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At least 73 records · Page 4

Seasonal Disappearance of Far-Infrared Haze in Titan's Stratosphere

A far-infrared emission band attributed to volatile or refractory haze in Titan's stratosphere has been decreasing in intensity since Cassini's arrival in 2004. The 220 cm(sup -1) feature, first seen by the Voyager Infrared Interferometer Spectrometer, has only been found in Titan's winter polar region. The emission peaks at about 140 km altitude near the winter stratospheric temperature minimum. Observations recorded over the period 2004-2012 by the Composite Infrared Spectrometer on Cassini show a decrease in the intensity of this feature by about a factor of four. Possible seasonal causes of this decline are an increase in photolytic destruction of source chemicals at high altitude, a lessening of condensation as solar heating increased, or a weakening of downwelling of vapors. As of early 2012, the 220 cm(sup -1) haze has not yet been detected in the south. The haze composition is unknown, but its decrease is similar to that of HC3N gas in Titan's polar stratosphere, pointing to a nitrile origin.

Jennings, Donald E.↗

Photolytic Hazes in the Atmosphere of 51 Eri b

We use a 1D model to address photochemistry and possible haze formation in the irradiated warm Jupiter 51 Eridani b. The intended focus was to be carbon, but sulfur photochemistry turns out to be important. The case for organic photochemical hazes is intriguing but falls short of being compelling. If they form, they are likeliest to do so if vertical mixing in 51 Eri b is weaker than in Jupiter, and they would be found below the regions where methane and water are photolyzed. The more novel result is that photochemistry turns H2S into elemental sulfur, here treated as S8. In the cooler models, S8 is predicted to condense in optically thick clouds of solid sulfur particles, whilst in the warmer models S8 remains a vapor along with several other sulfur allotropes that are both visually striking and potentially observable. For 51 Eri b, the division between models with and without condensed sulfur is at an effective temperature of 700 K, which is within error its actual effective temperature; the local temperature where sulfur condenses is between 280 and 320 K. The sulfur photochemistry we have discussed is quite general and ought to be found in a wide variety of worlds over a broad temperature range, both colder and hotter than the 650-750 K range studied here, and we show that products of sulfur photochemistry will be nearly as abundant on planets where the UV irradiation is orders of magnitude weaker than it is on 51 Eri b.

stars: individual(51 Eri b)↗

Large Aerosol Particles Favor Haze Conditions Through Limitations on Water Budget and Activation Kinetics

Experiments in the Pi Convection‐Cloud Chamber conducted by systematically changing the diameter of injected dry aerosol particles while holding the temperature difference constant demonstrate that dry diameter strongly influences the onset of haze‐dominated conditions. Two factors contribute: the system becomes water‐limited, resulting in reduction of supersaturation by growing aerosol particles to the activation diameter; and the activation process becomes kinetically limited. Dry aerosol diameter exerts a strong influence on activation time, with a power‐law exponent of 9/2. Kinetically limited activation occurs when the ratio of the activation and droplet residence times is greater than unity. The findings demonstrate that a haze‐dominated state, where cloud formation is suppressed, can be achieved not only with weak supersaturation forcing and high aerosol concentration but also with large, hygroscopic aerosol particles. These results have implications for cloud formation in polluted environments, fog development near the ocean, and hygroscopic cloud seeding.

54 ENVIRONMENTAL SCIENCES↗

Interior radiances in optically deep absorbing media. 3: Scattering from Haze L

The interior radiances are calculated within an optically deep absorbing medium scattering according to the Haze L phase function. The dependence on the solar zenith angle, the single scattering albedo, and the optical depth within the medium is calculated by the matrix operator method. The development of the asymptotic angular distribution of the radiance in the diffusion region is illustrated through a number of examples; it depends only on the single scattering albedo and on the phase function for single scattering. The exact values of the radiance in the diffusion region are compared with values calculated from the approximate equations proposed by Van de Hulst. The variation of the radiance near the lower boundary of an optically thick medium is illustrated with examples. The attenuation length is calculated for various single scattering albedos and compared with the corresponding values for Rayleigh scattering. The ratio of the upward to the downward flux is found to be remarkably constant within the medium. The heating rate is calculated and found to have a maximum value at an optical depth of two within a Haze L layer when the sun is at the zenith.

