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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

One-pot rapid synthesis of high aspect ratio silver nanowires for transparent conductive electrodes

Highlights: • We improved a method of preparation of silver nanowires. • The effects of PVP molecular weight and concentration on the morphology and aspect ratio of AgNWs were investigated. • The preferred orientation growth mechanism of AgNWs was also discussed briefly. • We got transparent conductive films by spin-coating silver nanowires dispersion which is compared to ITO films. • The effects of silver nanowires density and heating time on the sheet resistance and transmittance were investigated. - Abstract: Silver nanowires (AgNWs) with high aspect ratio were rapidly one-pot synthesized by a polyol process in the presence of polyvinylpyrrolidone (PVP) as a stabilizer as well as the anisotropic agent, and the corresponding transparent conductive films were prepared by spin-coating method. The effects of PVP molecular weight and concentration on the morphology and aspect ratio of AgNWs were investigated in detail, and the optoelectrical properties of the transparent conductive films were briefly introduced. The presence of PVP induces the growth of silver directed to form high aspect-ratio nanowires by a high anisotropic mode. Appropriate PVP molecular weight and concentration allows the rapid synthesis of AgNWs with the diameter of about 78.2 nm, the length of 79.52 μm and the aspect ratio as high as 1009.2. The as-prepared AgNWs films possess a transmittance of 81.6% and a sheet resistance of 11.36 Ω/sq. The resultant AgNWs with high aspect ratio can be applied to prepare transparent conductive electrodes.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2019

Exploring the Effect of Aspect to Inform Future Earthcasts of Climate-Driven Changes in Weathering of Shale

Projections of future conditions within the critical zone—earthcasts—can be used to understand the potential effects of changes in climate on processes affecting landscapes. We are developing an approach to earthcast how weathering will change in the future using scenarios of climate change. As a first step here, we use the earthcasting approach to model aspect-related effects on soil water chemistry and weathering on hillsides in a well-studied east-west trending watershed (Shale Hills, Pennsylvania, USA). We completed model simulations of solute chemistry in soil water with and without the effect of aspect for comparison to catchment observations. With aspect included, aqueous weathering fluxes were higher on the sunny side of the catchment. But the effect of aspect on temperature (0.8 °C warmer soil on sunny side) and recharge (100 mm/year larger on shaded side) alone did not explain the magnitude of the observed higher weathering fluxes on the sunny side. We note modeled aspect-related differences in weathering fluxes only approach field observations when we incorporated the measured differences in clay content observed in augered soils on the two hillslopes. We also had to include a biolifting module to accurately describe cation concentrations in soil water versus depth. Biolifting lowered some mineral dissolution rates while accelerating kaolinite precipitation. These short-duration simulations also highlighted that the inherited differences in particle size on the two sides of the catchment might in themselves be explained by weathering under different microclimates caused by aspect—over longer durations than simulated with our models.

58 GEOSCIENCES↗
DOE OSTI2023

Effect of aspect ratio on plasma response to resonant magnetic perturbations in tokamak devices

A systematic numerical study is carried out, computing and comparing the plasma response to the resonant magnetic perturbation (RMP) field, applied for controlling edge localized modes (ELMs), in a series of tokamak plasmas with varying aspect ratio and utilizing the MARS-F code. The aspect ratio is scanned either by varying the plasma major radius at a fixed minor radius or by varying the latter while fixing the former. Both approaches yield similar results when compared in terms of quantities with proper normalizations. In general, a non-monotonic dependence of the resonant response field (normalized by the vacuum counterpart) near the plasma edge is found with varying aspect ratio, indicating that a given ELM control coil current configuration strongly favors plasmas with a certain aspect ratio. This optimal aspect ratio, on the other hand, depends on the toroidal as well as poloidal (i.e., coil phasing) spectra of the applied RMP field. The equilibrium (edge) safety factor, the plasma shape, and the plasma toroidal flow are all fixed to ensure that the effects identified here are predominantly due to the plasma aspect ratio.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1995

