Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “NOX”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 703 records · Page 39

Comparison of Surface and Column Variations of CO2 Over Urban Areas for Future Active Remote CO2 Sensors

High resolution in-situ CO2 measurements were recorded onboard the NASA P-3B during the DISCOVER-AQ (Deriving Information on Surface Conditions from Column and Vertically Resolved Observations Relevant to Air Quality) Field Campaign, to investigate the ability of space-based observations to accurately assess near surface conditions related to air quality. This campaign includes, Washington DC/Baltimore, MD (July 2011), San Joaquin Valley, CA (January - February 2013), Houston, TX (September 2013), and Denver, CO (July-August 2014). Each of these campaigns consisted of missed approaches and approximately two hundred vertical soundings of CO2 within the lower troposphere (surface to about 5 km). In this study, surface (0 - 1 km) and column-averaged (0 - 3.5 km) CO2 mixing ratio values from the vertical soundings in the four geographically different urban areas are used to investigate the temporal and spatial variability of CO2 within the different urban atmospheric emission environments. Tracers such as CO, CH2O, NOx, and NMHCs are used to identify the source of CO2 variations in the urban sites. Additionally, we apply nominal CO2 column weighting functions for potential future active remote CO2 sensors operating in the 1.57-microns and 2.05-microns measurement regions to convert the in situ CO2 vertical mixing ratio profiles to variations in CO2 column optical depths, which is what the active remote sensors actually measure. Using statistics calculated from the optical depths at each urban site measured during the DISCOVER-AQ field campaign and for each nominal weighting function, we investigate the natural variability of CO2 columns in the lower troposphere; relate the CO2 column variability to the urban surface emissions; and show the measurement requirements for the future ASCENDS (Active Sensing of CO2 Emissions over Nights, Days, and Seasons) in the continental U.S. urban areas.

Choi, Yonghoon↗

Application of Deterministic and Probabilistic System Design Methods and Enhancements of Conceptual Design Tools for ERA Project

This report documents work done by the Aerospace Systems Design Lab (ASDL) at the Georgia Institute of Technology, Daniel Guggenheim School of Aerospace Engineering for the National Aeronautics and Space Administration, Aeronautics Research Mission Directorate, Integrated System Research Program, Environmentally Responsible Aviation (ERA) Project. This report was prepared under contract NNL12AA12C, "Application of Deterministic and Probabilistic System Design Methods and Enhancement of Conceptual Design Tools for ERA Project". The research within this report addressed the Environmentally Responsible Aviation (ERA) project goal stated in the NRA solicitation "to advance vehicle concepts and technologies that can simultaneously reduce fuel burn, noise, and emissions." To identify technology and vehicle solutions that simultaneously meet these three metrics requires the use of system-level analysis with the appropriate level of fidelity to quantify feasibility, benefits and degradations, and associated risk. In order to perform the system level analysis, the Environmental Design Space (EDS) [Kirby 2008, Schutte 2012a] environment developed by ASDL was used to model both conventional and unconventional configurations as well as to assess technologies from the ERA and N+2 timeframe portfolios. A well-established system design approach was used to perform aircraft conceptual design studies, including technology trade studies to identify technology portfolios capable of accomplishing the ERA project goal and to obtain accurate tradeoffs between performance, noise, and emissions. The ERA goal, shown in Figure 1, is to simultaneously achieve the N+2 benefits of a cumulative noise margin of 42 EPNdB relative to stage 4, a 75 percent reduction in LTO NOx emissions relative to CAEP 6 and a 50 percent reduction in fuel burn relative to the 2005 best in class aircraft. There were 5 research task associated with this research: 1) identify technology collectors, 2) model technology collectors in EDS, 3) model and assess ERA technologies, 4) LTO and cruise emission prediction, and 5) probabilistic analysis of technology collectors and portfolios.

Mavris, Dimitri N.↗

An Overview of Low-Emission Combustion Research at NASA Glenn

An overview of research efforts at NASA Glenn Research Center (GRC) in low-emission combustion technology that have made a significant impact on the nitrogen oxides (NOx) emission reduction in aircraft propulsion is presented. The technology advancements and their impact on aircraft emissions are discussed in the context of NASA's Aeronautics Research Mission Directorate (ARMD) high-level goals in fuel burn, noise and emission reductions. The highlights of the research presented here show how the past and current efforts laid the foundation for the engines that are flying today as well as how the continued technology advancements will significantly influence the next generation of aviation propulsion system designs.

