Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “Plasma”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 73 records · Page 4

Time-resolved imaging of atoms and molecules in laser-produced uranium plasmas

Gas-phase oxidation of uranium (U), plume chemistry, and its impact on optical emission features of the uranium plasma are investigated. Plasmas were produced via nanosecond laser ablation of a natural uranium target in a chamber where uranium oxidation was controlled by varying the oxygen partial pressure within argon cover gas. Monochromatic imaging of uranium atoms and monoxide molecules was performed using narrowband optical filters, which clearly reveals the spatio-temporal evolution of these species in the plasma. Uranium oxides are found to be formed at the plasma edges, where lower temperatures favor molecular recombination. Segregation between the distribution of uranium atoms and monoxide species is observed at later times of plasma evolution, and is more apparent at lower oxygen partial pressures. At higher oxygen partial pressures, significant variation in plume morphology is noticed for UO species, which is attributed to higher rate of oxide (UxOy) formation at the plume edges. The monochromatic images of U atoms and molecules and corresponding spectral features at various oxygen partial pressures presented here provide a unique insight into gas-phase, high-temperature uranium oxidation, and its chemistry and have implications for a wide range of nuclear applications, from stand-off detection of radioisotopes to forensics and safeguards.

(140.3440) Laser-induced breakdown, (280.4788) Opt↗

Exploring the crossover between high-energy-density plasma and ultracold neutral plasma physics

In this paper, we present ideas that were part of the miniconference on the crossover between High Energy Density Plasmas (HEDP) and Ultracold Neutral Plasmas (UNPs) at the 60th Annual Meeting of the American Physical Society Division of Plasma Physics, November 2018. We give an overview of UNP experiments with an emphasis on measurements of the time-evolving ion density and velocity distributions, the electron-ion thermalization rate, and plasma self-assembly—all just inside the strongly coupled plasma regime. We also present theoretical and computational models that were developed to understand a subset of HEDP experiments. However, because HEDP experiments display similar degrees of strong coupling, many aspects of these models can be vetted using precision studies of UNPs. This comparison is important because some statistical assumptions used for ideal plasmas are of questionable validity in the strongly coupled plasma regime. We summarize two theoretical approaches that extend kinetic theories into the strong-coupling regime and show good agreement for momentum transfer and self-diffusion. As capabilities improve, both computationally and experimentally, UNP measurements may help guide the ongoing development of HEDP-appropriate plasma models. Future opportunities in viscosity, energy relaxation, and magnetized plasmas are discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The 2022 Plasma Roadmap: low temperature plasma science and technology

Abstract The 2022 Roadmap is the next update in the series of Plasma Roadmaps published by Journal of Physics D with the intent to identify important outstanding challenges in the field of low-temperature plasma (LTP) physics and technology. The format of the Roadmap is the same as the previous Roadmaps representing the visions of 41 leading experts representing 21 countries and five continents in the various sub-fields of LTP science and technology. In recognition of the evolution in the field, several new topics have been introduced or given more prominence. These new topics and emphasis highlight increased interests in plasma-enabled additive manufacturing, soft materials, electrification of chemical conversions, plasma propulsion, extreme plasma regimes, plasmas in hypersonics, data-driven plasma science and technology and the contribution of LTP to combat COVID-19. In the last few decades, LTP science and technology has made a tremendously positive impact on our society. It is our hope that this roadmap will help continue this excellent track record over the next 5–10 years.

plasma diagnostics↗

Plasma-based global pathway analysis to understand the chemical kinetics of plasma-assisted combustion and fuel reforming

