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All sourcesNASA NTRSDOE OSTI
NASA NTRS1994

Multifrequency emission from hot ion disks

The discovery of a large number of gamma-emitting active galactic nuclei (AGNs) by the EGRET instrument on the Compton Gamma Ray Observatory (CGRO) has spawned a lot of theoretical interest in the high-energy and multifrequency emission from these objects. Since most of them show evidence for relativistic outflow, jet models have received most of the attention so far. However, the presence of soft photons at the center of the active nucleus and the resulting Compton drag make it difficult to produce the observed amount of MeV/GeV emission. We explore hot, two-temperature accretion disks around Kerr black holes as an alternative to relativistic beam models for the production of the high-enerty emission. The decay of neutral pions created in the hot region produces photons with energies up to several hundred MeV. Relativistic pairs created as a result of charged pion decays produce additional inverse-Compton radiation in the range of approx. 1 keV-4 MeV if the pairs are exposed to UV radiation, or in the range of approx. 40 keV-150 MeV if the pairs are exposed to soft X-rays. This suggests that high-energy flares in AGNs may be triggered by changes in the disk structure (such as phase transitions or the development of electron scattering coronae) that temporarily shield the hot inner region from UV photons emitted at larger radii, thereby reducing the optical depth for MeV/GeV gamma-rays. Stochastic processes may also play a role in accelerating the utrarelativistic electrons responsible for producing the highest energy (GeV) emission.

Maisack, Michael↗
DOE OSTI2020

An updated estimate of the Mu2e experiment sensitivity

The Mu2e experiment at Fermilab will search for the conversion of a negative muon into an electron inside the field of a nucleus. This process does not conserve charged-lepton flavour and is heavily suppressed in the Standard Model (SM), with a branching ratio < 10-50. Any evidence of it would be an undeniable evidence of new physics beyond the SM. The project sets out to achieve a single event sensitivity of $\sim 3 × 10^{-17}$ on the ratio between the probability for a conversion of a negative muon into an electron and the one for a muon capture by the nucleus. Such a sensitivity would represent a 4 orders of magnitude improvement on the previous upper limit for the process, making possible to test predictions of different extensions of the SM. Mu2e uses three superconducting solenoids to produce and measure the muon conversions. In the first solenoid, the Production Solenoid, pions and kaons are produced, together with other secondary products, by 8 GeV kinetic energy proton interactions in a tungsten target. A gradient magnetic field is specifically designed to direct low momentum particles into the Transport Solenoid, an S-shaped magnet that filters out particles with unwanted charge and momentum. Muons, produced by pion and kaon decays, finally reach the aluminum Stopping Target in the Detector Solenoid, where they eventually stop and convert. The result of the conversion process is a monochromatic electron of ~105 MeV/c momentum. The Detector Solenoid also hosts the two main detectors: a straw tube tracker and two CsI calorimeter disks, both providing measurement of event kinematics. A germanium detector and a LaBr crystal are located downstream of the Detector Solenoid to measure the X and gamma rays produced by the muon captures in the Stopping Target. A veto system of scintillators covering the Detector Solenoid and half of the Transport Solenoid is used to identify and reject cosmic rays interactions. With respect to the initial project, the Mu2e running plan has evolved to a staged configuration with 2 years at reduced intensity before the 2025 accelerator shutdown for the neutrino beam upgrade and 2 or 3 years at full intensity after that. This, together with geometry changes and a better knowledge of detector performances obtained by the first slice tests, has required a full revision of the signal over background selection that is the subject of this thesis. In order to achieve a new estimate of Mu2e sensitivity, the simulation of the data corresponding to the first 2 years of data acquisition has been performed. This includes both conversion electrons (CE) and the main sources of background: cosmics, decay-in orbits (DIO), radiative pion captures (RPC) and antiprotons. The characteristics of the signal and of the main backgrounds have been studied to define the best selection variables for CE. A special effort has been devoted to the evaluation of the antiproton background. The lack of experimental data for antiproton production cross section makes the systematic uncertainty on this background significant. A new parameterization of the cross section has been developed to fit the existing data and to provide a more reliable estimate of the systematic uncertainty by comparing the results of the old and the new model. A special effort has been devoted to the optimization of the antiprotons Monte Carlo generator. This study has also revealed that the dominant component within this background is represented by antiprotons produced in the opposite direction with respect to the Transport Solenoid entrance and then redirected to it by back-scattering processes in the Production Target. This ultimately highlights the sensitivity of the background estimate to the G4 handling of antiproton interactions in the 1 to 3 GeV/c momentum range. Finally, the final experimental sensitivity has been studied. The momentum and time selection have been optimized to obtain the 5-sigma discovery reach or, in case of no signal, the upper limit on conversion probability. The results confirm that, in the firs t two years of data taking, Mu2e will be able to improve the current experimental sensitivity for muon-to-electron conversion in an atomic field by more than 3 order of magnitudes.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS2013

