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At least 703 records · Page 39

The Effects of Aircraft Wake Dynamics on Contrail Development

Results of large-eddy simulations of the development of young persistent ice contrails are presented, concentrating on the interactions between the aircraft wake dynamics and the ice cloud evolution over ages front a few seconds to approx. 30 min. The 3D unsteady evolution of the dispersing engine exhausts, trailing vortex pair interaction and breakup, and subsequent Brunt-Vaisala oscillations of the older wake plume are modeled in detail in high-resolution simulations, coupled with it bulk microphysics model for the contrail ice development. The simulations confirm that the early wake dynamics can have a strong influence on the properties of persistent contrails even at late times. The vortex dynamics are the primary determinant of the vertical extent of the contrail (until precipitate ton becomes significant): and this together with the local wind shear largely determines the horizontal extent. The ice density, ice crystal number density, and a conserved exhaust tracer all develop and disperse in different fashions from each other. The total ice crystal number can be significantly reduced due to adiabatic compression resulting from the downward motion of the vortex system, even for ambient conditions that are substantially supersaturated with respect to ice. The fraction of the initial ice crystals surviving, their spatial distribution and the ice mass distribution are all sensitive to the aircraft type, ambient humidity, assumed initial ice crystal number, and ambient turbulence conditions. There is a significant range of conditions for which a smaller transport such as a B737 produces as significant a persistent contrail as a larger transport such as a B747, even though the latter consumes almost five times as much fuel. The difficulties involved in trying to minimize persistent contrail production are discussed.

Lewellen, D. C.↗

The Cloud-resolving model Radar SIMulator (CR-SIM) Version 3.3: description and applications of a virtual observatory

Ground-based observatories use multi-sensor observations to characterize cloud and precipitation properties. One of the challenges is how to design strategies to best use these observations to understand these properties and evaluate weather and climate models. This paper introduces the Cloud resolving model Radar SIMulator (CR-SIM), which uses output from high-resolution cloud resolving models (CRMs) to emulate multi-wavelength, zenith-pointing, and scanning radar observables and multi-sensor (radar and lidar) products. CR-SIM allows direct comparison between an atmospheric model simulation and remote-sensing products using a forward-modeling framework consistent with the microphysical assumptions used in the atmospheric model. CR-SIM has the flexibility to easily incorporate additional microphysical modules, such as microphysical schemes and scattering calculations, and expand the applications to simulate multi-sensor retrieval products. In this paper, we present several applications of CR-SIM for evaluating the representativeness of cloud microphysics and dynamics in a CRM, quantifying uncertainties in radar-lidar integrated cloud products and multi-Doppler wind retrievals, and optimizing radar sampling strategy using observing system simulation experiments. These applications demonstrate the application of CR-SIM as a virtual observatory operator on high-resolution model output for a consistent comparison between model results and observations to aid interpretation of the differences and improve understanding of the representativeness errors due to the sampling limitations of the ground-based measurements. CR-SIM is licensed under the GNU GPL package and both the software and the user guide are publicly available to the scientific community.