The Global Pathway Analysis (GPA) algorithm helps analyze the chemical kinetics of complex combustion systems by identifying important global reaction pathways connecting a source species to a sink species through various important intermediate species (i.e., hub species). Here, the present work aims to extend GPA algorithm to plasma-assisted combustion and fuel reforming systems to identify the dominant global pathways in such systems at various conditions. In addition, the present study extends the ability of GPA algorithm to identify reaction cycles involving the excitation of high-concentration species (e.g., O 2 , N 2 , and fuel) to their vibrational and electronic states and the subsequent de excitation to their ground state, based on their significance on the reactivity of plasma-assisted systems in terms of gas heating and radical production. Provisions are made in the GPA algorithm to evaluate the reactivity of identified re action pathways and cycles based on the element-flux transfer (i.e., dominance), heat release, and radical production rate. The newly developed Plasma-based Global Pathway Analysis (PGPA) algorithm is then used to analyze the plasma assisted combustion of ammonia and reforming of methane. The PGPA analyses elucidated the significance of vibrational-translational cycles on the reactivity of NH 3 /air mixtures. Further, analyses on the production of NO ascribed the early reforming of NH 3 to N 2 and H 2 in impeding the production of NO during plasma-assisted NH 3 ignition. Lastly, the enhanced reforming of CH 4 /N 2 mixtures using plasma has been attributed to electron impact dissociation of CH 4 when compared to thermal reforming. In contrast, conventional path-Flux analysis (PFA) was found to require significant manual effort and pre-analysis intuitions from expert knowledge, making it arduous to provide valuable in sights into plasma chemistry. The user-friendly and automated nature of PGPA thus provides a valuable tool for assessing the kinetics of plasma-assisted systems helpful in analyzing and, further, a foundation in reducing plasma-assisted chemistry, without the needs of expert knowledge.

33 ADVANCED PROPULSION SYSTEMS↗

Characterizing the plasma-induced thermal loads on a 200 kW light-ion helicon plasma source via infra-red thermography

The light-ion helicon plasma source of the Proto-MPEX linear plasma device has been recently upgraded to enable pulsed (0.5–1 s) operation up to 200 kW. The main objective of this work is to report on the plasma-induced surface heat fluxes incident on the helicon window during high power operation (60–150 kW net power) for the purpose of the design of the upcoming material plasma exposure eXperiment (MPEX). The IR imaging system and associated physics models for the extraction of surface heat fluxes are presented. Furthermore, experimental results demonstrate that the control of the plasma strike point via magnetic flux mapping and the use of dedicated limiters is effective at reducing the heat loads on the dielectric window. Moreover, it is found that the flux mapping must create a gap between the plasma and the dielectric window of at least the plasma radial decay length. Extrapolated to 200 kW net RF power, this mode of operation can reduce the power lost to the dielectric window by 33%. The results presented have direct application to the design of high-powered helicon plasma sources that operate in a steady state. Examples include linear divertor simulators such as MPEX, electric thrusters, negative ion sources for NBI and linear plasma–material interaction test stands.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Electric Field Measurements at the Surface of a Piezoelectric Transformer for Plasma Jet Formation using the Plasma Research Facility at Sandia National Laboratory (Final Report)

The overall goal of this research is to understand how low-temperature non-equilibrium plasmas form directly off the surface of piezoelectric crystals. Specifically, this project aims to temporally and spatially resolve how the electric field evolves on and near the surface of a piezoelectric transformer (PT) at conditions that produce an atmospheric-pressure air plasma jet emanating from the corner of the PT. In this work, we used the Plasma Research Facility (PRF) at Sandia National Laboratory to conduct temporally- and spatially-resolved electric field induced second harmonic (E-FISH) measurements of the electric field at and near the surface of a piezoelectric transformer, providing a fundamental understanding of how piezoelectric crystals can be used for plasma generation. We carried out two Objectives: Objective 1 – The first objective was to measure the temporal and spatial evolution of the electric field along the surfaces approaching the corner of a rectangular PT just below conditions that lead to plasma jet formation. Such a measurement can be used to explain when and where the electric field peaks, leading to plasma formation; Objective 2 – The second objective was to measure the temporal and spatial evolution of the electric field along the surfaces approaching the corner of a rectangular PT just at conditions of plasma jet formation. This, in principle, gives a more accurate determination of how the electric field leads to plasma formation but is more difficult due to the relatively stochastic plasma jet behavior of a PT. This work was complemented by an award from the Sandia PRF, and we worked with Dr. Edward Barnat at the Sandia PRF to carry out these objectives.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Effect of boronization on plasma-facing graphite surfaces and its correlation with the plasma behavior in NSTX-U

