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At least 73 records · Page 4

Tunable and angle-insensitive plasmon resonances in graphene ribbon arrays with multispectral diffraction response

Plasmon resonances in graphene ribbon arrays are investigated numerically by means of the Finite Element Method. Numerical analysis shows that a series of multipolar resonances take place when graphene ribbon arrays are illuminated by a TM polarized electromagnetic wave. Moreover, these resonances are angle-independent, and can be tuned greatly by the width and the doping level of the graphene ribbons. Specifically, we demonstrate that for graphene arrays with several sets of graphene ribbons, which have different widths or doping levels, each of these multipolar resonances will be split into several ones. In addition, as plasmon resonances can confine electromagnetic field at the ribbon edges, graphene ribbons with different widths or doping levels offer intriguing application for electrically tunable spectral imaging.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Close Proximity to a Quantum Phase Transition in TmZn2⁢GaO5

TmZn2⁢GaO5 is a newly synthesized triangular lattice magnet that exhibits a unique quantum phase characterized by strong Ising anisotropy, a pseudodoublet crystal electric field ground state, and a low-energy gapped excitation at the 𝐾 point. Unlike its well-known counterparts, TmMgGa⁢O4 and YbMgGa⁢O4, this material crystallizes in a distinct hexagonal structure, leading to a platform for investigating frustrated magnetism. Magnetic susceptibility, heat capacity, and inelastic neutron scattering measurements confirm the absence of long-range magnetic order down to 50 mK, placing TmZn2⁢GaO5 in a distinct region of the transverse-field Ising model phase diagram. Theoretical calculations based on spin-wave theory and mean-field modeling reproduce key experimental observations, reinforcing the material’s placement in a quantum disordered or multipolar state near a quantum critical point that separates it from the low-energy phase of TmMgGa⁢O4. These results highlight its potential for exploring quantum disordered states, anisotropic excitations, and exotic quantum phases in frustrated spin systems.

Ennis, Matthew [Department of Physics, Duke Univer↗

High-speed bullet ejections during the AGB-to-planetary nebula transition: HST observations of the carbon star, v hydrae

The well-studied carbon star, V Hya, showing evidence for high-speed, collimated outflows and dense equatorial structures, is a key object in the study of the poorly understood transition of AGB stars into aspherical planetary nebulae. Using the Space Telescope Imaging Spectrograph instrument on board the Hubble Space Telescope, we have obtained high spatial-resolution long-slit optical spectra of V Hya that show high-velocity emission in [S ii] and [Fe ii] lines. Our data set, spanning three epochs spaced apart by a year during each of two periods (in 2002–2004 and 2011–2013), shows that V Hya ejects high-speed (∼200–250 km s{sup −1}) bullets once every ∼8.5 years. The ejection axis flip–flops around a roughly eastern direction, both in and perpendicular to the sky-plane, and the radial velocities of the ejecta also vary in concert between low and high values. We propose a model in which the bullet ejection is associated with the periastron passage of a binary companion in an eccentric orbit around V Hya with an orbital period of ∼8.5 years. The flip–flop phenomenon is likely the result of collimated ejection from an accretion disk (produced by gravitational capture of material from the primary) that is warped and precessing, and/or that has a magnetic field that is misaligned with that of the companion or the primary star. We show how a previously observed 17 year period in V Hya’s light-cycle can also be explained in our model. Additionally, we describe how the model proposed here can be extended to account for multipolar nebulae.

79 ASTRONOMY AND ASTROPHYSICS↗

Horizontal Flows in the Photosphere and Subphotosphere of Two Active Regions

We compare horizontal flow fields in the photosphere and in the subphotosphere (a layer 0.5 megameters below the photosphere) in two solar active regions: AR11084 and AR11158. AR11084 is a mature, simple active region without significant flaring activity, and AR11158 is a multipolar, complex active region with magnetic flux emerging during the period studied. Flows in the photosphere are derived by applying the Differential Affine Velocity Estimator for Vector Magnetograms (DAVE4VM) on HMI-observed vector magnetic fields, and the subphotospheric flows are inferred by time-distance helioseismology using HMI-observed Dopplergrams. Similar flow patterns are found for both layers for AR11084: inward flows in the sunspot umbra and outward flows surrounding the sunspot. The boundary between the inward and outward flows, which is slightly different in the photosphere and the subphotosphere, is within the sunspot penumbra. The area having inward flows in the subphotosphere is larger than that in the photosphere. For AR11158, flows in these two layers show great similarities in some areas and significant differences in other areas. Both layers exhibit consistent outward flows in the areas surrounding sunspots. On the other hand, most well-documented flux-emergence-related flow features seen in the photosphere do not have counterparts in the subphotosphere. This implies that the horizontal flows caused by flux emergence do not extend deeply into the subsurface.