Low-Emission↗

Analysis of Summer-Time Ozone and Precursor Species in the Southeast United States

Ozone (O3) is a greenhouse gas and toxic pollutant which plays a major role in air quality and atmospheric chemistry. The understanding and ability to model the horizontal and vertical structure of O3 mixing ratios is difficult due to the complex formation/destruction processes and transport pathways that cause large variability of O3. The Environmental Protection Agency has National Ambient Air Quality Standards for O3 set at 75 ppb with future standards proposed to be as low as 65 ppb. These lower values emphasize the need to better understand/simulate the transport processes, emission sources, and chemical processes controlling precursor species (e.g., NOx, VOCs, and CO) which influence O3 mixing ratios. The uncertainty of these controlling variables is particularly large in the southeast United States (US) which is a region impacted by multiple different emission sources of precursor species (anthropogenic and biogenic) and transport processes resulting in complex spatio-temporal O3 patterns. During this work we will evaluate O3 and precursor species in the southeast US applying models, ground-based and airborne in situ data, and lidar observations. In the summer of 2013, the UAH O3 Differential Absorption Lidar (DIAL) (part of the Tropospheric Ozone Lidar Network (TOLNet)) measured vertical O3 profiles from the surface up to approximately 12 km. During this period, the lidar observed numerous periods of dynamic temporal and vertical O3 structures. In order to determine the sources/processes impacting these O3 mixing ratios we will apply the CTM GEOS-Chem (v9-02) at a 0.25 deg x 0.3125 deg resolution. Using in situ ground-based (e.g., SEARCH Network, CASTNET), airborne (e.g., NOAA WP-3D - SENEX 2013, DC-8 - SEAC4RS), and TOLNet lidar data we will first evaluate the model to determine the capability of GEOS-Chem to simulate the spatio-temporal variability of O3 in the southeast US. Secondly, we will perform model sensitivity studies in order to quantify which emission sources (e.g., anthropogenic, biogenic, lighting, wildfire) and transport processes (e.g., stratospheric, long-range, local scale) are contributing to these TOLNet-observed dynamic O3 patterns. Results from the evaluation of the model and the study of sources/processes impacting observed O3 mixing ratios will be presented.

Optical Radar↗

An Observationally Constrained Evaluation of the Oxidative Capacity in the Tropical Western Pacific Troposphere

Hydroxyl radical (OH) is the main daytime oxidant in the troposphere and determines the atmospheric lifetimes of many compounds. We use aircraft measurements of O3, H2O, NO, and other species from the Convective Transport of Active Species in the Tropics (CONTRAST) field campaign, which occurred in the tropical western Pacific (TWP) during January-February 2014, to constrain a photochemical box model and estimate concentrations of OH throughout the troposphere. We find that tropospheric column OH (OHCOL) inferred from CONTRAST observations is 12 to 40% higher than found in chemical transport models (CTMs), including CAM-chem-SD run with 2014 meteorology as well as eight models that participated in POLMIP (2008 meteorology). Part of this discrepancy is due to a clear-sky sampling bias that affects CONTRAST observations; accounting for this bias and also for a small difference in chemical mechanism results in our empirically based value of OHCOL being 0 to 20% larger than found within global models. While these global models simulate observed O3 reasonably well, they underestimate NOx (NO +NO2) by a factor of 2, resulting in OHCOL approx.30% lower than box model simulations constrained by observed NO. Underestimations by CTMs of observed CH3CHO throughout the troposphere and of HCHO in the upper troposphere further contribute to differences between our constrained estimates of OH and those calculated by CTMs. Finally, our calculations do not support the prior suggestion of the existence of a tropospheric OH minimum in the TWP, because during January-February 2014 observed levels of O3 and NO were considerably larger than previously reported values in the TWP.

