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Aerosol-Cloud Interactions in the South-East Atlantic: Knowledge Gaps, Planned Observations to Address Them, and Implications for Global Climate Change Modeling

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles, yet the fate of these particles and their influence on regional and global climate is poorly understood. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical Stratocumulus (Sc) cloud decks in the world. The stratocumulus "climate radiators" are critical to the regional and global climate system. They interact with dense layers of BB aerosols that initially overlay the cloud deck, but later subside and are mixed into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects. As emphasized in the latest IPCC report, the global representation of these aerosol-cloud interaction processes in climate models is one of the largest uncertainty in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for global climate change scenarios. We discuss the current knowledge of aerosol and cloud property distributions based on satellite observations and sparse suborbital sampling, and describe planned field campaigns in the region. Specifically, we describe the scientific objectives and implementation of the following four synergistic, international research activities aimed at providing a process-level understanding of aerosol-cloud interactions over the SE Atlantic: 1) ORACLES (Observations of Aerosols above Clouds and their interactions), a five-year investigation between 2015 and 2019 with three Intensive Observation Periods (IOP), recently funded by the NASA Earth-Venture Suborbital Program, 2) CLARIFY-2016 (Cloud-Aerosol-Radiation Interactions and Forcing: Year 2016), a comprehensive observational and modeling programme funded by the UK's Natural Environment Research Council (NERC), and supported by the UK Met Office. 3) LASIC (Layered Atlantic Smoke Interactions with Clouds), a funded deployment of the DOE (Department of Energy) ARM Mobile Facility (AMF1) to Ascension Island, nominally for April 1 2016 - March 31 2017, and 4) ONFIRE (Observations of Fire's Impact on the southeast Atlantic Region), a proposed deployment of the NCAR C-130 aircraft to Sao Tome Island in 2017.

Aerosol-cloud

Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: Future Suborbital Activities to Address Knowledge Gaps in Satellite and Model Assessments

Southern Africa produces almost a third of the Earth's biomass burning (BB) aerosol particles. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical stratocumulus (Sc) cloud decks in the world. The SE Atlantic stratocumulus deck interacts with the dense layers of BB aerosols that initially overlay the cloud deck, but later subside and may mix into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects, and their global representation in climate models remains one of the largest uncertainties in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for global climate change scenarios. Our understanding of aerosol-cloud interactions in the SE Atlantic is hindered both by the lack of knowledge on aerosol and cloud properties, as well as the lack of knowledge about detailed physical processes involved. Most notably, we are missing knowledge on the absorptive and cloud nucleating properties of aerosols, including their vertical distribution relative to clouds, on the locations and degree of aerosol mixing into clouds, on the processes that govern cloud property adjustments, and on the importance of aerosol effects on clouds relative to co-varying synoptic scale meteorology. We discuss the current knowledge of aerosol and cloud property distributions based on satellite observations and sparse suborbital sampling. Recent efforts to make full use of A-Train aerosol sensor synergies will be highlighted. We describe planned field campaigns in the region to address the existing knowledge gaps. Specifically, we describe the scientific objectives and implementation of the five synergistic, international research activities aimed at providing some of the key aerosol and cloud properties and a process-level understanding of aerosol-cloud interactions over the SE Atlantic: NASA's ORACLES, the UK Met Office's CLARIFY-2016, the DoE's LASIC, NSF's ONFIRE, and CNRS' AEROCLO-SA.

aerosols

Observations of Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: First Results from the ORACLES Deployments in 2016 and 2017