The First FERMI-LAT Gamma-Ray Burst Catalog

In three years of observations since the beginning of nominal science operations in 2008 August, the Large Area Telescope (LAT) on board the Fermi Gamma-Ray Space Telescope has observed high-energy great than (20 MeV) gamma-ray emission from 35 gamma-ray bursts (GRBs). Among these, 28 GRBs have been detected above 100 MeV and 7 GRBs above approximately 20 MeV. The first Fermi-LAT catalog of GRBs is a compilation of these detections and provides a systematic study of high-energy emission from GRBs for the first time. To generate the catalog, we examined 733 GRBs detected by the Gamma-Ray Burst Monitor (GBM) on Fermi and processed each of them using the same analysis sequence. Details of the methodology followed by the LAT collaboration for the GRB analysis are provided. We summarize the temporal and spectral properties of the LAT-detected GRBs. We also discuss characteristics of LAT-detected emission such as its delayed onset and longer duration compared with emission detected by the GBM, its power-law temporal decay at late times, and the fact that it is dominated by a power-law spectral component that appears in addition to the usual Band model.

gamma-ray burst: general↗
DOE OSTI2022

Positron Emission Intensity in the Decay of 86 gY for Use in Dosimetry Studies

The β + -emitting radionuclide 86 gY (t 1/2 = 14.7 h) forms a matched-pair with the β – -emitting therapeutic radionuclide 90Y (t 1/2 = 2.7 d) for theranostic application in medicine. This approach demands a precise knowledge of the positron emission probability of the PET nuclide which was until recently rather uncertain for 86 gY. In this work, an 86 gY source of high radionuclidic purity was prepared and a direct measurement of the positron emission intensity per 100 decay of the parent (hereafter “positron emission intensity”) was performed using high-resolution HPGe detector γ-ray spectroscopy. The electron capture intensity was also determined as an additional check by measuring the K α and K β X-rays of energies 14.1 and 15.8 keV, respectively, using a low energy HPGe detector. From those measurements, normalized values of 27.2 ± 2.0% for β + -emission and 72.8 ± 2.0% for EC were obtained. These results are in excellent agreement with values recently reported in the literature based on a detailed decay scheme study.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2025

Binary neutron star mergers as potential sources for ultrahigh-energy cosmic rays and high-energy neutrinos

Recent studies suggest that the most energetic cosmic rays, exceeding 100 EeV, may primarily consist of 𝑟-process nuclei. This highlights binary neutron star mergers and collapsars as promising sources of ultrahigh-energy cosmic rays (UHECRs). Building on these insights, we examine the conditions that facilitate the efficient production of UHE 𝑟-process nuclei during the prompt radiation (PR), extended emission (EE), and plateau emission phases of short gamma-ray bursts (sGRBs) following neutron star mergers. Our study reveals that jets associated with the PR phase, characterized by typical bulk Lorentz factors (≳ 400–500), dissipation radii, and magnetic field strengths, can accelerate 𝑟-process nuclei to energies ≳ 100 EeV, while preserving them during propagation within the source. Additionally, we investigate the production of HE neutrinos from photomeson and hadronic interactions, as well as from the 𝛽 decay of accelerated 𝑟-process nuclei. We find that the HE neutrino fluxes from sGRBs, mainly produced via photomeson interactions, are significantly limited to preserve the accelerated heavy nuclei, leading to lower fluxes than the predictions without allowing for contributions to UHECRs. Our results suggest that sGRBs may potentially contribute to UHECRs during the PR phase and to HE neutrinos during the EE phase—a scenario that can be tested by future neutrino observatories.

