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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
NASA NTRS2016

In Situ Measurement of Atmospheric Krypton and Xenon on Mars with Mars Science Laboratory

Mars Science Laboratorys Sample Analysis at Mars (SAM) investigation has measured all of the stable isotopes of the heavy noble gases krypton and xenon in the martian atmosphere, in situ, from the Curiosity Rover at Gale Crater, Mars. Previous knowledge of martian atmospheric krypton and xenon isotope ratios has been based upon a combination of the Viking missions krypton and xenon detections and measurements of noble gas isotope ratios in martian meteorites. However, the meteorite measurements reveal an impure mixture of atmospheric, mantle, and spallation contributions. The xenon and krypton isotopic measurements reported here include the complete set of stable isotopes, unmeasured by Viking. The new results generally agree with Mars meteorite measurements but also provide a unique opportunity to identify various non-atmospheric heavy noble gas components in the meteorites. Kr isotopic measurements define a solar-like atmospheric composition, but deviating from the solar wind pattern at 80Kr and 82Kr in a manner consistent with contributions originating from neutron capture in Br. The Xe measurements suggest an intriguing possibility that isotopes lighter than 132Xe have been enriched to varying degrees by spallation and neutron capture products degassed to the atmosphere from the regolith, and a model is constructed to explore this possibility. Such a spallation component, however, is not apparent in atmospheric Xe trapped in the glassy phases of martian meteorites.

Conrad, P. G.↗
NASA NTRS1993

Evidence for a spatially extended component of gamma rays from solar flares

We present gamma-ray measurements of a large solar flare that occurred beyond the western solar limb on September 29, 1989. The gamma-ray spectrum shows a neutron capture line which is much stronger than predicted by limb-darkening curves that fit the measurements for flares on the visible hemisphere. We show that this strong neutron capture line can be explained if, in addition to the compact impulsive phase component that normally dominates the total fluence, there is a spatially extended component. For the September 29, 1989 flare we find that such a spatially extended region must subtend more than about 30 deg on the solar surface. We suggest that the extended component could be powered by particles that diffuse from a compact impulsive region or by particles that diffuse into the lower solar atmosphere from a large-scale acceleration site.

Vestrand, W. T.↗
NASA NTRS2003

Cautionary Notes on Cosmogenic W-182 and Other Nuclei in Lunar Samples

Leya et al. (2000) showed that neutron capture on Ta-181 results in a production rate of Ta-182 (decays with a half-life of 114 days to W-182) sufficiently high to cause significant shifts in W-182 abundances considering the neutron fluences due to the cosmic ray cascade that were known to occur near the lunar surface. Leya et al. concluded that this cosmogenic production of W-182 may explain the large positive epsilon(sub W-182) values that Lee et al. (1997) had reported in some lunar samples rather than being produced from decay of now extinct Hf-182 (bar tau = 13 x 10(exp 6) yr). If the large range in epsilon(sub W-182) of lunar samples (0 to +11 in whole rock samples) was due to decay of now extinct Hf-182, it would require a very early time of formation and differentiation of the lunar crust-mantle system (with high Hf/W ratios) during the earliest stages of Earth s accretion. This result was both surprising and difficult to understand. The ability to explain these results by a more plausible mechanism is therefore very attractive. In a recent report Lee et al. (2002) showed that there were excesses of W-182 and that epsilon(sub W-182) was correlated with the Ta/W ratios in the mineral phases of individual lunar rock samples. This is in accord with W-182 variations in lunar samples being produced by cosmic-ray induced neutron capture on Ta-182.

Yin, Qingzhu↗
NASA NTRS1983

Steady flow approximations to the helium r-process

A steady flow approximation to the r-process is presented and used for numerical experiments with physical quantities to determine the sensitivity of the process to variations in those quantities. The effect of neutron capture cross sections along the capture path and of recently available improved beta decay rates on the r-process are discussed. The peaks in the observed r-process yield curve near mass numbers 80 and 130 are roughly characterized by a neutron number density of 10 to the 20th per cu/cm; the mean beta decay rates are about 10/s, and the freezing time is comparable to or less than 0.1 s. The peak near mass number 195 is roughly characterized by a neutron number density of 10 to the 21st/cm, the mean beta decay rates are about 100/s, and the freezing time is comparable to or less than 0.01 s. The flow path of the steady state r-process is sensitively dependent upon the neutron capture cross sections in the flow network and on the values of the beta decay rates.

