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At least 685 records · Page 38

A Method to Analyze How Various Parts of Clouds Influence Each Other's Brightness

This paper proposes a method for obtaining new information on 3D radiative effects that arise from horizontal radiative interactions in heterogeneous clouds. Unlike current radiative transfer models, it can not only calculate how 3D effects change radiative quantities at any given point, but can also determine which areas contribute to these 3D effects, to what degree, and through what mechanisms. After describing the proposed method, the paper illustrates its new capabilities both for detailed case studies and for the statistical processing of large datasets. Because the proposed method makes it possible, for the first time, to link a particular change in cloud properties to the resulting 3D effect, in future studies it can be used to develop new radiative transfer parameterizations that would consider 3D effects in practical applications currently limited to 1D theory-such as remote sensing of cloud properties and dynamical cloud modeling.

Varnai, Tamas↗

Development of a Random-Forest Cloud-Regime Classification Model Based on Surface Radiation and Cloud Products

Various methods have been developed to characterize cloud type, otherwise referred to as cloud regime. These include manual sky observations, combining radiative and cloud vertical properties observed from satellite, surface-based remote sensing, and digital processing of sky imagers. While each method has inherent advantages and disadvantages, none of these cloud-typing methods actually includes measurements of surface shortwave or longwave radiative fluxes. Here, a method that relies upon detailed, surface-based radiation and cloud measurements and derived data products to train a random-forest machine-learning cloud classification model is introduced. Measurements from five years of data from the ARM Southern Great Plains site were compiled to train and independently evaluate the model classification performance. A cloud-type accuracy of approximately 80% using the random-forest classifier reveals that the model is well suited to predict climatological cloud properties. Furthermore, an analysis of the cloud-type misclassifications is performed. While physical cloud types may be misreported, the shortwave radiative signatures are similar between misclassified cloud types. From this, we assert that the cloud-regime model has the capacity to successfully differentiate clouds with comparable cloud–radiative interactions. Therefore, we conclude that the model can provide useful cloud-property information for fundamental cloud studies, inform renewable energy studies, and be a tool for numerical model evaluation and parameterization improvement, among many other applications.

54 ENVIRONMENTAL SCIENCES↗

Understanding and Utilizing PBL Height Data from Multiple Observing Systems in the GEOS System