Southern Africa produces almost a third of the Earths biomass burning (BB) aerosol particles. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical stratocumulus (Sc) cloud decks in the world. The SE Atlantic stratocumulus deck interacts with the dense layers of BB aerosols that initially overlay the cloud deck, but later subside and often mix into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects, and their global representation in climate models remains one of the largest uncertainties in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for regional and global climate change predictions.The low-level clouds in the SE Atlantic have limited vertical extent and therefore present favorable conditions for their exploration with remote sensing. On the other hand, the normal coexistence of BB aerosols and Sc clouds in the same scene also presents significant challenges to conventional remote sensing techniques. We describe first results from NASAs airborne ORACLES (ObseRvations of Aerosols Above Clouds and Their IntEractionS) deployments in September 2016 and August 2017. We emphasize the unique role of polarimetric observations by two instruments, the Research Scanning Polarimeter (RSP) and the Airborne Multi-angle SpectroPolarimeter Imager (AirMSPI), and describe how these instruments help address specific ORACLES science objectives. Initial assessments of polarimetric observation accuracy for key cloud and aerosol properties will be presented, in as far as the preliminary nature of measurements permits.

Redemann, Jens

Aerosol-Radiation-Cloud Interactions in the South-East Atlantic: First Results from the ORACLES-2016 Deployment and Plans for Future Activities

Southern Africa produces almost a third of the Earths biomass burning (BB) aerosol particles. Particles lofted into the mid-troposphere are transported westward over the South-East (SE) Atlantic, home to one of the three permanent subtropical stratocumulus (Sc) cloud decks in the world. The SE Atlantic stratocumulus deck interacts with the dense layers of BB aerosols that initially overlay the cloud deck, but later subside and may mix into the clouds. These interactions include adjustments to aerosol-induced solar heating and microphysical effects, and their global representation in climate models remains one of the largest uncertainties in estimates of future climate. Hence, new observations over the SE Atlantic have significant implications for regional and global climate change predictions.Our understanding of aerosol-cloud interactions in the SE Atlantic is severely limited. Most notably, we are missing knowledge on the absorptive and cloud nucleating properties of aerosols, including their vertical distribution relative to clouds, on the locations and degree of aerosol mixing into clouds, on the processes that govern cloud property adjustments, and on the importance of aerosol effects on clouds relative to co-varying synoptic scale meteorology.We describe first results from various synergistic, international research activities aimed at studying aerosol-cloud interactions in the region:NASAs airborne ORACLES (ObseRvations of Aerosols Above Clouds and Their IntEractionS) deployment in AugustSeptember of 2016,the DoEs LASIC (Layered Atlantic Smoke Interactions with Clouds) deployment of the ARM Mobile Facility to Ascension Island (June 2016 October 2017), the ground-based components of CNRS AEROCLO-sA (Aerosols Clouds and Fog over the west coast of southern Africa), and ongoing regional-scale integrative, process-oriented science efforts as part of SEALS-sA (Sea Earth Atmosphere Linkages Study in southern Africa).We expect to describe experimental setups as well as showcase initial aerosol and cloud property distributions. Furthermore, we discuss the implementation of future activities in these programs in coordination with the UK Met Offices CLARIFY (CLoud-Aerosol-Radiation Interactions and Forcing) experiment in 2017.

aerosol

ELASTIC STABILITY OF SIMPLY SUPPORTED CORRUGATED CORE SANDWICH CYLINDERS

Theoretical buckling coefficients are obtained for the general instability of simply supported, corrugated core sandwich circular cylinders under combined loads with the core oriented parallel to the longitudinal axis of the cylinder. Buckling curves are presented for axial compression, external lateral pressure, torsion, and some typical interactions. The differential equations of equilibrium used to obtain the buckling equations were derived from the small deflection equations of Stein and Mayer which include the effect of deformation due to transverse shear. These equations are solved by Galerkin's equation. Remarks are made concerning the probable validity of the results of the small deflection theory for sandwich shells.