Cameron, A. G. W.↗
NASA NTRS2010

Comparing Solar-Flare Acceleration of >-20 MeV Protons and Electrons Above Various Energies

A large fraction (up to tens of percent) of the energy released in solar flares goes into accelerated ions and electrons, and studies indicate that these two populations have comparable energy content. RHESSI observations have shown a striking close linear correlation between the 2.223 MeV neutron-capture gamma-ray line and electron bremsstrahlung emission >300 keV, indicating that the flare acceleration of >^20 MeV protons and >300 keV electrons is roughly proportional over >3 orders of magnitude in fluence. We show that the correlations of neutron-capture line fluence with GOES class or with bremsstrahlung emission at lower energies show deviations from proportionality, primarily for flares with lower fluences. From analyzing thirteen flares, we demonstrate that there appear to be two classes of flares with high-energy acceleration: flares that exhibit only proportional acceleration of ions and electrons down to 50 keV and flares that have an additional soft, low-energy bremsstrahlung component, suggesting two separate populations of accelerated electrons. We use RHESSI spectroscopy and imaging to investigate a number of these flares in detail.

Shih, Albert Y.↗
NASA NTRS1991

Determining the solar-flare photospheric scale height from SMM gamma-ray measurements

A connected series of Monte Carlo programs was developed to make systematic calculations of the energy, temporal and angular dependences of the gamma-ray line and neutron emission resulting from such accelerated ion interactions. Comparing the results of these calculations with the Solar Maximum Mission/Gamma Ray Spectrometer (SMM/GRS) measurements of gamma-ray line and neutron fluxes, the total number and energy spectrum of the flare-accelerated ions trapped on magnetic loops at the Sun were determined and the angular distribution, pitch angle scattering, and mirroring of the ions on loop fields were constrained. Comparing the calculations with measurements of the time dependence of the neutron capture line emission, a determination of the He-3/H ratio in the photosphere was also made. The diagnostic capabilities of the SMM/GRS measurements were extended by developing a new technique to directly determine the effective photospheric scale height in solar flares from the neutron capture gamma-ray line measurements, and critically test current atmospheric models in the flare region.

Lingenfelter, Richard E.↗
NASA NTRS1978

Isotopic anomalies from neutron reactions during explosive carbon burning

The possibility that the newly discovered correlated isotopic anomalies for heavy elements in the Allende meteorite were synthesized in the secondary neutron capture episode during the explosive carbon burning, the possible source of the O-16 and Al-26 anomalies, is examined. Explosive carbon burning calculations under typical conditions were first performed to generate time profiles of temperature, density, and free particle concentrations. These quantities were inputted into a general neutron capture code which calculates the resulting isotopic pattern from exposing the preexisting heavy seed nuclei to these free particles during the explosive carbon burning conditions. The interpretation avoids the problem of the Sr isotopic data and may resolve the conflict between the time scales inferred from 1-129, Pu-244, and Al-26.

Lee, T.↗
NASA NTRS1979

Xenon from intermediate zones of supernovae

The paper examines the photodisintegration and neutron capture in massive stars which show that the bulk of the p-isotopes of Xe is formed during the gamma-process of Woosley and Howard (1978) by stripping of the Xe + Be seeds. The environments in which the chondrites can be formed were determined by the neutron-capture calculations; they show that the Xe-124-rich gas must be associated at the sources with anomalously large overabundances of Nd-142, Sm-144, and possibly Ba-130, and with anomalously small overabundances of the p-isotopes of Se, Kr, Sr, and Mo.

