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Assessing feasible H2–CO2 sources in the US as Feedstocks for Sustainable Aviation Fuel Precursors: Acetic Acid and Ethanol Production via Hydrogenotrophic Pathways
The environmental impact of carbon dioxide emissions is significant, and research is focused on mitigating these emissions and developing eco-friendly technologies in line with green chemistry principles. Waste-to-energy technologies play a crucial role in converting waste into renewable energy and valuable biofuels and bioproducts. This study specifically explores the utilization of waste gas emissions, particularly carbon dioxide, from various sources in the United States for the production of sustainable aviation fuel (SAF) precursors, such as ethanol and acetic acid. The study categorizes and quantifies the volumes of carbon dioxide emissions into three types: non-biogenic, biogenic, and biogenic emissions from ethanol production facilities. Stoichiometric calculations are applied to compare the amounts of carbon dioxide from each category with the available hydrogen production capacity, determining if sufficient hydrogen is present for converting carbon dioxide into SAF precursors. The study reveals two key findings. Firstly, there is a significant reserve of carbon dioxide, approximately 1648 million metric tons per year (MMTy), combining all three categories, which would require a substantial increase of approximately 35–40 times in the existing hydrogen production capacity of 4.988 MMTy. This increased hydrogen production has the potential to yield approximately 1067.82 MMTy of acetic acid and 189.19 MMTy of ethanol annually. Secondly, upon analyzing the quality and application of the three sources of carbon dioxide with the currently available hydrogen production capacity, it is found that biogenic carbon dioxide from ethanol plants is the most suitable choice for immediate production of SAF precursors. This would theoretically result in an annual production of 1.36 MMTy of ethanol and 1.772 MMTy of acetic acid. The other two sources of carbon dioxide can be considered potential reserves for future utilization when additional hydrogen production facilities are established. The study provides a foundation for assessing the aggregation potential required for acetic acid and ethanol production. By optimizing the use of waste gases as raw materials, the study not only enables the production of SAF precursors but also contributes to the passive reduction of greenhouse gas emissions.
The effective magnetic moments of Co2+ and Co3+ in SrTiO3 investigated by temperature-dependent magnetic susceptibility
Not provided.
A high throughput optical method for studying compositional effects in electrocatalysts for CO2 reduction
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Aqueous interphase formed by CO2 brings electrolytes back to salt-in-water regime
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Optimized Performance and Cost Potential for Indirect Supercritical CO2 Coal Fired Power Plants
This presentation given at the 2021 ASME Turbo Expo (GT2021-58865) summarizes the techno-economic global optimization results of coal-fired utility scale power plants based on indirect sCO2 power cycles with and without carbon capture and storage (CCS).
Impact of Plant Siting on Performance and Economics of Indirect Supercritical CO2 Coal Fired Power Plants
This study presents the impact of plant siting on the performance and economics of coal-fired utility scale power plants based on indirect sCO2 power cycles with carbon capture and storage (CCS). Presentation of paper made at the 2021 ASME Turbo Expo, GT2021-58867.
A Case Study of Risk Considerations for Transitioning CO2-EOR Field to Dedicated CO2-storage
Case study that summarizes the risk consideration for class II to class VI well transition. Presented (Virtual) at the Rock Fluid Dynamics (t-Navigator) Technology Summit 2024, May 10, 2024, Houston, TX.
Case Study of Risk Considerations for Transitioning a CO2-EOR Field to Dedicated CO2-storage
This is the poster for 2024 FECM / NETL Carbon Management Research Project Review Meeting. The poster the is the work we have done in NRAP Task 2 for Class II to Class VI Well Transition Case Study. Such study will be a continuously help to EPA for their guidance documentation.
Effect of the EMIM Cation on the CO2 Reduction Reaction on Gold: For CO2 Capture and Conversion Membranes
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A Geospatial Cost Comparison of CO2 Plume Geothermal (CPG) Power and Geologic CO2 Storage
CO 2 Plume Geothermal (CPG) power plants can use gigatonne-levels of CO 2 sequestration to generate electricity, but it is unknown if the resources that support low-cost CPG power align with the resources that support low-cost CO 2 sequestration. Here, we estimate and compare the geospatially-distributed cost of CPG and CO 2 storage across a portion of North America. We find that the locations with lowest-cost CO 2 storage are different than the locations with lowest-cost CPG. There are also locations with low-cost CO 2 storage (<$5/tCO 2 ) that do not support CPG power generation due to insufficient reservoir transmissivity or temperature. Thus, CPG development may require electricity prices that are greater than the levelized cost of electricity (LCOE) to offset the increased cost of sequestration. We introduce the “Additional Cost of Electricity (ACOE)” metric to account for this cost and add it to the LCOE to calculate breakeven electricity prices that are required for CPG development. We find that breakeven prices are lower when new CO 2 injection wells are drilled specifically for CPG (i.e., “greenfield” CPG development) compared to if only existing CO 2 sequestration injection wells are used (i.e., “brownfield” CPG development). This is because comparatively few wells are needed for sequestration-only, and the increased power capacity from having more CPG wells outweighs the increased costs from more drilling. We also find that sequestered CO 2 could be used to approximately triple the United States geothermal electricity power capacity via a single CPG “sweet spot” in South Dakota, but that breakeven electricity price for this development is on the order of $200/MW e h.
Theoretical screening and synthesizing sorbent materials for capturing CO2 and oxidizing CO to CO2
Proceedings of 12th Applied Energy Conference
Potential Oil Supply and CO2 Demand for CO2 Enhanced Oil Recovery in the United States
This presentation was given at the 2020 Pittsburgh Coal Conference on Sept 10, 2020. It describes an analysis using the FE/NETL CO<sub>2</sub> EOR Evaluation System in order to develop price curves for both oil supply as well as CO<sub>2</sub> demand resulting from potential application of CO<sub>2</sub> EOR. The analysis was conducted on a dataset of conventional oil reservoirs in the lower-48 states.
Comparative Analysis of CO2 Transport, Storage, and Produced Water Management Options from a CO2 Source Perspective
Presented by NETL at the 2021 AAPG-IMAGE Annual Conference and Exhibition
REX-CO2: Re-using Existing wells for CO2 storage operations
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Methods and systems for emissions control in solvent-based CO2 capture processes using CO2
A method with corresponding systems for reducing emission of amines to the atmosphere. The method includes a a) introducing a gas containing CO 2 into an absorber; b) flowing the flue gas through an absorber having an absorbent with a water-lean solution having less than 50% water and one or more amines, with the absorbent capturing the CO 2 and forming a reduced CO 2 content gas having a baseline CO 2 content; and c) washing the reduced CO 2 content gas in a wash column with a wash solution comprising carbonic acid formed by addition of gaseous CO 2 into the wash solution. In this method, the washing removes the amines from the reduced CO 2 content gas and produces a reduced amine content gas exiting from the wash column.