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At least 73 records · Page 4
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Trace Adsorptive Removal of PFAS from Water by Optimizing the UiO‐66 MOF Interface

Abstract The confluence of pervasiveness, bioaccumulation, and toxicity in freshwater contaminants presents an environmental threat second to none. Exemplifying this trifecta, per‐ and polyfluoroalkyl substances (PFAS) present an alarming hazard among the emerging contaminants. State‐of‐the‐art PFAS adsorbents used in drinking water treatment, namely, activated carbons and ion‐exchange resins, are handicapped by low adsorption capacity, competitive adsorption, and/or slow kinetics. To overcome these shortcomings, metal–organic frameworks (MOFs) with tailored pore size, surface, and pore chemistry are promising alternatives. Thanks to the compositional modularity of MOFs and polymer–MOF composites, herein we report on a series of water‐stable zirconium carboxylate MOFs and their low‐cost polymer‐grafted composites as C 8 –PFAS adsorbents with benchmark kinetics and “parts per billion” removal efficiencies. Bespoke insights into the structure–function relationships of PFAS adsorbents are obtained by leveraging interfacial design principles on solid sorbents, creating a synergy between the extrinsic particle surfaces and intrinsic molecular building blocks.

Ilić, Nebojša↗
DOE OSTI2025

Solar Cell Efficiency Tables (Version 66)

Consolidated tables showing an extensive listing of the highest independently confirmed efficiencies for solar cells and modules are presented. Guidelines for inclusion of results into these tables are outlined, and new entries since January 2025 are reviewed.

14 SOLAR ENERGY↗
DOE OSTI2021

Substitution of virgin carbon fiber with low-cost recycled fiber in automotive grade injection molding polyamide 66 for equivalent composite mechanical performance with improved sustainability

Recycled carbon fiber has historically proven challenging to integrate into composite manufacturing due in no small part to the low-density, randomly oriented, discontinuous fiber format that results from typical recycling. Discontinuous fiber requires the use of alternative technologies than those traditionally applied to continuous fiber (e.g., hand lay-up, winding). Extrusion compounding is one such applicable technology, but material transfer into the system requires alternative feeding equipment or the use of an altered procedure as trialed in this research. In this study, an injection molding compound for automotive applications was prepared with recycled carbon fiber and compared against an existing commercial compound. Input fibers and molded compound were evaluated for mechanical performance, while relevant variables such as compounded fiber alignment and aspect ratio were compared to the existing baseline material to confirm a like-for-like composite material structure. Overall, analysis indicates that recycled fiber performs similarly to virgin fiber reinforcement, demonstrating that recycled fiber may be a viable drop-in replacement for short-fiber discontinuous applications.

42 ENGINEERING↗
DOE OSTI2017

Benzimidazole-functionalized Zr-UiO-66 nanocrystals for luminescent sensing of Fe{sup 3+} in water

Zr-based MOF structure UiO-66 exhibits unprecedented high thermal and chemical stability, making it to be one of the most used MOFs in various applications. Yet, the poor photoluminescent (PL) properties of UiO-66 limit its applications in luminescent sensing. Herein, a new benzimidazole-functionalized UiO-66 nanocrystal (UiO-66-BI) was successfully fabricated via microwave synthesis. UiO-66-BI displayed octahedral nanocrystal morphology with a diameter smaller than 200 nm and could disperse well in water and common organic solvents. UiO-66-BI demonstrated extended optical absorption in the visible-light region and efficiently improved PL emission compared with UiO-66 pristine. The sensing properties of UiO-66-BI nanocrystals towards different ions were studied, and the results demonstrated that UiO-66-BI showed excellent selective luminescent sensing of Fe{sup 3+} ions in water.

36 MATERIALS SCIENCE↗
DOE OSTI2011

THE MASSIVE PROGENITOR OF THE POSSIBLE TYPE II-LINEAR SUPERNOVA 2009hd IN MESSIER 66

We present early- and late-time photometric and spectroscopic observations of supernova (SN) 2009hd in the nearby spiral galaxy NGC 3627 (M66). This SN is one of the closest to us in recent years and provides an uncommon opportunity to observe and study the nature of SNe. However, the object was heavily obscured by dust, rendering it unusually faint in the optical given its proximity. We find that the observed properties of SN 2009hd support its classification as a possible Type II-Linear SN (SN II-L), a relatively rare subclass of core-collapse SNe. High-precision relative astrometry has been employed to attempt to identify an SN progenitor candidate, based on a pixel-by-pixel comparison between Hubble Space Telescope (HST) F555W and F814W images of the SN site prior to explosion and at late times. A progenitor candidate is identified in the F814W images only; this object is undetected in F555W. Significant uncertainty exists in the astrometry, such that we cannot definitively identify this object as the SN progenitor. Via insertion of artificial stars into the pre-SN HST images, we are able to constrain the progenitor's properties to those of a possible supergiant, with intrinsic absolute magnitude M {sup 0}{sub F555W} {approx}> -7.6 mag and intrinsic color (V - I){sup 0} {approx}> 0.99 mag. The magnitude and color limits are consistent with a luminous red supergiant (RSG); however, they also allow for the possibility that the star could have been more yellow than red. From a comparison with theoretical massive-star evolutionary tracks which include rotation and pulsationally enhanced mass loss, we can place a conservative upper limit on the initial mass for the progenitor of M{sub ini} {approx}< 20 M{sub Sun }. If the actual mass of the progenitor is near the upper range allowed by our derived mass limit, then it would be consistent with that for the identified progenitors of the SN II-L 2009kr and the high-luminosity SN II-Plateau (II-P) 2008cn. The progenitors of these three SNe may possibly bridge the gap between lower-mass RSGs that explode as SNe II-P and luminous blue variables, or more extreme RSGs, from which the more exotic SNe II-narrow may arise. Very late time imaging of the SN 2009hd site may provide us with more clues regarding the true nature of its progenitor.

79 ASTRONOMY AND ASTROPHYSICS↗