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At least 73 records · Page 4

Remediating neutron damage in large area planar Ge-DSSD with amorphous germanium contacts through annealing and pulse-height correction

Large area, position sensitive planar germanium detectors offer new opportunities in -ray spectroscopy. For in-beam studies remediating neutron damage is important. This work studied a mechanically cooled circular planar 9 × 1 cm wafer with orthogonal 16 × 16 amorphous germanium strip electrodes. Before neutron irradiation the wafer was heated in-cryostat to above 373 K for more than 24 h in order to test the robustness of the contacts and the mechanical cooler. No deterioration in performance was observed. The detector was then exposed to controlled doses of 2.2 MeV neutrons, produced from the 7 Li(p,n) 7 Be reaction until substantial damage was observed. Averaged over the surface of the wafer, a flux of 1.9(1) x 10 9 n/cm 2 was delivered. The detector then survived thermal cycling and 350 K (~77°C) annealing for 70 h which substantially reduced hole trapping. pulse-height correction is investigated to further mitigate the neutron damage. Higher temperature annealing at 365 K was not successful.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

LET spectra measurements from the STS-35 CPDs

Linear energy transfer (LET) spectra derived form automated track analysis system (ATAS) track parameter measurements for crew passive dosimeters (CPD's) flown with the astronauts on STS-35 are plotted. The spread between the seven individual spectra is typical of past manual measurements of sets of CPD's. This difference is probably due to the cumulative net shielding variations experienced by the CPD's as the astronauts carrying them went about their activities on the Space Shuttle. The STS-35 mission was launched on Dec. 2, 1990, at 28.5 degrees inclination and 352-km altitude. This is somewhat higher than the nominal 300-km flights and the orbit intersects more of the high intensity trapped proton region in the South Atlantic Anomaly (SAA). However, in comparison with APD spectra measured on earlier lower altitude missions (STS-26, -29, -30, -32), the flux spectra are all roughly comparable. This may be due to the fact that the STS-35 mission took place close to solar maximum (Feb. 1990), or perhaps to shielding differences. The corresponding dose and dose equivalent spectra for this mission are shown. The effect of statistical fluctuations at the higher LET values, where track densities are small, is very noticeable. This results in an increased spread within the dose rate and dose equivalent rate spectra, as compared to the flux spectra. The contribution to dose and dose equivalent per measured track is much greater in the high LET region and the differences, though numerically small, are heavily weighted in the integral spectra. The optimum measurement and characterization of the high LET tails of the spectra represent an important part of the research into plastic nuclear track detector (PNTD) response. The integral flux, dose rate, dose equivalent rate and mission dose equivalent for the seven astronauts are also given.

Source record↗

Measurements of the radiation dose to LDEF by means of passive dosimetry

A very simple experiment was fielded on LDEF to measure the energetic radiation dose by means of passive dosimetry. It consisted of two identical packets of 16 LiF thermoluminescent dosimeters (TLD) arranged in planar arrays. One array was placed on the leading edge of the spacecraft, the other on the trailing edge. These arrays were installed in opaque packets of 1 mil Al foil and Kapton tape mounted behind an Al plate of 30 mils thickness. The nominal energy thresholds were 14 MeV for protons and 650 keV for electrons. In addition to the flight arrays, two control arrays were prepared which were kept with the flight arrays as long as possible during experimental integration and then stored in the lab. The flight and control arrays were read out alternating in groups of four; it was found that the control dose was negligible. The flight and control detectors were exposed to a 55 MeV proton beam in order to provide a recalibration of the detectors. It was found that the post-flight and pre-flight calibrations were in good agreement. A comparison of results with the prediction shows that the measured dose was a factor of 4 to 5 low. It is possible that there was in-flight annealing of the TLDs as a result of the long mission and perhaps temperature excursions of the sensors. The East-West effect was larger than expected. The ratio of 1.65 is approximately what was expected for the protons alone. Electrons should reduce the dose ratio since electrons add equally to the leading and trailing edge dose. A possible explanation is that the electron dose was negligible compared to the proton dose.

