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Global terrestrial water storage (TWS) anomalies reached a record low of –9.94 cm in 2023, decreasing 0.80 cm from 2022. These reductions largely reflect ongoing TWS losses from glacial melt and groundwater use for irrigation, offset by gains in central and eastern Antarctica and La Niña-related tropical wetting.
Ion mobility separations are usually performed in linear channels, which, when extended, can have a large footprint. In this work, we explored the performance of an ion mobility device with a curved architecture which can have a more compact form. The Co-centric Ion Mobility Spectrometer (CIMS) works by manipulating ions between two co-centric surfaces, each containing a serpentine track. The mobility separation inside CIMS is achieved using traveling waveforms (TWs). We initially evaluated the device using ion trajectory simulations using SIMION, which indicated that when ions traveled circularly inside CIMS, they resulted in similar resolving powers and transmitted m/z range as traveling in a straight path in structures for lossless ion manipulations (SLIM). We then performed experimental validation of CIMS in conjunction with a TOF MS. The CIMS was made of 2 flexible printed circuit board materials folded into concentric cylinders separated by a gap of 2.8 mm. The device was about 50 mm diameter × 152 mm long and provided 1.846 m of serpentine path length. Three sets of mixtures (Agilent tune mixture, tetraalkylammonium salts, and 8 peptide mixture) and four traveling waveform profiles (square, sine, triangle, and sawtooth) were used. The sawtooth TW profile produced a slightly higher resolving power for the Agilent tuning mixture and tetraalkylammonium ions. The average resolving power for Agilent tune mixture ions ranged from 37 (using sawtooth TW) to 27 (using square TW). For tetraalkylammonium ions, the average resolving powers ranged from 45 (sawtooth TW) to 31 (square TW). For the peptide mixture ions, the resolving power was similar among the four TW profiles and ranged from 51 to 56. The average percent error in TW CCS for the peptide mixture ions ranged was about 0.4%. In conclusion, the new device showed promising results for a device made of a flexible printed circuit board material, but improvements are needed to further increase the resolving power.
Ground-based heat treatment tests are planned on an argon gas-filled tantalum cartridge developed as pan of a Diffusion Processes in Molten Semiconductors (DPIMS) experiment conducted on NASA's Space Shuttle. The possibility that the cartridge may creep during testing and touch the furnace walls is of real concern in this program. The present paper discusses the results of calculations performed to evaluate this possibility. Deformation mechanism maps were constructed using literature data in order to identify the creep mechanism dominant under the appropriate stresses and temperatures corresponding to the test conditions. These results showed that power-law creep was dominant when the grain size of the material exceeded 55 gm but Coble creep was the important mechanism below this value of grain size. Finite element analysis was used to analyze the heat treatment tWs assuming a furnace run away condition (which is a worst case scenario) using the appropriate creep parameters corresponding to grain sizes of 1 and 100 gm. Calculations were also conducted to simulate the effect of an initial 3 tilt of the cartridge assembly, the maximum possible tilt angle. The von Mises stress and su-ain distributions were calculated assuming that the cartridge was fixed at one end as it was heated from ambient temperature to 1823 K in 1.42 h, maintained at 1823 K for 9.5 h and then further heated to an over temperature condition of 2028 K in 0.3 h. The inelastic axial and radial displacements of the cartridge walls were evaluated by resolving the von Mises strain along the corresponding directions. These calculations reveal that the maximum axial and radial displacements are expected to be about 2.9 and 0.25 mm, respectively, for both fine and coarse-grained materials at 2028 K. It was determined that these displacements occur during heat-up to temperature and creep of the cartridge is likely to be relatively insignificant irrespective of grain size. Furthermore, with a 3' tilt of the cartridge, the deflection is increased by only 0.39 gm which is negligible. Since the gap between the furnace heating elements and the cartridge is about 7.5 mm and less than the maximum radial dilation of 0.25 mm at 2028 K, it is concluded that the cartridge is unlikely to touch the furnace walls during the experiments.