SHELL STABILITY

Validity of the Relation Between Spontaneous and Stimulated Emissions in Semiconductors

The Einstein relation between spontaneous emission and absorption was originally derived for a system consists of a two-state subsystem representing matter and harmonic fields representing radiation. The derivation is based on the detailed balance between these two subsystems under thermal equilibrium. The relationship was later investigated in connection with the interactions between radiation field and solids or semiconductors. The simple derivation dose not hold for semiconductors in general. In certain limiting cases, simple relation was obtained. The validity of this relation is important not only because of its fundamental role connecting two of the most fundamental optical processes in semiconductors, but mostly also because of its wide use as a practical method to measure the optical gain of a semiconductor. The validity of this relation for semiconductors has been an issue of controversial for some time. In this paper we numerically examine the validity of this relationship for several different lineshapes including Lorentzian, Gaussian, Sech, and a convoluted double Lorentzians (CDL). We find out that at relatively low density above transparency level, all first three lineshapes violate the Einstein relation. The relation is approximately valid at high density. At very high density, the validity of the Einstein relation holds well for all three lineshapes. The reason behind this observation is explained. The CDL lineshape has been shown analytically to obey the Einstein relationship previously. We show that for a 2D semiconductor with parabolic bands, the CDL lineshape can be integrated analytically. This analytic lineshape is compared with a simple Lorentzian lineshape.

Ning, Cun-Zheng

Models And Experiments Of Laminar Diffusion Flames In Non-Uniform Magnetic Fields

Non-uniform magnetic fields affect laminar diffusion flames as a result of the paramagnetic and diamagnetic properties of the products and reactants. Paramagnetism is the weak attraction to a magnetic field a material exhibits as a result of permanent magnetic dipole moments in the atoms of the material. Diamagnetism is the weak repulsion to a magnetic field exhibited by a material due to the lack of permanent magnetic dipole moments in the atoms of a material. The forces associated with paramagnetic and diamagnetism are several orders of magnitude less than the forces associated with the more familiar ferromagnetism. A typical example of a paramagnetic gas is oxygen while hydrocarbon fuels and products of combustion are almost always diamagnetic. The fact that magnets can affect flame behavior has been recognized for more than one hundred years. Early speculation was that such behavior was due to the magnetic interaction with the ionized gases associated with a flame. Using a scaling analysis, it was later shown that for laminar diffusion flames the magnetic field/ionized gas interaction was insignificant to the paramagnetic and diamagnetic influences. In this effort, the focus has been on examining laminar diffusion slot flames in the presence of non-uniform upward decreasing magnetic fields produced using permanent magnets. The principal reason for choosing slot flames was mathematical models of such flames show an explicit dependence on gravitational body forces, in the buoyancy-controlled regime, and an applied magnetic field would also impose a body force. In addition, the behavior of such flames was more easily visualized while maintaining the symmetry of the two-dimensional problem whereas it would have been impossible to obtain a symmetric magnetic field around a circular flame and still visually record the flame height and shape along the burner axis. The motivation for choosing permanent magnets to produce the magnetic fields was the assumption that space-related technologies based on the knowledge gained during this investigation would more likely involve permanent magnets as opposed to electromagnets. While no analysis has been done here to quantify the impact that an electric field, associated with an electromagnetic, would have relative to the paramagnetic and diamagnetic interactions, by using permanent magnets this potential effect was completely eliminated and thus paramagnetic and diamagnetic effects were isolated.

Baker, J.