Boronization is a Plasma Facing Component (PFC) conditioning technique widely used in tokamak machines. The National Spherical Torus Experiment-Upgrade (NSTX-U) applied this conditioning, using a plasma glow with a deuterated Trimethyl-boron (d-TMB) and He mixture. The use of boronization during the campaign improved the plasma performance, allowing longer plasma discharges and H-mode access. The chemical state of an ATJ graphite sample, used as a proxy for the NSTX-U PFCs, was monitored in-situ using the Materials Analysis Particle Probe (MAPP) diagnostic and X-ray Photoelectron Spectroscopy (XPS). The XPS data showed a progressive rise (from + fluence increased. Filterscopes were used to measure the light emitted by oxygen impurities in the plasma near the surface of the PFC. An increase in the registered magnitude of the OII line, normalized to the Dγ intensity, was observed as the concentration of O on the ATJ surface increased. The plasma performance was found to be strongly correlated to oxygen impurity concentrations at the plasma edge and on the PFC surface, as measured by the discharge length and access to the H-mode regime. In this work, we present a quantitative analysis of the evolution of the chemistry of the ATJ surface, and the oxygen presence in the plasma-material interface, and report relevant plasma parameters observed during the same period of time.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Plasma catalysis: separating plasma and surface contributions for an Ar/N 2 /O 2 atmospheric discharge interacting with a Pt catalyst

Atmospheric pressure non-equilibrium plasmas can form nitrogen oxide (NO x ) compounds directly from nitrogen and oxygen without a catalyst, and at lower catalyst temperatures than would be possible without plasma. In this work, the oxidation of plasma-produced NO from an Ar/N 2 /O 2 non-equilibrium atmospheric-pressure plasma-jet (APPJ) over a platinum-on-alumina powder catalyst was investigated with in-situ infrared spectroscopy. Products downstream of the catalyst bed were analyzed along with catalyst surface species. The catalyst was exposed to plasma at both constant temperature and a cyclic temperature ramp in order to study long-lasting and transient surface changes. Primary incident reactive species to the catalyst were assessed to be NO and O 3 . Pt-Al 2 O 3 at 350 °C increased oxidation of NO relative to Al 2 O 3 or an empty chamber. The surface state of Pt-Al 2 O 3 evolves during plasma-effluent exposure and requires upwards of 20 min exposure for stabilization compared to Al 2 O 3 . Once stable surface conditions are achieved, thermal cycling reveals a repeatable hysteresis pattern in downstream products. At low temperature, oxygen and NO x accumulate on the catalyst surface and react at elevated temperatures to form NO 2 . Increasing plasma power and O 2 :N 2 ratio increases the hysteresis of the heating relative to the cooling curves in the pattern of NO 2 formation. The limitation on NO oxidation at high temperatures was assessed to be Pt-O which is depleted as the catalyst is heated. Once stored species have been depleted, NO oxidation rates are determined by incoming reactants. Two overlapping NO oxidation patterns are identified, one determined by surface reactants formed at low temperature, and the other by reactants arriving at the surface at high temperature. As a result, the plasma is responsible for providing the reactants to the catalyst surface, while the catalyst enables reaction at high temperature or storage at low temperature for subsequent reaction.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Plasma production and ion heating systems for the Material Plasma Exposure eXperiment