Key properties of nanocrystals are determined by their real atomic structure, therefore a reasonable understanding and meaningful interpretation of their properties requires a realistic model of the structure. In this paper we present an evidence of a complex response of the lattice distances to external pressure indicating a presence of a complex structure of Sic nanopowders. The experiments were performed on nanocrystalline Sic subjected to hydrostatic or isostatic pressure using synchrotron and neutron powder diffraction. Elastic properties of the samples were examined based on X-ray diffraction data using a Diamond Anvil Cell (DAC) in HASYLAB at DESY. The dependence'of the lattice parameters and of the Bragg reflections width with pressure exhibits a ha1 nature of the properties (compressibilities) of the powders and indicates a complex structure of the grains. We interpreted tws behaviour as originating from different elastic properties of the grain interior and surface. Analysis of the dependence of individual interatomic distances on pressure was based on in-situ neutron diffraction measurements done with HbD diffractometer at LANSCE in Los Alamos National Laboratory with the Paris-Edinburgh cell under pressures up to 8 GPa (Qmax = 26/A). Interatomic distances were obtained by PDF analysis using the PDFgetN program. We have found that the interatomic distances undergo a complex, non-monotonic changes. Even under substantial pressures a considerable relaxation of the lattice may take place: some interatomic distances increase with an increase in pressure. We relate this phenomenon to: (1), changes of the microstructure of the densified material, in particular breaking of its fractal chain structure and, (2), its complex structure resembling that of a material composed of two phases, each with its distinct elastic properties.
The twin STEREO spacecrafi, launched in October 2006, are in heliocentric orbits near 4 AU with one spacecraft (Ahead) leading Earth in its orbit around the Sun and the other (Behind) trailing Earth. As viewed from the Sun, the STEREO spacecraft are continually separating from one another at about 45 degrees per year with Earth biseding the angle. At present, th@spaser=raft are a bit more than 45 degrees apart, thus they are able to each 'vie@ ground the limb's of the Sun by about 23 degrees, corresponding to about 1.75 days of solar rotation. Both spameraft contain an identical set of instruments including an extreme ultraviolet imager, two white light coronagraphs, tws all-sky imagers, a wide selection of energetic particle detectors, a magnetometer and a radio burst tracker. A snapshot of the real time data is continually broadcast to NOW-managed ground stations and this small stream of data is immediately sent to the STEREO Science Center and converted into useful space weather data within 5 minutes of ground receipt. The resulting images, particle, magnetometer and radio astronomy plots are available at ~ ~ j ~ g ~ ~ ~ i t , : gAs~ timqe~ co~n~ting ue~s ijnto~ ~ ~ ~ ~ . ~ g ~ solar cycle 24, the separation angle becomes 90 degrees in early 2009 and 180 degrees in early 201 1 as the activity heads toward maximum. By the time of solar maximum, STEREO will provide for the first time a view of the entire Sun with the mronagraphs and e*reme ultraviolet instruments. This view wilt allow us to follow the evolution of active regions continuously and also detect new active regions long before they pose a space weather threat to Earth. The in situ instruments will be able to provide about 7 days advanced notice of co-rotating structures in the solar wind. During this same intewal near solar maximum, the wide-angle imagers on STEREB will both be ;able to view EarlCP-dirsted CMEs in their plane-oPsky. When combined with Eat-lhorbiting assets available at that time, it seems solar cycle 24 will mark a great increase in our ability to understand and predict space weather.
Terrestrial water storage (TWS) information derived from Gravity Recovery and Climate Experiment (GRACE) measurements is assimilated into a land surface model over the Mackenzie River basin located in northwest Canada. Assimilation is conducted using an ensemble Kalman smoother (EnKS). Model estimates with and without assimilation are compared against independent observational data sets of snow water equivalent (SWE) and runoff. For SWE, modest improvements in mean difference (MD) and root mean squared difference (RMSD) are achieved as a result of the assimilation. No significant differences in temporal correlations of SWE resulted. Runoff statistics of MD remain relatively unchanged while RMSD statistics, in general, are improved in most of the sub-basins. Temporal correlations are degraded within the most upstream sub-basin, but are, in general, improved at the downstream locations, which are more representative of an integrated basin response. GRACE assimilation using an EnKS offers improvements in hydrologic state/flux estimation, though comparisons with observed runoff would be enhanced by the use of river routing and lake storage routines within the prognostic land surface model. Further, GRACE hydrology products would benefit from the inclusion of better constrained models of post-glacial rebound, which significantly affects GRACE estimates of interannual hydrologic variability in the Mackenzie River basin.