Hydroxyl radical↗

Tropospheric Ozone Source Attribution in Southern California during Summer 2014 Based on Lidar Measurements and Model Simulations

In the past decades, significant efforts have been made to increase tropospheric ozone long-term monitoring. A large number of ground-based, airborne and space-borne instruments are currently providing valuable data to contribute to better understand tropospheric ozone budget and variability. Nonetheless, most of these instruments provide in-situ surface and column-integrated data, whereas vertically resolved measurements are still scarce. Besides ozonesondes and aircraft, lidar measurements have proven to be valuable tropospheric ozone profilers. Using the measurements from the tropospheric ozone differential absorption lidar (DIAL) located at the JPL Table Mountain Facility, California, and the GEOS-Chem and GEOS-5 model outputs, the impact of the North American monsoon on tropospheric ozone during summer 2014 is investigated. The influence of the Monsoon lightning-induced NOx will be evaluated against other sources (e.g. local anthropogenic emissions and the stratosphere) using also complementary data such as backward-trajectories analysis, coincident water vapor lidar measurements, and surface ozone in-situ measurements.

Lidar↗

A51F-0123: Model Analysis of Tropospheric Aerosol Variability and Sources over the North Atlantic During NAAMES 2015-2016

The North Atlantic Aerosols and Marine Ecosystems Study (NAAMES) is a five-year Earth-Venture Suborbital-2 Mission to characterize the plankton ecosystems and their influences on remote marine aerosols, boundary layer clouds, and their implications for climate in the North Atlantic. While marine-sourced aerosols have been shown to make important contributions to surface aerosol loading, cloud condensation nuclei and ice nuclei concentrations over remote marine and coastal regions, it is still a challenge to differentiate the marine biogenic aerosol signal from the strong influence of continental pollution outflow. We examine here the spatiotemporal variability and quantify the sources of tropospheric aerosols over the North Atlantic during the first two phases (November 2015 and May-June 2016) of NAAMES using a state-of-the-art chemical transport model (GEOS-Chem). The model is driven by the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) from the NASA Global Modeling and Assimilation Office (GMAO). It includes sulfate-nitrate-ammonium aerosol thermodynamics coupled to ozone-NOx-hydrocarbon-aerosol chemistry, mineral dust, sea salt, elemental and organic carbon aerosols, and especially a recently implemented parameterization for the marine primary organic aerosol emission. The simulated aerosols over the North Atlantic are evaluated with available satellite (e.g., MODIS) observations of aerosol optical depths (AOD), and aircraft and ship aerosol measurements. We diagnose transport pathways for continental pollution outflow over the North Atlantic using carbon monoxide, an excellent tracer for anthropogenic pollution transport. We also conduct model perturbation experiments to quantify the relative contributions of terrestrial and oceanic sources to the aerosol loading, AOD, and their variability over the North Atlantic.

aerosols↗

Understanding the Laminar Distribution of Tropospheric Ozone from Ground-Based, Airborne, Spaceborne, and Modeling Perspectives

Laminar ozone structure is a ubiquitous feature of tropospheric-ozone distributions resulting from dynamic and chemical atmospheric processes. Understanding the characteristics of these ozone laminae and the mechanisms responsible for producing them is important to outline the transport pathways of trace gases and to quantify the impact of different sources on tropospheric background ozone. In this study, we present a new method to detect ozone laminae to understand their climatological characteristics of occurrence frequency in terms of thickness and altitude. We employ both ground-based and airborne ozone lidar measurements and other synergistic observations and modeling to investigate the sources and mechanisms such as biomass burning transport, stratospheric intrusion, lightning-generated NOx, and nocturnal low-level jets that are responsible for depleted or enhanced tropospheric ozone layers. Spaceborne (e.g., OMI (Ozone Monitoring Instrument), TROPOMI (Tropospheric Monitoring Instrument), TEMPO (Tropospheric Emissions: Monitoring of Pollution)) measurements of these laminae will observe greater horizontal extent and lower vertical resolution than balloon-borne or lidar measurements will quantify. Using integrated ground-based, airborne, and spaceborne observations in a modeling framework affords insight into how to gain knowledge of both the vertical and horizontal evolution of these ubiquitous ozone laminae.