Kattawar, G. W.↗

Multiple scattered radiation emerging from continental haze layers. 1: Radiance, polarization, and neutral points

The complete radiation field is calculated for scattering layers of various optical thicknesses. Results obtained for Rayleigh and haze scattering are compared. Calculated radiances show differences as large as 23% compared to the approximate scalar theory of radiative transfer, while the same differences are approximately 0.1% for a continental haze phase function. The polarization of reflected and transmitted radiation is given for various optical thicknesses, solar zenith angles, and surface albedos. Two types of neutral points occur for aerosol phase functions. Rayleigh-like neutral points arise from zero polarization that occurs at scattering angles of 0 deg and 180 deg. For Rayleigh phase functions, the position of these points varies with the optical thickness of the scattering layer. Non-Rayleigh neutral points are associated with the zeros of polarization which occur between the end points of the single scattering curve, and are found over a wide range of azimuthal angles.

Kattawar, G. W.↗

Effect of atmospheric haze and sun angle on automatic classification of ERTS-1 data

The effect of variations in sun angle and haze level on the accuracy of automatic classification of Earth Resources Technology Satellite-1 (ERTS-1) data was studied by classifying ERTS imagery in which such variations were computer-simulated. It was found that relatively small changes in sun angle and haze level can substantially reduce classification accuracy.

Potter, J.↗

A lower limit on the top of Jupiter's haze layer

Remote sensing observations of the Jovian atmosphere at wavelengths ranging from UV to the IR are affected by the presence of haze layers above the visible clouds. These layers are difficult to detect as they generally contain submicron particles. In the present paper, a sequence of Voyager images of high-latitude haze, which extends through the Jovian stratosphere into the mesosphere is presented and discussed.

Cook, A. F., II↗

UMR dual mode CCN counter (modes: CFD plus haze)

The chamber consists of two vertical plates 100 cm long in the vertical direction and 13 cm wide, with a 0.8 cm spacing between the plates. The haze mode is used for the nuclei active at supersaturations (S) from 0.0133 to 0.173%. In this mode the two plates are kept at the same temperature (25 C). In the CFD mode the supersaturation is determined by the temperature difference between the two plates. About 40 minutes is required to obtain a spectrum (5 values of S in the CFD mode, plus 7 values of S in the haze mode). About half of this time is used to adjust the temperatures and flows; the rest is used in actual counting of the nuclei. Comparisons of the counter to other types of counters are reported.

Alofs, D. J.↗

Polarization studies of the Venus UV contrasts - Cloud height and haze variability

The present investigation is concerned with the measurement of differences in the polarization of bright and dark areas on Venus. The differential polarization is matched by simple models in which the cloud height, amount of submicron haze above the clouds, and absorber amount in the clouds are varied. Physical and chemical models consistent with the findings are proposed. The differences in polarization between bright and dark ultraviolet features on Venus are found to have a straightforward interpretation in terms of known constituents of the atmosphere near the cloud tops. The observations of the polarization in four colors over 2 1/2 Venus years imply that the submicron haze and UV absorbers are anticorrelated, and that the clouds lie slightly (approximately 1 km) lower in the dark regions. These findings pose strong constraints on any model for the brightness variations in the UV.

Esposito, L. W.↗

Vertical distribution of scattering hazes in Titan's upper atmosphere

Radial intensity scans of a Voyager 2 high phase angle image of Titan have been inverted to yield vertical extinction profiles at 1 deg intervals around the limb. A detached haze layer with peak particle number densities of about 0.2 cu/cm exists at all latitudes south of about 45 N, and at an altitude of 300-350 km. The optical depth 0.01 level lies at a radius of 2932 + or - 5 km at the equator and at a radius of 2915 + or - 10 km over the poles (altitudes of 357 + or - 5 and 340 + or - 10 km, respectively). In addition to the haze layer at 300-350 km, there is a small enhancement in the extinction at about 450 km which exists at all latitudes between 75 deg S and about 60 deg N.

Rages, K.↗

Radiative effects of the arctic haze

During the recent Arctic Gas and Aerosols Sampling Project flight series, the absorption of solar radiation by the Arctic haze was measured directly for the first time. Absorpton was measured in three narrow band channels, and the measurements were used to calibrate a high resolution solar flux model, which was then used to compute atmospheric heating rates. Analyses of data from three flights with estimated optical depths of 0.26, 0.17, and 0.31 at 500 nm produced instantaneous solar heating rates of the order of 1.1 to 1.5 K/day. These rates are greater by a factor of 2 to 3 than heating in the absence of the haze. Possible climatic implications are briefly discussed.