Blake, J. B.↗

Sensitivity and Detection Limit of Spectroscopic-Grade Perovskite CsPbBr 3 Crystal for Hard X-Ray Detection

We report spectroscopic-grade single crystal detectors can register the energies of individual X-ray interactions enabling photon-counting systems with superior resolution over traditional photoconductive X-ray detection systems. Current technical challenges have limited the preparation of perovskite semiconductors for energy-discrimination X-ray photon-counting detection. Here, this work reports the deployment of a spectroscopic-grade CsPbBr 3 Schottky detector under reverse bias for continuum hard X-ray detection in both the photocurrent and spectroscopic schemes. High surface barriers of approximate to ≈ 1 eV are formed by depositing solid bismuth and gold contacts. The spectroscopic response under a hard X-ray source is assessed in resolving the characteristic X-ray peak. The methodology in enhancing X-ray sensitivity by controlling the X-ray energies and flux, and voltage, is described. The X-ray sensitivity varies between a few tens to over 8000 μC Gy air -1 cm -2 . The detectable dose rate of the CsPbBr 3 detectors is as low as 0.02 nGy air s -1 in the energy discrimination configuration. Finally, the unbiased CsPbBr 3 device forms a spontaneous contact potential difference of about 0.7 V enabling high quality of the CsPbBr 3 single crystals to operate in "passive" self-powered X-ray detection mode and the X-ray sensitivity is estimated as 14 μC Gy air -1 cm -2 . The great potential of spectroscopic-grade CsPbBr 3 devices for X-ray photon-counting systems is anticipated in this work.

36 MATERIALS SCIENCE↗

Preliminary results of radiation measurements on EURECA

The eleven-month duration of the EURECA mission allows long-term radiation effects to be studied similarly to those of the Long Duration Exposure Facility (LDEF). Basic data can be generated for projections to crew doses and electronic and computer reliability on spacecraft missions. A radiation experiment has been designed for EURECA which uses passive integrating detectors to measure average radiation levels. The components include a Trackoscope, which employs fourteen plastic nuclear track detector (PNTD) stacks to measure the angular dependence of high LET (greater than or equal to 6 keV/micro m) radiation. Also included are TLD's for total absorbed doses, thermal/resonance neutron detectors (TRND's) for low energy neutron fluences and a thick PNTD stack for depth dependence measurements. LET spectra are derived from the PNTD measurements. Preliminary TLD results from seven levels within the detector array show that integrated does inside the flight canister varied from 18.8 +/- 0.6 cGy to 38.9 +/- 1.2 cGy. The TLD's oriented toward the least shielded direction averaged 53% higher in dose than those oriented away from the least shielded direction (minimum shielding toward the least shielded direction varied from 1.13 to 7.9 g/cm(exp 2), Al equivalent). The maximum dose rate on EURECA (1.16 mGy/day) was 37% of the maximum measured on LDEF and dose rates at all depths were less than measured on LDEF. The shielding external to the flight canister covered a greater solid angle about the canister than the LDEF experiments.

