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At least 703 records · Page 39

On the effectiveness of neural operators at zero-shot weather downscaling

Machine-learning (ML) methods have shown great potential for weather downscaling. These data-driven approaches provide a more efficient alternative for producing high-resolution weather datasets and forecasts compared to physics-based numerical simulations. Neural operators, which learn solution operators for a family of partial differential equations, have shown great success in scientific ML applications involving physics-driven datasets. Neural operators are grid-resolution-invariant and are often evaluated on higher grid resolutions than they are trained on, i.e., zero-shot super-resolution. Given their promising zero-shot super-resolution performance on dynamical systems emulation, we present a critical investigation of their zero-shot weather downscaling capabilities, which is when models are tasked with producing high-resolution outputs using higher upsampling factors than are seen during training. To this end, we create two realistic downscaling experiments with challenging upsampling factors (e.g., 8x and 15x) across data from different simulations: the European Centre for Medium-Range Weather Forecasts Reanalysis version 5 (ERA5) and the Wind Integration National Dataset Toolkit. While neural operator-based downscaling models perform better than interpolation and a simple convolutional baseline, we show the surprising performance of an approach that combines a powerful transformer-based model with parameter-free interpolation at zero-shot weather downscaling. We find that this Swin-Transformer-based approach mostly outperforms models with neural operator layers in terms of average error metrics, whereas an Enhanced Super-Resolution Generative Adversarial Network-based approach is better than most models in terms of capturing the physics of the ground truth data. We suggest their use in future work as strong baselines.

17 WIND ENERGY↗

From Latent Dynamics to Meaningful Representations

While representation learning has been central to the rise of machine learning and artificial intelligence, a key problem remains in making the learnt representations meaningful. For this the typical approach is to regularize the learned representation through prior probability distributions. However such priors are usually unavailable or are ad hoc. To deal with this, recent efforts have shifted towards leveraging the insights from physical principles to guide the learning process. In this spirit, we propose a purely dynamics-constrained representation learning framework. Instead of relying on predefined probabilities, we restrict the latent representation to follow overdamped Langevin dynamics with a learnable transition density — a prior driven by statistical mechanics. We show this is a more natural constraint for representation learning in stochastic dynamical systems, with the crucial ability to uniquely identify the ground truth representation. We validate our framework for different systems including a real-world fluorescent DNA movie dataset. Here, we show that our algorithm can uniquely identify orthogonal, isometric and meaningful latent representations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Episodic Magma Hammers for the 15 January 2022 Cataclysmic Eruption of Hunga Tonga‐Hunga Ha'apai

Understanding the forces and magma system dynamics on timescales of seconds to minutes remains challenging. In the January 2022 phreatoplinian Hunga Tonga-Hunga Ha'apai eruption, four remarkably similar seismic subevents within a 5-min interval occurred during the intensifying early eruptive phase. The subevents are similar in waveforms and durations (~25 s each). Each subevent begins with an unusual negative P-wave polarity which is inferred, using full-wave seismic modeling, to be caused by an upward single-force mechanism at the volcano created by a magma hammer likely in response to magma flow blockage/constriction during the early part of the eruption as discharge rapidly increased over orders of magnitude with concomitant conduit geometry evolution and instability. Our proposed episodic magma hammer model is consistent with thermodynamic and phase properties of the magmatic mixture, and yields an estimate of conduit mass flow in agreement with vent discharge rates derived from satellite imagery of plume heights.