CFD Analysis of Modular Thrusters Performance

The effective performance of modular thrusters in an aerospike configuration is difficult to determine. Standard analytical tools are applicable to conventional nozzle shapes, but are limited when applied to an aerospike nozzle (An aerospike nozzle is an altitude compensating external nozzle). Three baseline nozzle shapes are derived using standard analytical procedures. The baseline nozzle sizes are restricted to fill a volume envelope. The three shapes are an axi-symmetric round nozzle, a two dimensional planar square exit nozzle, and a super elliptic round to nearly square nozzle. The integrated (thruster/aerospike) performance of the three nozzles is determined through the use of three dimensional viscous computational fluid dynamic (CFD) calculation where complex features of the flow field can be accurately captured. The resulting installed performance is then used to evaluate the efficiency of these nozzle shapes for aerospike applications. The determination of effective performance of a thruster nozzle integrated into an aerospike nozzle require the solution of the three dimensional turbulent Navier-Stokes equations. The model used in this study consisted of two zones; one of the upstream thruster cowl surface so freestream conditions can be accurately predicted, and two, the aerospike surface beginning with the thruster outflow and extending to the end of the aerospike surface. The numerical grid consisted of over 120,000 nodes and used symmetry on the thruster centerline and edge. A two species non-reacting chemistry model was used to capture the variation of fluid properties between the hot plume base and freestream air. From the results of the three baseline nozzle aerospike calculations, the effictive performance of the nozzle was determined. The flow fields of these calculations do show some variation between the cases. Recirculation zones on the cowl surface is predicted for the two dimensional planar nozzle and a smaller one for the super elliptic nozzle. The recirculation is caused by the strong pressure gradient between the plume and freestream flows. The axi-symmetric nozzle results indicate recirculation zones on the thruster face. These recirculation zones smooth the pressure gradient between the plume and freestream flow limiting the formation of recirculation on the cowl surface. Thruster to thruster interaction is evident for the axi-symmetric and supper elliptic calculation while the two dimensional planar nozzle did not have any lateral expansion in the nozzle, so thruster to thruster interaction is limited. The integrated performance results, at the altitude choosen, show very little variation between the three thruster shapes. This result allows for nozzle shape determination based on additional considerations (thermal, structural, weight) besides performance.

Ungewitter, Ronald J.

The NASA Inductrack Model Rocket Launcher at the Lawrence Livermore National Laboratory

The Inductrack magnetic levitation system, developed at the Lawrence Livermore National Laboratory, is being studied for its possible use for launching rockets. Under NASA sponsorship, a small model system is being constructed at the Laboratory to pursue key technical aspects of this proposed application. The Inductrack is a passive magnetic levitation system employing special arrays of high-field permanent magnets (Halbach arrays) on the levitating carrier, moving above a "track" consisting of a close-packed array of shorted coils with which are interleaved with special drive coils. Halbach arrays produce a strong spatially periodic magnetic field on the front surface of the arrays, while canceling the field on their back surface. Relative motion between the Halbach arrays and the track coils induces currents in those coils. These currents levitate the carrier cart by interacting with the horizontal component of the magnetic field. Pulsed currents in the drive coils, synchronized with the motion of the carrier, interact with the vertical component of the magnetic field to provide acceleration forces. Motional stability, including resistance to both vertical and lateral aerodynamic forces, is provided by having Halbach arrays that interact with both the upper and the lower sides of the track coils. In its completed form the model system that is under construction will have a track approximately 100 meters in length along which the carrier cart will be propelled up to peak speeds of Mach 0.4 to 0.5 before being decelerated. Preliminary studies of the parameters of a full-scale system have also been made. These studies address the problems of scale-up, including means to simplify the track construction and to reduce the cost of the pulsed-power systems needed for propulsion.

Tung, L. S.

Hypersonic aerodynamics and entry-maneuver: Aerothermodynamic interactions for two lifting entry vehicles

The longitudinal, directional, and lateral static stability and control characteristics of a delta lifting body and a delta-wing body were obtained at a Mach number of 20 in helium for operational Reynolds numbers over an angle-of-attack range of -4 deg to 55 deg. The aerodynamic characteristics of the wing body were then evaluated in an entry study to examine the effects of vehicle performance on the aerothermodynamic parameters associated with constant and variable angle-of-attack modes for a 1500-n. mi. cross range. The experimental results indicated that the vehicles were stable, except for neutral directional stability for the wing-body shape, and could be trimmed over the operational angle-of-attack range; however, the wing-body vehicle had adverse yaw due to roll control. This roll-yaw coupling was not examined for the lifting body. The trajectory analysis indicated that a 17-percent decrease in performance required little change in the constant angle-of-attack entry mode and, in turn, resulted in a small decrease in the total heat load. For the pitch-modulated entry, the performance decrease required the pitch maneuver to begin earlier during entry and to last longer in order to meet the 1500-n. mi. cross range without a major heating penalty. The performance reduction also had little effect on the maximum laminar radiation equilibrium temperature over a major portion of the lower surface of the wing-body vehicle regardless of the entry mode.