54 ENVIRONMENTAL SCIENCES↗

Optimal Aerosol Parameterization for Remote Sensing Retrievals

We have developed a new algorithm for the retrieval of aerosol and gases from SAGE It1 solar transmission measurements. This algorithm improves upon the NASA operational algorithm in several key aspects, including solving the problem non-linearly and incorporating a new methodology for separating the contribution of aerosols and gases. In order to extract aerosol information we have built a huge database of aerosol models for both stratospheric and tropospheric aerosols, and polar stratospheric cloud particles. This set of models allows us to calculate a vast range of possible extinction spectra for aerosols. and from these, derive a set of eigenvectors which then provide the basis set used in our inversion algorithm. Our aerosol algorithm and retrievals are described in several articles (listed in References Section) published under this grant. In particular they allow us to analyze the spectral properties of aerosols and PSCs and ultimately derive their microphysical properties. We have found some considerable differences between our spectra and the ones derived from the SAGE III operational algorithm. These are interesting as they provide an independent check on the validity of published aerosol data and, in particular, on their associated uncertainties. In order to understand these differences, we are assembling independent aerosol data from other sources with which to make comparisons. We have carried out extensive comparisons of our ozone retrievals with both SAGE III and independent lidar, ozonesonde, and satellite measurements (Polyakov et al., 2004). These show very good agreement throughout the stratosphere and help to quantify differences which can be attributed to natural variation in ozone versus that produced by algorithmic differences. In the mid - upper stratosphere, agreement with independent data was generally within 5 - 20%. but in the lower stratosphere the differences were considerably larger. We believe that a large proportion of this discrepancy in the lower stratosphere is attributable to natural variation, and is also seen in comparisons between lidar and ozonesonde measurements. NO2 profiles obtained with our algorithm were compared to those obtained through the SAGE III operational algorithm and exhibited differences of 20 - 40%. Our retrieved profiles agree with the HALOE NO2 measurements significantly better than those of the operational retrieval. In other work (described below), we are extending our aerosol retrievals into the infrared regime and plan to perform retrievals from combined uv-visible-infrared spectra. This work will allow us to use the spectra to derive the size and composition of aerosols, and we plan to employ our algorithms in the analysis of PSC spectra. We are presently also developing a limb-scattering algorithm to retrieve aerosol data from limb measurements of solar scattered radiation.

Newchurch, Michael J.↗

Inference of cirrus cloud properties using satellite-observed visible and infrared radiances. I - Parameterization of radiance fields

The impact of using phase functions for spherical droplets and hexagonal ice crystals to analyze radiances from cirrus is examined. Adding-doubling radiative transfer calculations are employed to compute radiances for different cloud thicknesses and heights over various backgrounds. These radiances are used to develop parameterizations of top-of-the-atmosphere visible reflectance and IR emittance using tables of reflectances as a function of cloud optical depth, viewing and illumination angles, and microphysics. This parameterization, which includes Rayleigh scattering, ozone absorption, variable cloud height, and an anisotropic surface reflectance, reproduces the computed top-of-the-atmosphere reflectances with an accruacy of +/- 6 percent for four microphysical models: 10-micron water droplet, small symmetric crystal, cirrostratus, and cirrus uncinus. The accuracy is twice that of previous models.

Minnis, Patrick↗

On the Estimation of In-Cloud Vertical Air Motion Using Radar Doppler Spectra

Measurements of in-cloud vertical air motion are key to quantitatively describe cloud dynamics and their role in cloud microphysics. Here, a retrieval technique for estimating the in-cloud vertical air motion using the upward edge of the radar Doppler spectrum is presented. An additional broadening correction factor that depends on the signal-to-noise ratio (SNR) is introduced. A variety of independent measurements are used to assess the performance of the new technique. The vertical air motion is unbiased with an uncertainty of 0.2 m s –1 for SNR <30. Here, the properties of in-cloud vertical air motion are investigated from 1 year of ground-based observations of warm marine boundary layer clouds. Clouds with higher LWP are characterized by stronger vertical air motions compared to those having lower LWP values.

42 ENGINEERING↗

TPSAS-NF1676L-20101-DND

Aerosols influence climate through their direct and indirect effects. The aerosol indirect effect is based on the way they interact with surrounding clouds. During cloud formation and development, aerosols act as cloud nucleation nuclei (CCN) or ice nuclei, which modifies cloud micro-, macro-physical and radiative properties, and hence helps to shape the Earth's radiation budget. Dominant sources of ocean-derived aerosols that may serve as CCN include sea spray and biogenic aerosol. In this study, we used 10-years global observations from the A-Train satellites to show seasonal variations of cloud droplet number concentrations (CDNC), ocean chlorophyll concentrations, aerosol angstrom parameter, and rainfall. Potential cloud-aerosol interactions are further discussed based on seasonal and spatial correlations between microphysics of clouds and aerosols. Emphasis for this study is placed on the southern ocean and tropical Pacific.