Cosmic ray sources↗
DOE OSTI2023

Recommended Nuclear Structure and Decay Data for A = 200 Isobars

Evaluated nuclear structure and decay data for all nuclei with mass number A = 200 ( 200 Os, 200 Ir, 200 Pt, 200 Au, 200 Hg, 200 Tl, 200 Pb, 200 Bi, 200 Po, 200 At, 200 Rn, and 200 Fr), are presented. All available experimental data are compiled and evaluated, and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities and transition probabilities, as well as other nuclear properties, are recommended. Inconsistencies and discrepancies that exist in the literature are discussed. A number of computer codes (https://www-nds.iaea.org/public/ensdf pgm/) developed by members of the NSDD network were used during the evaluation process. In conclusion, this work supersedes the earlier evaluation by F.G. Kondev and S. Lalkovski (2007Ko42), published in Nuclear Data Sheets 108, 1471 (2007).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
NASA NTRS2012

In-situ Measurements of the Radiolytic Destruction of Glycine in Ices: Applications to the Martian Subsurface

Amino acids and other organic molecules are thought to be easily destroyed on the surface of Mars by the high flux of incident ultraviolet rays or by chemical interactions with oxidizing substances in the soil. However, organic molecules may survive in the subsurface, where chemical processes are driven by penetrating galactic cosmic rays such as MeV protons. Models of the radiation dose as a function of depth on Mars have shown that the contribution of galactic cosmic rays dominates from about one centimeter to a few meters [1 J. Theoretical models have also been published to aid in understanding molecular destruction at these depths, but these usually are based on room-temperature laboratory data, studies of single-component samples, and ex-situ methods of chemical analysis. Recent studies of amino-acid survivability include those involving UV photolysis [2, 3J and gamma radiolysis [4], but nearly all chemical and kinetic analyses from such experiments involved room-temperature measurements on samples irradiated and then removed from sealed containers. We report new laboratory studies of the radiation-induced destruction of glycine-containing ices. In-situ infrared spectroscopy was used to study decay rates as a function of temperature and initial glycine concentrations. Our results indicate that glycine's destruction rate depends on temperature, the presence of H20-ice, and the initial relative abundance of glycine. These trends are not obvious in previous work, suggesting that room-temperature measurements on pure glycine's radiation stability are not directly applicable to Mars and other environments.

Gerakines, Perry A.↗
DOE OSTI2020

Confronting Dark Matter with the Multiwavelength Sky (Final Technical Report)

The existence of dark matter is a key clue to new fundamental physics, yet its nature and non-gravitational interactions remain mysterious. In the course of this five-year project (spanning July 2015 - July 2020), we have developed novel analysis techniques to separate dark matter signals from astrophysical backgrounds in the inner Galaxy, and measured hitherto-unknown properties of the Fermi Bubbles and the Galactic Center excess in gamma-rays from the inner Milky Way. We have improved predictions for the spatial distribution and energy spectra of photon signals from dark matter, and set new limits from astrophysical and cosmological datasets on dark matter inhabiting complex dark sectors, multi-particle dark matter annihilation, and tiny primordial black holes. We have successfully adapted effective field theory techniques from collider physics to make high-precision predictions for signals from heavy weakly-interacting DM, allowing us to essentially exclude the possibility that DM is a thermal wino, and have discovered novel theoretical and observational implications for dark matter bound states and self-interactions. We have developed a comprehensive public code package for modeling the effects of exotic energy injections, such as from dark matter annihilation and decay, on the ionization and temperature history of the early cosmos, and have used these tools to set robust, powerful and broadly-applicable constraints on models of light dark matter.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2000

GRB970228: A Supernova Gamma-Ray Burst

We present B-, V-, R(sub c)-, I(sub c)-, J-, H-, and K-band observations of the optical transient (OT) associated with GRB970228 based on a reevaluation of published data. and present yet unpublished data. In order to minimize small calibration differences we collected and analyzed most of the photometry and determined the magnitude of the OT relative to a set of secondary field stars. We confirm that the early decay of the light curves (before March 6. 1997) was faster than that at later times (between March 6 and April 7. 1997). The early-time observations of GRB 970228 are consistent with relativistic blast wave models but the late-time observations are hard to understand in this framework. The observations are well explained by an initial power law decay with alpha = -1.46 +/- 0.33 modified at later times by a type-I(sub c) supernova light curve. together with the evidence for GRB980326 and GRB 980425 this is further evidence that at least some GRBs are associated with an unusual class of core-collapse supernovae.

