Pulsed Optically Pumped Magnetometry with Spin-Squeezing for Remote Monitoring
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Schwindt, Peter [Sandia National Laboratories (SNL↗
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Anisotropic ultrahigh gain emission observed in rotational transitions in optically pumped HF gas.
Gain and laser oscillations are obtained on rotational transitions of the first excited vibrational state of HF gas at room temperature, resonantly pumped by the 2.7-micron lines of a pulsed HF laser. Pumping the P-branch transitions connecting the ground and first excited vibrational states produces gain at the coupled rotational transitions at 36, 42, 51, 63, 84, and 126 microns. The gain exhibits directional properties characteristic of a unidirectional amplifier predicted by a recent theory. The incremental gains of these lines are very large, in excess of 1/cm, and the lines oscillate easily without mirrors (superradiance).
Skribanowitz, N.↗
Laser head for simultaneous optical pumping of several dye lasers
The invention is a laser head for simultaneous pumping several dye lasers with a single flash lamp. The laser head includes primarily a multi-elliptical cylinder cavity with a single flash lamp placed along the common focal axis of the cavity and with capillary tube dye cells placed along each of the other focal axes of the cavity. The inside surface of the cavity is polished. Hence, the single flash lamp supplies the energy to the several dye cells.
Mumola, P. B.↗
Stark effect applicable to optically pumped far-infrared laser
Absorption measurements at CO2 laser frequencies were carried out as a function of Stark fields and CH3OH gas pressures to assess the effect of low electric field Stark tuning on methanol absorption at the P(12) 9.4 micron CO2 laser line, in a continuing search for coherent emitters at submillimeter wavelengths (far infrared). The line center absorption coefficient is found to increase five-fold with a 2.3 kV/cm Stark field at the 220 mtorr methanol pressure optimal for methanol far infrared lasing. The low electric field Stark tuning encourages efforts to enhance the pumping efficiency of a methanol far infrared laser at its normal optimum operating pressure, and suggests that significant Stark field induced frequency modulation of the far IR laser output is feasible.
Claspy, P. C.↗
Approximate analytic solutions for the optical pumping of fluorescent dyes
A general technique for solving a system of rate equations describing the interaction of an electromagnetic field and a molecular system is presented. The method is used to obtain approximate time-dependent solutions for the upper-level population of fluorescent dyes in the presence of a pump field.
Lawandy, N. M.↗
Analysis and design of optically pumped far infrared oscillators and amplifiers
A waveguide laser oscillator was designed and experimental measurements made of relationships among output power, pressure, pump power, pump frequency, cavity tuning, output beam pattern, and cavity mirror properties for various active gases. A waveguide regenerative amplifier was designed and gain measurements were made for various active gases. An external Fabry-Perot interferometer was fabricated and used for accurate wavelength determination and for measurements of the refractive indices of solids transparent in the far infrared. An electronic system was designed and constructed to provide an appropriate error signal for use in feedback control of pump frequency. Pump feedback from the FIR laser was decoupled using a vibrating mirror to phase modulate the pump signal.
Galantowicz, T. A.↗
Semiclassical approach to collision-induced emission in the presence of intense laser radiation - An aspect in the study of cooperative chemical and optical pumping
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Lam, K.-S.↗
Approximate analytic solutions for the optical pumping of fluorescent dyes
A general technique for solving a system of rate equations describing the interaction of an electromagnetic field and a molecular system is presented. The method is used to obtain approximate time-dependent solutions for the upper-level populations of fluorescent dyes in the presence of a pump field.
Lawandy, N. M.↗
Temperature dependence of optically pumped far-infrared /FIR/ laser output power
The temperature dependence of the small signal gain and saturation power are derived using temperature-dependent rates in a four-level model. An expression is developed for the output power of a far-infrared oscillator as a function of temperature for both fixed pressure and fixed density. The results are valid in the regime of homogeneous broadening of the rotational transition and Doppler broadening of the pump transition. It is shown that, for most lasers, both the small signal gain and the saturation power decrease with increasing temperature. These effects have the overall result of increasing output power with decreasing temperatures.
Lawandy, N. M.↗
Optically pumped carbon dioxide laser mixtures
This work explores the concept of blackbody radiation pumping of CO2 gas as a step toward utilization of solar radiation as a pumping source for laser action. To demonstrate this concept, an experiment was performed in which laser gas mixtures were exposed to 1500 K thermal radiation for brief periods of time. A gain of 2.8 x 10 to the -3rd reciprocal centimeters has been measured at 10.6 microns in a CO2-He gas mixture of 1 Torr pressure. A simple analytical model is used to describe the rate of change of energy of the vibrational modes of CO2 and to predict the gain. Agreement between the prediction and experiment is good.