Shan Zeng↗

Evolution of a Florida Cirrus Anvil

This paper presents a detailed study of a single thunderstorm anvil cirrus cloud measured on 21 July 2002 near southern Florida during the Cirrus Regional Study of Tropical Anvils and Cirrus Layers--Florida Area Cirrus Experiment (CRYSTAL-FACE). NASA WB-57F and University of North Dakota Citation aircraft tracked the microphysical and radiative development of the anvil for 3 h. Measurements showed that the cloud mass that was advected downwind from the thunderstorm was separated vertically into two layers: a cirrus anvil with cloud-top temperatures of -45?C lay below a second, thin tropopause cirrus (TTC) layer with the same horizontal dimensions as the anvil and temperatures near -70?C. In both cloud layers, ice crystals smaller than 50 ?m across dominated the size distributions and cloud radiative properties. In the anvil, ice crystals larger than 50 ?m aggregated and precipitated while small ice crystals increasingly dominated the size distributions; as a consequence, measured ice water contents and ice crystal effective radii decreased with time. Meanwhile, the anvil thinned vertically and maintained a stratification similar to its environment. Because effective radii were small, radiative heating and cooling were concentrated in layers approximately 100 m thick at the anvil top and base. A simple analysis suggests that the anvil cirrus spread laterally because mixing in these radiatively driven layers created horizontal pressure gradients between the cloud and its stratified environment. The TTC layer also spread but, unlike the anvil, did not dissipate--perhaps because the anvil shielded the TTC from terrestrial infrared heating. Calculations of top-of-troposphere radiative forcing above the anvil and TTC showed strong cooling that tapered as the anvil evolved.

Garrett, T. J.↗

Synergy of Satellite-Surface Observations for Studying the Properties of Absorbing Aerosols in Asia

Through interaction with clouds and alteration of the Earth's radiation budget, atmospheric aerosols significantly influence our weather and climate. Monsoon rainfalls, for example, sustain the livelihood of more than half of the world's population. Thus, understanding the mechanism that drives the water cycle and freshwater distribution is high-lighted as one of the major near-term goals in NASA's Earth Science Enterprise Strategy. Every cloud droplet/ice-crystal that serves as an essential element in portraying water cycle and distributing freshwater contains atmospheric aerosols at its core. In addition, the spatial and temporal variability of atmospheric aerosol properties is complex due to their dynamic nature. In fact, the predictability of the tropical climate system is much reduced during the boreal spring, which is associated with the peak season of biomass burning activities and regional/long-range transport of dust aerosols. Therefore, to accurately assess the impact of absorbing aerosols on regional-to-global climate requires not only modeling efforts but also continuous observations from satellites, aircraft, networks of ground-based instruments and dedicated field experiments. Since 1997 NASA has been successfully launching a series of satellites the Earth Observing System - to intensively study, and gain a better understanding of, the Earth as an integrated system. Through participation in many satellite remote-sensing/retrieval and validation projects over the years, we have gradually developed and refined the SMART (Surface-sensing Measurements for Atmospheric Radiative Transfer) and COMMIT (Chemical, Optical & Microphysical Measurements of In-situ Troposphere) mobile observatories, a suite of surface remote sensing and in-situ instruments that proved to be vital in providing high temporal measurements, which complement the satellite observations. In this talk, we will present SMART-COMMIT which has played key roles, serving as network or supersite, in major international research projects such as the Joint Aerosol Monsoon Experiment (JAM EX), a core element of the Asian Monsoon Years (AMY, 2008-2012). SMART-COMMIT deployments during 2008 AMY/JAMEX were conducted in northwestern China to characterize the properties of dust-laden aerosols and in the vicinity of Beijing for mega-city aerosols. In 2009, SMART-COMMIT also participated in the JAMEX/RAJO-MEGHA (Radiation, Aerosol Joint Observations-Monsoon Experiment in the Gangetic-Himalayan Area; Sanskrit for Dust-Cloud) to study the aerosol properties, solar absorption and the associated atmospheric warming, and the climatic impact of elevated aerosols during the pre-monsoon season in South Asia. We will show results from these field experiments, as well as discuss a new initiative of 7-SEAS (7 South East Asian Studies) to study the interaction of anthropogenic aerosols with regional meteorology, particularly with clouds.

