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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
NASA NTRS2011

Active Neutron and Gamma-Ray Instrumentation for In Situ Planetary Science Applications

We describe the development of an instrument capable of detailed in situ bulk geochemical analysis of the surface of planets, moons, asteroids, and comets. This instrument technology uses a pulsed neutron generator to excite the solid materials of a planet and measures the resulting neutron and gamma-ray emission with its detector system. These time-resolved neutron and gamma-ray data provide detailed information about the bulk elemental composition, chemical context, and density distribution of the soil within 50 cm of the surface. While active neutron scattering and neutron-induced gamma-ray techniques have been used extensively for terrestrial nuclear well logging applications, our goal is to apply these techniques to surface instruments for use on any solid solar system body. As described, experiments at NASA Goddard Space Flight Center use a prototype neutron-induced gamma-ray instrument and the resulting data presented show the promise of this technique for becoming a versatile, robust, workhorse technology for planetary science, and exploration of any of the solid bodies in the solar system. The detection of neutrons at the surface also provides useful information about the material. This paper focuses on the data provided by the gamma-ray detector.

Parsons, A.↗
DOE OSTI2024

Absolute Neutron Rate Measurement and Non-Thermal/Thermonuclear Fusion Differentiation

The goal of fusion energy is to produce significantly more energy from fusion reactions than is input into the device. One of the products of fusion reactions is neutrons, which, due to their lack of charge, provide a unique view into the parameters of the device. Lawrence Livermore National Laboratory (LLNL) in collaboration with the University of California, Berkeley (UCB) have designed, assembled, and fielded a robust and portable neutron detection system known as PANDA (Portable and Adaptable Neutron Diagnostics for ARPA-E). This detector suite consists of three LaBr activation detectors that are calibrated to give a total neutron yield on shot, and twenty-four scintillators coupled to photo-multiplier tubes (SPMT). The SPMTs can be configured to attain spatial, temporal and/or energy information from fusion neutrons. The system was designed to be portable and is compartmentalized so that individual components can be used at different fusion facilities. During the duration of this work, part of the system was installed at the FuZE facility, a part of Zap Energy. Another component was installed that the CESZAR facility at the University of California, San Diego (UCSD) to support experiments by Magneto-Inertial Fusion Technologies, Inc. (MIFTI). The diagnostics were successful at both locations and the LLNL/UCB team supported the data analysis by creating and running analysis scripts and Monte-Carlo calculations. At Zap Energy the diagnostics demonstrated that the fusion from the FuZE device is thermonuclear in nature, a result that resulted in an invited talk at the American Physical Society Division of Plasma Physics and an invited paper. Additionally, temporal and spatial data was taken using the SPMTs to understand the duration and length of fusion production. At UCSD the neutron yield from the diagnostics was used to show improvements to fusion yields on their gas puff Z-pinch when using a gas shell surrounding the fuel. The success in this diagnostic has led to continued work at both Zap Energy and MIFTI, as well as follow on funding and interest at other fusion energy companies.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS2005

Method for Determination of Less Than 5 ppm Oxygen in Sodium Samples

Alkali metals used in pumped loops or heat pipes must be sufficiently free of nonmetallic impurities to ensure long heat rejection system life. Life issues are well established for alkali metal systems. Impurities can form ternary compounds between the container and working fluid, leading to corrosion. This Technical Memorandum discusses the consequences of impurities and candidate measurement techniques to determine whether impurities have been reduced to suf.ciently low levels within a single-phase liquid metal loop or a closed two-phase heat transfer system, such as a heat pipe. These techniques include the vanadium wire equilibration, neutron activation analysis, plug traps, distillation, and chemical analysis. Conceptual procedures for performing vanadium wire equilibration purity measurements on sodium contained in a heat pipe are discussed in detail.