Yesil, O.↗
Broad-band gain in optically pumped S2
The broad fluorescence spectrum and Franck-Condon shift of the B-X system of S2 are exploited in broad-band-gain experiments using the absorption of 308-nm XeCl excimer radiation to pump the level (upsilon-prime = 4) in an S2 vapor with and without Ar. The fluorescence spectra are examined to determine the effects of gas collisions, and the intense near-UV and visible bands are attributed to the redistribution of the population among the upsilon-prime levels resulting from S2-Ar collisions. Broad-band gain is observed on the rare-gas relaxation bands (2,17) (about 475 nm) and (3,18) (480 nm), while absorption is found in the (0,6), (0,7), and (0,8) near-UV (about 360-380-nm) bands where a transient population cascading down the X-state manifold fills the lower levels. It is inferred from the achievement of gain over much of the S2 fluorescence bandwidth that nonselective pumping mechanisms like discharges, solar energy, or flashlamps can be used with S2 as the tunable, chemically stable 'dye'.
Epler, J. E.↗
Coupled Lorenz systems in an optically pumped CH3F laser
The output emission of a short CH3F metallic waveguide laser pumped by an injection-locked CO2 transversely excited atmosphere laser is studied experimentally. The output is found to be extremely unpredictable when lasing occurs in both the excited and ground vibrational states on two separate transitions (496 and 452 microns, respectively). The dynamics and sensitivity to initial conditions are explained in terms of two Lorenz lasers with pump coupled population inversions.
Rabinovich, W. S.↗
A stable, high power optically pumped far infrared laser system
The generation of 1.25 watts of CW laser power at the 119-micron (2522.8 GHz) methanol line is reported. The maximum frequency fluctuation of the free running laser is less than + or - 100 kHz per hour. This laser has also been tested on numerous other lines ranging from 403.7 GHz (HCOOH) to 5260 GHz (CH3OD) with improved power and stability.
Farhoomand, Jam↗
Nd:LNA laser optical pumping of He-4 - Application to space magnetometers
Results obtained from laser pumping in a helium magnetometer sensor, using a tunable Nd:LNA laser pumped with a high-power diode laser, are reported. It is shown that it was possible to observe both the Hanle signals and the n = 0, p = 1 parametric resonance by monitoring the pumping radiation passing through the cell. As the diode laser-pumped Nd:LNA laser was tuned through the D0, D1, and D2 transitions, three distinct resonance signals were produced. A comparison of the slope of lamp-pumped signals and laser-pumped D1 signals showed that, under otherwise identical conditions, the slope of the D1 laser signal was 45 times greater than the lamp-pumped signal.
Slocum, R. E.↗
An investigation of a mathematical model of an optically pumped Ti(3+):Al2O3 laser system
During the last several years, solid state lasers were developed that have the potential for meeting rigorous performance requirements for space-based remote sensing of the atmosphere. In order to design a stable and efficient laser and to understand the effect on laser output of changes in the physical and design parameters, an understanding of the development of the dynamical processes of the laser is necessary. Typically, the dynamical processes in a laser system are investigated via rate equations describing the evolution of the occupancy in the electronic levels and of the photon density in the laser cavity. There are two approaches to this type of study. Most often, for the sake of simplicity, the spatial variations of the dynamic variables in the laser system are disregarded and the mathematical model consists of a system of first order nonlinear ordinary differential equations (ODE). The second approach is to take into account both spatial and temporal variations in the dynamic variables in the laser cavity. The resulting model consists of a first order semilinear system of partial differential equations (PDE). The model which was studied was studied was generic in the sense that it was a four-level laser system, but the parameters used in the numerical study were specific to Titanium-doped sapphire. For simplicity, a constant, spatially uniform pumping scheme was considered. In addition, a simplification of the model was made so that it treats a single lasing wavelength with a narrow bandwidth. The purpose was to investigate both versions of the mathematical model and to determine whether the numerical solutions are similar both qualitatively and quantitatively. The systems of ordinary differential equations were solved numerically using a Runge-Kutta-Fehlberg algorithm which was very efficient for typical values of the physical parameters. A numerical scheme, based on the Modified Euler method, for computing solutions to the system of partial differential equations was developed and implemented. The PDE model was solved numerically at the expense of greatly increased computer time.
Roberts, Lila F.↗
Computing Temperatures In Optically Pumped Laser Rods
Computer program presents new model solving temperature-distribution problem for laser rods of finite length and calculates both radial and axial components of temperature distributions in these rods. Contains several self-checking schemes to prevent over-writing of memory blocks and to provide simple tracing of information in case of trouble. Written in Microsoft FORTRAN 77.
Farrukh, Usamah O.↗
Actively Pumped Optical Filters at 532 nm
The operation of two narrow-band optical filters at 532.33 nm is presented. Both of these filters operate on the 4P(sub 1/2) to 8S(sub 1/2) excited-state transition in potassium vapor. One of the filters is based on excited-state Faraday effect, and requires the application of an external axial magnetic field. The peak transmission of this filter is approximately 3.5% with a linewidth of less than 10 GHz. The second filter does not require a magnetic field for its operation, but readily attains peak transmissions of 25-30%. The 4P(sub 1/2) state is excited by a 769.9 nm light pulse which is linearly polarized for the first scheme and circularly polarized for the second.
Billmers, Richard I.↗