SOLAR↗

ON THE GLOBAL STRUCTURE OF PULSAR FORCE-FREE MAGNETOSPHERE

The dipolar magnetic field structure of a neutron star is modified by the plasma originating in the pulsar magnetosphere. In the simplest case of a stationary axisymmetric force-free magnetosphere, a self-consistent description of the fields and currents is given by the well-known pulsar equation. Here we revise the commonly used boundary conditions of the problem in order to incorporate the plasma-producing gaps and to provide a framework for a truly self-consistent treatment of the pulsar magnetosphere. A generalized multipolar solution of the pulsar equation is found, which, as compared to the customary split monopole solution, is suggested to better represent the character of the dipolar force-free field at large distances. In particular, the outer gap location entirely inside the light cylinder implies that beyond the light cylinder the null and critical lines should be aligned and become parallel to the equator at a certain altitude. Our scheme of the pulsar force-free magnetosphere, which will hopefully be followed by extensive analytic and numerical studies, may have numerous implications for different fields of pulsar research.

79 ASTRONOMY AND ASTROPHYSICS↗

Surface configuration as an explanation for lithology-related cross-polarized radar image anomalies

One problem that has persisted since the development of multipolarized radar is the cause or causes of differential depolarization which is expressed as tonal reversals between like- and cross-polarized images of certain outcrops. Rocks producing anomalously low returns on the cross-polarized image could be classed into three general types: (1) certain geologically recent lava flows (late Pleistocene and Holocene), (2) some tertiary volcanics and (3) certain massive sandstones. Differential depolarization has been produced by volcanic rocks of various compositions including rhyolite, rhyodacite, dacite, andesite, and basalt. This has led to the conclusion that differential depolarization is not directly caused by any compositional factor. However, the study of aerial photos and subsequent field observation have led to the conclusion that the weathering and other surface characteristics of the outcrops are responsible for their appearance on multipolarized imagery.

Mccauley, J. R.↗

Communication: Dielectric properties of condensed systems composed of fragments

Here, the dielectric properties of molecules and nanostructures are usually modified in a complex manner, when assembled into a condensed phase. We propose a first-principles method to compute polarizabilities of sub-entities of solids and liquids, which accounts for multipolar interactions at all orders and is applicable to semiconductors and insulators. The method only requires the evaluation of induced fields in the condensed phase, with no need of multiple calculations for each constituent. As an example, we present results for the molecular polarizabilities of water in a wide pressure and temperature range. We found that at ambient conditions, the dipole-induced-dipole approximation is sufficiently accurate and the Clausius-Mossotti relation may be used, e.g., to obtain molecular polarizabilities from experimental refractive indexes. However with increasing pressure, this approximation becomes unreliable and in the case of ice X the Clausius-Mossotti relation is not valid.

36 MATERIALS SCIENCE↗

Quantum spin ice response to a magnetic field in the dipole-octupole pyrochlore Ce 2 Zr 2 O 7

