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DRiFT Current Mode, Trigger Settings and Flexible Detector Specifications Applied to Scintillator Arrays

MCNP radiation transport output is post-processed by DRiFT, a Detector Response Function Toolkit to simulate detailed nuclear instrumentation response. DRiFT can be used to assess the performance and potential limitations of scintillator, gas, and semiconductor detectors under a variety of simulated conditions not easily achievable in a laboratory setting. This work describes new updates in DRiFT for scintillator simulations which focus on the capability to simulate scintillators in current mode, an expansion of trigger options, and the ability to customize individual detector properties in a simulation. These improvements are designed to facilitate the ability to model large arrays of scintillator detectors with higher fidelity than was previously possible and are demonstrated in three examples. The first shows the difference between operating DRiFT in current and pulse mode. In the second example, which is intended to demonstrate deviations in individual detector performance, each detector has properties (PMT gain, optical transport, scintillation yield, etc.) that vary between detectors and are specified in DRiFT. A final example examines how DRiFT could be used to optimize digitizer settings in high rate measurements with split signals using the new common trigger option.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND

Recent development in organic scintillators

Discussion on recent developments of organic scintillators includes studies of organic compounds that form glass-like masses which scintillate and are stable at room temperature, correlations between molecular structure of organic scintillators and self-quenching, recently developed fast scintillators, and applications of liquid-scintillation counters.

Horrocks, D. L.

High latitude scintillation effects on very high frequency /vhf/ and S-band satellite transmissions.

A scintillation study was conducted with the purpose to define the extent of scintillation activity in the S-band region, and to determine if such activities at higher frequencies are caused by ionospheric irregularities similar to those causing scintillations at vhf and lower frequencies. Simultaneous transmissions at 137 and 1695 MHz from polar orbiting satellites were used in this study. Scintillations were found to be present at S-band frequencies in the polar regions; it is concluded that they are caused by ionospheric characteristics similar to those causing scintillations at lower frequencies.

Pope, J. H.

Research Investigation on Dense Scintillation Glass for Use in Total Absorption Nuclear Cascade Detectors

Three approaches to the development of a high density scintillation glass were investigated: They include the increase of density of glass systems containing cerium - the only systems which were known to show scintillation, the testing of a novel silicate glass system containing significant concentrations of silver produced by ion exchange and never tested previously, and the hot pressing of a diphasic compact of low density scintillation glass with high density passive glass. In first two cases, while ultraviolet excited fluorescence was maintained in the glasses showing high density, scintillation response to high energy particles was not retained in the case of the cerium containing glasses or developed in the case of the silver containing glasses. In the case of the compacts, the extremely long path length caused by the multiple internal reflections which occur in such a body resulted in attenuation even with glasses of high specific transmission. It is not clear why the scintillation efficiency is not maintained in the higher density cerium containing glasses.

Hensler, J. R.

Ionospheric irregularities causing scintillation of GHz frequency radio signals

Consideration of the recently observed phenomenon of scintillation of satellite signals at GHz frequency range. Based on the scintillation data and results from in situ measurements, several ionospheric irregularity models with different power spectra are studied. Scintillation index is computed for the various models and compared with observed results. Both magnitude and frequency dependence of the scintillation index are investigated. It is found that a thick irregularity slab of the order of 200 km with an electron density fluctuation of about 20 per cent of its background value and with a nonmonotonic power spectrum may account for the maximum observed values of the scintillation index as well as its frequency dependence. Some future observations and measurements are suggested.

Wernik, A. W.

Interstellar scattering of pulsar radiation. 1: Scintillation

An investigation of the intensity fluctuations of 28 pulsars near 0.4 GHz indicates that scintillation spectra have a Gaussian shape, scintillation indices are near unity, and the scintillation bandwidth depends linearly on dispersion measure. Observations near 2.5 GHz suggest a strong dependence of the frequency at which scintillation indices fall below unity on dispersion measure. Multistation measurements of scintillation provide values or limits for the scale size of the scattering diffraction pattern. The dependences of scattering parameters on dispersion measure is discussed in terms of the current models. It is suggested that any line of sight through the galaxy encounters increasingly rare, increasingly large deviations of thermal electron density on the scale of 10 to the 11th power cm.

Backer, D. C.

Ionospheric scintillations associated with equatorial E-region

Amplitude scintillations at 40, 140, and 360 MHz recorded at an equatorial station Ootacamund (dip 4 deg N) during the ATS-6 phase II and the ionograms at a nearby station Kodaikanal (dip 3.5 deg N) are examined for the scintillation activity. Various sporadic E events, but not the Es-q, are associated with intense daytime scintillations. There are no scintillations at times of normal E-layer or cusp type of Es. Scintillations are also present at times of night Es.

Chandra, H.