Tropospheric Ozone↗

Nitrous Oxides Ozone Destructiveness Under Different Climate Scenarios

Nitrous oxide (N2O) is an important greenhouse gas and ozone depleting substance as well as a key component of the nitrogen cascade. While emissions scenarios indicating the range of N2O's potential future contributions to radiative forcing are widely available, the impact of these emissions scenarios on future stratospheric ozone depletion is less clear. This is because N2O's ozone destructiveness is partially dependent on tropospheric warming, which affects ozone depletion rates in the stratosphere. Consequently, in order to understand the possible range of stratospheric ozone depletion that N2O could cause over the 21st century, it is important to decouple the greenhouse gas emissions scenarios and compare different emissions trajectories for individual substances (e.g. business-as-usual carbon dioxide (CO2) emissions versus low emissions of N2O). This study is the first to follow such an approach, running a series of experiments using the NASA Goddard Institute for Space Sciences ModelE2 atmospheric sub-model. We anticipate our results to show that stratospheric ozone depletion will be highest in a scenario where CO2 emissions reductions are prioritized over N2O reductions, as this would constrain ozone recovery while doing little to limit stratospheric NOx levels (the breakdown product of N2O that destroys stratospheric ozone). This could not only delay the recovery of the stratospheric ozone layer, but might also prevent a return to pre-1980 global average ozone concentrations, a key goal of the international ozone regime. Accordingly, we think this will highlight the importance of reducing emissions of all major greenhouse gas emissions, including N2O, and not just a singular policy focus on CO2.

stratospheric ozone depletion↗

Overview of Low Emission Combustion Research At NASA Glenn

An overview of research efforts at NASA Glenn Research Center (GRC) in low-emission combustion technology that have made a significant impact on the nitrogen oxides (NOx) emission reduction in aircraft propulsion is presented. The technology advancements and their impact on aircraft emissions are discussed in the context of NASA's Aeronautics Research Mission Directorate (ARMD) high-level goals in fuel burn, noise and emission reductions. The highlights of the research presented here show how the past and current efforts laid the foundation for the engines that are flying today as well as how the continued technology advancements will significantly influence the next generation of aviation propulsion system designs.

Combustion↗

Spatial and Temporal Variability of Ground and Satellite Column Measurements of NO2 and O3 over the Atlantic Ocean During the Deposition of Atmospheric Nitrogen to Coastal Ecosystems Experiment

In situ measurements of O3 and nitrogen oxides (NO + NO2=NOx) and remote sensing measurements of total column NO2 and O3 were collected on a ship in the North Atlantic Ocean as part of the Deposition of Atmospheric Nitrogen to Coastal Ecosystems (DANCE) campaign in July August 2014,100 km east of the mid-Atlantic United States. Relatively clean conditions for both surface in situ mixing ratio and total column O3 and NO2 measurements were observed throughout the campaign. Increased surface and column NO2 and O3 amounts were observed when a terrestrial air mass was advected over the study region. Relative to ship-based total column measurements using a Pandora over the entire study, satellite measurements overestimated total column NO2 under these relatively clean atmospheric conditions over offshore waters by an average of 16. Differences are most likely due to proximity, or lack thereof, to surface emissions; spatial averaging due to the field of view of the satellite instrument; and the lack of sensitivity of satellite measurements to the surface concentrations of pollutants. Total column O3 measurements from the shipboard Pandora showed good correlation with the satellite measurements(r 0.96), but satellite measurements were 3 systematically higher than the ship measurements, in agreement with previous studies. Derived values of boundary layer height using the surface in situ and total column measurements of NO2 are much lower than modeled and satellite-retrieved boundary layer heights, which highlight the differences in the vertical distribution between terrestrial and marine environments.

Martins, Douglas K.↗

Nitrogen Dioxide Observations from the Geostationary Trace Gas and Aerosol Sensor Optimization (GeoTaso) Airborne Instrument: Retrieval Algorithm and Measurements During DISCOVER-AQ Texas 2013