Valero, F. P. J.↗

The absorption of solar radiation by the Arctic atmosphere during the haze season and its effects on the radiation balance

Measurements of broadband spectral absorption of solar radiation by the Arctic atmosphere during haze events are reported. A preliminary analysis of the data indicates that large changes occur in the radiative transfer processes in the Arctic during haze events. For example, the planetary albedo is estimated to increase by 2.5 percent over the ocean and to decrease by 9 percent over the ice cap. Changes of such magnitude in the radiative parameters have the potential for significant climatic effects. The need for further experimental and modeling efforts is emphasized.

Valero, F. P. J.↗

Martian north polar hazes and surface ice - Results from the Viking Survey/Completion mission

The character of both the retreating polar cap edge and the accompanying atmospheric ice haze has been determined during the 1979-1980 Viking Survey/Completion mission observations of the Martian north polar regions. The ability of these Viking IR observations to distinguish haze from surface condensate yields a more accurate seasonal regression for the polar cap than can be determined from visual images. The transition from ice-free ground to a predominantly ice-covered surface at the cap edge spans 5-10 deg of latitude.

Christensen, P. R.↗

Titan - Far-infrared and microwave remote sensing of methane clouds and organic haze

Titan's surface and plausible atmospheric thermal opacity sources, which include gaseous N2, CH4, and H2, together with CH4 clouds and organic haze, are sufficient to match available earth-based and Voyager observations of Titan's thermal emission spectrum. Dominant thermal emission sources are the surface, at greater than 1 cm wavelengths, atmospheric N2 for the 1-200 micron range, condensed and gaseous CH4 for 200-20 microns, and molecular bands and organic haze at less than 20 microns.

Thompson, W. R.↗

Arctic haze and the radiation balance

Airborne measurements of the absorption of solar radiation by the Arctic haze indicate atmospheric heating rates of 0.15 to 0.25/Kday at latitudes between 72.6 and 74.0 N during the early spring. The haze interaction with solar radiation alters the radiative balance of the atmosphere-surface system. Generally, this interaction results in an increase of the solar energy absorbed by the atmosphere and in a decrease of the radiation absorbed by the ground. The cumulative deposition of black carbon over the surface produces a change in the optical properties of the ice which may results in an accelerating rate of ice melt. Experimental evidence of the magnitude of this effect is necessary to properly evaluate its consequences. An extended monitoring program is suggested.

Valero, Francisco P. J.↗

Nature of the stratospheric haze on Uranus - Evidence for condensed hydrocarbons

The characteristics and origin of lower-stratosphere haze on Uranus are investigated on the basis of high-phase-angle images obtained at 430-600 nm with the wide-angle and narrow-angle cameras of Voyager 2 during its encounter with Uranus in January 1986. The data-reduction and model-fitting procedures are explained in detail, and the results are presented in extensive tables and graphs. The data are found to be best matched by a haze consisting of particles of modal radius 130 + or - 20 nm and number density 2 + or - 1 per cu cm at the 44-mbar level; such aerosols could be formed by the stratospheric condensation of photochemically produced hydrocarbon gases (locally formed diacetylene and ethane, acetylene, and diacetylene formed at higher altitudes). A total aerosol production rate of (2-15) x 10 to the -17th g/sq cm sec is estimated.

Pollack, James B.↗

The effects of the Arctic haze as determined from airborne radiometric measurements during AGASP II

The effect of the Arctic-haze aerosol on the parameters of solar radiation was investigated using airborne radiometric measurements of radiation parameters during the second Arctic Gas and Aerosol Sampling Project. Simultaneously with absorption measurements, optical depths and total, direct, and scattered radiation fields were determined. The experimentally determined parameters were used to define an aerosol model, which was then used to calculate atmospheric heating rate profiles. It was found that, besides the increased absorption (30 to 40 percent) and scattering of radiation by the atmosphere, Arctic haze reduces the surface absorption of solar energy by 6 to 10 percent, and the effective planetary albedo over ice surfaces by 3 to 6 percent.

Valero, Francisco P. J.↗

A study of photopolarimeter system UV absorption data on Jupiter, Saturn, Uranus, and Neptune - Implications for auroral haze formation

The present investigation of the dark hazes of Jupiter, Saturn, Uranus, and Neptune on the basis of Voyager 2 UV data notes a geographic correlation between the auroral zones of Jupiter and Saturn and UV-dark polar regions. While the auroral fluxes and penetration depths on Jupiter and Saturn may suffice for a darkening of the polar regions by auroras' action on methane, Uranus and Neptune are found to be bright at all latitudes. In the former case, this brightness is in keeping with auroral electron energies too small to reach the CH4 homopause at which haze production occurs; in the latter case, a UV-dark band exists from 30 deg S to 5 deg N which is probably unrelated to auroral processes.

Pryor, Wayne R.↗