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At least 73 records · Page 4

Pinatubo and pre-Pinatubo optical-depth spectra: Mauna Loa measurements, comparisons, inferred particle size distributions, radiative effects, and relationship to lidar data

The Ames airborne tracking sunphotometer was operated at the National Oceanic and Atmospheric Administration (NOAA) Mauna Loa Observatory (MLO) in 1991 and 1992 along with the NOAA Climate Monitoring and Diagnostics Laboratory (CMDL) automated tracking sunphotometer and lidar. June 1991 measurements provided calibrations, optical-depth spectra, and intercomparisons under relatively clean conditions; later measurements provided spectra and comparisons for the Pinatubo cloud plus calibration checks. June 1991 results are similar to previous MLO springtime measurements, with midvisible particle optical depth at the near-background level of 0.012 +/- 0.006 and no significant wavelength dependence in the measured range (lambda = 0.38 to 1.06 micrometers). The arrival of the Pinatubo cloud in July 1991 increased midvisible particle optical depth by more than an order of magnitude and changed the spectral shape of to an approximate power law with an exponent of about -1.4. By clearly September 1991, the spectrum was broadly peaked near 0.5 micrometers, and by July 1992, it was peaked near 0.8 micrometers. Our optical-depth spectra include corrections for diffuse light. NOAA- and Ames Research Center (ARC)-measured spectra are in good agreement. Columnar size distributions inverted from the spectra show that the initial (July 1991) post-Pinatubo cloud was relatively rich in small particles (r less than 0.25 micrometers), which were progressively depleted in the August-September 1991 and July 1992 periods. Conversely, both of the later periods had more of the optically efficient medium-sized particles (0.25 less than r less than 1 micrometers) than did the fresh July 1991 cloud. These changes are consistent with particle growth by condensation and coagulation. Photometer-inferred column backscatter values agree with those measured by the CMDL lidar on nearby nights. Combining lidar-measured backscatter profiles with photometer-derived backscatter-to-area ratios gives peak particle areas that could cause rapid heterogeneous loss of ozone, given sufficiently low particle acidity and suitable solar zenith angles (achieved at mid- to high latitudes). Top-of-troposphere radiative forcings for the September 1991 and July 1992 optical depths and size distributions over MLO are about -5 and -3 W/sq m, respectively (hence comparable in magnitude but opposite in sign to the radiative forcing caused by the increase in manmade greenhouse gases since the industrial revolution). Heating rates in the Pinatubo layer over MLO are 0.55 +/- 0.13 and 0.41 +/- 0.14 K/d for September 1991 and July 1992, respectively.

Russell, P. B.↗

Pinatubo and Pre-Pinatubo Optical-Depth Spectra: Mauna Loa Measurements, Comparisons, Inferred Particle Size Distributions, Radiative Effects, and Relationship to Lidar Data

