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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4

Measuring Electron Diffusion and Constraining the Neutral Current $\pi^0$ Background for Single-Photon Events in MicroBooNE

Liquid Argon Time Projection Chambers (LArTPCs) are a rising technology in the field of experimental neutrino physics. LArTPCs use ionization electrons and scintillation light to reconstruct neutrino interactions with exceptional calorimetric and position resolution capabilities. Here, I present two analyses conducted in the MicroBooNE LArTPC at Fermilab: a measurement of the longitudinal electron diffusion coefficient, $D_L$, in the MicroBooNE detector and a constraint of the systematic uncertainty on MicroBooNE's single-photon analysis due to the dominant neutral current (NC) \piz{} background. Longitudinal electron diffusion modifies the spatial and timing resolution of the detector, and measuring it will help correct for these effects. Furthermore, current measurements of $D_L$ in liquid argon are sparse and in tension with one another, making the MicroBooNE measurement especially valuable. We report a measurement of $3.74^{+0.28}_{-0.29}$ cm$^2$/s. MicroBooNE is searchin g for si ngle-photon events as a potential explanation for the MiniBooNE low-energy excess (LEE) of electron neutrino-like events, which has been interpreted as evidence for low-mass sterile neutrinos. However, this search is overwhelmed by a large NC \piz{} background. By performing a sideband selection of NC \piz{} events, we apply a data-driven rate constraint to the single-photon analysis to reduce the systematic uncertainties. At present, this constraint improves the single-photon analysis' median sensitivity to the LEE-like signal from 0.9$\sigma$ to $1.5\sigma$. This sensitivity is expected to improve significantly as more data become available. Both of these measurements will not only benefit MicroBooNE, but also inform future LArTPC experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Damage and recovery characteristics of lithium-containing solar cells.

Damage and recovery characteristics were measured on lithium-containing solar cells irradiated by 1-MeV electrons. Empirical expressions for cell recovery time, diffusion-length damage coefficient immediately after irradiation, and diffusion-length damage coefficient after recovery were derived using results of short-circuit current, diffusion-length, and reverse-bias capacitance measurements. The damage coefficients were expressed in terms of a single lithium density parameter, the lithium gradient. A fluence dependence was also established, this dependence being the same for both the immediate-post-irradiation and post-recovery cases. Cell recovery rates were found to increase linearly with lithium gradient.

Faith, T. J.↗

Operando Topography and Mechanical Property Mapping of CO 2 Reduction Gas-Diffusion Electrodes Operating at High Current Densities

Electrochemical atomic force microscopy (EC-AFM) enables measurement of electrode topography and mechanical properties during electrochemical reactions. However, for aqueous-based reactions that make gas products, such as CO 2 reduction and water splitting into CO/H 2 , current densities below 1 mA cm −2 have been necessary to prevent formation of bubbles at the electrode; such bubbles can stick to the AFM probe and prevent further AFM imaging. Here, we demonstrate a novel cell design with a gas-diffusion electrode (GDE) to exhaust the gas products, thereby enabling high current density EC-AFM measurements at 1, 10, and 100 mA cm −2 that are not disturbed by bubble formation at the electrode surface. These experiments revealed a stable morphological structure of Cu catalysts deposited on GDEs during high current density operation. Systematic spatially resolved maps of deformation and adhesion showed no signs of a gas-liquid interface between catalyst particles of the GDE.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Stormtime transport of ring current and radiation belt ions

A dynamical guiding-center simulation model is used to study the stormtime ion transport which leads to the formation of the ring current and diffusion in the radiation belts. Representative ions guiding-center motion in response to model storm-associated impulses in the convection electric field is traced for a range of ion mu values. The present numerical results are compared with previously formulated limiting idealization of particle transport in order to assess the limits of validity of these approximations. For ions having drift periods that exceed the duration of the main phase of the storm, their inward transport to form the stormtime ring current is appropriately described as direct convective access. For ions having drift periods comparable to the duration of the main phase of the storm, there is a transition between direct convective access and transport that resembles radial diffusion. Lower-energy ring-current ions at L of about 3 are freshly injected there from open adiabatic trajectories, whereas the higher-energy ring-current population consists of a mixture of freshly injected and previously trapped ions.