Galama, T. J.↗
NASA NTRS1990

Measurement of the 0.3-8.5 MeV Galactic gamma-ray spectrum from the Galactic center direction

The low-energy gamma-ray spectrum from the direction of the Galactic center is determined using data obtained with the SMM Gamma-Ray Spectrometer. It is found that the diffuse gamma-ray spectrum from the Galactic center region can be interpreted in a straightforward way as the sum of five components of a presented equation. The components include a hard power law dominating the continuum at high energies caused principally by cosmic ray electron bremsstrahlung radiation, two narrow lines due to Al-26 decay and positron annihilation, an excess continuum component below 0.511 MeV consistent with the annihilation of positrons by formation of Ps, and a soft power law at low energies which is consistent with an extrapolation upward in energy of known hard X-ray sources in the Galactic center region.

Harris, M. J.↗
NASA NTRS1992

A liquid xenon imaging telescope for gamma ray astrophysics: Design and expected performance

A high resolution telescope for imaging cosmic x ray sources in the MeV region, with an angular resolution better than 0.5 deg is being developed as balloon-borne payload. The instrument consists of a 3-D liquid xenon TPC as x ray detector, coupled with a coded aperture at a distance of 1 meter. A study of the actual source distribution of the 1.809 MeV line from the decay of Al-26 and the 511 keV positron-electron annihilation line is among the scientific objectives, along with a search for new x ray sources. The telescope design parameters and expected minimum flux sensitivity to line and continuum radiation are presented. The unique capablity of the LXe-TPC as a Compton Polarimeter is also discussed.

Aprile, E.↗
NASA NTRS1986

Cosmic gamma-ray lines

Recent observations of gamma-ray line emissions from gamma-ray bursts, the ISM, the Galactic center, and solar flares are reviewed, and the implications of these observations for high-energy processes in these sources are discussed. Line observations suggest that magnetized neutron stars are probably the best candidate objects for burst sources. Observations of the 1.809-MeV line from Al-26 decay provide evidence for ongoing nucleosynthesis in the Galaxy and information on the spatial distribution of nucleosynthetic sites. The compact 0.511-MeV line source is probably a black hole at or close to the Galactic center. Solar-flare studies have provided new information on the confinement and escape of charged particles at the sun and on multiple acceleration phases in solar flares.

Ramaty, R.↗
NASA NTRS1988

Gamma-ray observations of Co-56 in SN 1987A

During observations of SN 1987A 286 days after the supernova explosion using a JPL high-resolution gamma-ray spectrometer, a line feature was found in the net supernova spectrum at an energy of 1240.8 + or - 1.7 keV, with an intrinsic width of 8.2 + or - 3.4 keV FWHM, and a net flux of 0.0021 + or - 0.0007 photons/sq cm per s. This feature is interpreted as the 1238 keV line from the decay of Co-56 in the supernova remnant. The blueshift and intrinsic broadening of the 1238 keV line are consistent with models incorporating mixing of the radioactive cobalt in the expanding eject.