The accuracy of PBL height simulation is a key issue in many applications including forecasting near surface meteorology and air quality, however, it is a very challenging problem due to the lack of not only comprehensive, global Planetary Boundary Layer (PBL) observations but also a strategy and infrastructure to utilize PBL height data from a variety of sensors. Following the designation of PBL as an incubation class observable in the 2017 Decadal Survey, the PBL Incubation Study Team Report [14] made clear that “a future global PBL observing system requires modeling and data assimilation as essential components.” There is an urgent need for global modeling development in order to utilize Program of Record (POR) observations, assess their impacts, and identify gaps to be filled by future PBL missions. Our overall objective is to develop PBL data assimilation capabilities in the NASA Global Earth Observing System (GEOS), focusing on PBL height from multiple observing systems, to support the assessment and use of future PBL observations. The NASA GEOS system is composed of the GEOS global atmospheric general circulation model (AGCM) and the atmospheric data assimilation system (ADAS). The PBL parameterizations include the “Lock” K-profile scheme driven by surface and cloud-top buoyancy fluxes ([4]), and the “Louis” local scheme for stable conditions based on the Richardson number ([5]). Above the mixed layer defined by the Lock surface plume, shallow cumulus convection is represented by the mass flux scheme of [9]. Additional parameterizations are summarized in [1]. The ADAS employs the hybrid 4D Ensemble- Variational (EnVar) configuration ([15]), with the ensemble providing flow-dependent background error covariance information. The resultant analysis increments are fed back to the forecast model through the 4D incremental analysis update (IAU) approach ([11]). In this study, PBL height data are being or have been generated from radiosondes, GNSS RO, satellite (CATS, CALIPSO and ICESat-2) and ground-based (MPLNET) lidars, and wind profiler. Investigations have been conducted to specify quality marks for PBL height retrievals for the data assimilation purpose. These PBL height data have different strengths and weaknesses ([2], [3], [6], [7], [8], [10]), and the satellite PBL height data provide better global coverage and complement in-situ PBL height data. Radiosondes offer high accuracy and in situ measurement of temperature and humidity profiles, but with poor spatio-temporal sampling. The in-situ observing systems like MPLNET and wind profiler provide long history of PBL height records at each station. The GNSS RO based PBL height is retrieved based on the sharp gradients in refractivity profile that represent the fine vertical structure of temperature and moisture changes above the PBL. However, not all RO refractivity profiles reach the surface depending on location and regime, and RO refractivity retrievals can be negatively biased below 2km. The PBL height data from satellite lidars provide high resolution along track PBL height retrievals, but over land they are affected by previous day convective PBL aerosol and strongly associated with mixing layer and retrievals cannot be made below thick, attenuating clouds. A successful assimilation of PBL height data requires a thorough understanding of the observing method and the retrieval algorithm for each observing system in order to use the PBL height data from multiple observing systems properly. Due to the sensitivity of PBL height data to the observing method and choice of algorithm, it is important to use a model definition appropriate for each observation type to compute differences between PBL height data and model PBL height (OmFs). The GEOS model currently includes two PBL height definitions suitable for direct comparison with observed PBL height, and additional definitions are being added in this study. Evaluation of different model PBL height definitions is underway. Meanwhile, efforts have been made in the GEOS data assimilation system to develop PBL height data assimilation capability. PBL height data can be assimilated using two different approaches. The traditional approach is to construct an observation operator and its tangent linear and adjoint, which link control variables to PBL height data from each observing system. This observation operator can be very complicated, e.g., the lidar-based PBL height observation operator includes the backscatter lidar forward observation operator, the algorithm to derive PBL height from attenuated total backscatter, interpolation, and calculations handling the mismatch between observed and model scales. The other approach is to augment PBL height to the control variable vector, and it is adopted in this study. The latter approach was also used in previous studies, e.g., the assimilation of PBL height data from radiosonde and aircraft in the Real Time Mesoscale Analysis (RTMA) system for a dispersion modelling study ([13]); the PBL height assimilation study using lidar PBL height data at Greensburg, Kansas for a field campaign ([12]). The PBL height assimilation from multiple observing systems in this study allows us to take advantage of the diverse PBL height data that provide much better global coverage collectively under different meteorological conditions and with different temporal and spatial scales. As all the PBL heights are tightly coupled with the PBL thermodynamic variables, the strong correlations, which are provided by the 4D ensemble forecast, enable PBL height data from various sources to interact and combine coherently and provide additional information for PBL temperature and moisture fields. The results of comparisons among PBL height data from different sources and the evaluation of the model PBL height definitions with the PBL height data will be presented, and the PBL height data synergy strategies and preliminary results will also be discussed at the conference.

Y. Zhu↗

Understanding Effective Diameter and Its Application to Terrestrial Radiation in Ice Clouds

The cloud property known as "effective diameter" or "effective radius", which in essence is the cloud particle size distribution (PSD) volume at bulk density divided by its projected area, is used extensively in atmospheric radiation transfer, climate modeling and remote sensing. This derives from the assumption that PSD optical properties can be uniquely described in terms of their effective diameter, D(sub e), and their cloud water content (CWC), henceforth referred to as the D(sub e)-CWC assumption. This study challenges this assumption, showing that while the D(sub e)-CWC assumption appears generally valid for liquid water clouds, it appears less valid for ice clouds in regions where (1) absorption is not primarily a function of either the PSD ice water content (IWC) or the PSD projected area, and (2) where wave resonance (i.e. photon tunneling) contributes significantly to absorption. These two regions often strongly coincide at terrestrial wavelengths when De less than ~60 m, which is where this D(sub e)-CWC assumption appears poorest. Treating optical properties solely in terms of D(sub e) and IWC may lead to errors up to 24%, 26% and 20% for terrestrial radiation in the window region regarding the absorption and extinction coefficients and the single scattering albedo, respectively. Outside the window region, errors may reach 33% and 42% regarding absorption and extinction. The magnitude and sign of these errors can change rapidly with wavelength, which may produce significant errors in climate modeling, remote sensing and other applications concerned with the wavelength dependence of radiation. Where the D(sub e)-CWC assumption breaks down, ice cloud optical properties appear to depend on D(sub e), IWC and the PSD shape. Optical property parameterizations in climate models and remote sensing algorithms based on historical PSD measurements may exhibit errors due to previously unknown PSD errors (i.e. the presence of ice artifacts due to the shattering of larger ice particles on the probe inlet tube during sampling). More recently developed cloud probes are designed to mitigate this shattering problem. Using realistic PSD shapes for a given temperature (and/or IWC) and cloud type may minimize errors associated with PSD shape in ice optics parameterizations and remote sensing algorithms. While this topic was investigated using two ice optics schemes (the Yang et al., 2005 database and the modified anomalous diffraction approximation, or MADA), a physical understanding of the limitations of the D(sub e)-IWC assumption was made possible by using MADA. MADA allows one to approximate the contribution of photon tunneling to absorption relative to other optical processes, which reveals that part of the error regarding the D(sub e)-IWC assumption can be associated with tunneling. By relating the remaining error to the radiation penetration depth in bulk ice (DELTA L) due to absorption, the domain where the D(sub e)-IWC assumption is weakest was described in terms of D(sub e) and DELTA L.

