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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Influence of neutrino-electron scattering and neutrino-pair annihilation on hypermassive neutron star

Here, we investigate the influence of inelastic neutrino microphysics in general-relativistic magnetohydrodynamics simulations of a hypermassive neutron star. In particular, we include species/energy groups coupled neutrino-matter interactions, such as inelastic neutrino-electron scattering and electron-positron annihilation kernels, into simulations up to 50 ms. Neutrino-electron inelastic scattering is known to have effective neutrino-matter energy exchange. We show that, with neutrino-electron inelastic scattering, simulations predict 75% higher disc mass with slightly different mass-averaged compositions, and 18% more ejected mass with similar distributions. The enhancement of the mass of the disc and the ejecta results in stronger baryon pollution, leading to less favorable jet launching environments. Furthermore, neutrino luminosities are about 50%, 40%, and 30% higher for electron neutrino, electron antineutrino, and heavy-lepton neutrinos. In contrast, we do not see any significant impacts due to electron-positron annihilation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Signatures of Weyl Fermion Annihilation in a Correlated Kagome Magnet

The manipulation of topological states in quantum matter is an essential pursuit of fundamental physics and next-generation quantum technology. Here we report the magnetic manipulation of Weyl fermions in the kagome spin-orbit semimetal Co 3 Sn 2 S 2 , observed by high-resolution photoemission spectroscopy. We demonstrate the exchange collapse of spin-orbit-gapped ferromagnetic Weyl loops into paramagnetic Dirac loops under suppression of the magnetic order. We further observe that topological Fermi arcs disappear in the paramagnetic phase, suggesting the annihilation of exchange-split Weyl points. In conclusion, our findings indicate that magnetic exchange collapse naturally drives Weyl fermion annihilation, opening new opportunities for engineering topology under correlated order parameters.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Observation of the W -Annihilation Process D s + → ω ρ + and Measurement of D s + → ϕ ρ + in D s + → π + π + π − π 0 π 0 Decays

We present the first amplitude analysis and branching fraction measurement of the decay D s + → π + π + π − π 0 π 0 , using e + e − collision data collected with the BESIII detector at center-of-mass energies between 4.128 and 4.226 GeV corresponding to an integrated luminosity of 7.33 fb − 1 , and report the first observation of the pure W -annihilation decay D s + → ω ρ + with a branching fraction of ( 0.99 ± 0.0 8 stat − 0.07 + 0.05 syst ) % . In comparison to the low significance of the D wave in the decay D s + → ϕ ρ + , the dominance of the D wave over the S and P waves, with a fraction of ( 51.85 ± 7.2 8 stat − 7.90 + 4.83 syst ) % observed in the decay D s + → ω ρ + , provides crucial information for the “polarization puzzle,” as well as for the understanding of charm meson decays. The branching fraction of D s + → π + π + π − π 0 π 0 is measured to be ( 4.41 ± 0.1 5 stat ± 0.1 3 syst ) % . Moreover, the branching fraction of D s + → ϕ ρ + is measured to be ( 3.98 ± 0.3 3 stat − 0.19 + 0.21 syst ) % , and the R ϕ = B ( ϕ → π + π − π 0 ) / B ( ϕ → K + K − ) is determined to be ( 0.222 ± 0.01 9 stat − 0.016 + 0.016 syst ), which is consistent with the previous measurement based on charm meson decays, but deviates from the results from e + e − annihilation and K − N scattering experiments by more than 3 σ . Published by the American Physical Society 2025

Ablikim, M.↗
DOE OSTI2025

Novel experimental probes of QCD in SIDIS and e + e - annihilation (Final Technical Report)