The pyrochlore magnet Ce 2 Zr 2 O 7 has attracted much attention as a quantum spin ice candidate whose novelty derives in part from the dipolar-octupolar nature of the Ce 3+ pseudospin-1/2 degrees of freedom it possesses. We report heat capacity measurements on single crystal samples of Ce 2 Zr 2 O 7 down to T~0.1K in a magnetic field along the [$1,\bar{1},0$] direction. These measurements show that the broad hump in the zero-field heat capacity moves higher in temperature with increasing field strength and is split into two separate humps by the [$1,\bar{1},0$] magnetic field at ~2T. These separate features are due to the decomposition of the pyrochlore lattice into effectively decoupled chains for fields in this direction: One set of chains (α chains) is polarized by the field while the other (β chains) remains free. This situation is similar to that observed in the classical spin ices Ho 2 Ti 2 O 7 and Dy 2 Ti 2 O 7 , but with the twist that here the strong transverse exchange interactions produce substantial quantum effects. Our theoretical modeling suggests that the β chains are close to a critical state, with nearly-gapless excitations. We also report elastic and inelastic neutron scattering measurements on single crystal Ce 2 Zr 2 O 7 in [$1,\bar{1},0$] and [0,0,1] magnetic fields at temperatures down to T=0.03K. The elastic scattering behaves consistently with the formation of independent chains for a [$1,\bar{1},0$] field, while the [0,0,1] field produces a single field-induced elastic magnetic Bragg peak at (0,2,0) and equivalent wavevectors, indicating a polarized spin ice state for fields above ~3T. For both [$1,\bar{1},0$] and [0,0,1] magnetic fields, our inelastic neutron scattering results show an approximately dispersionless continuum of scattering that increases in both energy and intensity with increasing field strength. By modeling the complete set of experimental data using numerical linked cluster and semiclassical molecular dynamics calculations, we demonstrate the dominantly multipolar nature of the exchange interactions in Ce 2 Zr 2 O 7 and the smallness of the parameter θ, which controls the mixing between dipolar and octupolar degrees of freedom. Finally, these results support previous estimates of the microscopic exchange parameters and place strong constraints on the theoretical description of this prominent spin ice candidate.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Enhanced light confinement in nonlocal resonant metasurfaces with weak multipolar scatterers

Stronger light confinement can be enabled by nanoantennas in the nanostructure and result in efficient control of the directionality of the scattering. We report on an observation of the well-pronounced multipolar resonances from nickel nanoantennas originating from collective effects. We show that the collective coupling of multipolar modes from weak scatterers can substantially enhance the electric dipole and quadrupole resonances. We also demonstrate the generalized lattice Kerker effect in this nanoantenna array. Resonant multipolar excitations within nickel nanoantenna arrays can significantly enhance phenomena such as magneto-optical effects, indicating promising potential for advanced applications in the field of nanophotonics and sensing.

Physics↗

Spectroscopic Evidence of Kondo-Induced Quasiquartet in CeRh 2 As 2

CeRh 2 As 2 is a new multiphase superconductor with strong suggestions for an additional itinerant multipolar ordered phase. The modeling of the low-temperature properties of this heavy-fermion compound requires a quartet Ce 3 + crystal-field ground state. Here, we provide the evidence for the formation of such a quartet state using x-ray spectroscopy. Core-level photoelectron and x-ray absorption spectroscopy confirm the presence of Kondo hybridization in CeRh 2 As 2 . The temperature dependence of the linear dichroism unambiguously reveals the impact of Kondo physics for coupling the Kramer’s doublets into an effective quasiquartet. Nonresonant inelastic x-ray scattering data find that the | Γ 7 − ⟩ state with its lobes along the 110 direction of the tetragonal structure ( x y orientation) contributes most to the multiorbital ground state of CeRh 2 As 2 . Published by the American Physical Society 2024

Christovam, Denise S. (ORCID:0000000250698107)↗

Noncollinear Magnetic Structure and Multipolar Order in Eu 2 Ir 2 O 7

The magnetic properties of the pyrochlore iridate material Eu 2 Ir 2 O 7 (5d 5 ) have been studied based on first principles calculations, where the crystal field splitting Δ , spin-orbit coupling (SOC) λ, and Coulomb interaction U within Ir 5 d orbitals all play significant roles. The ground state phase diagram has been obtained with respect to the strength of SOC and Coulomb interaction U , where a stable antiferromagnetic ground state with all-in–all-out (AIAO) spin structure has been found. In addition, another antiferromagnetic state with energy close to AIAO has also been found to be stable. The calculated nonlinear magnetization of the two stable states both have the d -wave pattern but with a π/4 phase difference, which can perfectly explain the experimentally observed nonlinear magnetization pattern. Finally, compared with the results of the nondistorted structure, it turns out that the trigonal lattice distortion is crucial for stabilizing the AIAO state in Eu 2 Ir 2 O 7 . Furthermore, besides large dipolar moments, we also find considerable octupolar moments in the magnetic states.