Tsay, Si-Chee↗

Satellite Investigations of Aerosol Radiative Forcing

Biomass burning aerosols have a wide spatial distribution that is governed by the geographic distribution of their source regions and tropospheric circulation. Annually, more than 114 teragrams of smoke is produced that have residence times ranging from days to weeks depending upon their size and chemical composition. These aerosols reflect the incoming solar directly which is called the "direct effect" and they also modify the reflective properties of clouds which is called the "indirect effect". The direct top of atmosphere (TOA) globally averaged radiative forcing estimate range from -0.2 to -1.1 W/sq m . The uncertainties in this estimate are due to the various assumptions (see Introduction) involved in the calculations. While the TOA radiative forcing estimates provide valuable information on the effects of aerosols on climate, equally important are the downward shortwave irradiances (DSWI) at the surface and the atmospheric heating/cooling rate profiles. For example, the DSWI irradiance calculations show large discrepancies between measurements and calculations in the presence of biomass burning aerosols due to the inaccurate characterization of aerosols in radiative transfer models. The DSWI is an important component of the surface radiation balance and the atmospheric effects govern both local and regional circulation patterns. Very few studies have attempted to estimate the surface and atmospheric effects of biomass burning aerosols largely due to the lack of information on the microphysical and chemical properties of biomass burning aerosols. The major focus of this effort is to estimate the direct TOA radiative forcing of aerosols using satellite measurements.

Christopher, Sundar A.↗

Adaptive Data Screening for Multi-Angle Polarimetric Aerosol and Ocean Color Remote Sensing Accelerated by Automatic Differentiation

Remote sensing measurements from multi-angle polarimeters (MAPs) contain rich aerosol microphysical property information, and these sensors have been used to perform retrievals in optically complex atmosphere and ocean systems. Previous studies have concluded that, generally, five moderately separated viewing angles in each spectral band provide sufficient accuracy for aerosol property retrievals, with performance gradually saturating as angles are added above that threshold. The Hyper-Angular Rainbow Polarimeter (HARP) instruments provide high angular sampling with a total of 90-120 unique angles across four bands, a capability developed mainly for liquid cloud retrievals. In practice, not all view angles are optimal for aerosol retrievals due to impacts of clouds, sun glint, and other impediments. The many viewing angles of HARP can provide resilience to these effects, if the impacted views are screened from the dataset, as the remaining views may be sufficient for successful analysis. In this study, we discuss how the number of available viewing angles impacts aerosol and ocean color retrieval uncertainties, as applied to two versions of the HARP instrument. AirHARP is an airborne prototype that was deployed in the ACEPOL field campaign, while HARP2 is an instrument in development for the upcoming NASA Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission. Based on synthetic data, we find that a total of 20-30 angles across all bands (i.e. five to eight viewing angles per band) are sufficient to achieve good retrieval performance. Following from this result, we develop an adaptive multi-angle polarimetric data screening (MAPDS) approach to evaluate data quality by comparing measurements with their best-fitted forward model. The FastMAPOL retrieval algorithm is used to retrieve scene geophysical values, by matching an efficient, deep learning-based, radiative transfer emulator to observations. The data screening method effectively identifies and removes viewing angles affected by thin cirrus clouds and other anomalies, improving retrieval performance. This was tested with AirHARP data, and we found agreement with the High Spectral Resolution Lidar-2 (HSRL-2) aerosol data. The data screening approach can be applied to modern satellite remote sensing missions, such as PACE, where a large amount of multi-angle, hyperspectral, polarimetric measurements will be collected.

multi-angle polarimeter↗

The Development of Midlatitude Cirrus Models for MODIS Using FIRE-I, FIRE-II, and ARM In Situ Data