Benton, E. V.↗

Physical Properties of Candidate X-ray Detector Material Rb 4 Ag 2 BiBr 9

Recently, metal halide perovskites have emerged as promising semiconductor candidates for sensitive X-ray photon detection due to their suitable band gap energies, excellent charge transport properties, and low material cost afforded by their low-temperature solution-processing preparation. Furthermore, we report an improved methodology for single crystal growth and thermal and electrical properties of a two-dimensional (2D) layered halide material Rb 4 Ag 2 BiBr 9 , which has been identified as a potential candidate for X-ray radiation detection applications. The measured heat capacity for Rb 4 Ag 2 BiBr 9 implies that there are no structural phase transitions upon cooling. Temperature dependence of thermal transport measurements further suggests remarkably low thermal conductivities of Rb 4 Ag 2 BiBr 9 that are comparable to the lowest reported in literature. The bulk crystal resistivity is determined to be 2.59 × 10 9 Ω·cm from the current–voltage (I–V) curve. Density of trap states is estimated to be ~10 10 cm –3 using the space-charge-limited-current measurements. The fabricated Rb 4 Ag 2 BiBr 9 -based X-ray detector shows good operational stability with no apparent current drift, which may be ascribed to the 2D crystal structure of Rb 4 Ag 2 BiBr 9 . Finally, by varying the X-ray tube current to change the corresponding dose rate, the Rb4Ag2BiBr9 X-ray detector sensitivity is determined to be 222.03 μC Gy –1 cm –2 (at an electric field of E = 24 V/mm).

36 MATERIALS SCIENCE↗

Evaluation of planar silicon pixel sensors with the RD53A readout chip for the Phase-2 Upgrade of the CMS Inner Tracker

The Large Hadron Collider at CERN will undergo an upgrade inorder to increase its luminosity to7.5 × 10$^{34}$ cm$^{-2}$s$^{-1}$. The increased luminosityduring this High-Luminosity running phase, starting around 2029,means a higher rate of proton-proton interactions, hence a largerionizing dose and particle fluence for the detectors. The currenttracking system of the CMS experiment will be fully replaced inorder to cope with the new operating conditions. Prototype planarpixel sensors for the CMS Inner Tracker with square50 μm × 50 μm and rectangular100 μm × 25 μm pixels read out by theRD53A chip were characterized in the lab and at the DESY-II testbeamfacility in order to identify designs that meet the requirements ofCMS during the High-Luminosity running phase. A spatial resolutionof approximately 3.4 μm (2 μm) is obtained using themodules with 50 μm × 50 μm(100 μm × 25 μm) pixels at the optimalangle of incidence before irradiation. After irradiation to a 1 MeVneutron equivalent fluence ofΦ$_{eq}$ = 5.3 × 10$^{15}$ cm$^{-2}$, a resolution of9.4 μm is achieved at a bias voltage of 800 V using a modulewith 50 μm × 50 μm pixel size. All modulesretain a hit efficiency in excess of 99% after irradiation tofluences up to 2.1 × 10$^{16}$ cm$^{-2}$. Further studies ofthe electrical properties of the modules, especially crosstalk, arealso presented in this paper.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Biology and Medicine, Fall 1965 Semiannual report

Reports on radiation medicine, radiobiology, EPR STUDIES of OH radicals in ice, radiation doses on manned space missions, silicon detectors, and recovery of yeast after irradiation

X-RAY IRRADIATION↗

Criticality Accident Alarm System Modeling for the Uranium Processing Facility

The Criticality Accident Alarm System (CAAS) for the Uranium Processing Facility (UPF) provides coverage for two primary processing facilities. For UPF, detailed documentation and drawings of the design are readily available. While this design information allows for some CAAS modeling features to match the actual design with a high level of accuracy, assumptions and simplifications are necessary as it is unrealistic and unnecessary to replicate many aspects of the design. A set of modeling guidelines and techniques were used to develop consistency between the MCNP6 models. While ensuring conservatism, overly conservative choices must be avoided to demonstrate the minimum accident of concern can be detected. To ensure proper modeling choices were made for the final models, a group of parametric studies were performed to evaluate the impact on the dose rates detected at the individual detectors. Some of these modeling choices and/or associated parametric studies include: - Modeling the grid steel area above the detectors as homogeneous stainless steel and determining the impact on detectability with an increasing density. - Modeling the presence of equipment in close proximity to the CAAS detectors. - Determining an appropriate material density to represent miscellaneous items not specifically modeled. - Evaluating the impact of sprinkler activation. The results of UPF CAAS analyses show that the modeling assumptions made based on the detailed design and parametric studies are appropriate and demonstrate accurate yet conservative models have been developed for detecting minimum accident of concern within the UPF.

