agreement.

Gerakis, Alexandros [Luxembourg Institute of Scien↗