The research addressed with this award seeks to advance our understanding of the structure and dynamics underlying the properties of visible matter. In our current understanding the nucleons (protons and neutrons) are not fundamental but are comprised of quarks and gluons, which are collectively called partons. A static quark picture fails to explain the properties of the nucleons, such as their mass and intrinsic spin, which are thought to emerge dynamically from the quark-gluon interactions via the strong force. In this work, novel observables employing correlations of particles produced in the scattering of high energy electrons off protons at the CLAS12 experiment at Jefferson Lab were analyzed to probe quark-gluon interactions. The ultimate goal of this line of inquiry is to be able to describe the properties of protons and neutrons from first principles, similar to how studying the hydrogen atom has led to the formulation of the theory of Quantum Electrodynamics. Because quarks cannot be observed directly but only as part of more complex composite particles, a smaller, complimentary part of this work was the analysis of particle production in electron-positron annihilation at the Belle II experiment to understand the production of particles from initial quarks. This takes advantage of the fact that in e + e - annihilation the initial quark dynamics is known, unlike in the scattering of nucleons. Several new applications using Machine Learning algorithms for event tagging and reconstruction to support this program were developed as part of this award. In addition, we had a significant role in the development of the physics program for the future Electron-Ion Collider, which is a new collider to be build in the US within the next decade.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Harnessing the Population Statistics of Subhalos to Search for Annihilating Dark Matter

The Milky Way's dark matter halo is expected to host numerous low-mass subhalos with no detectable associated stellar component. Such subhalos are invisible unless their dark matter annihilates to visible states such as photons. One of the established methods for identifying candidate subhalos is to search for individual unassociated gamma-ray sources with properties consistent with the dark matter expectation. However, robustly ruling out an astrophysical origin for any such candidate is challenging. In this work, we present a complementary approach that harnesses information about the entire population of subhalos—such as their spatial and mass distribution in the Galaxy—to search for a signal of annihilating dark matter. Using simulated data, we show that the collective emission from subhalos can imprint itself in a unique way on the statistics of observed photons, even when individual subhalos may be too dim to be resolved on their own. Additionally, we demonstrate that, for the models we consider, the signal can be identified even in the face of unresolved astrophysical point-source emission of extragalactic and Galactic origin. Furthermore, this establishes a new search technique for subhalos that is complementary to established methods, and that could have important ramifications for gamma-ray dark matter searches using observatories such as the Fermi Large Area Telescope and the Cerenkov Telescope Array.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Current and Future γ-Ray Searches for Dark Matter Annihilation Beyond the Unitarity Limit

For decades, searches for electroweak-scale dark matter (DM) have been performed without a definitive detection. This lack of success may hint that DM searches have focused on the wrong mass range. A proposed candidate beyond the canonical parameter space is ultraheavy DM (UHDM). In this work, we consider indirect UHDM annihilation searches for masses between 30 TeV and 30 PeV—extending well beyond the unitarity limit at ~100 TeV—and discuss the basic requirements for DM models in this regime. We explore the feasibility of detecting the annihilation signature, and the expected reach for UHDM with current and future very-high-energy (VHE; >100 GeV) γ-ray observatories. Specifically, we focus on three reference instruments: two Imaging Atmospheric Cherenkov Telescope arrays, modeled on VERITAS and CTA-North, and one extended air shower array, motivated by HAWC. With reasonable assumptions on the instrument response functions and background rate, we find a set of UHDM parameters (mass and cross section) for which a γ-ray signature can be detected by the aforementioned observatories. Here, we further compute the expected upper limits for each experiment. With realistic exposure times, the three instruments can probe DM across a wide mass range. At the lower end, it can still have a point-like cross section, while at higher masses the DM could have a geometric cross section, indicative of compositeness.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Evaluation of adsorption and mechanical strength of 13X zeolite mixtures with phyllosilicate binders using molecular dynamics simulation and positron annihilation spectroscopy