A majority of the countries in the Middle East and North Africa (MENA) region suffer from water scarcity due in part to widespread rainfall deficits, unprecedented levels of water demand, and the inefficient use of renewable freshwater resources. Since a majority of the water withdrawal in the MENA is used for irrigation, there is a desperate need for improved understanding of irrigation practices and agricultural water use in the region. Here, satellite-derived irrigation maps and crop-type agricultural data are applied to the Land Data Assimilation System for the MENA region (MENA LDAS), designed to provide regional, gridded fields of hydrological states and fluxes relevant for water resources assessments. Within MENA-LDAS, the Catchment Land Surface Model (CLSM) simulates the location, timing, and amount of water applied through agricultural irrigation practices over the region from 2002-2012. In addition to simulating the irrigation impact on evapotranspiration, soil moisture, and runoff, we also investigate regional changes in terrestrial water storage (TWS) observed from the Gravity Recovery and Climate Experiment (GRACE) and simulated by CLSM.
Observations from recent soil moisture missions (e.g. SMOS) have been used in innovative data assimilation studies to provide global high spatial (i.e. 40 km) and temporal resolution (i.e. 3-days) soil moisture profile estimates from microwave brightness temperature observations. In contrast with microwave-based satellite missions that are only sensitive to near-surface soil moisture (0 - 5 cm), the Gravity Recovery and Climate Experiment (GRACE) mission provides accurate measurements of the entire vertically integrated terrestrial water storage column but, it is characterized by low spatial (i.e. 150,000 km2) and temporal (i.e. monthly) resolutions. Data assimilation studies have shown that GRACE-TWS primarily affects (in absolute terms) deeper moisture storages (i.e., groundwater). This work hypothesizes that unprecedented soil water profile accuracy can be obtained through the joint assimilation of GRACE terrestrial water storage and SMOS brightness temperature observations. A particular challenge of the joint assimilation is the use of the two different types of measurements that are relevant for hydrologic processes representing different temporal and spatial scales. The performance of the joint assimilation strongly depends on the chosen assimilation methods, measurement and model error spatial structures. The optimization of the assimilation technique constitutes a fundamental step toward a multi-variate multi-resolution integrative assimilation system aiming to improve our understanding of the global terrestrial water cycle.
Freshwater availability is changing worldwide. Here we quantify 34 trends in terrestrial water storage (TWS) observed by the Gravity Recovery and Climate Experiment (GRACE) satellites during 2002-2016 and categorize their drivers as natural interannual variability, unsustainable groundwater consumption, or climate change. Several of these trends had been lacking thorough investigation and attribution, including massive changes in northwestern China and the Okavango delta. Others are consistent with climate model predictions. This observation-based assessment of how the world's water landscape is responding to human impacts and climate variations provides a blueprint for evaluating and predicting emerging threats to water and food security.
Terrestrial water storage can be defined as the summation of all water on the land surface and in the subsurface. It includes surface soil moisture, root zone soil moisture, groundwater, snow,ice, water stored in the vegetation, river and lake water. Terrestrial water storage (TWS) changes have been observed by the Gravity Recovery and Climate Experiment (GRACE) mission since 2002. GRACE has provided an unprecedented view of the terrestrial water storage variations at large scales. Extremes in water storage often are associated with droughts and flooding events because they are driven by the surplus or deficit of water. Few hydrologic observing networks yield sufficient data for comprehensive monitoring of changes in the total amount of water stored in a region. GRACE observations have helped to fill this gap. This book chapter is divided into 4 sections.Section 1 provides an overview of the GRACE mission. Section 2 reviews the terrestrial water storage solutions that are available. Section 3 describes regional to global applications of GRACE for monitoring extremes in the terrestrial water storage, including droughts and flooding events. Conclusions and future directions are reported in Section 4.
We evaluate the impact of Gravity Recovery and Climate Experiment data assimilation (GRACE-DA) on seasonal hydrological forecast initialization over the United States, focusing on groundwater storage. GRACE-based terrestrial water storage (TWS) estimates are assimilated into a land surface model for the2003–16 period. Three-month hindcast (i.e., forecast of past events) simulations are initialized using states from the reference (no data assimilation) and GRACE-DA runs. Differences between the two initial hydrological condition (IHC) sets are evaluated for two forecast techniques at 305 wells where depth to water table measurements are available. Results show that using GRACE-DA-based IHC improves seasonal groundwater forecast performance in terms of both RMSE and correlation. While most regions show improvement, degradation is common in the High Plains, where withdrawals for irrigation practices affect groundwater variability more strongly than the weather variability, which demonstrates the need for simulating such activities. These findings contribute to recent efforts toward an improved U.S. drought monitoring and forecast system.