Algorithms for high aspect ratio oriented triangulations

Grid generation plays an integral part in the solution of computational fluid dynamics problems for aerodynamics applications. A major difficulty with standard structured grid generation, which produces quadrilateral (or hexahedral) elements with implicit connectivity, has been the requirement for a great deal of human intervention in developing grids around complex configurations. This has led to investigations into unstructured grids with explicit connectivities, which are primarily composed of triangular (or tetrahedral) elements, although other subdivisions of convex cells may be used. The existence of large gradients in the solution of aerodynamic problems may be exploited to reduce the computational effort by using high aspect ratio elements in high gradient regions. However, the heuristic approaches currently in use do not adequately address this need for high aspect ratio unstructured grids. High aspect ratio triangulations very often produce the large angles that are to be avoided. Point generation techniques based on contour or front generation are judged to be the most promising in terms of being able to handle complicated multiple body objects, with this technique lending itself well to adaptivity. The eventual goal encompasses several phases: first, a partitioning phase, in which the Voronoi diagram of a set of points and line segments (the input set) will be generated to partition the input domain; second, a contour generation phase in which body-conforming contours are used to subdivide the partition further as well as introduce the foundation for aspect ratio control, and; third, a Steiner triangulation phase in which points are added to the partition to enable triangulation while controlling angle bounds and aspect ratio. This provides a combination of the advancing front/contour techniques and refinement. By using a front, aspect ratio can be better controlled. By using refinement, bounds on angles can be maintained, while attempting to minimize the number of Steiner points.

Posenau, Mary-Anne K.↗
NASA NTRS1961

Aerodynamic Characteristics of Low-Aspect-Ratio Wings in Close Proximity to the Ground

A wind-tunnel investigation has been conducted to determine the effect of ground proximity on the aerodynamic characteristics of thick highly cambered rectangular wings with aspect ratios of 1. 2, 4, and 6. The results showed that, for these aspect ratios, as the ground war, approached all wings experienced increases in lift-curve slope and reductions in induced drag which resulted in increases in lift-drag ratio. Although an increase in lift-curve slope was obtained for all aspect ratios as the ground was approached, the lift coefficient at an angle of attack of 0 deg for any given aspect ratio remained nearly constant. The experimental results were in general agreement with Wieselsberger's ground-effect theory (NACA Technical Memorandum 77). As the wings approached the ground, there was an increase in static longitudinal stability at positive angles of attack. When operating in ground effect, all the wings had stability of height at positive angles of attack and instability of height at negative angles of attack. Wing-tip fairings on the wings with aspect ratios of 1 and 2 produced small increases in lift-drag ratio in ground effect. End plates extending only below the chord plane on the wing with an aspect ratio of 1 provided increases in lift coefficient and in lift-drag ratio in ground effect.

Fink, Marvin P.↗
NASA NTRS1947

Drag Measurements at Transonic Speeds of NACA 65-009 Airfoils Mounted on a Freely Falling Body to Determine the Effects of Sweepback and Aspect Ratio

Drag measurements at transonic speeds on rectangular airfoils and on airfoils swept back 450 are reported. These airfoils, which were mounted on cylindrical test bodies, are part of a series being tested in free drops from high altitude to determine the effect of variation of basic airfoil parameters on airfoil drag characteristics at transonic speeds. These rectangular and swept-back airfoils had the same span, airfoil section (NACA 65-009), and chord perpendicular to the leading edge. The tests were made to compare the drag of rectangular and sweptback airfoils at a higher aspect ratio than had been used in a similar comparison reported previously. The results showed that the drag of the swept-back airfoil was less than 0.15 that of the rectangular airfoil at a Mach number of 1.00 and less than 0.30 that of the rectangular airfoil at a Mach number of 1.17. A comparison of these swept-back airfoils with similar airfoils of lower aspect ratio previously tested by the same method indicated that in the investigated speed range reduction in aspect ratio results in increased drag. In the highest part of the investigated speed range, however, the drag coefficient of the high-aspect-ratio swept-back airfoils showed a tendency to approach that of the lower-aspect-ratio swept-back airfoils. A similar comparison for the rectangular airfoils showed that delay in the drag rise and a reduction in drag at supercritical speeds can be realIzed through reduction in aspect ratio. These results confirm those reported in NACA ACR No. L5J16.