Reid, R. S.↗
DOE OSTI2024

Detection of uranium-photofission neutrons with a 4 He scintillation detector

The use of photon active interrogation to detect special nuclear material has held significant theoretical promise, as the interrogating source particles, photons, are fundamentally different from one of the main signatures of special nuclear material: neutrons produced in nuclear fission. However, neutrons produced by photonuclear reactions in the accelerator target, collimator, and environment can obscure the fission neutron signal. These (γ, n) neutrons could be discriminated from fission neutrons by their energy spectrum, but common detectors sensitive to the neutron spectrum, like organic scintillators, are typically hampered by the intense photon background characteristic of photon-based active interrogation. In contrast, high-pressure 4 ⁢He-based scintillation detectors are well-suited to photon active interrogation, as they are similarly sensitive to fast neutrons and can measure their spectrum, but show little response to gamma rays. Here, in this work, a photon active interrogation system utilizing a 4 ⁢He scintillation detector and a 9 MeV linac-bremsstrahlung x-ray source was experimentally evaluated. The detector was shown to be capable of operating in intense gamma-ray environments and detecting photofission neutrons from 238 ⁢U when interrogated by this x-ray source. The photofission neutrons show clear spectral separation from (γ, n) neutrons produced in lead, a common shielding material.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

The UCLA Cosmochemistry Database

Abstract The UCLA Cosmochemistry Database was initiated as part of a data-rescue and -storage project aimed at archiving a variety of cosmochemical data acquired at University of California, Los Angeles (UCLA). The data collection includes elemental compositions of extraterrestrial materials analyzed by UCLA cosmochemists over the last five decades. The analytical techniques include atomic absorption spectrometry (AAS) and neutron activation analysis (NAA) at UCLA. The data collection is stored on the Astromaterials Data System (Astromat). We provide both interactive tables and downloadable datasheets for users to access all data. The UCLA Cosmochemistry Database archives cosmochemical data that are essential tools for increasing our understanding of the nature and origin of extraterrestrial materials. Future studies can reference the data collection in the examination, analysis, and classification of newly acquired extraterrestrial samples.

Science & Technology - Other Topics↗
NASA NTRS2023

The UCLA Cosmochemistry Database

The UCLA Cosmochemistry Database was initiated as part of a data-rescue and -storage project aimed at archiving a variety of cosmochemical data acquired at University of California, Los Angeles (UCLA). The data collection includes elemental compositions of extraterrestrial materials analyzed by UCLA cosmochemists over the last five decades. The analytical techniques include atomic absorption spectrometry (AAS) and neutron activation analysis (NAA) at UCLA. The data collection is stored on the Astromaterials Data System (Astromat). We provide both interactive tables and downloadable datasheets for users to access all data. The UCLA Cosmochemistry Database archives cosmochemical data that are essential tools for increasing our understanding of the nature and origin of extraterrestrial materials. Future studies can reference the data collection in the examination, analysis, and classification of newly acquired extraterrestrial samples.

Bidong Zhang↗
NASA NTRS2001

Integration of Lunar Polar Remote-Sensing Data Sets: Evidence for Ice at the Lunar South Pole

In order to investigate the feasibility of ice deposits at the lunar south pole, we have integrated all relevant lunar polar data sets. These include illumination data, Arecibo ground-based monostatic radar data, newly processed Clementine bistatic radar data, and Lunar Prospector neutron spectrometer measurements. The possibility that the lunar poles harbor ice deposits has important implications not only as a natural resource for future human lunar activity but also as a record of inner solar system volatiles (e.g., comets and asteroids) over the past billion years or more. We find that the epithermal neutron flux anomalies, measured by Lunar Prospector, are coincident with permanently shadowed regions at the lunar south pole, particularly those associated with Shackleton crater. Furthermore, these areas also correlate with the beta=0 circular polarization ratio (CPR) enhancements revealed by new processing of Clementine bistatic radar echoes, which in turn are colocated with areas of anomalous high CPR observed by Arecibo Observatory on the lower, Sun-shadowed wall of Shackleton crater. Estimates of the extent of high CPR from Arecibo Observatory and Clementine bistatic radar data independently suggest that approximately 10 square kilometers of ice may be present on the inner Earth-facing wall of Shackleton crater. None of the experiments that obtained the data presented here were ideally suited for definitively identifying ice in lunar polar regions. By assessing the relative merits of all available data, we find that it is plausible that ice does occur in cold traps at the lunar south pole and that future missions with instruments specifically designed to investigate these anomalies are worthy.

