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NASA NTRS1992

Airborne Lidar Observations of the Stratosphere After the Pinatubo Eruption

The eruption of Mt. Pinatubo in June 1991 injected the largest mass of gases and ash into the stratosphere observed since lidar and satellite monitoring of the stratosphere became possible in the middle 1960's. Because of early indications of the significance of the eruption, NASA mounted an airborne mission to survey the stratospheric plume soon after the eruption. The NASA Wallops Electra aircraft was outfitted with a depolarization lidar, a correlation spectrometer (for SO2 measurements), a total-direct-diffuse spectral radiometer, and a Fourier transform spectrometer. Six flights were made during the period July 7-14.

Winker, David M.↗
NASA NTRS1992

Two Wavelength Measurements of the Pinatubo Aerosol Above Toronto, Canada

Since March 1991 our group has been routinely operating a Differential Absorption Lidar system in Toronto, Canada. The system is based on a XeCl Excimer laser. We have also been running a Backscatter Lidar based on a NdYAG laser. In the period from March 1991 to March 1992 measurements have been taken during about 40 nights with the DIAL system and more than 90 nights with the NdYAG system. In all measurements after July 21, 1991 we have observed aerosol layers in the stratosphere, resulting from the Mt. Pinatubo eruptions around June 15, 1992. These aerosol layers interfere significantly with many optical remote sensing techniques, and we have been investigating their properties with our two Lidar systems. In this paper we present a summary of these measurements.

Steinbrecht, W.↗
NASA NTRS1992

Correction of DIAL Stratospheric Ozone Measurements in the Presence of Pinatubo Aerosols

NASA Langley's airborne lidar system measured aerosol and ozone distributions in the stratosphere from Jan. - Mar. 1992 as part of the Airborne Arctic Stratospheric expedition (AASE-2). The eruption of Mount Pinatubo in Jun. 1991 has increased the aerosol burden of the stratosphere and thereby increased the importance of applying an aerosol correction to the ozone measurements. The correction relies on a Bernoulli solution to derive a backscatter correction to the differential absorption lidar (DIAL) returns at two wavelengths in the ultraviolet spectral region (lambda(sub on) = 301.5 nm, lambda(sub off) = 310.87 nm) as described in earlier works. This paper discusses how the parameters for the correction were optimized for application to the AASE-2 data set.

Fenn, Marta A.↗
NASA NTRS1992

Lidar Observations of Stratospheric Clouds After Volcanic Eruption of Pinatubo

A very large increase of backscattered light from the stratospheric aerosol layer was observed by using a ruby laser in Beijing (39 degrees 54 minutes N, 116 degrees 27 minutes E) from the end of July 1991 to March 1992. It was concluded that this increase was almost certainly due to the volcanic eruption of Mt. Pinatubo in the Philippines in June 1991. The measuring instruments used are described. Information is given in graphical form for vertical profiles, fluctuation of the maximum backscattering ratio above 20 km during the nine month period, and the time variation of the integrated backscattering coefficient at a height of 15 to 30 km.

Sun, Jinhui↗
NASA NTRS1991

Simulation of the Pinatubo aerosol cloud in general circulation model

The global transport and dispersion of the Pinatubo aerosol cloud are simulated by means of a high-resolution stratospheric version of the NCAR Community Climate Model (CCM2) with an annual cycle. A passive tracer was injected into the model stratosphere over the Philippine Islands on June 15, and the transport was simulated for 180 d using an accurate semi-Lagrangian advection scheme. The simulated volcanic aerosol cloud initially drifted westward and expanded in longitude and latitude. The bulk of the aerosol cloud dispersed zonally to form a continuous belt in longitude, and remained confined to the tropics, centered near the 20-mb level for the entire 180-d model run, although a small amount was transported episodically into the upper troposphere in association with convective disturbances. Aerosol transported to the troposphere was dispersed within a few weeks into the Northern Hemisphere extratropics. In the Southern Hemisphere, the aerosol was mixed into the region equatorward of the core of the polar night jet during the first 50 d, but penetration into southern polar latitudes was delayed until the final warming in November.

Boville, Byron A.↗
NASA NTRS1992

SAGE II measurements of early Pinatubo aerosols

SAGE II satellite measurements of the Mt. Pinatubo eruption cloud in the stratosphere during June, July, and early August 1991 show that aerosols in the tropics reached as high as 29 km altitude with most of the cloud between 20 and 25 km. The most optically thick portions of the cloud covered latitudes from 10 deg S to 30 deg N during the early part of this period. By late July, high stratospheric optical depths were observed to at least 70 deg N, with the high values north of about 30 deg N from layers below 20 km. High pressure systems in both hemispheres were observed to be correlated with the movement of volcanic material at 21 km into the westerly jet stream at high southern latitudes and similarly to high northern latitudes at 16 km. By August, the entire Southern Hemisphere had experienced a 10-fold increase in optical depth relative to early July due to layers above 20 km. Initial mass calculations using SAGE II data place the aerosol produced from this eruption at 20 to 30 megatons, well above the 12 megatons produced by El Chichon.