Mathews, Charles W.↗
NASA NTRS2017

Cause and Cure - Deterioration in Accuracy of CFD Simulations With Use of High-Aspect-Ratio Triangular Tetrahedral Grids

Traditionally high-aspect ratio triangular/tetrahedral meshes are avoided by CFD re-searchers in the vicinity of a solid wall, as it is known to reduce the accuracy of gradient computations in those regions and also cause numerical instability. Although for certain complex geometries, the use of high-aspect ratio triangular/tetrahedral elements in the vicinity of a solid wall can be replaced by quadrilateral/prismatic elements, ability to use triangular/tetrahedral elements in such regions without any degradation in accuracy can be beneficial from a mesh generation point of view. The benefits also carry over to numerical frameworks such as the space-time conservation element and solution element (CESE), where triangular/tetrahedral elements are the mandatory building blocks. With the requirement of the CESE method in mind, a rigorous mathematical framework that clearly identities the reason behind the difficulties in use of such high-aspect ratio triangular/tetrahedral elements is presented here. As will be shown, it turns out that the degree of accuracy deterioration of gradient computation involving a triangular element is hinged on the value of its shape factor Gamma def = sq sin Alpha1 + sq sin Alpha2 + sq sin Alpha3, where Alpha1; Alpha2 and Alpha3 are the internal angles of the element. In fact, it is shown that the degree of accuracy deterioration increases monotonically as the value of Gamma decreases monotonically from its maximal value 9/4 (attained by an equilateral triangle only) to a value much less than 1 (associated with a highly obtuse triangle). By taking advantage of the fact that a high-aspect ratio triangle is not necessarily highly obtuse, and in fact it can have a shape factor whose value is close to the maximal value 9/4, a potential solution to avoid accuracy deterioration of gradient computation associated with a high-aspect ratio triangular grid is given. Also a brief discussion on the extension of the current mathematical framework to the tetrahedral-grid case along with some of the practical results of this extension is also provided. Furthermore, through the use of numerical simulations of practical viscous problems involving high-Reynolds number flows, the effectiveness of the gradient evaluation procedures within the CESE framework (that have their basis on the analysis presented here) to produce accurate and stable results on such high-aspect ratio meshes is also showcased.

CESE Method↗
DOE OSTI2023

System efficiency of packed bed TES with radial flow vs. axial flow – Influence of aspect ratio

Here, this paper compares the net system efficiency, including thermal efficiency and pressure drop effects, of radial versus axial flow packed beds for thermal energy storage. The traditional packed bed system is a cylindrical geometry where fluid flows axially from one end to another. However, issues of thermal stratification and high-pressure drop have led to recent studies on radial flow systems. One potential benefit is the reduced pressure drop in a radial flow system. This paper compares the performance of radial flow and axial flow systems at a range of aspect ratios (AR = H/D bed ) from 0.21 to 1.92 using a numerical model where the storage volume is held constant in all cases. When the radial flow bed is at a low aspect ratio (short/wide), the thermal front is improved but the pressure drop is high. At a high aspect ratio, the velocity is reduced in radial flow, leading to decreased pressure drop but an increased spreads in the thermal front that lowers thermal efficiency. The opposite trends are noted in axial flow. Thermal efficiencies of 83–91 % were noted for radial flow, while they ranged from 85 to 94 % in axial flow. Net efficiencies including pressure drop ranged from 74 to 82 % for radial flow and 80–87 % for axial flow. In both systems, a peak net efficiency was noted between the highest and lowest aspect ratio. While some aspect ratios with radial flow outperform axial flow from a net efficiency perspective, the results show that the highest net efficiency from axial flow is higher than that from radial flow. Overall, this paper highlights the importance of innovative TES designs and their potential to improve energy efficiency.