61 RADIATION PROTECTION AND DOSIMETRY↗

A Compact Electron-Proton Spectrometer for Moon / Mars Surface Space Weather Monitoring and Crew Protection (CEPS)

Small mass/low-power sensors are needed for autonomous Moon/Mars surface ops that provide alerts to impending adverse space weather conditions. In order to use current operational forecasting tools, a sensor capable of measuring both high-energy electrons and protons is needed. By combining high-TRL Timepix technology with a CdTe layer, this project leverages known technology to fill a critical gap for surface operations. Typical space weather sensors are at least an order of magnitude higher in mass than is expected from Timepix-based devices and are deployed on robotic assets away from human crews. High fidelity measurements at the crew location and subsequent ability are needed to provide warnings to crews to shelter with a device that can easily be carried on the Lunar and Martian surfaces.​ The aim of this project is the development of compact, low power space weather sensors for crew protection based on the combination of AES flight heritage Timepix hardware with novel CdTe (Cadmium Telluride) sensors. CdTe technology has only recently matured to a point where it can be reliably used with Timepix detectors. These detectors will be able to measure electron spectra in an energy range relevant to the RELEASE model, which is used operationally by NASA to provide crew early warning of Solar Energetic Particle Events as well as protons in the energy ranges relevant to human health allowing for event ‘nowcasting’ and total event crew dose prediction. Compared to existing solutions these detectors will be compact enough to travel with crew, providing a significant advantage to space environment situation awareness. Project results indicate that CdTe-based Timepix sensors respond well to energetic electrons, and particle tracks are sufficiently distinct to be able to measure in a mixed radiation field. Thermal testing results point to a needed design modification to mitigate high temperatures the detector will see in space. Radiation susceptibility testing was conducted to assess the radiation hardness of the CdTe-Timepix assembly. Overall, the assembly continued to operate up to 100 kRad of gamma-ray exposure. The system calibration did show drift over time but recovered once exposure was complete.

Dan James Fry↗

CEPS – A Compact Electron-Proton Spectrometer

Small mass/low-power sensors are needed for autonomous Moon/Mars surface ops that provide alerts to impending adverse space weather conditions. In order to use current operational forecasting tools, a sensor capable of measuring both high-energy electrons and protons is needed. By combining high-TRL Timepix technology with a CdTe layer, this project leverages known technology to fill a critical gap for surface operations. Typical space weather sensors are at least an order of magnitude higher in mass than is expected from Timepix-based devices and are deployed on robotic assets away from human crews. High fidelity measurements at the crew location and subsequent ability are needed to provide warnings to crews to shelter with a device that can easily be carried on the Lunar and Martian surfaces.​ The aim of this project is the development of compact, low power space weather sensors for crew protection based on the combination of AES flight heritage Timepix hardware with novel CdTe (Cadmium Telluride) sensors. CdTe technology has only recently matured to a point where it can be reliably used with Timepix detectors. These detectors will be able to measure electron spectra in an energy range relevant to the RELEASE model, which is used operationally by NASA to provide crew early warning of Solar Energetic Particle Events as well as protons in the energy ranges relevant to human health allowing for event ‘nowcasting’ and total event crew dose prediction. Compared to existing solutions these detectors will be compact enough to travel with crew, providing a significant advantage to space environment situation awareness. Project results indicate that CdTe-based Timepix sensors respond well to energetic electrons, and particle tracks are sufficiently distinct to be able to measure in a mixed radiation field. Detector response functions were developed for both electrons and protons. Measurement results showed response to both electrons and protons in the energy range of interest for human space flight.