Mccormick, M. P.↗
NASA NTRS1992

Airborne lidar observations of the Pinatubo volcanic plume

A dual-polarization lidar aboard the NASA Electra aircraft was used in July 1991 to survey the stratospheric plume from the recent Mt. Pinatubo eruption. Many distinct layers were observed, ranging from 17 to 26 km in altitude. Peak scattering ratios of as high as 80 at 532 nm were recorded. Total particle mass of the plume 27 days after the eruption is estimated from these measurements to be on the order of 8 megatonnes, with perhaps half the original SO2 converted to aerosol at that point.

Winker, D. M.↗
NASA NTRS1992

Preliminary analysis of observations of the Pinatubo volcanic plume with a polarization-sensitive lidar

A dual-polarization lidar aboard the NASA Electra aircraft was used in July 1991 to survey the stratospheric plume from the recent Mt. Pinatubo eruption. Both depolarizing and non-depolarizing volcanic layers were observed, ranging from 17 to 26 km in altitude. Differences in the depolarization signatures of the layers indicates differences in the composition or physical state of the particles in the layers.

Winker, D. M.↗
NASA NTRS1992

Airborne observations of SO2, HCl, and O3 in the stratospheric plume of the Pinatubo volcano in July 1991

A high-resolution IR spectrometer aboard the NASA Electra aircraft to measure the total column amount of SO2, O3, and HCl above the aircraft while flying over the Caribbean three weeks after the June 15 eruption of Mt. Pinatubo in the Philippines. South of 20 deg N latitude columns of SO2 were observed ranging from 2.0-3.7 x 10 exp 16 molecules/sq cm. In addition, the column amount of HCl averaged 1.5 x 10 exp 15 molecules/sq cm in the region of the plume. This represents a small increase in HCl above the amount, estimated from the previous measurements, that would have been presented had there been no volcanic eruption, but the increase is substantially less than that seen following the 1982 eruptions of El Chichon.

Mankin, William G.↗
NASA NTRS1992

Mt. Pinatubo SO2 column measurements from Mauna Loa

Absorption features of the nu sub 1 band of SO2 are identified in high-resolution IR solar-absorption spectra recorded from Mauna Loa, Hawaii, on July 9 and 12, 1991, shortly after the arrival of the first eruption plume from the Mt. Pinatubo volcano. A total SO2 vertical column amount of (5.1 +/- 0.5) x 10 exp 16 molecules/sq cm on July 9 is retrieved based on nonlinear least-squares spectral fittings of 9 selected SO2 absorption features with an updated set of SO2 spectral parameters. A SO2 total-column upper limit of 0.9 x 10 exp 16 molecules/sq cm deduced from measurements on September 20-24, 1991, is consistent with the dispersion of the SO2 cloud and the rapid conversion of the SO2 vapor into volcanic aerosol particles.

Goldman, A.↗
NASA NTRS1992

Stratospheric temperature increases due to Pinatubo aerosols

Northern-Hemisphere stratospheric temperatures at 30 and 50 mb beginning in June 1991 are compared with 20-year (1965-1984) and 26-year (1964-1989) monthly means. Significant temperature increases are shown in July, August, September, and October for latitudes from approximately 30 deg N to the equator. In September and October deviations are observed for large areas between the equator and 30 deg N, with temperature increases as high as + 3.5 C occurring at some locations. The monthly averaged zonal mean 30-mb temperatures at 20 deg N in September and October were approximately 2.5 C higher that the 26-year mean, with some daily zonal mean increases of almost 3 C. Higher values occurred equatorward of 20 deg N. These warmings are due to absorption of radiation by the aerosols produced from the June eruptions of the volcano Pinatubo (15.1 deg N, 120.4 deg E) in the Philippines. Stratospheric warmings are expected to be occurring simultaneously at southern latitudes, especially from the equator to about 20 deg S, based on satellite and lidar measurements of the locations of the new aerosol layers. These localized temperature increases should decrease in magnitude and become more global as the cloud disperses globally and spreads in altitude.

Labitzke, K.↗
NASA NTRS1992

Observations of reduced ozone concentrations in the tropical stratosphere after the eruption of Mt. Pinatubo

Two independent sets of data, one of aerosols from an airborne lidar system, and one of ozone from ozonesonde measurements indicate that significant ozone decreases may have happened as a result of the injection of debris by the Mt. Pinatubo volcano in June 1991. The amount of this reduction maximizes at 24-25 km, near the peak of the aerosol distribution, though a deficit is seen throughout the lower stratosphere between 19 and 28 km. The greatest differences observed prior and subsequent to the eruptions at these altitudes is 18-20 percent.