Detailed in situ data from cirrus clouds have been collected during dedicated field Campaigns, but the use of the size and habit distribution data has been lagging in the development of more realistic cirrus scattering models. In this study, the authors examine the use of in situ cirrus data collected during three field campaigns to develop more realistic midlatitude cirrus microphysical models. Data are used from the First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment (FIRE)-I (1986) and FIRE-II (1991) campaigns and from a recent Atmospheric Radiation Measurement (ARM) Program campaign held in March-April of 2000. The microphysical models are based on measured vertical distributions of both particle size and particle habit and are used to develop new scattering models for a suite of moderate-resolution imaging spectroradiometer (MODIS) bands spanning visible. near-infrared, and infrared wavelengths. The sensitivity of the resulting scattering properties to the underlying assumptions of the assumed particle size and habit distributions are examined. It is found that the near-infrared bands are sensitive not only to the discretization of the size distribution but also to the assumed habit distribution. In addition. the results indicate that the effective diameter calculated from a given size distribution tends to be sensitive to the number of size bins that are used to discretize the data and also to the ice-crystal habit distribution.

Nasiri, Shaima L.↗

Chapter 10 - Remote Sensing Measurements of Aerosol Properties

Satellite instruments have proven especially capable at monitoring the quantity of airborne particles in columns of atmosphere, globally. This chapter describes the principles of satellite measurements and retrieval algorithms, and surveys current instruments and their capabilities. We outline the issues associated with retrieval algorithms, such as surface characterization and aerosol proximity to clouds, and the challenges with interpretation of the results. The relationship between measured aerosol properties and climate-relevant aerosol properties simulated in models is outlined, as well as how measurements are used to evaluate models. Most space-based aerosol instruments are passive sensors that measure reflected sunlight at multiple wavelengths, some at multiple viewing angles. A few are active sensors that send out their own laser light and measure the returned signal. Except when clouds are present, the excess amount of light scattered back to space, beyond that expected from the surface and atmospheric gas, is attributed to aerosol. Satellite measurements are used in many ways in aerosol research. They often provide the only method for monitoring hazardous phenomena such as major wildfire and volcanic eruption plumes, especially in remote areas. Stable, long-term, near-global-scale satellite data records make it possible to identify regional and global aerosol trends. Aerosol radiative effects on climate can be quantified on a near-global scale and used to estimate the strength of aerosol–radiation and aerosol–cloud interactions as well as to evaluate climate model simulations of these interactions. Aerosol-type mapping from satellite imagery is helpful for source attribution, model validation, and to constrain particle light-absorption properties that are essential for radiative forcing calculations. The range of aerosol properties retrieved from satellite observations has grown considerably since the first global estimates of aerosol optical depth (τ a) over ocean were made in the late 1970s. Methods for retrieving particle size and light-absorption properties were explored in the 1990s using multispectral, multi-angle observations, and polarization in visible and near-infrared wavelengths. Sensitivity to particle light absorption, primarily from black or brown carbon content, improved with the inclusion of UV channels, and sensitivity to very thin aerosol layers in the upper troposphere and lower stratosphere was advanced with the use of limb-sounding instruments and active sensors. There are limitations to every measurement technique, including satellite aerosol remote sensing. For wide-swath, passive instruments, aerosol retrievals near clouds can present substantial challenges as far as 15 km away due to cloud-scattered light contaminating the signal. In nearly all cases, retrievals over bright snow and ice surfaces are precluded because surface reflectance uncertainties can overwhelm the aerosol signal. Similarly, meteorological cloud is identified and masked out where possible. Data from passive sensors also lack vertical resolution except those that view toward the limb or where multi-angle imagery is acquired over plumes from wildfires, erupting volcanoes, and wind-blown dust. Yet, passive sensors provide vastly more coverage than the active instruments that mitigate these issues. Particle microphysical information is qualitative from all remote sensing techniques, relying on proxies to infer particle composition, hygroscopicity, and the amount of light-absorbing material. Further, particles smaller than about 200 nm diameter cannot be distinguished from atmospheric gas molecules with remote sensing, which hinders studies of cloud condensation nuclei and their effects on clouds. Most satellite instruments dedicated to aerosol observations are in low-Earth, near-polar, sun-synchronous orbits, which means they cross the equator at the same local time each day. Most are set on cycles that repeat approximately every 16 days, which makes it difficult to monitor aerosol evolution locally. Geostationary satellites make it possible to observe changes occurring from minutes to hours over regions up to 8000 km in size, but lack coverage of high latitudes, and often provide more limited constraints on aerosol properties. Ground-truth data are vital for satellite aerosol-retrieval validation. The AErosol RObotic NETwork (AERONET) of sun photometers was created in 1993 and has become an established global network of over 350 instruments for validating satellite measurements. The network, as well as global networks of ground-based lidars, solar flux radiometers and other sun photometers, are widely used for evaluating global satellite retrievals and model simulations. NASA's Earth Observing System (EOS) program beginning in 1999 led to improvements in reliability, spatial resolution, and spectral resolution (and hence, to improved particle size discrimination and light absorption properties). Satellite payloads include advanced broad-swath and multi-angle imagers, along with the first space-based active sensor focused largely on long-term aerosol monitoring. Since about 2002, Europe's SENTINEL and operational meteorological satellite fleets are also providing sustained aerosol observations, with planned continuation until at least 2030. Satellite remote sensing instruments offer valuable data for evaluating aerosol representations in global climate models. They have been used to assess aerosol optical and physical properties, trends and distributions, and are applied increasingly as direct model constraints in data assimilation to create global aerosol reanalysis products. Aerosol optical depth is the most common quantity adopted for routine model evaluation, including multiwavelength data to loosely constrain particle-size distributions. These evaluations of multiple models have revealed general biases in their regional aerosol amounts and seasonal patterns of transport and removal. Although satellite measurements have near-global coverage, substantial errors can be introduced into the model observation comparison unless attention is paid to spatial and temporal collocation, cloud screening, subgrid-scale variability, and measurement uncertainties that vary with retrieval conditions.