The Geostationary Trace gas and Aerosol Sensor Optimization (GeoTASO) airborne instrument is a test bed for upcoming air quality satellite instruments that will measure backscattered ultraviolet, visible and near-infrared light from geostationary orbit. GeoTASO flew on the NASA Falcon aircraft in its first intensive field measurement campaign during the Deriving Information on Surface Conditions from Column and Vertically Resolved Observations Relevant to Air Quality (DISCOVER-AQ) Earth Venture Mission over Houston, Texas, in September 2013. Measurements of backscattered solar radiation between 420 and 465 nm collected on 4 days during the campaign are used to determine slant column amounts of NO2 at 250 m x 250 m spatial resolution with a fitting precision of 2.2 x 10(exp 15) molecules/sq cm. These slant columns are converted to tropospheric NO2 vertical columns using a radiative transfer model and trace gas profiles from the Community Multiscale Air Quality (CMAQ) model. Total column NO2 from GeoTASO is well correlated with ground-based Pandora observations (r = 0.90 on the most polluted and cloud-free day of measurements and r = 0.74 overall), with GeoTASO NO2 slightly higher for the most polluted observations. Surface NO2 mixing ratios inferred from GeoTASO using the CMAQ model show good correlation with NO2 measured in situ at the surface during the campaign (r = 0.85). NO2 slant columns from GeoTASO also agree well with preliminary retrievals from the GEO-CAPE Airborne Simulator (GCAS) which flew on the NASA King Air B200 (r = 0.81, slope = 0.91). Enhanced NO2 is resolvable over areas of traffic NOx emissions and near individual petrochemical facilities.

Aerosol Sensor Optimization↗

Model Validation for Propulsion - On the TFNS and LES Subgrid Models for a Bluff Body Stabilized Flame

With advances in computational power and availability of distributed computers, the use of even the most complex of turbulent chemical interaction models in combustors and coupled analysis of combustors and turbines is now possible and more and more affordable for realistic geometries. Recent more stringent emission standards have enticed the development of more fuel-efficient and low-emission combustion system for aircraft gas turbine applications. It is known that the NOx emissions tend to increase dramatically with increasing flame temperature. It is well known that the major difficulty, when modeling the turbulence-chemistry interaction, lies in the high non-linearity of the reaction rate expressed in terms of the temperature and species mass fractions. The transport filtered density function (FDF) model and the linear eddy model (LEM), which both use local instantaneous values of the temperature and mass fractions, have been shown to often provide more accurate results of turbulent combustion. In the present, the time-filtered Navier-Stokes (TFNS) approach capable of capturing unsteady flow structures important for turbulent mixing in the combustion chamber and two different subgrid models, LEM-like and EUPDF-like, capable of emulating the major processes occurring in the turbulence-chemistry interaction will be used to perform reacting flow simulations of a selected test case. The selected test case from the Volvo Validation Rig was documented by Sjunnesson.

bluff body↗

NASA Environmentally Responsible Aviation's Highly-Loaded Front Block Compressor Demonstration

The ERA project was created in 2009 as part of NASAs Aeronautics Research Mission Directorates (ARMD) Integrated Systems Aviation Program (IASP). The purpose of the ERA project was to explore and document the feasibility, benefit, and technical risk of vehicles concepts and enabling technologies to reduce aviations impact on the environment. The metrics for this technology is given in Figure 1 with the N+2 metrics highlighted in green. It is anticipated that the United States air transportation system will continue to expand significantly over the next few decades thus adversely impacting the environment unless new technology is incorporated to simultaneously reduce nitrous oxides (NOx), noise and fuel consumption. In order to achieve the overall goals and meet the technology insertion challenges, these goals were divided into technical challenges that were to be achieved during the execution of the ERA project. Technical challenges were accomplished through test campaigns conducted by Integrated Technology Demonstration (ITDs). ERAs technical performance period ended in 2015.

Environment↗

Fuel and Combustor Concerns for Future Commercial Combustors

Civil aircraft combustor designs will move from rich-burn to lean-burn due to the latter's advantage in low NOx and nvPM emissions. However, the operating range of lean-burn is narrower, requiring premium mixing performance from the fuel injectors. As the OPR increases, the corresponding combustor inlet temperature increase can benefit greatly with fuel composition improvements. Hydro-treatment can improve coking resistance, allowing finer fuel injection orifices to speed up mixing. Selective cetane number control across the fuel carbon-number distribution may allow delayed ignition at high power while maintaining low-power ignition characteristics.