Grant, W. B.↗
NASA NTRS1992

Raman lidar measurements of Pinatubo aerosols over southeastern Kansas during November-December 1991

Raman lidar measurements over southeastern Kansas of stratospheric aerosols produced by the June 1991 eruptions of Mt. Pinatubo were made on 10 nights during November and December 1991. Both aerosol backscattering and extinction profiles were derived simultaneously from the lidar data since this system detects Raman scattering from nitrogen and oxygen as well as the backscattered light from aerosols and molecules. Aerosols scattering ratios greater than 3(at 351 nm) were measured on several nights. Peak aerosol concentrations were located between 19-22 km and varied significantly from night to night. Aerosol extinction/backscatter ratios computed from the lidar data and averaged over the altitude region of enhanced aerosol scattering between 15-25 km varied between 18-28 sr. Mie computations show these values to be consistent with scattering by aerosol particles with mode radii between 0.3 to 0.5 micron and that the ratios would increase to 40-65 sr at 694 nm. Aerosol optical thicknesses derived from the lidar extinction measurements at 351 nm varied between 0.04 and 0.06.

Ferrare, R. A.↗
NASA NTRS1992

Pinatubo eruption winter climate effects: Model versus observations

Large volcanic eruptions, in addition to the well-known effect of producing global cooling for a year or two, have been observed to produce shorter-term responses in the climate system involving non-linear dynamical processes. In this paper, we use the ECHAM2 general circulation model forced with stratospheric aerosols to test some of these ideas. Run in a perpetual-January mode, with tropical stratospheric heating from the volcanic aerosols typical of the 1982 El Chichon eruption or the 1991 Pinatubo eruption, we find a dynamical response with an increased polar night jet in the Northern Hemisphere (NH) and stronger zonal winds which extended down into the troposphere. The Azores High shifts northward with increased tropospheric westerlies at 60N and increased easterlies at 30N. Surface temperatures are higher both in northern Eurasia and North America, in agreement with observations for the NH winters or 1982-83 and 1991-92 as well as the winters following the other 10 largest volcanic eruptions since 1883.

Graf, HANS-F.↗
NASA NTRS1992

Buffering of stratospheric circulation by changing amounts of tropical ozone - A Pinatubo case study

Stratospheric aerosol from Mount Pinatubo heated the tropical lower stratosphere by about 0.3 K/day mainly due to absorption of terrestrial infrared radiation. This heating was dissipated by: (1) an observed increase in stratospheric temperatures, which enhanced the radiation cooling; (2) additional mean upward motion, observed for the aerosol cloud, which led to adiabatic cooling; and (3) reductions in ozone concentrations resulting from enhanced upward motions. Each of these processes operated on a different time scale: maximum temperatures were observed after about 90 days; maximum ozone losses of about -1.5 ppm occurred after 140 days when the enhanced vertical velocities effectively lifted the ozone profile by about 2 km. We believe this shows that ozone plays an important role in buffering vertical motion in the tropical lower stratosphere, and hence the residual Brewer Dobson circulation of the whole stratosphere.

Kinne, S.↗
NASA NTRS1992

Observations of a new SAGE II aerosol extinction mode following the eruption of Mt. Pinatubo

In the aftermath of the eruption of Mt. Pinatubo, multiwavelength stratospheric aerosol extinction measurements by the satellite-borne Stratospheric Aerosol and Gas Experiment (SAGE II) revealed the presence of a previously unobserved mode of aerosol that exhibited high extinction but a small inferred particle size. This mode may represent a transitional phase between the very small aerosol created by gas-to-particle conversion and a quasi-steady state, post-volcanic aerosol that exhibits both large extinction and large particle size. The presence of a transitional small aerosol mode may have a significant impact on chemical and radiative processes in the stratosphere.

Thomason, Larry W.↗
NASA NTRS1993

Tropical ozone loss following the eruption of Mt. Pinatubo

Total Ozone Mapping Spectrometer (TOMS) measurements of equatorial total ozone following the eruption of Mt. Pinatubo show a decrease of up to 6 percent over climatology. Ozone losses begin approximately a month following the eruption, consistent with the time required for the SO2 to convert to sulfuric acid aerosol. The thick aerosol layer interferes with the TOMS retrieval, but this interference is small and easily accounted for in the retrieval. Ozone values remain below climatology until December, 1991. Ozonesonde data from Natal, Brazil taken before and two months after the eruption support TOMS observations of ozone loss. These sondes show that the ozone loss region is confined to a 2-3 km thick layer between 24 and 28 km.

Schoeberl, Mark R.↗
NASA NTRS1993

Radiative climate forcing by the Mount Pinatubo eruption

Radiative flux anomalies derived from the NASA spaceborne Earth Radiation Budget Experiment were used to determine the volcanic radiative forcing that followed the eruption of Mount Pinatubo in June 1991. They are the first unambiguous, direct measurements of large-scale volcanic forcing. The volcanic aerosols caused a strong cooling effect immediately; the amount of cooling increased through September 1991 as shortwave forcing increased relative to the longwave forcing. The primary effects of the aerosols were a direct increase in albedo over mostly clear areas and both direct and indirect increases in the albedo of cloudy areas.

Minnis, P.↗