aerosol properties↗

Atmospheric ice nuclei concentration measurements over a high altitude-station in the Western Ghats, India

Mixed-phase and ice clouds play a significant role in modulating the Indian summer monsoon rainfall, and modeling studies suggest that inaccurate representation of ice nucleating particles (INP) is one of the factors, which have resulted in a deficiency in the prediction of cloud properties and hydrological cycle. We do not understand the ice nucleation mechanisms to represent the ice formation in the model, and therefore more INP measurements at various supercooled temperatures are needed. This study reports for the first time real-time INP concentration at a high altitude station in the Western Ghats region of India, and these results will be used to constrain the ice nucleation parameterizations in the model. The variation of INP for any particular cloud condition can have strong microphysical responses of mixed-phase precipitation formation processes. Also, to improve the representation of heterogeneous ice nucleation, INP measurements of various types of aerosols commonly observed over the Indian region are needed. This study presents, the INP concentrations and daily concentration of non-refractory chemical composition (organics, sulfate, nitrate, ammonium, and chloride), cloud condensation nuclei (CCN), and aerosol size distribution. Spectrometer for Ice Nuclei (SPIN) was operated to measure INP concentration at the mountain site from August to December 2018. INP measurements were performed at three different temperatures (-25, -30, and - 34 °C) in the immersion freezing mode relevant for mixed-phase cloud conditions. The average INP concentrations approximately varied from 0.18 to 12.4 L-1, 0.39 to 24 L-1, 1.1 to 40.2 L-1 at -25, -30, and - 34 °C, respectively. These concentrations are within the concentrations reported in the literature from different regions across the globe. The air mass back trajectory analysis showed that continental air mass contains more INP compared to maritime air mass. The information on INP concentration and chemical characteristics of aerosol will help to improve heterogeneous ice nucleation parameterization in numerical models.

Kumar, Anil V.↗

Examining conditions supporting the development of anomalous charge structures in supercell thunderstorms in the Southeastern United States