Equatorial scintillations - A review

Scintillation observations of equatorial irregularities by techniques such as in situ, radar backscatter, airglow, and total electron content are reviewed, with an emphasis on GHz measurements. New aspects of the spread-F analysis from ionograms are mentioned, followed by a discussion of scintillation morphology, and the longitudinal control of the equatorial scintillations is emphasized. A coordinated multitechnique observation of the equatorial irregularities is described in detail, the study being divided into two parts: (1) an examination of the large field-aligned irregularity structures and their association with discrete patches of scintillation activity, and (2) an investigation of the coexistence of km-scale-irregularities with meter scales and a description of the evolution of the irregularity and scintillation spectra during the various phases of irregularity generation and decay. Unsolved problems are also reviewed, e.g., it is stated that the effects of steep spatial gradients in the electron density structures and their subsequent erosion on both CW and pulse propagation need to be evaluated both from the point of view of theory and experiments.

Basu, S.

High pressure gas scintillation drift chambers with wave shifter fiber readout. I

The authors present results from a prototype xenon-gas scintillation drift chamber. It was operated at pressures up to 20 atm, and the scintillation light yield was measured at various pressures and reduced fields. Scintillation-reduced fields ranged from 1.3 to 3 kV/cm/atm in a 5.4-mm scintillation gap. Drift fields ranged from 45 to 100 V/cm/atm in an 8-cm drift region. The chamber was exposed to an 241Am source in a port either 2.7 or 5.4 cm from the secondary scintillation region. The authors also describe the high-voltage problems encountered during operation at high pressures. Further tests with the wave shifter fiber readout showed that the problem of gas contamination by the fibers is manageable but that the interaction between the optical fibers and the high-pressure xenon gas can lead to fiber damage. A solution to this problem is described.

Parsons, A.

Results from a study of scintillation behavior at 12, 20, and 30 GHz using the results from the Virginia Tech Olympus receivers

Tropospheric scintillations are rapid fluctuations of signal caused by multiple scattering from the small scale turbulent refractive index inhomogeneities in the troposphere. They can strongly impair satellite communications links operating at frequency above 10 GHz. The VA Tech OLYMPUS propagation experiment which includes 12, 20, and 30 GHz beacon receivers at an elevation angle of 14 degrees provides us with valuable multifrequency scintillation data. A long term analysis of tropospheric scintillation results from the VA Tech OLYMPUS experiment is presented. It includes statistics of both the scintillation intensity and the attenuation relative to clear air as well as seasonal, diurnal and meteorological trends. A comparison with the Consultative Committee for International Radio (CCIR) predictive model for scintillation fading is presented.

Pratt, Timothy

Silicon Photo-Multiplier Readouts for Scintillators in High-Energy Astronomy

New scintillator materials have recently been shown to hold great potential for low-cost, reliable gamma-ray detectors in high-energy astronomy. New devices for the detection of scintillation light promise to make scintillator-based instruments even more attractive by reducing mass and power requirements,in particular, silicon photo-multipliers (SiPMs) are starting to become commercially available that offer gains and quantum efficiencies similar to those of photo-multiplier tubes (PMTs), but with greatly reduced mass, high ruggedness, low voltage requirements, and no sensitivity to magnetic fields. We have conducted laboratory tests of a sample of commercially available SiPMs coupled to LaBr3;Ce, a scintillator of relevance to to future high-energy astrophysics missions. We present results for gamma-ray spectroscopy. compare the SiPM performance to that of a PMT, and discuss the extent to which SiPMs offer significant advantages for scintillator-based space missions.

Bloser, Peter F.

Tests of Multibeam Scintillation Mitigation on Laser Uplinks

A report presents additional details about parts of the program of research and development that is the topic of the immediately preceding article. The report emphasizes those aspects of the program that pertain to the use of multiple uplink laser beams in a ground-to-spacecraft optical communication system to reduce (relative to the case of a single uplink laser beam) the depth and frequency of occurrence of fades in the uplink signal received at the spacecraft. The underlying multibeam scintillation-mitigation concept was described in "Multiple-Beam Transmission for Optical Communication" (NPO-20384), NASA Tech Briefs, Vol. 22, No. 11 (November 1998), page 56. The report discusses the need for mitigating uplink scintillation; briefly describes the Optical Communications Telescope Laboratory and its role as the ground station in the research; summarizes prior experiments in uplink scintillation and multibeam mitigation of scintillation in ground-to-spacecraft laser communications; and describes key experiments planned to be performed in the next five years. The report then elaborates somewhat on the initial experiments, which are to be dedicated to understanding and perfecting the multibeam scintillation-mitigation strategy.