25 ENERGY STORAGE↗
DOE OSTI2016

Microwave synthesis and photocatalytic activities of ZnO bipods with different aspect ratios

Highlights: • We synthesized linked ZnO nanorods by a facile microwave method. • The effect of reaction parameters on ZnO was investigated. • ZnO bipods with different aspect ratios were prepared. • The photocatalytic performance of ZnO bipods was evaluated. - Abstract: Linked ZnO nanorods have been successfully prepared via a facile microwave method without any post-synthesis treatment. The X-ray diffraction (XRD) patterns indicated the precursor had completely transformed into the pure ZnO crystal. The images of field emitting scanning electron microscope (FESEM) and transmission electron microscope (TEM) showed that linked ZnO nanorods consisted predominantly of ZnO bipods. The formation process of the ZnO bipods was clearly discussed. ZnO bipods with different aspect ratios have been obtained by tuning the concentrations of reagents and microwave power. Moreover, the photocatalytic performance of ZnO bipods with different aspect ratios for degradation of methylene blue was systematically evaluated. The results of photocatalytic experiments showed that the photocatalytic activity increased with the aspect ratios of ZnO bipods increased. The reason is that ZnO bipods with larger aspect ratio have higher surface area, which can absorb more MB molecules to react with ·OH radicals.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Aspect ratio control and photocatalytic properties analysis of anatase TiO2 nanoparticles

Highlights: • TiO{sub 2} nanoparticles with different aspect ratio were prepared and characterized. • Their aspect ratio is tuned by varying surfactants molar ratio and concentration. • TiO{sub 2} nanoparticles show photocatalytic activities in degradation of methylene blue. - Abstract: Anatase TiO{sub 2} nanoparticles with tuning size and aspect ratio were successfully prepared by a simple solvothermal method, using ethanol as a solvent, titanium butoxide as a precursor, and oleic acid and oleylamine as anionic and cationic capping agents, respectively. The average size and aspect ratio of these nanoparticles can be greatly regulated by varying the oleic acid/oleylamine molar ratio while keeping their total molar content constant and finely adjusted by increasing the total capping agents molar concentration in solvent at constant molar ratio (oleic acid/oleylamine molar ratio = 1:1). The variation of molar ratio or molar concentration enables a manipulation of the growth rate along different facets of TiO{sub 2} nanoparticles and, consequently, a control of the aspect ratio of these nanoparticles. Moreover, the photocatalytic degradation rate of methyl blue for sample prepared with molar ratio of oleic acid to oleylamine at 6:24 is over 11% higher than that for the other samples.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
NASA NTRS1949

Investigation at low speeds of the effect of aspect ratio and sweep on rolling stability derivatives of untapered wings

A low scale wind tunnel investigation was conducted in rolling flow to determine the effects of aspect ratio and sweep (when varied independently) on the rolling stability derivatives for a series of untapered wings. Test results indicate that when the aspect ratio was held constant, an increase in the sweepback angle caused a significant reduction in the damping in roll at low lift coefficients for only the higher aspect ratios that were tested. This result was in agreement with available swept wing theory which indicated no effect of sweep for aspect ratios near zero. The result of the linear theory that the damping in roll is independent of lift coefficient and that the yawing moment and lateral force due to rolling are directly proportional to the lift coefficient was found to be valid for only a very limited lift coefficient range when the wings were highly swept. For such wings, the damping was found to increase in magnitude and the yawing moment due to rolling, to change from negative to positive at moderate lift coefficients. The effect of wing tip suction, not acounted for by present theory, was found to be very important with regard to the yawing moment due to rolling, particularly for low aspect ratio swept wings. An empirical means of correcting present theory for the effect of tip suction is suggested.