Hypotheses regarding favorable conditions for anomalous charging have primarily resulted from studies within the Great Plains region of the United States, where the efficiency of warm precipitation processes is thought to be fundamental. Rare observations of anomalous charge structures in the Southeastern region challenge existing conceptual models used to explain anomalous charging. As a rigorous evaluation of conditions that support anomalous charge structures, environmental characteristics and bulk kinematic and microphysical properties of two normal and two anomalous supercell thunderstorms observed in the Southeast were compared in this paper. Within the anomalous supercells, greater quantities of precipitation ice were identified at higher altitudes and colder temperatures, suggesting a greater depth of riming growth and increased vertical transport of rimed hydrometeors. Deeper anomalous supercell updrafts were larger and stronger in the upper mixed-phase and glaciated regions. However, normal supercells were characterized by more robust low-level updrafts, resulting in comparable warm cloud residence times that suggested warm precipitation processes were not necessarily less efficient in the anomalous supercells. Indications of enhanced mixed-phase liquid water content in favor of anomalous charging were observed in the anomalous supercells, though contrasts in related environmental parameters were not as large as observed in other comparative studies. Anomalous supercell environments were characterized by increased instability, shallower warm cloud depth, as well as lower relative humidity in the 700 mb to 500 mb layer. Evidence of impacts from dry air in anomalous storm structures suggested that water vapor content may have affected particle-scale charge transfer in support of anomalous charge structure development.

54 ENVIRONMENTAL SCIENCES↗

Global Land Surface Emissivity Retrieved From Satellite Ultraspectral IR Measurements

Ultraspectral resolution infrared (IR) radiances obtained from nadir observations provide information about the atmosphere, surface, aerosols, and clouds. Surface spectral emissivity (SSE) and surface skin temperature from current and future operational satellites can and will reveal critical information about the Earth s ecosystem and land-surface-type properties, which might be utilized as a means of long-term monitoring of the Earth s environment and global climate change. In this study, fast radiative transfer models applied to the atmosphere under all weather conditions are used for atmospheric profile and surface or cloud parameter retrieval from ultraspectral and/or hyperspectral spaceborne IR soundings. An inversion scheme, dealing with cloudy as well as cloud-free radiances observed with ultraspectral IR sounders, has been developed to simultaneously retrieve atmospheric thermodynamic and surface or cloud microphysical parameters. This inversion scheme has been applied to the Infrared Atmospheric Sounding Interferometer (IASI). Rapidly produced SSE is initially evaluated through quality control checks on the retrievals of other impacted surface and atmospheric parameters. Initial validation of retrieved emissivity spectra is conducted with Namib and Kalahari desert laboratory measurements. Seasonal products of global land SSE and surface skin temperature retrieved with IASI are presented to demonstrate seasonal variation of SSE.

