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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Ultrafast Yttrium Hydride Chemistry at High Pressures via Non-equilibrium States Induced by an X-ray Free Electron Laser

Controlling the formation and stoichiometric content of the desired phases of materials has become of central interest for a variety of fields. The possibility of accessing metastable states by initiating reactions by X-ray-triggered mechanisms over ultrashort time scales has been enabled by the development of X-ray free electron lasers (XFELs). Utilizing the exceptionally high-brilliance X-ray pulses from the EuXFEL, we report the synthesis of a previously unobserved yttrium hydride under high pressure, along with nonstoichiometric changes in hydrogen content as probed at a repetition rate of 4.5 MHz using time-resolved X-ray diffraction. Furthermore, exploiting non-equilibrium pathways, we synthesize and characterize a hydride in a Weaire–Phelan structure type at pressures as low as 125 GPa, predicted using a crystal structure search, with a hydrogen content of 4.0–5.75 hydrogens per cation, that is enthalpically metastable on the convex hull.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Poincaré beams from a free electron laser

Poincaré beams are light beams that have spatially inhomogeneous polarization structure that spans a finite portion of the Poincaré sphere. This feature bestows the beams with intriguing topological properties and has led to a surge in research on their fundamental characteristics, their controlled generation and on emerging applications. Here we present an experimental demonstration of a Poincaré beam generated in the extreme ultraviolet (16.7 nm) at the FERMI free electron laser (FEL). The ‘star’ type Poincaré beam is generated by exploiting the phase and intensity structure intrinsic to FEL radiation without relying on optical elements. Here, we controlled the spatial polarization distribution through a precise overlap and power balance between two FEL pulses, each with different transverse phase distributions and orthogonal circular polarizations. The spatial polarization structure was mapped in detail and shows extensive coverage of the Poincaré sphere, in agreement with analytic predictions. This method of in situ Poincaré beam production in FELs enables straightforward flexibility in the orientation and balance of polarization states, and can readily be extended to other vector beams and to shorter wavelengths enabling novel science applications in modern light sources.

Morgan, Jenny [SLAC National Accelerator Laborator↗
DOE OSTI2024

Protocols for x-ray transient grating pump/optical probe experiments at x-ray free electron lasers

Abstract Transient grating spectroscopy is a specialized application of the four-wave-mixing methodology and constitutes a versatile technique for investigating the dynamics of vibrational, magnetic and electronic degrees of freedom of matter in a background-free fashion. Recent developments in free-electron laser sources have enabled the extension of this technique into the extreme ultraviolet range. Ongoing efforts to expand transient grating spectroscopy into the x-ray regime promise numerous advantages: (1) substantial penetration depths that allow for probing bulk material properties, (2) element specificity via specific core-excited states, and (3) short wavelengths that allow for excitation gratings with higher momentum transfer and improved spatial resolution. In this study, we comprehensively outline the procedures for conducting x-ray transient grating pump/optical probe experiment. The process encompasses the design and alignment of the experimental setup, as well as the subsequent steps involved in data acquisition and analysis. This paper is intended as a comprehensive guide for researchers interested in implementing x-ray transient grating spectroscopy, providing valuable insights into the intricacies of the experimental workflow required for this novel technique. Furthermore, we discuss the potential for extending this methodology to an x-ray pump/x-ray probe scheme, envisioning a future direction that holds promise for enhancing the capabilities and scope of x-ray transient grating spectroscopy, opening new opportunities for studying ultrafast processes with unprecedented temporal and spatial resolutions.

Optics↗
DOE OSTI2024

Finite element procedure for thermomechanical and structural integrity analysis of beam intercepting devices subjected to free electron laser

High-energy particles, including photons (x-ray, γ-ray, bremsstrahlung), electrons, and protons, possess the capability to penetrate materials and deposit energy within them. The degree of absorption depends on both the energy and type of particles, as well as the properties of the materials with which they interact. This energy deposition can manifest either at the material's surface or throughout its volume, potentially resulting in various failure modes. The primary aim of this paper is to establish a structured analysis methodology for evaluating the structural integrity of beam-intercepting devices when subjected to high-energy particles. Here, the paper also reviews some of the underlying physics, pertinent to the scope of the thermomechanical analysis, potential failure modes, and introduces verification and validation methodologies. Engineers and researchers can utilize the guidelines presented in this paper to effectively plan the development of beam intercepting devices, thereby ensuring their reliability and performance in the presence of high-energy particle exposure.

Finite element analysis↗
NASA NTRS1982

Free-electron laser from wave-mechanical beats of 2 electron beams

It is possible, though technically difficult, to produce beams of free electrons that exhibit beats of a quantum mechanical nature. (1) the generation of electromagnetic radiation, e.g., light, based on the fact that the beats give rise to alternating charge and current densities; and a frequency shifter, based on the fact that a beam with beats constitutes a moving grating. When such a grating is exposed to external radiation of suitable frequency and direction, the reflected rediation will be shifted in frequency, since the grating is moving. A twofold increase of the frequency is readily attainable. It is shown that it is impossible to generate radiation, because the alternating electromagnetic fields that accompany the beats cannot reform themselves into freely propagating waves. The frequency shifter is useless as a practical device, because its reflectance is extremely low for realizable beams.

Lichtenstein, R. M.↗
DOE OSTI2025

Imaging a light-induced molecular elimination reaction with an X-ray free-electron laser

Tracking the motion of individual atoms during chemical reactions represents a severe experimental challenge, especially if several competing reaction pathways exist or if the reaction is governed by the correlated motion of more than two molecular constituents. Here we demonstrate how ultrashort X-ray pulses combined with coincident ion imaging can be used to trace molecular iodine elimination from laser-irradiated diiodomethane (CH 2 I 2 ), a reaction channel of fundamental importance but small relative yield that involves the breaking of two molecular bonds and the formation of a new one. We map bending vibrations of the bound molecule, disentangle different dissociation pathways, image the correlated motion of the iodine atoms and the methylene group leading to molecular iodine ejection, and trace the vibrational motion of the formed product. Our results provide a quantitative mechanistic picture behind previously suggested reaction mechanisms and prove that a variety of geometries are involved in the molecular bond formation.