Chen, Margaret W.↗

Diffuse cloud chemistry

The current status of models of diffuse interstellar clouds is reviewed. A detailed comparison of recent gas-phase steady-state models shows that both the physical conditions and the molecular abundances in diffuse clouds are still not fully understood. Alternative mechanisms are discussed and observational tests which may discriminate between the various models are suggested. Recent developments regarding the velocity structure of diffuse clouds are mentioned. Similarities and differences between the chemistries in diffuse clouds and those in translucent and high latitude clouds are pointed out.

Van Dishoeck, Ewine F.↗

Limitations on solar cell open-circuit voltage and efficiency

Techniques used to determine the open-circuit voltage of solar cells are analyzed. It is noted that the computational procedures for determining the output characteristics of a solar cell depend on a thorough understanding of the behavior of individual components. However, amorphous materials and combination solar cells exhibit increasingly complex behaviors and theoretical analyses therefore are continually more dependent on experimental data for verification. Formulations are defined for the base region and for diffusion length measurement. Experimental results are cited to show that, for low resistivity, planar surface cells, the dark current from the emitter is the dominant factor limiting increases in the Voc, which can be enhanced by improving the efficiency of the doping levels and profile to minimize the effects of bandgap narrowing, junction recombination current, and diffusion length of the emitter region.

Meulenberg, A., Jr.↗

Simulation of magnetic field line stochasticity at the magnetopause

We have conducted a three-dimensional particle simulation to study the magnetic field line stochasticity at the magnetopause current layer. Our results show that the magnetic field lines become stochastic due to the overlap of the destabilized multiple tearing mode islands, which agrees with the percolation model suggested by Galeev et al. (1986). After the field lines become stochastic, these tearing modes grow even 2-3 times faster than in the linear stage and saturate at an amplitude level 3-4 times bigger than the single tearing mode without mode-mode coupling. The field line stochasticity also causes a strong particle diffusion across the current layer. The diffusion coefficient reaches to 10(exp 9) sq m/s for typical magnetopause parameters. Associated with the particle diffusion, the current layer becomes broader in width. As a result, the magnetic energy is dissipated into particle energy by heating parallel to the local magnetic field. The particle energy increases by 60%, while the magnetic helicity, which has always been regarded as a good invariant, changes by 20%.

Wang, Zhi↗

Ion Behaviors in the Reconnection Diffusion Region of a Corrugated Magnetotail Current Sheet

The current sheet structure and ion behaviors in a magnetotail reconnection diffusion regionare investigated. The multispacecraft analysis suggests a corrugated current sheet structure, interpretedas due to a apping motion that propagates along geocentric solar magnetospheric along the +y direction inthe Geocentric Solar Magnetospheric (GSM) coordinate. The electric eld (E) and ion distributions havesimilarities with those in a planar current sheet. Energetic ions move along the current direction, suggestingthe acceleration by the observed reconnection E during the meandering motion. Counterstreaming ionsalong the current sheet normal suggest the acceleration by the Hall E that is observed to be the dominantcomponent. However, at certain locations, E and counterstreaming ions signicantly deviate from the localnormal direction, and more than one pair of counterstreaming populations exist, possibly because thecorrugated current sheet enables ions entering the current sheet at different locations with differentvelocities to mix together

Wang, Shan↗

BRDF Calibration of Sintered PTFE in the SWIR

Satellite instruments operating in the reflective solar wavelength region often require accurate and precise determination of the Bidirectional Reflectance Distribution Function (BRDF) of laboratory-based diffusers used in their pre-flight calibrations and ground-based support of on-orbit remote sensing instruments. The Diffuser Calibration Facility at NASA's Goddard Space Flight Center is a secondary diffuser calibration standard after NEST for over two decades, providing numerous NASA projects with BRDF data in the UV, Visible and the NIR spectral regions. Currently the Diffuser Calibration Facility extended the covered spectral range from 900 nm up to 1.7 microns. The measurements were made using the existing scatterometer by replacing the Si photodiode based receiver with an InGaAs-based one. The BRDF data was recorded at normal incidence and scatter zenith angles from 10 to 60 deg. Tunable coherent light source was setup. Broadband light source application is under development. Gray-scale sintered PTFE samples were used at these first trials, illuminated with P and S polarized incident light. The results are discussed and compared to empirically generated BRDF data from simple model based on 8 deg directional/hemispherical measurements.