Arrington, J. P.

Unsuccessful Concepts for Aircraft Wake Vortex Minimization

Exploratory concepts are described which were investigated to achieve a reduction in the vortex induced rolling upsets produced by heavy aircraft trailing vortexes. The initial tests included the use of mass injection, oscillating devices, wingtip shape design, interacting multiple vortexes, and end plates. Although later refinements of some of these concepts were successful, initial test results did not indicate a capability of these concepts to significantly alter the vortex induced rolling upset on a following aircraft.

Dunham, R. E., Jr.

Basic avionics module design for general aviation aircraft

The design of an advanced digital avionics system (basic avionics module) for general aviation aircraft operated with a single pilot under IFR conditions is described. The microprocessor based system provided all avionic functions, including flight management, navigation, and lateral flight control. The mode selection was interactive with the pilot. The system used a navigation map data base to provide operation in the current and planned air traffic control environment. The system design included software design listings for some of the required modules. The distributed microcomputer uses the IEEE 488 bus for interconnecting the microcomputer and sensors.

Smyth, R. K.

Design of a simulation environment for laboratory management by robot organizations

This paper describes the basic concepts needed for a simulation environment capable of supporting the design of robot organizations for managing chemical, or similar, laboratories on the planned U.S. Space Station. The environment should facilitate a thorough study of the problems to be encountered in assigning the responsibility of managing a non-life-critical, but mission valuable, process to an organized group of robots. In the first phase of the work, we seek to employ the simulation environment to develop robot cognitive systems and strategies for effective multi-robot management of chemical experiments. Later phases will explore human-robot interaction and development of robot autonomy.

Zeigler, Bernard P.

Experimental and analytical study on fluid whirl and fluid whip modes

Fluid whirl and fluid whip are rotor self-excited, lateral vibrations which occur due to rotor interactions with the surrounding fluid. There exist various modes of fluid whirl and fluid whip. These modes are close to rotor modes corresponding to free vibrations (based on the linear model). Small differences are due to nonlinearities in the system. This paper presents experimental and analytical results on the lowest modes of fluid whirls and fluid whip. Examples of rotors supported in fluid lubricated bearings show the variations of rotor deflection amplitudes and phases in the whirl and whip modes with changes of rotative speeds and/or changes in lumped mass locations along the shaft.

Muszynska, Agnes

Wind Tunnel Measurements and Calculations of Aerodynamic Interactions Between Tiltrotor Aircraft

Wind tunnel measurements and calculations of the aerodynamic interactions between two tiltrotor aircraft in helicopter mode are presented. The measured results include the roll moment and thrust change on the downwind aircraft, as a function of the upwind aircraft position (longitudinal, lateral, and vertical). Magnitudes and locations of the largest interactions are identified. The calculated interactions generally match the measurements, with discrepancies attributed to the unsteadiness of the wake and aerodynamic forces on the airframe. To interpret the interactions in terms of control and power changes on the aircraft, additional calculations are presented for trimmed aircraft with gimballed rotors.