Nozette, Stewart↗
DOE OSTI2023

Fission product yields from the 238 U ( n,f ) reaction at E n = 4.6 MeV

Here, we present cumulative fission product yields from the 238 U (n, f) reaction at an incident energy of 4.6 MeV for fission products with half-lives from less than one second to several hours. We employed direct γ-ray spectroscopy to measure unseparated fission products with a conventional neutron activation analysis and a cyclic activation technique using the RApid Belt-driven Irradiated Target Transfer System (RABITTS). Yields were determined for 78 isotopes and isomers, covering the mass range 84 ≤ A ≤ 148 and the charge range from 33(As) ≤ Z ≤ 58(Ce). Our experimental cumulative yields are compared to the literature and evaluated data at E n ≈0.5 MeV from ENDF/B-VIII.0 and JEFF-3.3 libraries and with theoretical models using the GEF and FREYA codes at E n =4.6 MeV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS1977

Test of a model for trace element partition during closed-system solidification of a silicate liquid

Trace-element concentrations in separated minerals and rock fragments from a coarsely crushed and sieved sample of medium-grained lunar basalt are determined by high-precision instrumental neutron activation analysis for three main purposes. These are: (1) to test a previously proposed model for describing trace-element behavior during solidification of a silicate liquid under conditions of a closed system; (2) to compare trace-element concentrations among different size fractions of a comminuted basalt; and (3) to investigate small-scale heterogeneity within a single medium-grained basalt. It is found that an excellent mass balance for the whole rock is attained in terms of the trace-element concentrations of the component minerals and mesostasis, that the mixing model describing this mass balance yields a superior modal analysis for the whole rock, and that different size fractions of the coarsely crushed basalt vary in mineral composition. The closed-system model is shown to account properly for the average behavior of the trace elements during solidification of the basalt, and values of distribution coefficients are obtained for incompatible elements in that rock.

Haskin, L. A.↗
NASA NTRS1995

The Dripping Handrail Model: Transient Chaos in Accretion Systems

We define and study a simple dynamical model for accretion systems, the "dripping handrail" (DHR). The time evolution of this spatially extended system is a mixture of periodic and apparently random (but actually deterministic) behavior. The nature of this mixture depends on the values of its physical parameters - the accretion rate, diffusion coefficient, and density threshold. The aperiodic component is a special kind of deterministic chaos called transient chaos. The model can simultaneously exhibit both the quasiperiodic oscillations (QPO) and very low frequency noise (VLFN) that characterize the power spectra of fluctuations of several classes of accretion systems in astronomy. For this reason, our model may be relevant to many such astrophysical systems, including binary stars with accretion onto a compact object - white dwarf, neutron star, or black hole - as well as active galactic nuclei. We describe the systematics of the DHR's temporal behavior, by exploring its physical parameter space using several diagnostics: power spectra, wavelet "scalegrams," and Lyapunov exponents. In addition, we note that for large accretion rates the DHR has periodic modes; the effective pulse shapes for these modes - evaluated by folding the time series at the known period - bear a resemblance to the similarly- determined shapes for some x-ray pulsars. The pulsing observed in some of these systems may be such periodic-mode accretion, and not due to pure rotation as in the standard pulsar model.

Young, Karl↗
DOE OSTI2025

Burnup Monitoring for Pebble Bed Reactor Systems

A pebble burnup monitoring system is a required component for domestic reactor safety and safeguards applications associated with pebble bed reactors (PBRs). One of the main requirements of a PBR burnup monitoring system is that it needs to be capable of rapid measurements to assess the burnup of each individual pebble to determine whether to recirculate it in the reactor or discard it as spent fuel. This report considers three different approaches for a burnup monitoring system for pebbles discharged from the reactor core in a pebble bed modular reactor-400: • passive gamma spectrometry measurement, • passive neutron coincidence measurement, and • active neutron counter based on the differential die-away technique. Conceptual designs have been created for each of these detectors, and preliminary analysis has been performed using Monte Carlo N-Particle and Oak Ridge Isotope Generation code simulations. The advantages and practical limitations (e.g., high radiation background) of each system were identified. Simulations suggest that each of the three measurement techniques can be successfully employed to distinguish between pebbles based on their number of passes through the core and to quantify the burnup of pebbles.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2021

Development of a versatile, high-temperature, high-throughput ion irradiation system