Georgiev, Georgi T.↗

Effect of eddy diffusivity on wind-driven currents in a two-layer stratified lake

The steady state wind-driven circulation was numerically calculated in a rectangular stratified lake. The lake is composed of two layers having uniform but unequal densities and eddy diffusivities. The position in thermocline and the three-dimensional velocities in both layers calculated using shallow lake equations. The results show that, as the eddy diffusivity in the hypolimnion is increased, the thermocline tilt and hypolimnetic velocities increase. The effect of the other variables such as wind stress, density, basin length, and mean thermocline depth are also shown.

Gedney, R. T.↗

Porosity Measurement in Laminated Composites by Thermography and FEA

This paper presents the correlation between the through-thickness thermal diffusivity and the porosity of composites. Finite element analysis (FEA) was used to determine the transient thermal response of composites that were subjected to laser heating. A series of finite element models were built and thermal responses for isotropic and orthographic materials with various thermal diffusivities subjected to different heating conditions were investigated. Experiments were conducted to verify the models and to estimate the unknown parameters such as the amount of heat flux. The analysis and experimental results show good correlation between thermal diffusivity and porosity in the composite materials. They also show that both laser and flash heating can be used effectively to obtain thermal diffusivity. The current infrared thermography system is developed for use with flash heating. The laser heating models and the FEA results can provide useful tools to develop practical thermal diffusivity measurement scheme using laser heat.

Chu, Tsuchin Philip↗

Structural Tuning of Self‐Conductive Polymer as Gas Diffusion Layer for Electrocatalytic Reactions at High Current

Electrocatalytic conversions offer a promising route for sustainable chemical production using renewable energy. Gas diffusion layers (GDLs) enable selective product formation at high current densities but suffer from electrolyte flooding, and polytetrafluoroethylene (PTFE)-based GDLs typically require metal conductive layers, which constrain catalyst development. A recently developed GDL configuration, electropolymerized poly(3,4-ethylenedioxythiophene) (PEDOT)-coated PTFE, demonstrates notable flooding resistance, but suffers from gas diffusion limitations at elevated currents due to limited gas diffusion through the PEDOT layer. Here, different dopants in PEDOT are exploited to modify the physical properties and enhance gas transport. ClO 4 − -doped PEDOT exhibits superior performance due to optimized physical structure, leading to increased gas permeance and faradaic efficiency (FE) for CO production during electrocatalytic CO 2 reduction. Further optimization of coverage and thickness achieved by adjusting charge density led to an optimal configuration at 33 mC cm −2 . This GDL supports various metal electrocatalysts and demonstrates FE CO of > 90% for over 150 h at −200 mA cm −2 using a commercial silver electrocatalyst. This work highlights the importance of GDL engineering in enhancing performance and durability for long-term electrocatalytic processes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

The Shuttle Orbiter high resolution accelerometer package experiment - Preliminary flight results

A description of the High Resolution Accelerometer Package (HiRAP) experiment, designed to measure rarefied flow aerodynamic accelerations, is given. The ground test calibration factors, as well as post-flight data processing techniques to extract aerodynamic accelerations, are discussed and applied to the recorded reentry data of the recent STS-6 Shuttle Orbiter flight. The ratio of the measured normal-to-axial aerodynamic accelerations during reentry is used to obtain the first flight measurement of the lift-to-drag ratio (L/D) of a winged entry vehicle in the rarefied flow flight regime. The preliminary result for the free-molecule flow L/D is 0.10 + or - 0.03. The initial flight results on L/D are compared with current predictions which are based upon theoretical and empirical considerations. The measured free-molecule flow L/D value is higher than predicted by a factor of about three, indicating that surface reflection is not completely diffuse as currently assumed. In the rarefied flow transition regime, the Shuttle data book-bridging formula fits the flight data adequately. Upper altitude density profiles are also deduced from the measurements and presented. The density profiles show a wave phenomena with amplitude of about 60 percent, relative to a standard model.

