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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Towards Resilient Design of Leader-following Consensus with Attack Identification and Privacy Preservation Capabilities

This paper considers a leader-following consensus in the presence of unknown but bounded cyber-attacks. Specifically, we consider the following cyber-attack scenarios: (i) an attacker aims to destabilize the consensus dynamics by injecting exogenous signals to both the actuators of the followers and/or the communication network, (ii) an eavesdropper adversary aims to obtain information on the physical state of the agents. To this end, a novel resilient leader-following consensus algorithm based on a competitive interaction method is proposed. In addition, it is demonstrated that by appropriately choosing the information exchanged between the agents, the proposed control framework also enables the cooperative system to either distributively identify the compromised communication links in real-time or to protect the privacy of the physical state of the agents from the eavesdropper. Here, a numerical example is provided to illustrate the proposed resilient control algorithms.

Gusrialdi, Azwirman↗
DOE OSTI2024

Identification and Suppression of Point Defects in Bromide Perovskite Single Crystals Enabling Gamma‐Ray Spectroscopy

Abstract Methylammonium lead tribromide (MAPbBr 3 ) stands out as the most easily grown wide‐band‐gap metal halide perovskite. It is a promising semiconductor for room‐temperature gamma‐ray ( γ ‐ray) spectroscopic detectors, but no operational devices are realized. This can be largely attributed to a lack of understanding of point defects and their influence on detector performance. Here, through a combination of crystal growth design and defect characterization, including positron annihilation and impedance spectroscopy, the presence of specific point defects are identified and correlated to detector performance. Methylammonium (MA) vacancies, MA interstitials, and Pb vacancies are identified as the dominant charge‐trapping defects in MAPbBr 3 crystals, while Br vacancies caused doping. The addition of excess MABr reduces the MA and Br defects and so enables the detection of energy‐resolved γ ‐ray spectra using a MAPbBr 3 single‐crystal device. Interestingly, the addition of formamidinium (FA) cations, which converted to methylformamidinium (MFA) cations by reaction with MA + during crystal growth further reduced MA defects. This enabled an energy resolution of 3.9% for the 662 keV 137 Cs line using a low bias of 100 V. The work provides direction toward enabling further improvements in wide‐bandgap perovskite‐based device performance by reducing detrimental defects.

Ni, Zhenyi↗
DOE OSTI2021

Surface Functionalization of Black Phosphorus with Nitrenes: Identification of P=N Bonds Using Isotopic Labeling

Abstract: Surface functionalization of two-dimensional crystals is a key path to tuning their intrinsic physical and chemical properties. However, synthetic protocols and experimental strategies to directly probe chemical bonding in modified surfaces are scarce. Introduced here is a mild, surface-specific protocol for the surface functionalization of few-layer black phosphorus nanosheets using a family of photolytically generated nitrenes (RN) from the corresponding azides. By embedding spectroscopic tags in the organic backbone, a multitude of characterization techniques are employed to investigate in detail the chemical structure of the modified nanosheets, including vibrational (infrared, Raman), Xray (emission, photoelectron), CPMAS NMR, and UV-vis spectroscopy. To directly probe the functional groups introduced on the surface, R fragments were selected such that in conjunction with vibrational spectroscopy, 15N-labeling experiments, and DFT methods, diagnostic P=N vibrational modes indicative of iminophosphorane units on the nanosheet surface could be conclusively identified.

Walz, Kendall↗
DOE OSTI2019

Identification and mapping of riverbed sediment facies in the Columbia River through integration of field observations and numerical simulations

In the Hanford Reach of the Columbia River, a thin layer of recent alluvium overlies the sedimentary formations that comprise the unconfined groundwater aquifer. Experimental and modeling studies have demonstrated that this alluvial layer exerts significant control on the exchange of groundwater and surface water (hydrologic exchange flux), and is associated with elevated levels of biogeochemical activity. This layer is also observed to be strongly heterogeneous, and quantifying the spatial distribution of properties over the range of scales of interest is challenging. Facies are elements of a sediment classification scheme that groups complex geologic materials into a set of discrete classes according to distinguishing features. Facies classifications have been used as a framework for assigning heterogeneous material properties to grid cells of numerical models of flow and reactive transport in subsurface media. The usefulness of such an approach hinges on being able to relate facies to quantitative properties needed for flow and reactive transport modeling, and on being able to map facies over the domain of interest using readily available information. While aquifer facies have been used in various modeling contexts, application of this concept to riverbed sediments is relatively new. Here we describe an approach for categorizing and mapping recent alluvial (riverbed) sediments based on the integration of diverse observations with numerical simulations of river hydrodynamics. The facies have distinct distributions of sediment texture which correspond to variations in hydraulic properties, and therefore provide a useful framework for assigning heterogeneous properties in numerical simulations of hydrologic exchange flows and biogeochemical processes.

Hou, Zhangshuan↗
DOE OSTI2016

Identification of high transverse momentum top quarks in pp collisions at $ \sqrt{s}=8 $ TeV with the ATLAS detector

This study presents studies of the performance of several jet-substructure techniques, which are used to identify hadronically decaying top quarks with high transverse momentum contained in large-radius jets. The efficiency of identifying top quarks is measured using a sample of top-quark pairs and the rate of wrongly identifying jets from other quarks or gluons as top quarks is measured using multijet events collected with the ATLAS experiment in 20.3 fb -1 of 8 TeV proton-proton collisions at the Large Hadron Collider. Predictions from Monte Carlo simulations are found to provide an accurate description of the performance. The techniques are compared in terms of signal efficiency and background rejection using simulations, covering a larger range in jet transverse momenta than accessible in the dataset. Finally and additionally, a novel technique is developed that is optimized to reconstruct top quarks in events with many jets.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