We report ion irradiation has long been used as a surrogate for neutron irradiation experiments which are comparatively slower, more expensive, and often can leave materials activated and difficult to handle post-irradiation. However, with the growing use of combinatorial synthesis methods and high-throughput, automated characterization techniques, ion irradiation facilities will need to upgrade their capabilities to be able to accommodate these new material platforms. To address this challenge, a high-throughput ion irradiation system has been developed at the University of Wisconsin-Madison Ion Beam Laboratory (IBL). The system is capable of accommodating large sample arrays of arbitrary geometries and heat samples individually using an infrared laser to enable high-temperature, high-throughput ion irradiation while mitigating the risk of annealing the irradiation damage in nearby samples. To control stage motion, laser power, and beam current measurement, among other tasks, the program Chronos was developed which enables automated high-throughput irradiation experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Analysis of Second Target Station Target Removal Dose Rates

The Second Target Station (STS) project at Oak Ridge National Laboratory’s spallation neutron source is a crucial initiative for maintaining U.S. leadership in neutron sciences. The STS aims to create the world’s brightest pulsed cold neutron source, enabling cutting-edge research across various scientific disciplines. To ensure safe and efficient maintenance operations, understanding the effects of shutdown dose rates from activated components within the STS target systems is essential. This study establishes a computational framework for calculating decay gamma sources and subsequent shutdown dose rates utilizing advanced methods to account for all activation channels, including high-energy interactions down to thermal neutron capture. This study describes a novel integration of multiple tools and provides an effective means of analyzing activation and shutdown dose rates at spallation neutron facilities. A custom-developed script automates the decay gamma source generation process, ensuring proper sampling during the variance reduction phase, which is critical for accurate predictions of shutdown dose rates.

Transmutation↗
NASA NTRS1981

Pulsar disk systems

It is proposed that radio pulsars have the same basic physical features as X-ray pulsars. Specifically, it is suggested that active radio pulsars are rotating neutron stars surrounded by fossil disks left over from the collapse event and that energy is extracted from the rotation of the neutron star by interaction with the disk to produce pulsar luminosity. Attention is given to a model in which the neutron star acts as a unipolar generator (or Faraday disk dynamo) and the disk acts as a load. The self-excitation of the disk/pulsar system is considered along with aspects of disk persistence, pulsed emission, and magnetically field aligned currents to the disk. An investigation is conducted regarding the possibility of a deposition of material in the form of a disk about a pulsar, taking into account questions concerning disk survival. It is found that there are some promising features regarding a disk system.

Michel, F. C.↗
NASA NTRS1976

The abundances of zirconium and hafnium in the solar system

The concentrations of zirconium and hafnium have been determined in the Orgueil, Murchison, Allende, Bruderheim, and Alais meteorites by radiochemical neutron activation analysis. The mean Zr/Hf weight ratio in the first four of these meteorites is 31.3 (plus or minus 2.2), indicating no major fractionation of Zr from Hf. Alais contains anomalously high amounts of many refractory lithophile elements, including Zr and Hf. Orgueil contains 3.1 ppm Zr and 0.11 ppm Hf, corresponding to 9.0 and 0.16 atoms, respectively, relative to 1 million Si atoms.

Ganapathy, R.↗
DOE OSTI2024

Towards the Development of Molten Salt Reactor Multiphysics Modeling Capabilities: Depletion, Thermochemistry, Reactor Dynamics, and Species Tracking

This report documents the simulation and modeling work performed under the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program, utilizing the tools and codes developed under the program. The focus in this Fiscal Year (FY) is on the depletion, thermochemistry, reactor dynamics, and species transport in MSRs. The fission products travelling in the entire primary loop is unique in MSRs. There are many physical/chemical mechanisms that can significantly affect the fission products concentration in the fuel salt, e.g., diffusion into gas bubbles, diffusion in the core moderators, deposition on the surface of structures/pipes, etc. The fission product concentration in the fuel salt can potentially affect the neutronics, system dynamics, chemical potentials, etc., so accurately predicting the fission products distribution in the primary loop is important. Under the main objective, different activities are pursued to assess the NEAMS tools applicability for a variety of areas on species transport, including the depletion analyses using Griffin (fission product source), the redox potential assessment at different depletion points, the assessment of xenon transport effect on the neutronics and reactor dynamics, a survey of correlations for calculating the mass transfer coefficient of different fission products, etc.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2020