Johnson, Wayne

Fluorophilic Sigma(σ)‐Lock Self‐Healable Copolymers

Abstract Although F‐Containing molecules and macromolecules are often used in molecular biology to increase the binding with Lewis acidic groups by introducing favorable C−F dipoles, there is virtually no experimental evidence and limited understanding of the nature of these interactions, especially their role in synthetic polymeric materials. These studies elucidate the molecular origin of inter‐ and intra‐Chain interactions responsible for self‐healing of F‐Containing copolymers composed of pentafluorostyrene and n‐butyl acrylate units (p(PFS/nBA). Guided by dynamic surface oscillating force (SOF) and spectroscopic measurements supported by molecular dynamics (MD) simulations, these studies show that the reformation of σ‐σ orbitals in −C−F of PFS and CH 3 CH 2 − of nBA units enables the recovery of entropic energy via fluorophilic‐σ‐lock van der Waals forces when PFS/nBA molar ratios are ~50/50. The strength of these interactions determined experimentally for self‐healable PFS/nBA compositions is in the order ~0.3 kcal/mol which primarily comes from fluorophilic‐σ‐lock (~70 %) contributions. These interactions are significantly diminished for non‐self‐healable counterparts. Strongly polarized −C−F σ orbitals create lateral dipolar forces enhancing the affinity towards −C−H orbitals, facilitating energetically favorable interactions. Entropic recovery driven by non‐Covalent bonding offers a valuable tool in designing materials with unique functionalities, particularly self‐healable batteries and energy storage devices.

Gaikwad, Samruddhi

Fluorophilic Sigma(σ)‐Lock Self‐Healable Copolymers

Although F-Containing molecules and macromolecules are often used in molecular biology to increase the binding with Lewis acidic groups by introducing favorable C−F dipoles, there is virtually no experimental evidence and limited understanding of the nature of these interactions, especially their role in synthetic polymeric materials. These studies elucidate the molecular origin of inter- and intra-Chain interactions responsible for self-healing of F-Containing copolymers composed of pentafluorostyrene and n-butyl acrylate units (p(PFS/nBA). Guided by dynamic surface oscillating force (SOF) and spectroscopic measurements supported by molecular dynamics (MD) simulations, these studies show that the reformation of σ-σ orbitals in −C−F of PFS and CH 3 CH 2 − of nBA units enables the recovery of entropic energy via fluorophilic-σ-lock van der Waals forces when PFS/nBA molar ratios are ~50/50. The strength of these interactions determined experimentally for self-healable PFS/nBA compositions is in the order ~0.3 kcal/mol which primarily comes from fluorophilic-σ-lock (~70 %) contributions. These interactions are significantly diminished for non-self-healable counterparts. Strongly polarized −C−F σ orbitals create lateral dipolar forces enhancing the affinity towards −C−H orbitals, facilitating energetically favorable interactions. Entropic recovery driven by non-Covalent bonding offers a valuable tool in designing materials with unique functionalities, particularly self-healable batteries and energy storage devices.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH

Scale disparity and spectral transfer in anisotropic numerical turbulence

To study the effect of cancellations within long-range interactions on local isotropy at the small scales, we calculate explicitly the degree of cancellation in distant interactions in the simulations of Yeung & Brasseur and Yeung, Brasseur & Wang using the single scale disparity parameter 's' developed by Zhou. In the simulations, initially isotropic simulated turbulence was subjected to coherent anisotropic forcing at the large scales and the smallest scales were found to become anisotropic as a consequence of direct large-small scale couplings. We find that the marginally distant interactions in the simulation do not cancel out under summation and that the development of small-scale anisotropy is indeed a direct consequence of the distant triadic group, as argued by Yeung, et. al. A reduction of anisotropy at later times occurs as a result of the isotropizing influences of more local energy-cascading triadic interactions. Nevertheless, the local-to-nonlocal triadic group persists as an isotropizing influence at later times. We find that, whereas long-range interactions, in general, contribute little to net energy transfer into or out of a high wavenumber shell k, the anisotropic transfer of component energy within the shell increases with increasing scale separations. These results are consistent with results by Zhou, and Brasseur & Wei, and suggest that the anisotropizing influences of long range interactions should persist to higher Reynolds numbers. The residual effect of the forced distant group in this low-Reynolds number simulation is found to be forward cascading, on average.

Zhou, YE