Goodman, Alex↗
NASA NTRS1947

Calculations of the Supersonic Wave Drag of Nonlifting Wings with Arbitrary Sweepback and Aspect Ratio: Wings Swept Behind the Mach Lines

On the basis of a recently developed theory for finite sweptback wings at supersonic speeds, calculations of the supersonic wave drag at zero lift were made for a series of wings having thin symmetrical biconvex sections with untapered plan forms and various angles of sweepback and aspect ratios. The results are presented in a unified form so that a single chart permits the direct determination of the wave drag for this family of airfoils for an extensive range of aspect ratio and sweepback angle for stream Mach numbers up to a value corresponding to that at which the Mach line coincides with the wing leading edge. The calculations showed that in general the wave-drag coefficient decreased with increasing sweepback. At Mach numbers for which the Mach lines are appreciably ahead of the wing leading edge, the 'wave-drag coefficient decreased to an important extent with increases in aspect ratio or slenderness ratio. At Mach numbers for which the Mach lines approach the wing leading edge (Mach numbers approaching a value equal to the secant of the angle of sweepback), the wave-drag coefficient decreased with reductions in aspect ratio or slenderness ratio. In order to check the results obtained by the theory, a comparison was made with the results of tests at the Langley Memorial Aeronautical Laboratory of sweptback wing attached to a freely falling body. The variation of the drag with Mach number and aspect ratio as given by the theory appeared to be in reasonable

Harmon, Sidney M↗
NASA NTRS1997

Comparison of High Aspect Ratio Cooling Channel Designs for a Rocket Combustion Chamber

An analytical investigation on the effect of high aspect ratio (height/width) cooling channels, considering different coolant channel designs, on hot-gas-side wall temperature and coolant pressure drop for a liquid hydrogen cooled rocket combustion chamber, was performed. Coolant channel design elements considered were: length of combustion chamber in which high aspect ratio cooling was applied, number of coolant channels, and coolant channel shape. Seven coolant channel designs were investigated using a coupling of the Rocket Thermal Evaluation code and the Two-Dimensional Kinetics code. Initially, each coolant channel design was developed, without consideration for fabrication, to reduce the hot-gas-side wall temperature from a given conventional cooling channel baseline. These designs produced hot-gas-side wall temperature reductions up to 22 percent, with coolant pressure drop increases as low as 7.5 percent from the baseline. Fabrication constraints for milled channels were applied to the seven designs. These produced hot-gas-side wall temperature reductions of up to 20 percent, with coolant pressure drop increases as low as 2 percent. Using high aspect ratio cooling channels for the entire length of the combustion chamber had no additional benefit on hot-gas-side wall temperature over using high aspect ratio cooling channels only in the throat region, but increased coolant pressure drop 33 percent. Independent of coolant channel shape, high aspect ratio cooling was able to reduce the hot-gas-side wall temperature by at least 8 percent, with as low as a 2 percent increase in coolant pressure drop. The design with the highest overall benefit to hot-gas-side wall temperature and minimal coolant pressure drop cooling can now be done in relatively short periods of time with multiple iterations.

Wadel, Mary F.↗
NASA NTRS1959

Effect of Stator and Rotor Aspect Ratio on Transonic-Turbine Performance

The effect of stator and rotor aspect ratio on transonic-turbine performance was experimentally investigated. The stator aspect ratios covered were 1.6. 0.8, and 0.4, while the rotor aspect ratios investigated were 1.46 and 0.73. It was found that the observed variation in turbine design-point efficiency was negligible. Thus, within the range of aspect ratio investigated, these results verify for turbines operating in the transonic flow range the finding of a reference report, which showed analytically that, if blade shape and solidity are held constant, the aspect ratio may be varied over a wide range without appreciable change in turbine efficiency.

Wong, Robert Y.↗
NASA NTRS2003

Aeroacoustics of a High Aspect-Ratio Jet

Circulation control wings are a type of pneumatic high-lift device that have been extensively researched as to their aerodynamic benefits. However, there has been little research into the possible airframe noise reduction benefits of a circulation control wing. The key element of noise is the jet noise associated with the jet sheet emitted from the blowing slot. This jet sheet is essentially a high aspect-ratio rectangular jet. Thus, to fully understand the noise of a circulation control wing, the noise of high aspect-ratio rectangular jets must also be understood. A high aspect-ratio nozzle was fabricated to study the general characteristics of high aspect-ratio jets with aspect ratios from 100 to 3000. The jet noise of this nozzle was proportional to the 8" power of the jet velocity. It was also found that the jet noise was proportional to the slot height to the 312 power and slot width to the 1/2 power.