Mahoney, W. A.↗
DOE OSTI2021

Efficient Prompt Scintillation and Fast Neutron-Gamma Ray Discrimination Using Amorphous Blends of Difluorenylsilane Organic Glass and in-situ Polymerized Vinyltoluene

High performance radiation detection materials are an integral part of national security, medical imaging, and nuclear physics applications. Those that offer compositional and manufacturing versatility are of particular interest. In this work, we report a new family of radiological particle-discriminating scintillators containing bis(9,9-dimethyl-9H-fluoren-2- yl)diphenylsilane (compound “P2”) and in-situ polymerized vinyltoluene (PVT) that is phase stable and mechanically robust at any blend ratio. The gamma-ray light yield increases nearly linearly across the composition range, to ~16,400 photons/MeV at 75 % wt. P2. These materials are also capable of γ/n pulse shape discrimination (PSD) and between 20-50 % P2 loading are competitive with the PSD quality of commercially-available plastic scintillators. The 137 Cs scintillation rise and decay times are sensitive to P2 loading and approach the values for “pure” P2. Additionally, the radiation detection performance of P2-PVT blends can be made stable in 60°C air for at least 1.5 months with the application of a thin film of poly(vinylalcohol) to the scintillator surfaces.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1973

Energy spectra of cosmic gamma-ray bursts

Spectral measurements of six cosmic gamma-ray bursts in the energy region of 0.1 to 1.2 MeV, made using a semi-omnidirectional X-ray detector on IMP-6 are reported. These measurements confirm the hard X-ray or gamma-ray nature of the bursts, as inferred from the original observations by Klebesadel et al., (1973), and show that their maximum energy release is in this several hundred keV region. Each burst consists of several 1 or 2-second pulses each with the characteristic spectrum of approximately 150-keV exponential, followed by a softer decay. There is no evidence of line structure in this energy region, or for a marked change in the energy spectrum within a given pulse. Event size spectra are estimated for galactic and extragalactic models; the total emission is consistent with present measurements of the diffuse background, and unlikely to account for any spectral feature in the few-MeV region.

Cline, T. L.↗
NASA NTRS1986

Results of a search for a new class of GRBS in the SMM data

The results of a search for the soft and short Gamma-Ray Bursts (GRBs) in the data of the Hard X-Ray Burst Spectrometer (HXRBS) on the Solar Maximum Mission (SMM) are presented. Data for four events are presented, including their time profiles and spectral characteristics. In one case the instrument time resolution reveals a total burst duration of 55 ms with rise and decay times of less than about 5 ms.

Kouveliotou, C.↗
NASA NTRS1991

GRIS instrument continuum results from SN1987A

Results on the continuum emission from SN1987A from two balloon flights of gamma-ray imaging spectrometer over Alice Springs, Australia, in the spring and fall of 1988 are presented. The durations of the two observations were 11.2 and 11.7 hours, respectively. The measured continuum spectra (95-2560 keV for the spring and 55-2560 keV for the fall) are consistent with Compton scattering of the Co-56 decay lines. The 10HMM model agrees well with continuum data in the energy dependence of the continuum both in the slope of the spectra and the step increases below the 2599, 1238, and 847 keV Co-56 decay lines.

Barthelmy, S.↗
DOE OSTI2024

Elucidating the Radiation-Induced Redox Chemistry of Plutonium Under Used Nuclear Fuel Reprocessing Conditions

Plutonium plays a critical role in the development of sustainable nuclear fuel cycles, and yet, our fundamental understanding of this element’s inherent radiation-induced redox chemistry and associated impacts on nuclear fuel cycle technologies is limited. Unanticipated changes in oxidation state distribution can influence the speciation and transport of plutonium in a given process. Control of these parameters is especially important for used nuclear fuel reprocessing technologies, wherein the separation and recovery of plutonium is typically achieved by the selective formation, maintenance, and complexation of specific oxidation states. Furthermore, plutonium’s inherent radiation-induced redox chemistry has the capacity to influence the radiolytic behavior of its complexes, the longevity of which are critical in the design of efficient and cost-effective advanced reprocessing technologies. These radiation-induced processes are unavoidable under fuel cycle conditions owing to the inherency of ionizing radiation fields to the decay of plutonium’s isotopes and to the various other radioisotopes generated by nuclear fission and neutron-capture process and the subsequent radioactive decay of their products. As such, mechanistically understanding the response of plutonium’s multiple oxidation states to multi-component ionizing radiation fields is essential for predicting the behavior of this critical element under used nuclear fuel reprocessing conditions. Here, through a combination of time-resolved (electron pulse) and steady-state (alpha and gamma) irradiation experiments complemented by quantitative, multiscale modeling calculations, we present advances in our understanding of radiation-induced plutonium redox chemistry!

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