Blanchard, R. C.↗

Junction characteristics of silicon solar cells. Part 1: Nonilluminated case

Precise values of the reverse saturation currents in silicon solar cells and magnitudes of the diffusion and recombination components have been obtained. The recombination current as well as leakage current due to shunting are shown to be nonuniform across the cell. The diffusion lengths calculated from the diffusion current components agree well with diffusion lengths measured independently in similar material. Models are given demonstrating the effect of recombination and shunting currents on the dark current-voltage characteristics of solar cells.

Stirn, R. J.↗

The plasma wave environment of an auroral arc - Electrostatic ion cyclotron waves in the diffuse aurora

Electric field plasma wave observations were made with a sounding rocket payload in and near a quiet auroral arc. This payload was launched on March 9, 1978 from Poker Flat, Alaska. The payload trajectory was close to the magnetic meridian and passed over a 40 kR auroral arc. The present investigation is concerned with ac electric field observations in the ELF and lower VLF covering a frequency range from 2.5 Hz to 8 kHz. Attention is given to aspects of instrumentation, the general situation, a data analysis, and the obtained results. Waves were observed at low altitude in a region of downward parallel current and diffuse aurora. These waves had properties consistent with those expected for hydrogen and oxygen electrostatic ion cyclotron (EIC) waves.

Bering, E. A.↗

Carrier diffusion in long wavelength InGaN quantum well LEDs after injection through V-defects

The efficiency of operation of GaN-based light emitting diodes (LEDs) to a large degree relies on realization of a uniform hole distribution between multiple quantum wells (QWs) of the active region. Since the direct thermionic transport between the QWs is inefficient, the hole injection through semipolar {$10\bar{1}1$} QWs that form on the facets of V-defects has been suggested as an alternative approach. However, for an efficient LED operation, the carrier distribution should be uniform not only vertically, between the QWs but also laterally, within individual QWs. In this work, the lateral carrier distribution in long wavelength InGaN/GaN QW LEDs is studied by the scanning near-field optical microscopy. The measurements have shown that emission is concentrated around the V-defect injectors. At high currents, the diffusion length of holes in polar QWs was found to be ∼0.6–1 μm and the hole diffusion coefficient ∼0.6 cm 2 /s. The obtained data should aid design of the V-defect injectors for a laterally uniform carrier distribution in the active region QWs.

Current crowding↗

Interactions Between Climate and Species Drive Future Forest Carbon and Water Balances

Global change is altering forest carbon and water balances; however, the extent to which tree species shape ecosystem‐scale responses to climate, particularly in biodiverse forests, remains unclear. To address this, we simulated the effects of an envelope of future climate conditions on watershed carbon and water balances and quantified the contributions of tree species based on their xylem anatomy. We accomplished this by incorporating species‐level transpiration calculations into a landscape‐scale ecosystem process model. Our revised model linked the effects of forest succession, species composition, and climate change on water and carbon. Calibration of forest water fluxes using sap flux measurements and catchment water balances captured variability in species transpiration and interannual ET in biodiverse, humid temperate forest catchments in the southern Blue Ridge Mountains, USA. Across wet and dry future climate projections, ET increased, and streamflow and net carbon uptake decreased, particularly under a scenario of increasing drought. Despite accounting for just 30% of current biomass, diffuse‐porous tree species were the main driver of carbon and water flux responses now and in the future, thus intensifying the increase in ET and decline in streamflow. As diffuse‐porous biomass continues to increase, these forests will be increasingly sensitive to drought, amplifying losses of carbon sequestration and freshwater delivery.

54 ENVIRONMENTAL SCIENCES↗