Plasma production and ion heating in the Material Plasma Exposure eXperiment (MPEX), whose design is nearing completion, is accomplished using continuous wave RF power with average power density up to 1.6 MW/m2 at the plasma interface. Plasma is produced using helicon waves coupled through a single helical antenna at 13.56 MHz with power supplied by three 100 kW fixed-frequency RF generators feeding a power combiner network followed by the matching network and launcher. The helicon source can utilize various gasses including hydrogen, deuterium, and helium, with a magnetic field strength in the source region up to 0.2 T, and maximum device |B| of 2.5 T. Power is coupled to ions via ion cyclotron heating at the fundamental resonance using a pair of phased helical antennas operating in the frequency range 4-9 MHz, that launch waves towards the resonance from the antenna region where ω > ωci. ICH power is supplied by a single 500 kW tunable RF transmitter through a 90° power splitter and matching/decoupling network. In the case of both the helicon and ICH systems the antennas are located external to the vacuum, with power transferred through novel water-cooled coaxial vacuum windows consisting of fused quartz outer cylinders and silicon nitride inner cylinders with forced convection water cooling between them. The antenna enclosures are pressurized with dry air to 3 bar absolute for voltage standoff.Several 3-D COMSOL models have been created to simulate the two systems. A model of the helicon region utilizing a cold plasma dielectric tensor with accurate magnetic field and realistic plasma density profiles has been used to calculate the plasma loading/complex antenna input impedance at the launcher feed for various ne and |B| values, for the purpose of estimating power handling. It also incorporates the geometry of all launcher structures relevant to this determination. A still more detailed model of the launcher together with a lossy dielectric plasma surrogate has been used to determine RF electric field values and power losses in the device components.Similar models have been produced to predict the performance and power handling of the ICH launcher. For this device the impedance matrix of the two-element antenna array is calculated using a warm plasma model, necessary to properly determine the wave propagation and absorption.

Goulding, Richard↗

Non-linear dependence of ion heat flux on plasma density at the L–H transition of JET NBI-heated deuterium–tritium plasmas

Abstract Recent JET D–T campaigns opened the possibility of unique isotope studies to investigate the L–H transition physics in view of reactor plasmas and to study the origin of the observed power threshold minimum. In the present paper, we characterise L–H transitions in the low and high-density branches of JET NBI-heated D–T plasmas. As discussed in the paper, L–H transition has been hypothesised to be determined by the transport power losses of plasma ions, i.e. the so-called ion heat flux ( Q i ). We present the first power balance analysis of JET NBI-heated D–T plasmas to evaluate the ion heat flux at the transition. Due to the experimental setting being similar to previous JET D experiments, we also directly compare the results, discussing the isotope effect and similarities between datasets. First, we find an isotope effect between D and D–T Q i , with a lower Q i in D–T plasmas. We confirm that the ion heat flux deviates from density linearity compared to the linear trend observed in wave-heated D plasmas of other tokamaks. The deviation we observe in NBI-heated L–H transitions happens at an isotope-dependent density. Plasma edge rotation correlates with Q i deviation from density linearity in the low-density branch. However, further investigations would be required to assess the role of rotation on Q i and the power threshold minimum at JET. At low plasma density, NBI power dominates Q i , while increasing the density makes the equipartition power dominant. We finally compare our results with hypotheses proposed from evidence in other tokamaks to present a complete overview of ion heat flux analyses in D and D–T NBI-heated plasmas at JET.

Vincenzi, P. (ORCID:0000000251564354)↗

Experimental Investigation of the Effects of Magnetic Mirrors on Plasma Transport in the Prototype Material Plasma Exposure Experiment

The Prototype Material Plasma Exposure eXperiment (Proto-MPEX) at Oak Ridge National Laboratory is developing a helicon radio frequency (RF) source for plasma production along with microwave electron heating and RF ion heating. Proto-MPEX has several magnetic mirrors that affect plasma transport. The magnetic field near the helicon source is ~ 0.05 T, and the peak magnetic field in Proto-MPEX is ~ 1.8 T, which results in a large magnetic well for particles sourced at the helicon transporting toward the target region. Keeping the helicon source field and the target field constant, experiments have been conducted by methodically changing the magnetic field, at a local axial location, within the source and the target. Plasma flow measurements using Mach probes have shown a decrease in the flow as a function of the magnetic mirror ratio. Plasma flows were further investigated with ion cyclotron resonant heating (ICH). Results with the addition of ICH measured upstream of the antenna have shown a decrease in Mach number as a function of mirror ratio when compared to helicon discharges. Such flow behavior demonstrated slowing down of the plasma due to the increased reverse plasma flow toward the helicon plasma source. However, in high magnetic fields, when the resonant magnetic field moved away from the ICH antenna, no effects on the plasma flow due to ICH were observed.