There is growing interest in developing zeolites with novel internal structures that have optimal adsorptive capacity and high mechanical strength, while offering advantages, such as being light weight. We integrate computational and experimental methods to explore the effect of binder/zeolite types, and weight percentages on the mechanical strength of 13X zeolite and adsorption capacities of N 2 , H 2 O, and CO 2 for additive manufacturing (AM) applications with the goal of maximizing both adsorption and strength. Zeolite 13X mixtures and phyllosilicate binders (either bentonite or kaolin) are combined using molecular dynamics (MD) simulations to create structures with various binder/zeolite weight percentages. Further, adsorption capabilities and mechanical strength are assessed using the grand canonical Monte Carlo (GCMC) and ReaxFF modules, respectively. Our modeling shows that an optimized zeolite/binder ratio for N 2 adsorption is around 15 wt% for kaolin and roughly 10 wt% for bentonite. The resulting parameters can be applied to facilitate macro-scale computational fluid dynamics (CFD) and finite element method (FEM) simulations of an AM zeolite structure. We also performed Positron Annihilation Lifetime Spectroscopy (PALS) measurements on zeolite samples to explore the effect of changes in the internal volume. The results show an inverse relationship between the free volume and the solid loading and adding a binder changes the morphology of the zeolite-binder compound and decreases open-volume area significantly.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Visible-Light-Initiated Free-Radical Polymerization by Homomolecular Triplet-Triplet Annihilation

Polymerization reactions initiated by ultraviolet light are ubiquitous in scores of industrial applications but would markedly benefit from visible-light activation to overcome stability, energy consumption, light penetration, and sample geometry limitations. The current work leverages visible-light-driven homomolecular triplet-triplet annihilation (TTA) in zinc(II) meso-tetraphenylporphyrin (ZnTPP) to initiate facile free-radical polymerization in trimethylolpropane triacrylate (TMPTA) and methyl acrylate (MA) monomers through ultrafast electron transfer quenching. Selective Q-band (S 1 ) excitation of ZnTPP in the green or yellow sensitizes TTA occurring between two 3 ZnTPP* energized chromophores, ultimately generating the highly reducing S 2 excited state on one ZnTPP molecule (E red = –2.13 V versus saturated calomel electrode, SCE). Subsequently, this S 2 state engages in electron transfer with TMPTA or MA, thereby initiating the radical polymerization process. Bimolecular electron transfer was confirmed through optically gated fluorescence upconversion. In conclusion, FT-IR and EPR spin-trapping experiments verified visible-light-initiated polymerization leading to the formation of well-defined macro- and microscopic objects.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Enhanced defect annihilation capability of the graphene/copper interface: An in situ study

It is well known that energetic heavy ion irradiations can often induce defects and ultimately lead to material degradations. Interfaces, such as high-angle grain boundaries (HAGBs), are generally used as defect sinks for alleviating the irradiation damage. However, HAGBs are often unstable during radiation. Here we investigate the interfacial irradiation responses of the graphene (Gr)/Cu composites by using in situ Kr ++ ions irradiation under transmission electron microscopy. The results revealed that the Gr/Cu interface exhibits higher defect annihilation capability compared to the HAGBs in Cu. Moreover, the atomistic simulations suggested a slightly higher and larger range of stress field for the Gr/Cu interface, which contributes to the enhanced defects absorption capability. The present findings are essential to understand and design a new class of carbon/metal composites with superior irradiation tolerance.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Hydrated doped-BaZrO 3 proton conductors studied by positron annihilation lifetime spectroscopy

The study of defect chemistry for doped BaZrO 3 proton conductors is of particular interest because of defect interactions that can affect the proton conductivity of the material. Protons incorporated due to the material's hydration can be trapped by negatively charged immobile dopants, reducing proton mobility. The reduction of the proton conduction impedes using BaZrO 3 materials in energy conversion applications at intermediate temperatures (300°C – 600°C). The probing of proton trapping in doped BaZrO 3 is hindered by the limited availability of techniques sensitive to defect chemistries. In this work, we used positron annihilation lifetime spectroscopy (PALS) to study the defect chemistry of Y-doped and Sc-doped BaZrO 3 . Using a two-state positron trapping model we showed that PALS can be used to study the defect chemistry of hydrated dense proton conductors. Positron trapping rates and lifetimes were correlated with doping levels of the materials. Probability significance t-tests were carried out for PALS parameters to verify whether there are differences/similarities for various populations: non-doped/doped, level and type of doping, high temperature, and surface effects. Further, the results revealed that the initial doping generates a significant number of traps available for positrons. Doping in yttrium increased the positron trapping rate, while this effect was not observed with scandium. Low-temperature hydration affects specimens significantly inhibiting positron trapping at undoped BaZrO 3 material and highly doped specimens. Positronium formation in rough surface layers, and highly doped specimens was detected but does not exceed 1%.