Mitchell, D. L.↗

Linking Deep and Shallow Convective Mass Fluxes via an Assumed Entrainment Distribution in CAM5‐CLUBB: Parameterization and Simulated Precipitation Variability

Abstract We modify the Zhang‐McFarlane (ZM) deep convection scheme in the Community Atmosphere Model version 5 to couple it with a unified parameterization for boundary‐layer turbulence and shallow convection, that is, Cloud Layers Unified by Binormals (CLUBB). By assuming a lognormal distribution of entrainment rate across the entire moist convective regimes, we link mass fluxes between shallow and deep convection, which are partitioned by the entrainment rate of the shallowest deep convective plume. Hence, a new deep convective closure is established which is coupled to the sub‐grid vertical motion variability in CLUBB. The convection feedback (or memory) effects are also considered to decrease the entrainment spectrum width and enhance the vertical velocity variability that further affect deep convection. Results show that the revised scheme improves the precipitation simulations in terms of the mean state and variability at various timescales, such as the alleviated double‐intertropical convergence zone and more realistic simulations of the seasonal variation of monsoon precipitation over East Asia, Madden‐Julian Oscillation, and precipitation diurnal phase propagations downstream of large terrains. The improvements are still seen in many aspects such as the mean‐state precipitation when turning off the convection feedback impacts in the revised scheme, emphasizing the benefits of using the modified mass‐flux closure. However, the convection feedbacks have considerable effects on the precipitation diurnal cycle simulations over regions with late‐afternoon precipitation peaks. Overall, the revised scheme provides a unified treatment for sub‐grid vertical motions across regimes of boundary‐layer turbulence, shallow convection, and deep convection, leading to better‐simulated precipitation at various timescales.

54 ENVIRONMENTAL SCIENCES↗

Examining the Ice-Nucleating Particles from the Southern Great Plains Field Campaign Report

The recent U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility field campaign, named Examining the Ice-Nucleating Particles from Southern Great Plains (ExINP-SGP), targeted experimentally characterizing abundance and other properties of ambient ice-nucleating particles (INPs) at the SGP site in Oklahoma (36° 36' 18" N, 97° 29' 6" W) during the period of October 1 to November 14, 2019. This campaign was funded through the DOE Office of Science Early Career Research Program (DE-SC0018979) as one of three major campaigns to be conducted at three ARM observatories, including the Eastern North Atlantic (ENA) station in 2020–2021 and North Slope of Alaska (NSA) site in 2021–2023, besides SGP. Different INP episodes were assessed to develop an SGP-relevant ice nucleation parameterization that would help understand convective and mixed-phase cloud systems typically observed in this region.

54 ENVIRONMENTAL SCIENCES↗

Rapid saturation of cloud water adjustments to shipping emissions

Abstract. Human aerosol emissions change cloud properties by providing additional cloud condensation nuclei. This increases cloud droplet numbers, which in turn affects other cloud properties like liquid-water content and ultimately cloud albedo. These adjustments are poorly constrained, making aerosol effects the most uncertain part of anthropogenic climate forcing. Here we show that cloud droplet number and water content react differently to changing emission amounts in shipping exhausts. We use information about ship positions and modeled emission amounts together with reanalysis winds and satellite retrievals of cloud properties. The analysis reveals that cloud droplet numbers respond linearly to emission amount over a large range (1–10 kg h−1) before the response saturates. Liquid water increases in raining clouds, and the anomalies are constant over the emission ranges observed. There is evidence that this independence of emissions is due to compensating effects under drier and more humid conditions, consistent with suppression of rain by enhanced aerosol. This has implications for our understanding of cloud processes and may improve the way clouds are represented in climate models, in particular by changing parameterizations of liquid-water responses to aerosol.