Kafle, Nischal↗

Plasma turbulence enhanced current collection: Results from the plasma motor generator electrodynamic tether flight

The plasma motor generator (PMG) experiment, launched June 26, 1993, was a tethered system of two identical plasma contactors connected via a 500-m conducting tether. The experiment was designed to demonstrate the ability of plasma contactors to provide a low-impedance connection between a spacecraft and the ionosphere for both the electron emission and collection. The flight data indicate that plasma contactors enhance electron collection and emission by both neutralizing the electron space charge and scattering electrons across the geomagnetic field lines. Up to a 0.3 A steady current flowed along the tether in a curcuit completed through the ionosphere. An analytical model for plasma contactor interaction with a background plasma which incorporates electron scattering by plasma waves is compared with the flight data. Good agreement between the model and the data is achieved for an effective scattering frequency equal to one twentieth of the local plasma contactor plasma frequency.

Katz, I.↗

Investigations of Remote Plasma Irregularites by Radio Sounding: Applications of the Radio Plasma Imager on IMAGE

The Radio Plasma Imager (RPI) on the Imager for Magnetopause-to-Aurora Global Exploration (IMAGE) mission operates like a radar by transmitting and receiving coherent electromagnetic pulses. Long-range echoes of electromagnetic sounder waves are reflected at remote plasma cutoffs. Thus, analyses of RPI observations will yield the plasma parameters and distances to the remote reflection points. These analyses assume that the reflecting plasma surfaces are cold and are sufficiently smooth that they effectively behave as plane mirrors to the incoming sounder waves, i.e., that geometric optics can be used. The RPI will employ pulse compression and spectral integration techniques, perfected in ground-based ionospheric digital sounders, in order to enhance the signal-to-noise ratio in long-range magnetospheric sounding. When plasma irregularities exist in the remote magnetospheric plasmas that are being probed by the sounder waves, echo signatures may become complicated. Ionospheric sounding experience indicates that while topside sounding echo strengths can actually be enhanced by the presence of irregularities, ground-based sounding indicates that coherent detection techniques can still be employed. In this paper we investigate the plasma conditions that will allow coherent signals to be detected by the RPI and the signatures to be expected, such as scattering and plasma resonances, in the presence of multi-scale irregularities, may possibly have on RPI signals. Sounding of irregular plasma structures in the plasmasphere, plasmapause and magnetopause are also discussed.

Fung, Shing F.↗

Particle charge distributions in the effluent of a flow-through atmospheric pressure low temperature plasma

Atmospheric pressure low-temperature plasmas are often utilized to perform particle synthesis, treatment, and removal. It is well-known that dust particles are highly negatively charged in these plasmas; however, little is known about dust particle charging behavior as particles leave the plasma volume and pass through the spatial afterglow region. In this work, monodisperse particles of various sizes and work functions were introduced into an atmospheric pressure radiofrequency capacitively coupled flow-through plasma. Dust particle electrical mobility distributions downstream of the flow-through plasma were measured utilizing a differential mobility analyzer in conjunction with a condensation particle counter at various gas flow velocities. Charge distributions were determined from the measured electrical mobility distributions. Experiments confirm that particles become less negatively charged, and even net-positively charged after leaving the plasma volume, with a distribution that follows a shifted Boltzmann charge distribution. Additionally, particle charge in the effluent of the flow-through plasma is negligibly dependent on work function but highly size and flow velocity dependent. Larger particles were shown to have a higher magnitude of charge under all studied conditions; however, particle polarity was switchable by varying gas flow velocity. The charging dynamics were simulated utilizing a constant number Monte Carlo model that accounts for electron temperature decay and the transition from ambipolar to free diffusion of electrons and ions in the spatial afterglow. Simulation results also suggest that, at the same flow velocity, larger particles obtain a greater magnitude of charge, negative or positive. Furthermore, the decrease in electron mobility and the difference between ion and electron convective loss rates create an ion-rich region in the plasma effluent that promotes ion–particle collisions and drives particle charge removal and even reversal of polarity. Larger particles more favorably collide with energetic species in these environments, which results in higher charge states.