58 GEOSCIENCES↗

Lagrangian Characterization of Surface Transport From the Equatorial Atlantic to the Caribbean Sea Using Climatological Lagrangian Coherent Structures and Self‐Organizing Maps

Abstract This study presents an assessment of the transport of suspended material by surface ocean currents, which have a critical role in determining the connectivity and distribution of living and non‐living material. Lagrangian experiments reveal pathways from the Equatorial Atlantic to 10 strategic regions within the Caribbean Sea, determined by considering the space‐time variability of climatological Lagrangian Coherent Structures, which act as recurrent attracting pathways and transport barriers. Due to windage or Stokes drift, wind forcing is a significant factor in determining the spatial locations where particles cluster and the time needed to reach the Caribbean from the Equatorial Atlantic. Pathways shift westward within the Caribbean and take less time to arrive with increasing wind influence. Depending on the wind effect, the particles show higher confluence in different areas of the Caribbean. A case study is presented for the Mexican Caribbean nearshore area, isolated from ocean‐current trajectories. Here, wind weakens the transport barrier responsible for this isolation and causes particle confluence toward that region. Spatial patterns of the Eulerian velocity identified through Self‐Organizing Maps, with time dependence given by their best matching units, can reproduce the characteristic Lagrangian patterns of surface current climate variability. Our study demonstrates the application of tools from dynamical systems and unsupervised neural networks to understand Lagrangian patterns and identify the processes that drive them. These findings improve our understanding of transport mechanisms of suspended material by surface ocean currents in the Western Atlantic and the Caribbean Sea, which is essential for managing and conserving marine ecosystems.

Allende‐Arandía, Ma. Eugenia↗

Causally‐Informed Deep Learning to Improve Climate Models and Projections

Abstract Climate models are essential to understand and project climate change, yet long‐standing biases and uncertainties in their projections remain. This is largely associated with the representation of subgrid‐scale processes, particularly clouds and convection. Deep learning can learn these subgrid‐scale processes from computationally expensive storm‐resolving models while retaining many features at a fraction of computational cost. Yet, climate simulations with embedded neural network parameterizations are still challenging and highly depend on the deep learning solution. This is likely associated with spurious non‐physical correlations learned by the neural networks due to the complexity of the physical dynamical system. Here, we show that the combination of causality with deep learning helps removing spurious correlations and optimizing the neural network algorithm. To resolve this, we apply a causal discovery method to unveil causal drivers in the set of input predictors of atmospheric subgrid‐scale processes of a superparameterized climate model in which deep convection is explicitly resolved. The resulting causally‐informed neural networks are coupled to the climate model, hence, replacing the superparameterization and radiation scheme. We show that the climate simulations with causally‐informed neural network parameterizations retain many convection‐related properties and accurately generate the climate of the original high‐resolution climate model, while retaining similar generalization capabilities to unseen climates compared to the non‐causal approach. The combination of causal discovery and deep learning is a new and promising approach that leads to stable and more trustworthy climate simulations and paves the way toward more physically‐based causal deep learning approaches also in other scientific disciplines.

Meteorology & Atmospheric Sciences↗

A Non‐Intrusive Machine Learning Framework for Debiasing Long‐Time Coarse Resolution Climate Simulations and Quantifying Rare Events Statistics

Abstract Due to the rapidly changing climate, the frequency and severity of extreme weather is expected to increase over the coming decades. As fully‐resolved climate simulations remain computationally intractable, policy makers must rely on coarse‐models to quantify risk for extremes. However, coarse models suffer from inherent bias due to the ignored “sub‐grid” scales. We propose a framework to non‐intrusively debias coarse‐resolution climate predictions using neural‐network (NN) correction operators. Previous efforts have attempted to train such operators using loss functions that match statistics. However, this approach falls short with events that have longer return period than that of the training data, since the reference statistics have not converged. Here, the scope is to formulate a learning method that allows for correction of dynamics and quantification of extreme events with longer return period than the training data. The key obstacle is the chaotic nature of the underlying dynamics. To overcome this challenge, we introduce a dynamical systems approach where the correction operator is trained using reference data and a coarse model simulation nudged toward that reference. The method is demonstrated on debiasing an under‐resolved quasi‐geostrophic model and the Energy Exascale Earth System Model (E3SM). For the former, our method enables the quantification of events that have return period two orders longer than the training data. For the latter, when trained on 8 years of ERA5 data, our approach is able to correct the coarse E3SM output to closely reflect the 36‐year ERA5 statistics for all prognostic variables and significantly reduce their spatial biases.