Verification of Special Nuclear Material (SNM) using Active Well Coincidence Counter (AWCC) and a High Purity Germanium (HPGe) Detector

SNM verification can be accomplished via two methods i.e. destructive analysis (DA) or nondestructive analysis (NDA). The DA modes are much more accurate compared to NDA modes; nevertheless, the sample's physical integrity is destroyed in the process. Techniques such as ICP-MS, ID-ICP-MS, TI-MS are few examples of DA, where a bulk material is ground and mixed with a solution (some form of acid) to acquire a homogenous sample. In contrast, NDA modes utilize signals emitted by the sample such as gamma, neutrons, light, or heat to analyze samples under investigation. HPGe detectors are some of the most frequently used gamma detectors to assay SNM. However, in a high activity scenario it provides a large uncertainty and sometimes becomes unfeasible to measure low energy gamma rays. Meanwhile, neutron detectors are not affected by the gamma background, therefore they can be used in addition to the gamma detectors to verify total fissile mass ({sup 235}U + {sup 239}Pu) of SNM. The AWCC is one of the thermal neutron NDA systems developed at the Los Alamos National Laboratory (LANL). It consists of 42 {sup 3}He detectors to measure gross neutrons (singles), coincidence neutrons (doubles), higher order multiplicity counting (triples, quadruples, etc.). It can effectively operate in both active and passive neutron interrogation modes. It can utilize AmLi, AmBe, or {sup 252}Cf active interrogation neutron sources. It is used to verify declared fissile mass ({sup 235}U or {sup 239}Pu) present in SNM. Objectives: Calibrate HPGe and AWCC for lightly irradiated (with enough {sup 137}Cs gamma background) ∼93% enriched HEU fuels; Verify fissile mass ({sup 235}U +{sup 239}Pu) content using AWCC and HPGe; Model and benchmark AWCC in MCNP6. Neutron coincidence and multiplicity counting: Two or more neutrons are coincident if they are detected by the system within the specified gate window; In AWCC: Gate window is 128 μsec; Induced fission in fissile material such as {sup 235}U and {sup 239}Pu - emission of time correlated neutrons - Singles, Doubles, Triples, or Quadruples; No induced fission in non-fissile materials- no correlated neutrons - only singles. SNM can be verified with high accuracy and precision using gamma and neutron NDA instruments such as HPGe and AWCC. Interaction with thermal neutrons. Non-fissile atoms - do not emit correlated neutrons. Fissile atoms - emit correlated neutrons during induced fission events. The time correlated neutrons can be detected by using coincidence or multiplicity counters such as AWCC. Likewise, {sup 235}U produces 186 keV gamma peak that can be measured by a HPGe gamma detector. Counts under 186 keV gamma peak provide information about {sup 235}U content. Combining AWCC and HPGe results can provide better understanding of special nuclear material under investigation.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2025

Real-Space Local Dynamics in 1,2,3-Triazole Using Inelastic Neutron Scattering

Enhancing proton transport in polymer electrolytes is crucial for advancing next-generation solid-state batteries, yet our understanding of proton conductivity in nonaqueous environments remains limited due to a lack of atomic-scale insights. Here, in this study, we investigated the atomic-scale dynamics of 1,2,3-triazole, a small molecule capable of dynamic hydrogen bonding, as a model system for proton hopping in nonaqueous environments. Using the real-space correlation function determined by the double Fourier transformation of inelastic neutron scattering spectra, we identified that the self-motion of protons and intermolecular dynamics occur on comparable time scales. Furthermore, we observed that the activation energy associated with the intermolecular dynamics matches the energy barrier for molecular rotations determined through Density Functional Theory calculations. These findings underscore the importance of controlling molecular dynamics at the atomic scale to control proton transport. Additionally, we demonstrated that intermolecular dynamics in systems involving protons can be studied using inelastic neutron scattering even without deuteration, thereby providing a broader avenue for studying atomic-scale dynamics in soft matter systems.

Shinohara, Yuya [Oak Ridge National Laboratory (OR↗