atmospheric pressure low temperature plasma↗

Plasma steering to avoid disruptions in ITER and tokamak power plants

Steering tokamak plasmas is commonly viewed as a way to avoid disruptions and runaway electrons. Plasma steering sounds as safe as driving to work but will be shown to more closely resemble driving at high speed through a dense fog on an icy road. The long time required to terminate an ITER discharge compared to time over which dangers can be foreseen is analogous to driving in a dense fog. Here, the difficulty of regaining plasma control if it is lost resembles driving on an icy road. Disruptions and runaways are associated with three issues—a solution to one tends to complicate the solution to the other two: loss of plasma position control, excessive heat deposition, and wall melting due to runaway electrons. All three risks must be addressed for ITER to achieve its mission and essentially eliminated before tokamak power plants can be deployed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Plasma potential shaping using end-electrodes in the Large Plasma Device

We perform experiments in the Large Plasma Device at the University of California, Los Angeles, studying how different end-electrode biasing schemes modify the radial potential profile in the machine. We impose biasing profiles of different polarities and gradient signs on a set of five concentric electrodes placed 12 m downstream from the plasma source. We find that imposing concave-down profiles (negative potential radial gradient) on the electrodes creates radial potential profiles halfway up the plasma column that are comparable to those imposed on the electrodes and a few electron temperature in height, regardless of the biasing polarity. On the other hand, imposing concave-up profiles (positive potential radial gradient) leads to non-monotonic radial potential profiles. This observation can be explained by the current drawn through the electrodes and the parallel plasma resistivity, highlighting their important role in controlling the rotation of plasma. Concave-down plasma potential profiles, obtained by drawing electrons on the axis, are predicted to drive azimuthal drift velocities that can approach significant fractions of the ion sound speed in the central region of the plasma column.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Three-dimensional measurements of plasma parameters in an inductively coupled plasma processing chamber

Inductively coupled plasmas (ICPs) are extensively used for materials processing and microelectronics fabrication. However, their electromagnetic properties have not been fully characterized. In this regard, we have performed fully three dimensional (3D), time dependent measurements of the magnetic field, electron density, and electron temperature for an ICP sustained in argon in an industrial reactor designed for plasma etching in microelectronics fabrication. These measurements were compared to modeling results. The plasma was generated using pulsed power delivered at 2 MHz by a planar coil. The magnetic field was measured using a three axis magnetic probe at 15 366 locations throughout the plasma volume during the H-mode portion of the pulse at temporal intervals of 2 ns. A swept Langmuir probe was used to measure plasma parameters at the same locations. The plasma density measurement was calibrated with line-integrated densities obtained using a 96 GHz interferometer. During a single radio frequency (RF) cycle, the 3D current density [derived from B(r→,t)]is initially maximum just below the coil and moves downward toward the center of the chamber. Isosurfaces of current are nearly symmetric toroids. The total electric field, space charge field, and inductive electric field were derived and used to calculate the dissipated power, plasma current, and Poynting flux. Computer modeling of the experiment reproduces the phase dependent behavior. Animations showing the time dependent 3D measurements are presented in the supplementary material.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Research and Development to Reduce Impurity Production and Transport of the Impurities to the Target in Linear Plasma Devices Using Helicon Plasma Sources

Linear plasma devices used to test plasma facing materials (PFMs) and components for fusion reactors are often suffering under the production of intrinsic impurities from the plasma source system. Most linear plasma devices use internal electrodes (hollow cathodes, reflex arc, or cascading arc), which typically are the source of the main impurities. The next-generation plasma generators use radio frequency (RF) plasma sources like helicons to avoid internal electrodes. However, high power operation of helicons has proven to result in impurity production due to the high rectified sheath voltages created. Depending on the plasma parameters and magnetic configuration, these impurities can be transported to the target and deposited there to unacceptable high levels. Here, in this contribution, the experimental results from Proto-MPEX are summarized, and the conclusions of the impurity source physics are given. Methods to reduce the impurity production, the impurity transport, and the net deposition on the target are presented. These methods to reduce the impurity production include Faraday screens to reduce the sheath voltage drop, high-Z refractory coatings to reduce the erosion yield, and wall conditioning methods. Methods to reduce the impurity transport include changes in the magnetic configuration as well as electron heating to change axial and radial temperature profiles. Preliminary results on the effectiveness of some of these methods are presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