Barthel Sorensen, B.↗

A New Framework for the Attribution of Air‐Sea CO 2 Exchange

Abstract The air‐sea transfer of carbon dioxide can be viewed as a dynamic system through which atmospheric and oceanic processes push surface waters away from thermodynamic equilibrium, while diffusive gas transfer pulls them back toward local equilibrium. These push/pull processes drive significant sub‐seasonal, seasonal, and interannual variability in air‐sea carbon fluxes, the quantification of which is critical both for diagnosing the ocean response to fossil fuel emissions and for attempts to mitigate anthropogenic climate disruption through intentional modification of surface ocean biogeochemistry. In this study, we present a new approach for attributing air‐sea carbon fluxes to specific mechanisms. The new framework is first applied to a two‐box ocean nutrient and carbon cycle model as an illustrative example. Next, outputs from a regional eddy‐resolving model of the Southern Ocean are analyzed. The roles of multiple physical and biogeochemical processes are identified. The decomposition of the seasonal air‐sea carbon flux shows the dominant role of biological carbon pumps that are partially compensated by the transport convergence. Finally, the framework is used to diagnose the response to mesoscale iron and alkalinity release, explicitly quantifying transport feedback and eventual impacts on net air‐sea carbon flux. Ocean carbon transport has divergent influences between iron and alkalinity release, due to opposing near‐surface gradients of dissolved inorganic carbon. We suggest that our attribution framework may be a useful analytical technique for monitoring natural ocean carbon fluxes and quantifying the impacts of human intervention on the ocean carbon cycle.

Ito, Takamitsu [School of Earth and Atmospheric Sc↗

Discovering the Multisectoral Impacts of Global Energy Sector Outcomes Through Multiple Ensemble Aggregation Measures

Understanding complex human-Earth system interactions often involves analyzing large scenario ensembles that encompass a wide range of plausible futures. These ensembles often require aggregation to summarize information based on specific criteria or conditions. However, previous research using global change scenario ensembles has largely overlooked how the choice of aggregation method influences the interpretation of results. To address this gap, we leverage a large ensemble data set designed to capture broad energy system dynamics generated using the Global Change Analysis Model. We first explore how energy-related uncertainties are propagated to both global and regional water-energy-food sectors. We then conduct a rank correlation analysis across seven ensemble aggregation measures and demonstrate the need to consider multiple measures in global change scenarios. Our results suggest that global water and food sector outcomes in the 21st century vary widely depending on different scenario assumptions. The global energy productivity is projected to improve by the end of the century across all scenarios. Moreover, regions facing water scarcity challenges in 2100 do not always overlap with those facing extreme energy and food sector outcomes. Although rank correlations across seven aggregation measures are relatively stable across sectors, we identify cases where relying on a single measure leads to losing critical information in the full ensemble. Reliance on a single aggregation measure can distort the interpretation of global change scenario outcomes. Instead, adopting multiple ensemble aggregation measures provides a more holistic understanding of global change scenario ensembles.

Kim, Gijoo↗

Imaging grain microstructure in a model ceramic energy material with optically generated coherent acoustic phonons

Characterization of microstructure, chemistry and function of advanced energy materials remains a challenge for instrumentation science with tremendous opportunity for new discoveries. This active area of research is starting to make considerable strides with examples ranging from methodologies that employ bright X-rays, electron microscopy and optical spectroscopy. However, further development of instruments, capable of multimodal measurements, is necessary to fully reveal complex microstructure evolution in realistic environments and dynamical systems that are far from equilibrium. In this regard, laser-based instruments have a unique advantage as multiple measurement methodologies are easily combined into a single instrument using standard optics. A new pump-probe method that uses optically generated acoustic phonons is expanding standard optical characterization by providing depth resolved information. Here we report on a noteworthy extension of this pump-probe method to image grain microstructure in ceria. Rich information regarding the orientation of individual crystallites is obtained by monitoring acoustic phonon velocities and noting how the polarization of the probe beam influences the detected signal amplitude. When paired with other optical microscopies, this methodology will provide new perspectives for optical characterization of ceramic materials.