Atomic and molecular interactions with photons↗
DOE OSTI2024

ORBITAL ANGULAR MOMENTUM BEAMS RESEARCH USING A FREE-ELECTRON LASER OSCILLATOR

Strong Hadron Cooling (SHC), utilizing the coherent electron cooling scheme, has been extensively investigated for the Electron Ion Collider (EIC). Throughout our cooling optimization studies, we realized that a Super-Gaussian electron bunch offers enhanced performance in comparison to a Gaussian bunch. Our approach involves initiating the electron beam distribution in a double peak form, transitioning them into a Super-Gaussian distribution due to the longitudinal space charge. Subsequently, a chicane within the linac section compresses the bunch to meet the required bunch length. We tuned a third harmonic cavity amplitude to reduce the nonlinear term of the chicane. Moreover, given the low initial current leading to a small but non-uniform slice energy spread, we evaluated utilizing laser heating techniques to achieve a uniformly distributed slice energy spread. In this report, we discuss the concepts and simulation results

Wang, E.↗
DOE OSTI2024

ORBITAL ANGULAR MOMENTUM BEAMS RESEARCH USING A FREE-ELECTRON LASER OSCILLATOR

We present a Fixed-Field-Alternating (FFA) permanent magnet racetrack electron accelerator with energy range between 10-60 GeV for the future LHeC. Electron beam is brought back to the linac by the single beam line without requiring electric power REDUCING estimated wall power of 100 MW in the present LHeC design to a negligible power for arcs as the permanent magnets are used. The design is based on experience from the very successful commissioning of the Cornell University and Brookhaven National Laboratory Energy Recovery Test Accelerator ? ?CBETA?. The proposal supports sustainability efforts for LHeC by making a 'green' accelerator. It is an energy recovery linac with 99.9% energy efficiency and reduces the power consumption by using small permanent magnets. The FFA non-linear gradient design is a racetrack shape, where, as in the CBETA, the arcs are matched by adiabatic transition to the two (LHeC) or multiple straight sections. Two 10 GeV superconducting linacs are placed on both sides of the Interaction Region (IR) significantly reducing the power of synchrotron radiation loss.

Trbojevic, D.↗
NASA NTRS1984

Orbital stability in combined uniform axial and three-dimensional wiggler magnetic fields for free-electron lasers

Zachary Phys. Rev. A 29 (6), 3224 (1984) recently analyzed the instability of relativistic-electron helical trajectories in combined uniform axial and helical wiggler magnetic fields when the radial variation of the wiggler field is taken into account. It is shown here that the type 2 instability comprised of secular terms growing linearly in time, identified by Zachary and earlier by Diament Phys. Rev. A 23 (5), 2537 (1981), is an artifact of simple perturbation theory. A multiple-time-scale perturbation analysis reveals a nonsecular evolution on a slower time scale which accommodates an arbitrary initial perturbation. It is shown that, in the absence of exponential instability, the electron seeks a modified helical orbit more appropriate to its perturbed state and oscillates stably about it. Thus, the perturbed motion is oscillatory but nonsecular, and hence the helical orbits are stable.

Johnston, S.↗
NASA NTRS1989

An ultraviolet gas-loaded free-electron laser

By loading the wiggler cavity of an FEL with hydrogen gas, it is possible to tune the FEL to below 130 nm, just above the electronic resonance of molecular hydrogen. The change in wavelength results from the refractive index of the gas, which alters the phase velocity of the wave and so modifies the synchronism condition. Using the parameters of the wiggler on the beamline of the Stanford Superconducting Accelerataor, this FEL can be tuned from 500 to 130 nm with a pressure ranging from 0 to 55 torr. The calculated electronic gain varies between 5.6 and 11 percent over this wavelength interval, comparable to the gain in vacuum.

Reid, Max B.↗
NASA NTRS1993

The free-electron laser in a symmetrical confocal resonator

A tapered wiggler is used in a FEL oscillator to improve the saturation efficiency. During signal buildup the tapered wiggler does not provide optimum phase synchronism between the electron beam and the electromagnetic wave, resulting in an appreciable loss in small-signal gain. This problem can be ameliorated by using a multicomponent wiggler, which is a combination of a uniform wiggler and a tapered section. During buildup, gain is primarily contributed by the linear element, and at high power levels the gain and efficiency are enhanced by the taper. Ideally, one would like to have the optical waist location near the linear section at small-signal levels and at near the tapered section at high power levels. Placing the FEL in a symmetrical confocal resonator approaches this desired effect automatically since it has the unique characteristic that a stable mode exists for all locations of the waist of a Gaussian beam along the axis of the interferometer.

Ozcan, Meric↗
DOE OSTI2024

DOE Phase II Final Technical Report Bright Electron Source for X-ray Free Electron Lasers Award Number DE-SC0020607 Prepared for U.S. Department of Energy, Office of Science, SC-1 For the Period May 3, 2021 – August 2, 2024 Report Date November 25, 2024 Submitted by Harish B. Bhandari, Ph.D., Principal Investigator Report Contributors Dr. Oleg Maksimov, RMD Inc. Dr. Bryan Rachmilowitz, RMD Inc. Dr. Jared Maxson, Cornell University Dr. Hisato Yamaguchi, LANL

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Bhandari, Harish↗