54 ENVIRONMENTAL SCIENCES↗

The January and July performance of the OSU two-level atmospheric general circulation model

A modified version of the two-level atmospheric general circulation model has been developed and employed in the simulation of January and July global climates. The overall physical and numerical formation of the Oregon State University model is the same as that described by Gates and Schlesinger (1977), but in the new version water vapor at the upper level has been made a prognostic variable, the parameterizations of cumulus convection, large-scale condensation and evaporation, clouds, and radiative transfer have been changed, the surface snow mass and ground temperature have been made prognostic variables, and the treatment of the surface boundary layer has been revised. It is found that the model simulates most features of the large-scale distributions of observed January and July climate more accurately than before.

Schlesinger, M. E.↗

Infrared spectra of rotating protostars

Earlier calculations of the infrared emission expected from stars in the process of being made are corrected to include the most important observable effects of rotation and generalized. An improved version of the spherical model of a previous paper is developed, and the corresponding emergent spectral energy distributions are calculated for the theoretically expected mass infall rate in the cores of cool and quiescent molecular clouds. The dust grain opacity model and the temperature profile parameterization are improved. It is shown that the infrared spectrum of the IRAS source 04264+2426, which is associated with a Herbig-Haro object, can be adequately represented in terms of a rotating and accreting protostar. This strengthens the suggestion that collimated outflows in young stellar objects originate when a stellar wind tries to emerge and reverse the swirling pattern of infall which gave birth to the central star.

Adams, F. C.↗

A model of the tropical Pacific sea surface temperature climatology

A model for the climatological mean sea surface temperature (SST) of the tropical Pacific Ocean is developed. The upper ocean response is computed using a time dependent, linear, reduced gravity model, with the addition of a constant depth frictional surface layer. The full three-dimensional temperature equation and a surface heat flux parameterization that requires specification of only wind speed and total cloud cover are used to evaluate the SST. Specification of atmospheric parameters, such as air temperature and humidity, over which the ocean has direct influence, is avoided. The model simulates the major features of the observed tropical Pacific SST. The seasonal evolution of these features is generally captured by the model. Analysis of the results demonstrates the control the ocean has over the surface heat flux from ocean to atmosphere and the crucial role that dynamics play in determining the mean SST in the equatorial Pacific. The sensitivity of the model to perturbations in the surface heat flux, cloud cover specification, diffusivity, and mixed layer depth is discussed.

Seager, Richard↗

Comparison of GOES-Retrieved and In Situ Measurements of Deep Convective Anvil Cloud Microphysical Properties During the Tropical Composition, Cloud and Climate Coupling Experiment (TC(sup 4))

One of the main goals of the Tropical Composition, Cloud and Climate Coupling Experiment (TC(sup 4)) during July and August 2007 was to gain a better understanding of the formation and life cycle of cirrus clouds in the upper troposphere and lower stratosphere and how their presence affects the exchange of water vapor between these layers. Additionally, it is important to compare in situ measurements taken by aircraft instruments with products derived from satellite observations and find a meaningful way to interpret the results. In this study, cloud properties derived using radiance measurements from the Geostationary Operational Environmental Satellite (GOES) imagers are compared to similar quantities from aircraft in situ observations and are examined for meaningful relationships. A new method using dual \angle satellite measurements is used to derive the ice water content (IWC) for the top portion of deep convective clouds and anvils. The results show the in situ and remotely sensed mean microphysical properties agree to within approx.10 microns in the top few kilometers of thick anvils despite the vastly different temporal and spatial resolutions of the aircraft and satellite instruments. Mean particle size and IWC are shown to increase with decreasing altitude in the top few kilometers of the cloud. Given these relationships, it may be possible to derive parameterizations for effective particle size and IWC as a function of altitude from satellite observations

Yost, Christoher R.↗

Making Atmospheric Convective Parameterizations Obsolete with Machine Learning Emulation

Parameterizations of moist convection in atmospheric models are notoriously problematic, and while global cloud resolving models (GCRM) are often touted as the ultimate solution, the computational cost is a considerable hurdle to overcome. Machine learning emulation of GCRMs for predictive modelling can leverage the DOE’s computational resource investments and allow widespread use of GCRMs such that traditional parameterizations become obsolete for most applications.