Heymann, D.↗
NASA NTRS1993

Induced activation study of LDEF

Analysis of the induced radioactivity of the Long Duration Exposure Facility (LDEF) is continuing with extraction of specific activities for various spacecraft materials. Data and results of activation measurements from eight facilities are being collected for interpretation at Eastern Kentucky University and NASA/Marshall Space Flight Center. The major activation mechanism in LDEF components is the proton flux in the South Atlantic Anomaly (SAA). This flux is highly anisotropic, and could be sampled by taking advantage of the gravity-gradient stabilization of the LDEF. The directionally-dependent activation due to these protons was clearly observed in the data from aluminum experiment tray clamps (reaction product Na-22), steel trunnions (reaction product Mn-54 and others) and is also indicated by the presence of a variety of nuclides in other materials. A secondary production mechanism, thermal neutron capture, was observed in cobalt, indium, and tantalum, which are known to have large capture cross sections. Experiments containing samples of these metals and significant amounts of thermalizing low atomic number (Z) material showed clear evidence of enhanced activation of Co-60, In-114m, and Ta-182. Other mechanisms which activate spacecraft material that are not as easily separable from SAA proton activation, such as galactic proton bombardment and secondary production by fast neutrons, are being investigated by comparison to radiation environmental calculations. Deviations from one-dimensional radiation models indicate that these mechanisms are more important at greater shielding depths. The current status of the induced radioactivity measurements as of mid-year 1992 are reviewed. Specific activities for a number of materials which show SAA effects and thermal neutron capture are presented. The results for consistency by combining data from the participating institutions is also examined.

Harmon, B. A.↗
NASA NTRS1972

Lunar neutron stratigraphy.

Study of the isotopic composition of gadolinium and samarium in four soil and seven drill stem samples returned by the Apollo 15 mission. The results show the possibility to date sedimentary processes on the lunar surface for time scales of around 100 million years because of the particular dependence of neutron capture reactions on depth. The neutron flux has a distinct peak as a function of depth. This peak appears to lie below the level of shallow cratering for time scales of less than one billion years and consequently forms a readily identified marker layer of both depth and time.

Russ, G. P., III↗
NASA NTRS1974

Gamma ray lines from solar flares

The strongest line, both predicted theoretically and detected observationally at 2.2 MeV, is due to neutron capture by protons in the photosphere. The neutrons are produced in nuclear reactions of flare accelerated particles which also positrons and prompt nuclear gamma rays. From the comparison of the observed and calculated intensities of the lines at 4.4 or 6.1 MeV to that of the 2.2 MeV line, it is possible to deduce the spectrum of accelerated nuclei in the flare region; and from the absolute intensities of these lines, it is possible to obtain the total number of accelerated nuclei at the sun. The study of the 2.2 MeV line also gives information on the amount of He-3 in the photosphere. The study of the line at 0.51 MeV resulting from positron annihilation complements the data obtained from the other lines; in addition it gives information on the temperature and density in the annihilation region.

Ramaty, R.↗
NASA NTRS1975

Gamma-ray lines from solar flares

The theory of gamma-ray line production in solar flares is treated in detail. The strongest line, both predicted theoretically and detected observationally at 2.2 MeV, is due to neutron capture by protons in the photosphere. The neutrons are produced in nuclear reactions of flare-accelerated particles which also produce positrons and prompt nuclear gamma rays. From the comparison of the observed and calculated intensities of the lines at 4.4 or 6.1 MeV to that of the 2.2-MeV line, it is possible to deduce the spectrum of accelerated nuclei in the flare region; and from the absolute intensities of these lines, it is possible to obtain the total number of accelerated nuclei at the sun. The study of the 2.2-MeV line also gives information on the amount of He-3 in the photosphere. The study of the line at 0.51 MeV resulting from positron annihilation complements the data obtained from the other lines. In addition, it gives information on the temperature and density in the annihilation region and on the anisotropy of the accelerated electron beam which produces continuum gamma rays at energies greater than about 1 MeV.