36 MATERIALS SCIENCE↗

Neptune radio emission in dipole and multipole magnetic fields

We study Neptune's smooth radio emission in two ways: we simulate the observations and we then consider the radio effects of Neptune's magnetic multipoles. A procedure to deduce the characteristics of radio sources observed by the Planetary Radio Astronomy experiment minimizes limiting assumptions and maximizes use of the data, including quantitative measurement of circular polarization. Study of specific sources simulates time variation of intensity and apparent polarization of their integrated emission over an extended time period. The method is applied to Neptune smooth recurrent emission (SRE). Time series are modeled with both broad and beamed emission patterns, and at two frequencies which exhibit different time variation of polarization. These dipole-based results are overturned by consideration of more complex models of Neptune's magnetic field. Any smooth emission from the anticipated auroral radio source is weak and briefly observed. Dominant SRE originates complex fields at midlatitude. Possible SRE source locations overlap that of 'high-latitude' emission (HLE) between +(out) and -(in) quadrupoles. This is the first identification of multipolar magnetic structure with a major source of planetary radio emission.

Sawyer, C. B.↗

Controlling spins with surface magnon polaritons

Polaritons in metals, semimetals, semiconductors, and polar insulators can allow for extreme confinement of electromagnetic energy, providing many promising opportunities for enhancing typically weak light-matter interactions such as multipolar radiation, multiphoton spontaneous emission, Raman scattering, and material nonlinearities. These extremely confined polaritons are quasielectrostatic in nature, with most of their energy residing in the electric field. As a result, these “electric” polaritons are far from optimized for enhancing emission of a magnetic nature, such as spin relaxation, which is typically many orders of magnitude slower than corresponding electric decays. Here, we take concepts of “electric” polaritons into magnetic materials, and propose using surface magnon polaritons in negative magnetic permeability materials to strongly enhance spin relaxation in nearby emitters. Specifically, we provide quantitative examples with MnF 2 and FeF 2 , enhancing spin transitions in the THz spectral range. In this work we find that these magnetic polaritons in 100-nm thin films can be confined to lengths over 10 000 times smaller than the wavelength of a photon at the same frequency, allowing for a surprising 12 orders of magnitude enhancement in magnetic dipole transitions. This takes THz spin-flip transitions, which normally occur at timescales on the order of a year, and forces them to occur at sub-ms timescales. Our results suggest an interesting platform for polaritonics at THz frequencies, and more broadly, a way to use polaritons to control light-matter interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Active Plasmonics and Active Chiral Plasmonics through Orientation-Dependent Multipolar Interactions

While most active plasmonic efforts focus on responsive metamaterials to modulate optical response, we present a simple alternative based on applied orientation control that can likely be implemented for many passive plasmonic materials. Passive plasmonic motifs are simpler to prepare but cannot be altered postfabrication. Here, we show that such systems can be easily manipulated through substrate orientation control to generate both active plasmonic and active chiral plasmonic responses. Using gold nanocrescents as our model platform, we demonstrate tuning of optical extinction from -21% to +36% at oblique incidence relative to normal incidence. Variation of substrate orientation in relation to incident polarization is also demonstrated to controllably switch chiroptical handedness (e.g., Δg = ± 0.55). These active plasmonic responses arise from the multipolar character of resonant modes. In particular, we correlate magnetoelectric and dipole–quadrupole polarizabilities with different light-matter orientation-dependence in both near- and far-field localized surface plasmon activity. Additionally, the attribution of far-field optical response to higher-order multipoles highlights the sensitivity offered by these orientation-dependent characterization techniques to probe the influence of localized electromagnetic field gradients on a plasmonic response. The sensitivity afforded by orientation-dependent optical characterization is further observed by the manifestation in both plasmon and chiral plasmon responses of unpredicted structural nanocrescent variance (e.g., left- and right-tip asymmetry) not physically resolved through topographical imaging.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Evolution of non-Kramers doublets in magnetic field in PrNi 2 Cd 20 and PrPd 2 Cd 20