Wilson, Keith

Detection of scintillation light in noble gases with wavelength-shifting optical fibers

Wavelength-shifting (WLS) techniques enable particle detectors based on noble gases, whose scintillation light is predominantly emitted in the vacuum-ultraviolet. We investigate WLS fibers coated with tetraphenyl butadiene (TPB) for scintillation light detection in gaseous xenon and argon at pressures up to 8.5 bar, motivated by future high-pressure xenon time-projection chambers of the NEXT program. Two detector configurations are studied: an elongated high-pressure vessel with four PTFE panels equipped with WLS fibers read by temperature-stabilized SiPMs, and a compact box-shaped detector operated at 1 bar Xe with WLS fibers read out by PMTs. Both operate with continuous gas purification. The detector response is characterized using cosmic muons and alpha particles from a $^{241}$Am source. With the SiPM setup, we measure a light collection efficiency (LCE) of ${1.18 \pm 0.01~\mathrm{(sta.)}~^{+0.07}_{-0.09}~\mathrm{(sys.)}~\%}$ for xenon and ${1.07 \pm 0.01~\mathrm{(sta.)}~^{+0.06}_{-0.08}~\mathrm{(sys.)}~\%}$ for argon. With PMT readout, we measure a LCE of ${0.45 \pm 0.01~\mathrm{(sta.)} \pm 0.05~\mathrm{(sys.)}~\%}$ in xenon, in agreement with the SiPM result once photon detection efficiency is accounted for. Average scintillation waveforms in xenon and argon are studied to assess the time structure of the emitted light. Cosmic-muon measurements yield a mean energy required to produce a scintillation photon $45\pm7~\mathrm{(sta.)}~^{+4}_{-5}~\mathrm{(sys.)}~\mathrm{eV}$ at 1.5 bar, in agreement with the literature. The results demonstrate that TPB-coated WLS fiber systems can reliably detect scintillation light in high-pressure gaseous noble detectors, with a LCE representing an upper limit for realistic large-scale TPCs, where additional photon losses from materials and fiber attenuation are expected.

Soleti, S. R. [Donostia Intl. Phys. Ctr., San Seba

Characterization of a radiation detector based on opaque water-based liquid scintillator

Here, we present the characterization of a novel radiation detector based on an opaque water-based liquid scintillator. Opaque scintillators, also known as LiquidO, are made to be highly scattering, such that the scintillation light is effectively confined, and read out through wavelength-shifting fibers. The 1-liter, 32-channel prototype demonstrates the capability for both spectroscopy and topological reconstruction of point-like events. The design, construction, and evaluation of the detector are described, including modeling of the scintillation liquid optical properties and the detector’s response to gamma rays of several energies. A mean position reconstruction error of 4.4 mm for 1.6 MeV-equivalent events and 7.4 mm for 0.8 MeV-equivalent events is demonstrated using a simple reconstruction approach analogous to center-of-mass.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Czochralski Growth and Characterization of a Compositionally Complex Rare Earth Aluminum Garnet Scintillator: (Gd 1/4 Y 1/4 Tb 1/4 Lu 1/4 ) 3 Al 5 O 12 :Ce

Compositionally complex oxides have garnered increasing interest for their enhanced phase stability and tunable functional properties, yet their development as bulk single crystal scintillators remains limited. Herein, we report the Czochralski growth and characterization of (Gd 1/4 Y 1/4 Tb 1/4 Lu 1/4 ) 3 Al 5 O 12 :Ce (GYTLAG), a compositionally complex garnet incorporating four dodecahedrally coordinated principal rare earth elements. The garnet phase was confirmed by powder and single crystal X-ray diffraction, and macroscopic defects are described. X-ray absorption near-edge structure measurements confirm the 3+ oxidation state of all rare earths and support their occupation of the same crystallographic site; white line intensity variations correlate with the anticipated segregation behavior. Elemental segregation is quantified by SEM/EDS and ICP-OES, and a linear trend was established between the segregation coefficient and the difference between each rare earth’s ionic radius (r) and the average ionic radius (AIR) of the dodecahedral site. This trend offers a predictive framework for compositional control in future REAG crystals grown by the Czochralski method. Photoluminescence and radioluminescence measurements reveal both Ce 3+ and Tb 3+ emission. Scintillation pulses exhibit four-component decay with dominant ~230 µs and ~1.2 ms components, and the light yield is estimated to be up to 43,000 ph/MeV under 137Cs γ-ray excitation. GYTLAG also demonstrates a strong radioluminescence efficiency and 50% lower afterglow at 20 ms compared to a LuAG:Ce reference, underscoring its promise for scintillator applications.