36 MATERIALS SCIENCE↗

Molecular structure retrieval directly from laboratory-frame photoelectron spectra in laser-induced electron diffraction

Ubiquitous to most molecular scattering methods is the challenge to retrieve bond distance and angle from the scattering signals since this requires convergence of pattern matching algorithms or fitting methods. This problem is typically exacerbated when imaging larger molecules or for dynamic systems with little a priori knowledge. Here, we employ laser-induced electron diffraction (LIED) which is a powerful means to determine the precise atomic configuration of an isolated gas-phase molecule with picometre spatial and attosecond temporal precision. We introduce a simple molecular retrieval method, which is based only on the identification of critical points in the oscillating molecular interference scattering signal that is extracted directly from the laboratory-frame photoelectron spectrum. The method is compared with a Fourier-based retrieval method, and we show that both methods correctly retrieve the asymmetrically stretched and bent field-dressed configuration of the asymmetric top molecule carbonyl sulfide (OCS), which is confirmed by our quantum-classical calculations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Protons on the line

Stable regions in four-dimensional phase space were observed by following the motion of accelerated proton beams subject to nonlinear forces. Here, this provides insights into the physics of dynamical systems and may lead to improved accelerator designs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Stoichiometrically-informed symbolic regression for extracting chemical reaction mechanisms from data

A data-driven computational method is introduced to extract chemical reaction mechanisms from time series chemical concentration data. It is realized through the use of dynamic symbolic regression in which a sparse analytical form for a dynamical system is discoverable from the underlying data. We specifically develop the stoichiometrically-informed symbolic regression (SISR) method to address a standing challenge in complex chemical reaction networks: given a time-series dataset of concentrations of several components, what is the mechanism and the associated rate constants? SISR finds the optimal mechanism, kinetic equations and rate constants by combining differential optimization with a genetic optimization approach that searches a symbolic space of possible reaction mechanisms. Use of SISR in several paradigmatic examples spanning linear and nonlinear reaction schemes results in excellent agreement between true and predicted mechanisms, including when the method is applied to noisy data. The advantages of a stoichiometrically-informed approach such as SISR to address reaction discovery is illustrated through comparison with the use of generic state-of-the-art data-driven approaches.

36 MATERIALS SCIENCE↗

Tracing the outflow kinematics in Type 2 active galactic nuclei

Here, we used a sample of 577 spectra of active galactic nuclei Type 1.8-2 (z < 0.25) taken from the Sloan Digital Sky Survey to trace the influence of the outflow kinematics on the profiles of different emission lines (Hβ, [O III], Hα, [N II], [S II]). All considered lines were fitted with two Gaussian components: one that fits the core of the line, and another that fits the wings. We provide a procedure for decomposition of the Hα+[N II] wavelength band for spectra where these lines overlap. The influence of the gravitational and non-gravitational kinematics on the line components is investigated by comparing the dispersions of the line components with stellar velocity dispersion. We find that wing components of all the considered emission lines have pure non-gravitational kinematics. The core components are consistent with gravitational kinematics for the Hα, [N II], and [S II] lines, while in the [O III] there is evidence for contribution from non-gravitational kinematics. We adopted the wing components as a proxy for the outflow contribution and investigated the outflow kinematics by analysing the correlations between the widths and shifts of the wing components of different lines. For this purpose, we used the subsets in which wing components are detected in both compared lines, and can be fitted independently. We find strong correlations between wing component shifts, as well as between wing component widths of all considered lines, with the exception of the Hβ wing component width. These correlations indicate that outflow dynamics systemically affect all emission lines in the spectrum. However, it reflects with a different strength in their profiles, which is observed as different widths of the wing components. This is investigated by comparison of the mean widths of the wing components in subsets where wing components are present in all lines. The strongest outflow signature is observed in the [O III] lines, which have the broadest wing components; weaker outflow signatures are found in Hα and [N II], and the weakest is found for [S II]. These results imply that the considered lines arise in different parts of an outflowing region.