The Ames airborne tracking sunphotometer was operated at the National Oceanic and Atmospheric Administration (NOAA) Mauna Loa Observatory (MLO) in 1991 and 1992 along with the NOAA Climate Monitoring and Diagnostics Laboratory (CMDL) automated tracking sunphotometer and lidar. June 1991 measurements provided calibrations, optical-depth spectra, and intercomparisons under relatively clean conditions; later measurements provided spectra and comparisons for the Pinatubo cloud plus calibration checks. June 1991 results are similar to previous MLO springtime measurements, with midvisible particle optical depth tau(sub p)(lambda = 0.526 microns) at the near-background level of 0.012 +/- 0.006 and no significant wavelength dependence in the measured range (lambda = 0.38 to 1.06 microns). The arrival of the Pinatubo cloud in July 1991 increased midvisible particle optical depth by more than an order of magnitude and changed the spectral shape of tau(sub p)(lambda) to an approximate power law with an exponent of about -1.4. By early September 1991, the spectrum was broadly peaked near 0.5 microns, and by July 1992, it was peaked near 0.8 microns. Our optical-depth spectra include corrections for diffuse light which increase postvolcanic midvisible tau(sub p) values by 1 to 3% (i.e., 0.0015 to 0.0023). NOAA- and Ames Research Center (ARC)-measured spectra are in good agreement. Columnar size distributions inverted from the spectra show that the initial (July 1991) post-Pinatubo cloud was relatively rich in small particles (r less than 0.25 microns), which were progressively depleted in the August-September 1991 and July 1992 periods. Conversely, both of the later periods had more of the optically efficient medium-sized particles (0.25 less than r less than 1 micron) than did the fresh July 1991 cloud. These changes are consistent with particle growth by condensation and coagulation. The effective, or area-weighted, radius increased from 0.22 +/- 0.06 micron in July 1991 to 0.56 +/- 0.12 micron in August-September 1991 and to 0.86 +/- 0.29 micron in July 1992. Corresponding column mass values were 4.8 +/- 0.7, 9.1 +/- 2.7, and 5.5 +/- 2 micro g/sq cm, and corresponding column surface areas were 4.4 +/- 0.5, 2.9 +/- 0.2, and 1.1 +/- 0.1 sq micron/sq cm,. Photometer-inferred column backscatter values agree with those measured by the CMDL lidar on nearby nights. Combining lidar-measured backscatter profiles with photometer-derived backscatter-to-area ratios gives peak particle areas that could cause rapid heterogeneous loss of ozone, given sufficiently low particle acidity and suitable solar zenith angles (achieved at mid- to high latitudes). Top-of-troposphere radiative forcings for the September 1991 and July 1992 optical depths and size distributions over MLO are about -5 and -3 W 1/sq m, respectively (hence comparable in magnitude but opposite in sign to the radiative forcing caused by the increase in manmade greenhouse gases since the industrial revolution). Heating rates in Pinatubo layer over MLO are 0.55 +/- 0.13 and 0.41 +/- 0.14 K/d for September 1991 and July 1992, respectively.

Russell, P. B.↗

Effect of particle size and particle size distribution on physical characteristics, morphology and crystal structure of explosively compacted high-T(sub c) superconductors

A superconductor, of composition Y(Ba,K,Na)2Cu3O(x)/F(y) and a composite of composition Y(Ba,K,Na)2Cu3O(x)/F(y) + Ag, with changing K, Na and F content but a constant silver content (Ag = 10 mass%) was prepared using a single heat treatment. the resulting material was ground in a corundum lined mill, separated to particle size fractions of 0-40 micron, 0-63 micron and 63-900 micron and explosively compacted, using an explosive pressure of 10(exp 4) MPa and a subsequent heat treatment. Best results were obtained with the 63-900 micron fraction of composition Y(Ba(1.95) K(0.01)Cu3O(x)F(0),(05)/Ag: porosity less than 0.01 cu cm/g and current density 2800 A/sq cm at 77K.

Kotsis, I.↗

Particle Size Distributions Obtained Through Unfolding 2D Sections: Towards Accurate Distributions of Nebular Solids in the Allende Meteorite

Size distributions of nebular solids in chondrites suggest an efficient sorting of these early forming objects within the protoplanetary disk. The effect of this sorting has been documented by investigations of modal abundances of CAIs (e.g., [1-4]) and chondrules (e.g., [5-8]). Evidence for aerodynamic sorting in the disk is largely qualitative, and needs to be carefully assessed. It may be a way of concentrating these materials into planetesimal-mass clumps, perhaps 100 fs of ka after they formed. A key parameter is size/density distributions of particles (i.e., chondrules, CAIs, and metal grains), and in particular, whether the radius-density product (rxp) is a better metric for defining the distribution than r alone [9]. There is no consensus between r versus rxp based models. Here we report our initial tests and preliminary results, which when expanded will be used to test the accuracy of current dynamical disk models.

Christoffersen, P. A.↗

Calibrations of phase abundance, composition, and particle size distribution for olivine-orthopyroxene mixtures from reflectance spectra

An analytical method for quantifying the characteristics (phase abundances, phase composition, and grain size) of an olivine-orthopyroxene mixture from reflectance spectra is described. The spectral parameters related to reflectance, wavelength position, and albedo are investigated; the absorption bands for the olivine-orthopyroxene mixture is also studied. Primary calibrations useful for the determination of the olivine-orthopyroxene mixture characteristics are examined.