Compositionally complex oxide, high entropy oxide,

Characterization of EJ-270 and Ce-doped LiCAF scintillators for the development of high-rate neutron reflectometer detectors

The Second Target Station of the Spallation Neutron Source at Oak Ridge National Laboratory is anticipated to provide a neutron source with ∼20 times increase in peak brightness than the First Target Station. The neutron reflectometers currently in operation at the First Target Station need to be upgraded due to the increased neutron flux. A prototype neutron detector module based upon a pixelated scintillator array readout by silicon photomultipliers is being developed to address the high-rate challenge faced with future neutron reflectometer instruments at the Second Target Station. Two types of scintillator materials were considered for this detector development, i.e., 6 Li-loaded EJ-270 plastic scintillator and Ce-doped LiCAF single crystal. This paper reports the scintillator characterization results, including light yield, pulse shape discrimination performance, capability to detect thermal neutrons in a high γ-ray field, and γ-ray sensitivity. The number of photons produced per neutron capture by EJ-270 and LiCAF:Ce was measured to be 2176 ± 91 and 2651 ± 108, respectively. EJ-270 demonstrated a good capability to discriminate between neutrons and γ-rays by employing the commonly used charge comparison method (figure-of-merit: 1.13 ± 0.01 for an energy cut of 292–426 keVee) and a reasonable performance when using the time-over-threshold techniques; however, no discrimination was observed from LiCAF:Ce regardless of the pulse shape discrimination approaches utilized, making pulse height discrimination necessary for LiCAF:Ce to differentiate between neutrons and γ-rays. Both EJ-270 and LiCAF:Ce exhibited an acceptable capacity to detect thermal neutrons at high exposure rates up to approximately 584 mR/h. Furthermore, the γ-ray sensitivities measured with a 60 Co source at an exposure rate of around 1145 mR/h were determined to be (6.11 ± 0.87) × 10 −6 and (7.64 ± 1.08) × 10 −7 for EJ-270 and LiCAF:Ce, respectively.

EJ-270

Scintillation properties of diamond powders and feasibility of using them in thermal neutron detectors

Diamond offers unique properties for radiation detection, including high radiation hardness, very low gamma sensitivity, and fast response. Conventional diamond detectors rely on charge collection, but this approach requires ultra-pure single crystals and suffers from radiation-induced degradation. Here, in this work, we demonstrate an alternative approach using diamonds as scintillators for detection of charged particles and thermal neutrons. Prototypes were fabricated from commercially available diamond powders bonded to glass substrates and coupled with 6 LiF converters and silicon photomultipliers (SiPMs) and conventional PMTs. We characterized their scintillation properties under alpha particle excitation, x-ray photoluminescence, and thermal neutrons. The tryout detectors exhibit strong scintillation light signals, nanosecond-scale response times, and neutron detection efficiencies up to approximately 14 %, evaluated by comparison to conventional 3 He detector with known efficiency. These results demonstrate the feasibility of cost-effective, lightweight and robust diamond scintillation detectors for applications in space and planetary science, nuclear security, safeguards and environmental monitoring requiring efficient, robust, gamma-blind neutron detectors.

47 OTHER INSTRUMENTATION

3D printed water-stable Cd-doped Cs 4 MnBi 2 Cl 12 /polylactic acid perovskite/polymer composites for high-flux X-ray scintillation

Stable and efficient X-ray scintillators are crucial for medical diagnostics, industrial, and defense applications. However, conventional scintillator technologies face a trade-off between stability, optimal performance, and sustainability. Herein, we introduce 3D-printed Cs 4 MnBi 2 Cl 12 (Pero1) and Cs 4 Cd 0.68 Mn 0.32 Bi 2 Cl 12 (Pero2) perovskite microcrystals embedded within a polylactic acid (PLA) polymer composite as X-ray scintillators, combining efficiency, stability, and sustainability. The orange luminescent perovskite powder phosphors exhibited poor water stability, which was successfully addressed through incorporation into PLA via filament extrusion and fused deposition modeling (FDM) 3D printing. The resulting composite films demonstrated remarkable water stability while maintaining uniform orange emission throughout the polymer matrix, as confirmed by 3D topography scanning and X-ray fluorescence mapping. Structural characterization revealed minimal chemical interaction between the perovskite and PLA matrix, with the composites retaining their crystalline properties. The PLA-Pero2 composite exhibited superior optical properties, with a photoluminescence quantum yield of 47%, nearly 17 times higher than that of PLA-Pero1 (2.8%), attributed to the effective suppression of non-radiative decay pathways through Cd 2+ doping. Under hard X-ray irradiation at synchrotron beamlines, both composites exhibited excellent radioluminescence, with emission peaks at 605 nm, a linear response across a wide X-ray flux range, and remarkable radiation stability, showing less than 3% intensity degradation after 600 seconds of continuous high-dose exposure. The PLA-Pero2 composite achieved a spatial resolution of 5 line pairs per millimeter and a contrast ratio of 0.255. These performance metrics, combined with the polymer's biodegradability and scalability through additive manufacturing, position PLA-based composites as a more sustainable alternative to conventional petroleum-based polymer scintillators for next-generation medical imaging, radiation monitoring, and industrial radiography applications.

3D Printing