Ramaty, R.↗
NASA NTRS1986

Production rates of neon xenon isotopes by energetic neutrons

As a first step in an experimental program to study the behavior of noble gases produced in situ in minerals, a suite of minerals and pure chemicals were irradiated with 14.5 MeV neutrons at LLNL's Rotating Target Neutron Source (RTNS-II) and production rates for noble gases were determined. While neutron effects in meteorites and lunar samples are dominated by low-energy neutron capture, more energetic cosmic-ray secondary neutrons can provide significant depth-dependent contributions to production of cosmogenic nuclides through endothermic reactions such as (n,2n), (n,np), (n,d) and (n,alpha). Production rates for nuclides produced by cosmic-ray secondary neutrons are therefore useful in interpreting shielding histories from the relative abundances of cosmogenic nuclides. Absolute production cross sections were calculated from isotope dilution analyses of NaCl, Mg, CsCl, and Ba(NO3)2 samples, assuming purity, stoichiometry, and quantitative noble gas retention and extraction. Relative production cross sections determined from neon isotopic ratios in the mineral samples were also considered in evaluating the neon production cross sections. Results are presented.

Leich, D. A.↗
NASA NTRS1981

I-Xe dating - Intercomparisons of neutron irradiations and reproducibility of the Bjurbole standard

Previously unpublished data from the stepwise heating analysis of the Valecitos 1 (V1) Bjurbole standard are presented together with the results of an isotopic dilution measurement of a KI monitor included in the V1 irradiation package. The results of these analyses are compared with the values observed in other irradiations. Apparent I-Xe 'formation' ages are reproducible for three different samples of Bjurbole, suggesting isotopic homogeneity for initial iodine in the bulk material. The systematics of neutron capture in Xe-135 (produced from U-235 neutron fission) are examined and verified in irradiated BCR-1.

Hohenberg, C. M.↗
NASA NTRS2008

Grazing-Incidence Neutron Optics based on Wolter Geometries

The feasibility of grazing-incidence neutron imaging optics based on the Wolter geometries have been successfully demonstrated. Biological microscopy, neutron radiography, medical imaging, neutron crystallography and boron neutron capture therapy would benefit from high resolution focusing neutron optics. Two bounce optics can also be used to focus neutrons in SANS experiments. Here, the use of the optics would result in lower values of obtainable scattering angles. The high efficiency of the optics permits a decrease in the minimum scattering vector without lowering the neutron intensity on sample. In this application, a significant advantage of the reflective optics over refractive optics is that the focus is independent of wavelength, so that the technique can be applied to polychromatic beams at pulsed neutron sources.

Gubarev, M. V.↗
NASA NTRS1978

Petrology, chemistry, age and irradiation history of Luna 24 samples

The results of petrological, chemical, isotopic age determination and irradiation studies of sample 24170 from the 170 cm depth of the regolith core returned from Mare Crisium by Luna 24 are presented. The sample is found to be comprised of fragments from a single igneous rock, with mineralogical evidence indicating it to be a mare basalt. The crystallization age is determined by Sm-Nd and Ar(40)-Ar(39) ages to be 3.30 AE, establishing the presence of relatively young flows. All soil samples show low trace element compositions with minimum contamination by KREEPUTh-rich materials. Rb-Sr and Sm-Nd relations reflect the absence of significant fractionation at ages younger than 4.5 AE. One soil sample shows extremely large neutron capture effects, imposing a new lower limit to the neutron production rate in the regolith and requiring the addition of irradiated materials from depth.

Wasserburg, G. J.↗
NASA NTRS1993

Redistribution of subsurface neutrons caused by ground ice on Mars

As part of an ongoing effort to understand data that will be returned by the Mars Observer Gamma Ray Spectrometer (MOGRS) experiment, we calculate neutron and gamma ray fluxes for simple models describing near-surface ground ice on Mars. Our goal is to determine the limits in information content of remotely sensed neutrons and gamma rays is delineating the abundance of ground ice and its distribution with depth. Such ice is expected based on simple theoretical calculations of the H2O environment of the martian surface and atmosphere. We find it produces a marked redistribution of neutrons with depth. Neutron-capture gamma ray production closely follows the flux of thermal neutrons and is likewise redistributed with depth. Calculated effects at Mars mapping orbit are sufficiently large that, if ice is present at the depths and in the quantities expected, the MOGRS should provide a robust detection of its presence. Although in the information content of gamma rays and neutrons alone is not sufficient to define the many parameters needed to specify its abundance and emplacement below the surface, their combined use might allow separation of the ice abundance from its vertical distribution within the regolith.

Feldman, W. C.↗