79 ASTRONOMY AND ASTROPHYSICS↗

Dynamics of bottlebrush polymers

Bottlebrushes are an interesting class of polymers which shows intriguing material properties often associated with dynamics. While dynamical phenomena in linear polymers are well understood and existing theories can describe them in a good way, bottlebrush dynamics have only rarely been investigated. Therefore, we performed dielectric spectroscopy and quasi-elastic neutron scattering to study the dynamics of polydimethylsiloxane-based bottlebrush polymers, PDMS-g-PDMS focusing mostly on the segmental dynamics of the side chains. Comparing the relaxation times of the α – relaxation, tracked with dielectric spectroscopy, of bottlebrush polymers with those of their respective linear side chains show a slowing down once the side chains are attached to the backbone. This effect diminishes and finally vanishes with increasing side chain length. The time and length scale, offered by quasi-elastic neutron scattering, fits for the segmental dynamics together with faster processes. The Q -dependence of the segmental relaxation times allows to classify bottlebrush polymers as heterogenous including a non-Gaussian character. For such a dynamical system, the mean square displacement needs to be separated into single processes before an overall mean square displacement can be generated by applying the time temperature superposition principle.

36 MATERIALS SCIENCE↗

An ideal MHD δW stability analysis that bypasses the Newcomb equation

In the following work, we demonstrate the efficacy of a Riccati δW ideal MHD stability analysis that bypasses the numerically intractable integration of the Newcomb equation. By transforming the linear Newcomb equation into a quadratic Riccati equation, an accurate and equivalent δW analysis is performed that is shown to enjoy some numerical advantages. Additionally, we demonstrate that the Riccati approach is better conditioned than its Newcomb counterpart at the magnetic axis, and we apply dynamical systems insights to examine its behavior at singular points. We further discuss the constraints involved in solving for the extremal admissible perturbations of a δW analysis.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

A broadband wavelet implementation for rapid ultrasound pulse-echo time-of-flight measurements

A broadband wavelet approach to ultrasonic pulse-echo time-of-flight measurements is described. The broadband approach significantly reduces the time required for frequency-dependent pulse-echo measurements, enabling studies of dynamic systems ranging from biological systems to solid-state phase transitions. The described broadband approach is demonstrated in parallel with the more traditional frequency stepping approach to perform ultrasound time-of-flight measurements inside a large volume Paris-Edinburgh press in-situ at a synchrotron source. The broadband wavelet data acquisition process was found to be 1-2 orders of magnitude faster than the steppedfrequency approach, with no compromise in data quality or determined results.

47 OTHER INSTRUMENTATION↗

Advances in coherent coupling between magnons and acoustic phonons

The interaction between magnetic and acoustic excitations have recently inspired many interdisciplinary studies ranging from fundamental physics to circuit implementation. Specifically, the exploration of their coherent interconversion enabled via the magnetoelastic coupling opens a new playground combining straintronics and spintronics, and provides a unique platform for building up on-chip coherent information processing networks with miniaturized magnonic and acoustic devices. In this Perspective, we will focus on the recent progress of magnon-phonon coupled dynamic systems, including materials, circuits, imaging and new physics. In particular, we highlight the unique features such as nonreciprocal acoustic wave propagation and strong coupling between magnons and phonons in magnetic thin-film systems, which provides a unique platform for their coherent manipulation and transduction. We will also review the frontier of surface acoustic wave resonators in coherent quantum transduction and discuss how the novel acoustic circuit design can be applied in microwave spintronics.

36 MATERIALS SCIENCE↗