Radiation↗

Large area vertical Ga 2 O 3 Schottky diodes for X-ray detection

In this work, the Schottky barrier diodes were fabricated from a bulk Sn-doped (001) n-type Ga 2 O 3 substrate with a Si-doped epitaxial layer grown by hydride vapor phase epitaxy (HVPE), which demonstrate a good response to X-rays. Circular metal contacts with diameters ranging from 50 to 1500 um and square metal contacts ranging from 100 X 100 to 1600 X 1600 um 2 were deposited on the wafer. The devices were characterized for their electrical performance including forward current–voltage (FIV), reverse current–voltage (RIV), and capacitance-voltage (CV) measurements. The best device showed a breakdown voltage of –804 V and the devices tested had an average ideality of 1.12. The devices exhibited a clear response to X-rays even at zero bias with an experimentally observed response time 1.03 s and a linear response of detector signal to the X-ray dose rate. The experimentally observed device response time improved to 0.25 s when bias voltage is applied. The device also survived a long-term stability test of over 2 h under a constant X-ray irradiation. The sensitivity and the lower limit of detection for X-ray by Ga2O3 epitaxial Schottky detectors were discussed and determined as 43.5 C/mGy cm –2 at –200 V and 8.31 nGy Air /s, respectively.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Depth distribution of absorbed dose on the external surface of Cosmos 1887 biosatellite

Significant absorbed dose levels exceeding 1.0 Gy day-1 have been measured on the external surface of the Cosmos 1887 biosatellite as functions of depth in stacks of thin thermoluminescent detectors (TLDs) of U.S.S.R. and U.S.A. manufacture. The dose was found to decrease rapidly with increasing absorber thickness, thereby indicating the presence of intensive fluxes of low-energy particles. Comparison between the U.S.S.R. and U.S.A. results and calculations based on the Vette Model environment are in satisfactory agreement. The major contribution to the dose under thin shielding thickness is shown to be from electrons. The fraction of the dose due to protons and heavier charged particles increases with shielding thickness.

NASA Discipline Number 04-10↗

Depth Dose Distribution Study within a Phantom Torso after Irradiation with a Simulated Solar Particle Event at NSRL

The adequate knowledge of the radiation environment and the doses incurred during a space mission is essential for estimating an astronaut's health risk. The space radiation environment is complex and variable, and exposures inside the spacecraft and the astronaut's body are compounded by the interactions of the primary particles with the atoms of the structural materials and with the body itself Astronauts' radiation exposures are measured by means of personal dosimetry, but there remains substantial uncertainty associated with the computational extrapolation of skin dose to organ dose, which can lead to over- or underestimation of the health risk. Comparisons of models to data showed that the astronaut's Effective dose (E) can be predicted to within about a +10% accuracy using space radiation transport models for galactic cosmic rays (GCR) and trapped radiation behind shielding. However for solar particle event (SPE) with steep energy spectra and for extra-vehicular activities on the surface of the moon where only tissue shielding is present, transport models predict that there are large differences in model assumptions in projecting organ doses. Therefore experimental verification of SPE induced organ doses may be crucial for the design of lunar missions. In the research experiment "Depth dose distribution study within a phantom torso" at the NASA Space Radiation Laboratory (NSRL) at BNL, Brookhaven, USA the large 1972 SPE spectrum was simulated using seven different proton energies from 50 up to 450 MeV. A phantom torso constructed of natural bones and realistic distributions of human tissue equivalent materials, which is comparable to the torso of the MATROSHKA phantom currently on the ISS, was equipped with a comprehensive set of thermoluminescence detectors and human cells. The detectors are applied to assess the depth dose distribution and radiation transport codes (e.g. GEANT4) are used to assess the radiation field and interactions of the radiation field with the phantom torso. Lymphocyte cells are strategically embedded at selected locations at the skin and internal organs and are processed after irradiation to assess the effects of shielding on the yield of chromosome damage. The initial focus of the present experiment is to correlate biological results with physical dosimetry measurements in the phantom torso. Further on, the results of the passive dosimetry within the anthropomorphic phantoms represent the best tool to generate reliable data to benchmark computational radiation transport models in a radiation field of interest. The presentation will give first results of the physical dose distribution, the comparison with GEANT4 computer simulations based on a Voxel model of the phantom, and a comparison with the data from the chromosome aberration study.