36 MATERIALS SCIENCE↗
DOE OSTI2022

An intermediate model for fitting triplet–triplet annihilation in phosphorescent organic light emitting diode materials

Triplet–triplet annihilation (TTA) is one of the primary contributors to efficiency roll-off and permanent material degradation in phosphorescent organic light-emitting diodes. Here, the two limiting case models typically used to quantify this quenching mechanism are multi-step Dexter and single-step Förster, which, respectively, assume ideal Fickian diffusion or perfect trapping of triplet excitons. For device-relevant guest doping levels (typically 5–12 vol. %), both significant diffusion of excitons and trapping due to spatial and energetic disorder exist, so neither conventional model fits experimental data well. We develop and validate an intermediate TTA model, which is a weighted average of the limiting cases of pure radiative decay (no TTA) and multi-step Dexter based TTA that returns an effective TTA rate constant and a parameter quantifying the portion of well-isolated excitons. Kinetic Monte-Carlo simulations and time-resolved photoluminescence measurements of an archetype host–guest system demonstrate that our intermediate model provides significantly improved fits with more realistic physical values, is more robust to variations in experimental conditions, and provides an analysis framework for the effects of trapping on TTA.

30 DIRECT ENERGY CONVERSION↗
DOE OSTI2024

Zeolite‐Based Catalysts for Conversion of Oxygenated Polymer Waste by Positron Annihilation

Positron Annihilation Lifetime Spectroscopy (PALS) has been employed to investigate the catalysts HZSM-5 and MESO−Y, which play a pivotal role in catalyzing and upgrading plastics, with a primary focus on oxygenated polymers, thereby transforming existing plastic materials into simpler, higher-quality value-added products. Here, in this study, PALS was systematically compared with other complementary analytical techniques. The research outcomes have successfully demonstrated the efficacy of PALS in elucidating the morphology and topology of zeolites at micro/meso-meter scales. The first experiment focuses on H-ZSM-5 zeolite subjected to treatments involving polyurethane and polypropylene. The second experiment delves into H-ZSM-5 zeolites with varying Si/Al ratios, both before and after conversion. The third experiment investigates Y zeolites that are surfactant templated to induce meso-porosity, examining their fresh state as well as their post-conversion condition. The PALS analysis was supplemented by BET (Brunauer-Emmett-Teller) analysis and NMR (Nuclear Magnetic Resonance) spectroscopies. Notably, PALS exhibits superior sensitivity, at the sub-nanometer scale, suggesting its potential as a preferred complementary method for catalysis studies. In conclusion, the integration of PALS into the repertoire of analytical tools enhances our understanding of catalyst behavior and catalytic processes, offering valuable insights for the advancement of plastic recycling and catalysis research.

32 - ENERGY CONSERVATION, CONSUMPTION, AND UTILIZA↗
DOE OSTI2024

The quintuplet annihilation spectrum

Abstract We extend the Effective Field Theory of Heavy Dark Matter to arbitrary odd representations of SU(2) and incorporate the effects of bound states. This formalism is then deployed to compute the gamma-ray spectrum for a5of SU(2): quintuplet dark matter. Except at isolated values of the quintuplet mass, the bound state contribution to hard photons with energy near the dark-matter mass is at the level of a few percent compared to that from direct annihilation. Further, compared to smaller representations, such as the triplet wino, the quintuplet can exhibit a strong variation in the shape of the spectrum as a function of mass. Using our results, we forecast the fate of the thermal quintuplet, which has a mass of ~13.6 TeV. We find that existing H.E.S.S. data should be able to significantly test the scenario, however, the final word on this canonical model of minimal dark matter will likely be left to the Cherenkov Telescope Array (CTA).