Praseodymium-based 1-2-20 cage compounds PrT 2 X 20 (T is generally Ti, V, Nb, Ru, Rh, Ir; and X is either Al, Zn, or Cd) provide yet another platform to study nontrivial electronic states of matter ranging from topological and magnetic orders to unconventional multipolar orders and superconductivity. In this paper, we report measurements of the electronic heat capacity in two Pr-based 1-2-20 materials: PrNi 2 Cd 20 and PrPd 2 Cd 20 . We find that the lowest-energy multiplet of the Pr 4f 2 valence configuration is a Γ 3 non-Kramers doublet and the first excited triplet is assumed to be a magnetic Γ 5 . By analyzing the dependence of the energy splitting between the ground and first excited singlet states on an external magnetic field, we found that the maximum in the heat capacity corresponding to the Schottky anomaly in PrPd 2 Cd 20 , unlike PrNi 2 Cd 20 , shows a pronounced linear dependence on an external magnetic field at higher field values. In conclusion, this effect is associated with the exchange interactions between the field-induced magnetic dipole moments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Asymptotic normalization of mirror states and the effect of couplings

Assuming that the ratio between asymptotic normalization coefficients of mirror states is model independent, charge symmetry can be used to indirectly extract astrophysically relevant proton capture reactions on proton-rich nuclei based on information on stable isotopes. The assumption has been tested for light nuclei within the microscopic cluster model. In this work we explore the Hamiltonian independence of the ratio between asymptotic normalization coefficients of mirror states when deformation and core excitation is introduced in the system. For this purpose we consider a phenomenological rotor+N model where the valence nucleon is subject to a deformed mean field and the core is allowed to excite. We apply the model to {sup 8}Li/{sup 8}B, {sup 13}C/{sup 13}N, {sup 17}O/{sup 17}F, {sup 23}Ne/{sup 23}Al, and {sup 27}Mg/{sup 27}P. Our results show that, for most studied cases, the ratio between asymptotic normalization coefficients of mirror states is independent of the strength and multipolarity of the couplings induced. The exception is for cases in which there is an s-wave coupled to the ground state of the core, the proton system is loosely bound, and the states have large admixture with other configurations. We discuss the implications of our results for novae.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Revealing the Nature of Antiferroquadrupolar Ordering in Cerium Hexaboride: CeB 6

The cerium hexaboride (CeB 6 ) f -electron compound displays a rich array of low-temperature magnetic phenomena, including a “magnetically hidden” order, identified as multipolar in origin via advanced x-ray scattering. From first-principles electronic-structure results, we find that the antiferroquadrupolar (AFQ) ordering in CeB 6 arises from crystal-field splitting and yields a band structure in agreement with experiments. With interactions of p electrons between Ce and B 6 being small, the electronic state of CeB 6 is suitably described as Ce(4 f 1 ) 3+ (e – )(B 6 ) 2– . The AFQ state of orbital spins is caused by an exchange interaction induced through spin-orbit interaction, which also splits the J = 5/2 state into a Γ 8 ground state and a Γ 7 excited state. Within the smallest antiferromagnetic (AFM) (111) configuration, an orbital-ordered AFQ state appears during charge self-consistency, and it supports the appearance of a “hidden” order. Furthermore hydrostatic pressure (either applied or chemically induced) stabilizes the AFM (AFQ) states over a ferromagnetic one, as observed at low temperatures.

36 MATERIALS SCIENCE↗

Multipolarization P-, L-, and C-band radar for coastal zone mapping - The Louisiana example

Multipolarization P-, L-, and C-band airborne SAR data sets were acquired over a coastal zone and a forested wetland of southern Louisiana. The data sets were used with field-collected surface-parameter data in order to determine the value of SAR systems in assessing and mapping coastal-zone surface features. The coastal-zone surface features in this study are sediments, sediment distribution, and the formation of new isles and banks. Results of the data analysis indicate that the P-band radar with 68-cm wavelength is capable of detecting the submerged sediment if the area is very shallow (i.e., a water depth of less than one meter). The penetration capability of P-band radar is also demonstrated in the forested wetland area. The composition and condition of the ground surface can be detected, as well as the standing water beneath dense tree leaves.

Wu, Shih-Tseng↗