Berger, Thomas↗

Evaluation of neutron dosimetry capabilities with the MC-15 portable multiplicity counter

This work proposes a preliminary neutron dose rate estimation method for a neutron multiplicity detector through measurement- and simulation-based analyses. Uncharacterized neutron-emitting sources may be encountered in situations such as nuclear emergency response, safeguards, and treaty verification. These circumstances may present irradiation risk to personnel conducting field assay, search, and characterization measurements. It is therefore of interest to provide a field neutron dosimetry capability with the existing neutron multiplicity counting (NMC) capabilities. To date, no commercially-available neutron detection systems are capable of both accurate NMC and real-time neutron dosimetry. This work will focus on estimating dose rate using input from a single fielded NMC called the MC-15. The energy-dependent neutron detection efficiency response of the MC-15 was quantified in monoenergetic neutron simulations and evaluated in response to two neutron-emitting sources and to a polyethylene-moderated source. The results were compared to existing neutron dosimeters and established the proof of concept for further investigation of the MC-15 for dose estimation. Measurement results were also replicated in simulations; additional simulations were then conducted to expand upon the limited empirical data. The initial empirical results provided a conversion factor appropriate for use when measuring 252 Cf neutrons that is independent of polyethylene shielding presence and thickness. The simulated data sets were then used to evaluate a fit equation allowing estimation of the neutron dose rate for less restricted geometric configurations and dependent only on the distance between the source and the detector. Additionally, the energy dependence of the efficiency response indicates that further empirical evaluations could provide energy-dependent conversion factors for broader neutron dosimetry capabilities with a wider range of neutron-emitting sources.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Evaluation of radiation interference in the Voyager Sun Sensor's cadmium sulfide detector

The simulation of radiation interference effects and the results of a radiation interference test on two Voyager Sun Sensor prototype detector assemblies are reported. The derivation of test levels and requirements are discussed and show that cobalt 60 gamma radiation is an effective and practical simulator of the ionization dose rate effects induced by high-energy electron flux incident on the spacecraft at a rate of 3.7 x 10 to the 8th e/sq cm-sec (10 rad(Si)/s) during closest approach to Jupiter. The test results provide information that is used to confirm an analytic correlation, and to predict satisfactory performance of a spacecraft sun sensing device having stringent angular resolution requirements. The measured detector response shows that at dose rates incident on the detector elements of 2 rad(Si)/sec, which is four times that expected during Jupiter encounter, the radiation-induced angle error is almost an order of magnitude less than that allowed by the acceptance criteria.

Clarke, T. C.↗

Low-dose high-resolution $\mathrm{TOF}$-$\mathrm{PET}$ using ionization-activated multi-state low-$\mathrm{Z}$ detector media

We propose PET scanners using low atomic number media that undergo a persistent local change of state along the paths of the Compton recoil electrons. Measurement of the individual scattering locations and angles, deposited energies, and recoil electron directions allows using the kinematical constraints of the 2-body Compton scattering process to perform a statistical time-ordering of the scatterings, with a high probability of precisely identifying where the gamma first interacted in the detector. In these cases the Line-of-Response is measured with high resolution, determined by the underlying physics processes and not the detector segmentation. There are multiple such media that act through different mechanisms. As an example in which the change of state is quantum-mechanical through a change in molecular configuration, rather than thermodynamic, as in a bubble chamber, we present simulations of a two-state photoswitchable organic dye, a ‘Switchillator’, that is activated to a fluorescent-capable state by the ionization of the recoil electrons. The activated state is persistent, and can be optically excited multiple times to image individual activated molecules. Energy resolution is provided by counting the activated molecules. Location along the LOR is implemented by large-area time-of-flight MCP-PMT photodetectors with single photon time resolution in the tens of ps and sub-mm spatial resolution. Simulations indicate a large reduction of dose.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