Cloutis, Edward A.↗

On the Use of the Log-Normal Particle Size Distribution to Characterize Global Rain

Although most parameterizations of the drop size distributions (DSD) use the gamma function, there are several advantages to the log-normal form, particularly if we want to characterize the large scale space-time variability of the DSD and rain rate. The advantages of the distribution are twofold: the logarithm of any moment can be expressed as a linear combination of the individual parameters of the distribution; the parameters of the distribution are approximately normally distributed. Since all radar and rainfall-related parameters can be written approximately as a moment of the DSD, the first property allows us to express the logarithm of any radar/rainfall variable as a linear combination of the individual DSD parameters. Another consequence is that any power law relationship between rain rate, reflectivity factor, specific attenuation or water content can be expressed in terms of the covariance matrix of the DSD parameters. The joint-normal property of the DSD parameters has applications to the description of the space-time variation of rainfall in the sense that any radar-rainfall quantity can be specified by the covariance matrix associated with the DSD parameters at two arbitrary space-time points. As such, the parameterization provides a means by which we can use the spaceborne radar-derived DSD parameters to specify in part the covariance matrices globally. However, since satellite observations have coarse temporal sampling, the specification of the temporal covariance must be derived from ancillary measurements and models. Work is presently underway to determine whether the use of instantaneous rain rate data from the TRMM Precipitation Radar can provide good estimates of the spatial correlation in rain rate from data collected in 5(sup 0)x 5(sup 0) x 1 month space-time boxes. To characterize the temporal characteristics of the DSD parameters, disdrometer data are being used from the Wallops Flight Facility site where as many as 4 disdrometers have been used to acquire data over a 2 km path. These data should help quantify the temporal form of the covariance matrix at this site.

Meneghini, Robert↗

Particle Size Distributions Measured in B757 Engine Plume During EXCAVATE

A ground-based test, the Experiment to Characterize Aircraft Volatile Aerosols and Trace Species Emissions (EXCAVATE), was conducted at NASA Langley Research Center, January 26 - 27, 2002, with a Boeing 757 aircraft. The aircraft was anchored on a tarmac and two probes were positioned downstream of the right-side engine, a Rolls Royce RB211-585. One probe was designed and fabricated by Arnold Engineering Development Center (AEDC) and had a 45.6 mm (1.794 in.) ID. A second probe, constructed of 6.4 mm (0.25 in.) stainless-steel tubing at NASA Langley Research Center, had a 6 mm (0.22 in.) ID. The engine was run on JP-5 with three different sulfur concentrations, 810 ppm, 1050 ppm, 1820 ppm; and was operated over a range of power settings from idle to near-full power. Particulate size-distributions and concentrations were measured at four downstream axial locations: 1 m and 10 m with the AEDC particulate probe, and 25 m and 35 m with the Langley probe. Fuel with various sulfur contents was tested to address the long-standing question of the role of sulfur in the formation of volatile species. Several experimental and modeling studies have shown a correlation between fuel sulfur-content and particulate-emissions. The object of EXCAVATE was to further study the effect of sulfur content on particulate number concentration and size-distribution as a function of location in the engine plume and engine operating conditions.

Sanders, Terry↗

Exploring the Climatic Impact of Bi-Modal Dust Particle Size Distributions During the MY34/2018 Global Dust Storm with the NASA Ames Mars Global Climate Model.

We have implemented a bi-modal dust lifting scheme in the NASA Ames Mars Global Climate Model (GCM) and investigated the climatic impact on the MY34/2018 Global Dust Storm (GDS). We found that the climate is measurably responsive to the inclusion of a second, smaller dust mode. Dust tends to be lifted through a deeper column in the atmosphere, which is reflected in the climate as changes to atmospheric temperature, tide amplitudes, and surface temperatures. Adding a modest fraction of a smaller dust mode improves simulations during the GDS compared to Curiosity semi-diurnal tide observations as well as Mars Climate Sounder (MCS) T15 brightness temperatures

R A Urata↗