Zhou, D. K.↗

Large Eddy Simulation of Cirrus Clouds

The Regional Atmospheric Modeling System (RAMS) with mesoscale interactive nested-grids and a Large-Eddy Simulation (LES) version of RAMS, coupled to two-moment microphysics and a new two-stream radiative code were used to investigate the dynamic, microphysical, and radiative aspects of the November 26, 1991 cirrus event. Wu (1998) describes the results of that research in full detail and is enclosed as Appendix 1. The mesoscale nested grid simulation successfully reproduced the large scale circulation as compared to the Mesoscale Analysis and Prediction System's (MAPS) analyses and other observations. Three cloud bands which match nicely to the three cloud lines identified in an observational study (Mace et al., 1995) are predicted on Grid #2 of the nested grids, even though the mesoscale simulation predicts a larger west-east cloud width than what was observed. Large-eddy simulations (LES) were performed to study the dynamical, microphysical, and radiative processes in the 26 November 1991 FIRE 11 cirrus event. The LES model is based on the RAMS version 3b developed at Colorado State University. It includes a new radiation scheme developed by Harrington (1997) and a new subgrid scale model developed by Kosovic (1996). The LES model simulated a single cloud layer for Case 1 and a two-layer cloud structure for Case 2. The simulations demonstrated that latent heat release can play a significant role in the formation and development of cirrus clouds. For the thin cirrus in Case 1, the latent heat release was insufficient for the cirrus clouds to become positively buoyant. However, in some special cases such as Case 2, positively buoyant cells can be embedded within the cirrus layers. These cells were so active that the rising updraft induced its own pressure perturbations that affected the cloud evolution. Vertical profiles of the total radiative and latent heating rates indicated that for well developed, deep, and active cirrus clouds, radiative cooling and latent heating could be comparable in magnitude in the cloudy layer. This implies that latent heating cannot be neglected in the construction of a cirrus cloud model. The probability density function (PDF) of w was analyzed to assist in the parameterization of cloud-scale velocities in large-scale models. For the more radiatively-driven, thin cirrus case, the PDFs are approximately Gaussian. However, in the interior of the deep, convectively unstable case, the PDFs of w are multi-modal and very broad, indicating that parameterizing cloud-scale motions for such clouds can be very challenging. The results of this research are described in detail in a paper submitted to the Journal of Atmospheric Science (Wu and Cotton, 1999), which is enclosed as Appendix 2. Using soundings extracted from a mesoscale simulation of the November 26, 1991 cirrus event, the radiative effects on vapor deposition/sublimation of ice crystals was studied using a two-dimensional cloud-resolving model (CRM) version of RAMS, coupled to an explicit bin-resolving microphysics. The CRM simulations of the November 26, 1991 cirrus event demonstrate that the radiative impact on the diffusional growth (or sublimation) of ice crystals is significant. In this case, the ice particles experienced radiative warming. Model results show that radiative feedbacks in the diffusional growth of ice particles can be very complex. Radiative warming of an ice particle will restrict the particle's diffusional growth. In the case of radiative warming, ice particles larger than a certain size will experience so much radiative warming that surface ice saturation vapor pressures become large enough to cause sublimation of the larger crystals, while smaller crystals are growing by vapor deposition. However, ice mass production can be enhanced in the case of radiative cooling of an ice particle. For the November 26, 1991 cirrus event, radiative feedback results in significant reduction in the total ice mass, especially in the production of large ice crystals, and consequently, both radiative and dynamic properties of the cirrus cloud are significantly affected. A complete description of this research has been submitted as a paper to the Journal of Atmospheric Science (Wu et al., 1999), and included as Appendix 3.

Wu, Ting↗

Cirrus Simulations of CRYSTAL-FACE 23 July 2002 Case

A key objective of the Cirrus Regional Study of Tropical Anvils and Cirrus Layers - Florida Area Cirrus Experiment (CRYSTAL-FACE) is to understand relationships between the properties of tropical convective cloud systems and the properties and lifecycle of the extended cirrus anvils they produce. We report here on a case study of 23 July 2002 where a sequence of convective storms over central Florida produced an extensive anvil outflow. Our approach is to use a suitably-initialized cloud-system simulation with MM5 to define initial conditions and time-dependent forcing for a simulation of anvil evolution using a two-dimensional fine-resolution (100 m) cirrus cloud model that explicitly accounts for details of cirrus microphysical development (bin or spectra model) and fully interactive radiative processes. The cirrus model follows Lin. Meteorological conditions and observations for the 23 July case are described in this volume. The goals of the present study are to evaluate how well we can simulate a cirrus anvil lifecycle, to evaluate the importance of various physical processes that operate within the anvil, and to evaluate the importance of environmental conditions in regulating anvil lifecycle. CRYSTAL-FACE produced a number of excellent case studies of anvil systems that will allow environmental factors, such as static stability or wind shear in the upper troposphere, to be examined. In the present study, we strive to assess the importance of propagating gravity waves, likely produced by the deep convection itself, and radiative processes, to anvil lifecycle and characteristics.

Starr, David↗

Studying Cloud and Radiative Impacts Through an Improved Physically Based Representation of Organic Aerosol in a Large-Scale Model (WRF-Chem) (Final Report)

The work performed under this award resulted in the development of a computationally-efficient kinetic model to simulate the chemistry, thermodynamics, and microphysics of organic aerosol. Versions of the kinetic model were used to study a suite of aerosol processes including, multigenerational gas-phase chemistry, phase-state influenced gas/particle partitioning, heterogeneous oxidation, oligomerization reactions, and experimental artifacts. The kinetic model has now been implemented into a regional chemistry-climate model (WRF-Chem) to further study the formation, evolution, properties, and spatiotemporal distribution of organic aerosol at urban, regional, and global scales.

54 ENVIRONMENTAL SCIENCES↗