Munro, Scott E.↗
DOE OSTI2015

Effects of aspect ratio and concentration on rheology of epoxy suspensions containing model plate-like nanoparticles

Hexagonal 2-dimensional α-zirconium phosphate crystals were prepared with lateral diameters ranging from 110 nm to 1.5 μm to investigate the effect of particle size on suspension rheology. The nanoplatelets were exfoliated to individual sheets with monodisperse thickness and dispersed in a Newtonian epoxy fluid. The steady shear response of dilute and semi-dilute suspensions was measured and compared to expressions obtained from theory for infinitely dilute suspensions. For suspensions containing the smaller nanoplatelets, aspect ratio ∼160, the low shear rate viscosity and transition to shear thinning behavior were well described by theory for loadings up to 0.5 vol. %. The agreement was improved by assuming a moderate polydispersity in lateral diameter, ∼30%–50%, which is consistent with experimental observation. For the higher aspect ratio nanoplatelets, good agreement between theory and experiment was observed only at high shear rates. At lower shear rate, theory consistently over-predicted viscosity, which was attributed to a progressive shift to non-isotropic initial conditions with increasing particle size. The results suggest that at a fixed Peclet number, there is an increasing tendency for the nanoplatelets to form transient, local stacks as particle size increases. The largest particles, aspect ratio ∼2200, showed unusual shear thinning and thickening behaviors that were attributed to particle flexibility. The findings demonstrate the surprising utility of theory for infinitely dilute suspensions to interpret, and in some cases quantitatively describe, the non-Newtonian viscosity of real suspensions containing high aspect ratio plate-like particles. A simple framework is proposed to interpret deviations from ideal behavior based on the local and collective behavior of the suspended nanoplatelets.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Synthesis of high aspect ratio ZnO nanowires with an inexpensive handcrafted electrochemical setup

In this work, high aspect ratio zinc oxide nanowires are synthesized using templated one-step electrodeposition technique. Electrodeposition of the nanowires is done using a handcrafted electronic system. Nuclear track-etched polycarbonate membrane is used as a template to form the high aspect ratio nanowires. The result of X-ray diffraction and scanning electron microscopy shows that nanowires with a good crystallinity and an aspect ratio of more than 30 can be achieved in a suitable condition. The height of electrodeposited nanowires reaches to about 11 μm. Based on the obtained results, high aspect ratio ZnO nanowires can be formed using inexpensive electrodeposition setup with an acceptable quality.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Addressing social aspects associated with wastewater treatment facilities

In wastewater treatment facilities (WWTF), technical and financial aspects have been considered a priority, while other issues, such as social aspects, have not been evaluated seriously and there is not an accepted methodology for assessing it. In this work, a methodology focused on social concerns related to WWTF is presented. The methodology proposes the use of 25 indicators as a framework for measuring social performance to evaluate the progress in moving towards sustainability. The methodology was applied to test its applicability and effectiveness in two WWTF in Mexico (urban and rural). This evaluation helped define the key elements, stakeholders and barriers in the facilities. In this context, the urban facility showed a better overall performance, a result that may be explained mainly by the better socioeconomic context of the urban municipality. Finally, the evaluation of social aspects using the semi-qualitative approach proposed in this work allows for a comparison between different facilities and for the identification of strengths and weakness, and it provides an alternative tool for achieving and improving wastewater management. - Highlights: • The methodology proposes 25 indicators as a framework for measuring social performance in wastewater treatment facilities. • The evaluation helped to define the key elements, stakeholders and barriers in the wastewater treatment facilities. • The evaluation of social aspects allows the identification of strengths and weakness for improving wastewater management. • It provides a social profile of the facility that highlights the best and worst performances.

54 ENVIRONMENTAL SCIENCES↗