Physics↗
DOE OSTI2024

Annihilation of electroweak dumbbells

We study the annihilation of electroweak dumbbells and the dependence of their dynamics on initial dumbbell length and twist. Untwisted dumbbells decay rapidly while maximally twisted dumbbells collapse to form a compact sphaleron-like object, before decaying into radiation. The decay products of a dumbbell include electromagnetic magnetic fields with energy that is a few percent of the initial energy. The magnetic field from the decay of twisted dumbbells carries magnetic helicity with magnitude that depends on the twist, and handedness that depends on the decay pathway.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

Topological freeze-out by semi-annihilation

We point out that a QCD-like dark sector can be coupled to the Standard Model by gauging the topological Skyrme current, which measures the dark baryon number in the infrared, to give a technically natural model for dark matter. This coupling allows for a semi-annihilation process χχ → χX μ , where X μ is the gauge boson mediator and χ a dark pion field, which plays the dominant role in setting the dark matter relic abundance. The topological interaction is purely p-wave and so free from indirect detection constraints. We show that the dark matter pion mass needs to be in the range 10 MeV ≲ m χ ≲ 1 TeV; towards the lighter end of this range, there can moreover be significant self-interactions. We discuss prospects for probing this scenario at collider experiments, ranging from the LHC to low-energy e + e − colliders, future Higgs factories, and beam-dump experiments.

Models for Dark Matter↗
DOE OSTI2023

Pileup and Infrared Radiation Annihilation (PIRANHA): a paradigm for continuous jet grooming

Jet grooming is an important strategy for analyzing relativistic particle collisions in the presence of contaminating radiation. Most jet grooming techniques introduce hard cutoffs to remove soft radiation, leading to discontinuous behavior and associated experimental and theoretical challenges. In this paper, we introduce Pileup and Infrared Radiation Annihilation (Piranha), a paradigm for continuous jet grooming that overcomes the discontinuity and infrared sensitivity of hard-cutoff grooming procedures. We motivate Piranha from the perspective of optimal transport and the Energy Mover’s Distance and review Apollonius Subtraction and Iterated Voronoi Subtraction as examples of Piranha-style grooming. We then introduce a new tree-based implementation of Piranha, Recursive Subtraction, with reduced computational costs. Finally, we demonstrate the performance of Recursive Subtraction in mitigating sensitivity to soft distortions from hadronization and detector effects, and additive contamination from pileup and the underlying event.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Positron annihilation spectroscopy of defects in nuclear and irradiated materials- a review

Positron is the only probe that can detect individual atomic vacancies and small and large vacancy clusters induced by irradiation with remarkable sensitivity, providing information about their size, concentration, and chemical environment. The focus of this review article is to provide guidance to facilitate applications of positron annihilation spectroscopy (PAS) in irradiation-induced defect studies to advance the development of new radiation-tolerant materials. The principle of PAS, its techniques, and data analysis methods are described. PAS studies of defects in nuclear and irradiated materials are reviewed and discussed in depth. Future developments to advance PAS applications in nuclear materials research and studies of materials under extreme environments are presented.

Atomic scale defects↗
DOE OSTI2021

Defect annihilation in heavy ion irradiated polycrystalline gold

In this study, we explore the interaction of electron wind force (EWF) with defects originating from ion irradiation in-situ inside a transmission electron microscope. Nanocrystalline gold specimens were self-ion irradiated to a dose of 5 × 10 15 ions/cm 2 (45 displacement per atom) to generate a high density of displacement damage. We also developed a molecular dynamics simulation model to understand the associated atomic scale mechanisms. Both experiments and simulations show that the EWF can impart significant defect mobility even at low temperatures, resulting in the migration and elimination of defects in a few minutes. Overall, we propose that the EWF interacts with defects to create highly glissile Shockley partial dislocations, which makes the fast and low temperature defect annihilation possible.

36 MATERIALS SCIENCE↗