Combustor↗

Advanced Environmental Barrier Coating Development for SiC-SiC Ceramic Matrix Composite Components

This presentation reviews the NASA advanced environmental barrier coating (EBC) system development for SiC-SiC Ceramic Matrix Composite (CMC) combustors particularly under the NASA Environmentally Responsible Aviation, Fundamental Aeronautics and Transformative Aeronautics Concepts Programs. The emphases have been placed on the current design challenges of the 2700-3000F capable environmental barrier coatings for low NOX emission combustors for next generation turbine engines by using advanced plasma spray based processes, and the coating processing and integration with SiC-SiC CMCs and component systems. The developments also have included candidate coating composition system designs, degradation mechanisms, performance evaluation and down-selects; the processing optimizations using TriplexPro Air Plasma Spray Low Pressure Plasma Spray (LPPS), Plasma Spray Physical Vapor Deposition and demonstration of EBC-CMC systems. This presentation also highlights the EBC-CMC system temperature capability and durability improvements under the NASA development programs, as demonstrated in the simulated engine high heat flux, combustion environments, in conjunction with high heat flux, mechanical creep and fatigue loading testing conditions.

CMAS↗

Production of Peroxy Nitrates in Boreal Biomass Burning Plumes over Canada During the BORTAS Campaign

The observations collected during the BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites (BORTAS) campaign in summer 2011 over Canada are analysed to study the impact of forest fire emissions on the formation of ozone (O3 and total peroxy nitrates (sigma)PNs, (sigma)ROONO2. The suite of measurements on board the BAe-146 aircraft, deployed in this campaign, allows us to calculate the production of O3 and of (sigma)PNs, a long-lived NOx reservoir whose concentration is supposed to be impacted by biomass burning emissions.In fire plumes, profiles of carbon monoxide (CO), which is a well-established tracer of pyrogenic emission, show concentration enhancements that are in strong correspondence with a significant increase of concentrations of (sigma)PNs, where as minimal increase of the concentrations of O3 and NO2 is observed. The (sigma)PN and O3 productions have been calculated using the rate constants of the first- and second-order react Pions of volatile organic compound (VOC) oxidation. The (sigma)PN and O3 productions have also been quantified by 0-D model simulation based on the Master Chemical Mechanism. Both methods show that in fire plumes the average production of (sigma)PNs and O3 are greater than in the background plumes, but the increase of (sigma)PN production is more pronounced than the O3 production. The average (sigma)PN production in fire plumes is from 7 to 12 times greater than in the background, whereas the average O3 production in fire plumes is from 2 to 5 times greater than in the background. These results suggest that, at least for boreal forest fires and for the measurements recorded during the BORTAS campaign,fire emissions impact both the oxidized NOy and O3;but (1)(sigma)PN production is amplified significantly more thanO3 production and (2) in the forest fire plumes the ratio between the O3 production and the (sigma)PN production is lower than the ratio evaluated in the background air masses, thus confirming that the role played by the (sigma)PNs produced during biomass burning is significant in the O3 budget. The implication of these observations is that fire emissions in some cases, for example boreal forest fires and in the conditions reported here, may influence more long-lived precursors of O3than short-lived pollutants, which in turn can be transported and eventually diluted in a wide area.

biomass burning↗

Air Quality Modeling Using the NASA GEOS-5 Multispecies Data Assimilation System

The NASA Goddard Earth Observing System (GEOS) data assimilation system (DAS) has been expanded to include chemically reactive tropospheric trace gases including ozone (O3), nitrogen dioxide (NO2), and carbon monoxide (CO). This system combines model analyses from the GEOS-5 model with detailed atmospheric chemistry and observations from MLS (O3), OMI (O3 and NO2), and MOPITT (CO). We show results from a variety of assimilation test experiments, highlighting the improvements in the representation of model species concentrations by up to 50% compared to an assimilation-free control experiment. Taking into account the rapid chemical cycling of NO2 when applying the assimilation increments greatly improves assimilation skills for NO2 and provides large benefits for model concentrations near the surface. Analysis of the geospatial distribution of the assimilation increments suggest that the free-running model overestimates biomass burning emissions but underestimates lightning NOx emissions by 5-20%. We discuss the capability of the chemical data assimilation system to improve atmospheric composition forecasts through improved initial value and boundary condition inputs, particularly during air pollution events. We find that the current assimilation system meaningfully improves short-term forecasts (1-3 day). For longer-term forecasts more emphasis on updating the emissions instead of initial concentration fields is needed.

Keller, Christoph A.↗