54 ENVIRONMENTAL SCIENCES↗

Improving GCM Predictability of Mixed-Phase Clouds and Aerosol Interactions at High Latitudes with ARM Observations

The overachieving goal of this project is to improve the predictability of mixed-phase clouds and aerosol interactions in the Community Atmosphere Model version 6 (CAM6) through comparison with the ARM observations. There are three main objectives of the proposed study: (1) Improve the representation of ice microphysical processes in mixed-phase clouds; (2) Test the performance of ice microphysics in CESM-CAM6 with the ARM observations in northern and southern high latitudes; and (3) Examine mixed-phase cloud microphysics-aerosol-turbulence-radiation interactions in CESM-CAM6. In this project, we have (1) Improved the representation of ice microphysical processes in mixed-phase clouds in CESM-CAM6 by implementing the marine organic aerosol (MOA) and treating the ice nucleating particles (INPs) from MOA and its impacts on mixed-phase clouds. We improved the treatment of ice depositional growth through the Wegener–Bergeron–Findeisen (WBF) process by considering the subgrid heterogeneous distributions between liquid droplets and ice crystals in mixed-phase clouds; (2) Tested the performance of ice microphysics in CESM-CAM6 with the ARM observations at high latitudes. We compared the simulated INP concentrations with the ARM observations, e.g., from M-PACE, ISDAC, INPOP, and other data (Mace Head, Zeppelin, CAPRICORN). We examined the impact of improved WBF treatment on model simulated Arctic mixed-phase clouds observed in the M-PACE field campaign. Seasonal variations of modeled mixed-phase cloud properties (LWO, IWP) are compared with the ground-based remote sensing retrievals at the ARM’s NSA $Utqia\dot{g}vik$ site; and (3) Examined mixed-phase cloud microphysics-aerosol-dynamics-radiation interactions in CESM-CAM6 that include the impacts of MOA INPs, and impacts of different model parameterizations (CLUBB versus UW turbulence & shallow convection schemes, MG2 versus MG1) on high-latitude mixed-phase cloud properties. Aerosol indirect effects of MOA through the liquid phase (droplet activation) and ice phase processes (e.g., the glaciation indirect effect) were investigated.

54 ENVIRONMENTAL SCIENCES↗

Using ARM Data to Retrieve Entrainment Rates in Stratocumulus Cloud Systems (Final Report)

A stratocumulus-topped boundary layer (STBL) is a shallow convecting layer in which both the updraft and the downdraft branches of the convective circulation are saturated (cloudy) in the upper part of the boundary layer. The convective circulation is vigorous, yet the cloud-top entrainment velocity, $w_e$, is small and difficult to measure. Differences between currently used parameterizations of $w_e$ in GCMs can lead to STBLs that differ by as much as a factor of two in climatologically important properties such as liquid water path and boundary layer depth. We have developed a new method to retrieve entrainment rates in STBLs which uses vertical velocity retrievals from surface-based cloud radar, in conjunction with other surface-based measurements. These new estimates will allow a more comprehensive evaluation of parameterizations of entrainment rate for STBLs. The new method will also provide ground-based estimates of entrainment in STBLs over long time periods. We use retrievals of vertical velocity and liquid water content profiles to estimate the turbulent liquid water flux, which is then used in combination with observed cloud-top jumps of temperature, water vapor, and calculated radiative flux profiles to estimate the entrainment rate. We present results for three days for which observational data was not significantly contaminated by drizzle. The resulting average entrainment rates are 0.58 cm/s, 1.51 cm/s, and 0.31 cm/s.

54 ENVIRONMENTAL SCIENCES↗

CGILS: Results from the First Phase of an International Project to Understand the Physical Mechanisms of Low Cloud Feedbacks in Single Column Models

1] CGILS-the CFMIP-GASS Intercomparison of Large Eddy Models (LESs) and single column models (SCMs)-investigates the mechanisms of cloud feedback in SCMs and LESs under idealized climate change perturbation. This paper describes the CGILS results from 15 SCMs and 8 LES models. Three cloud regimes over the subtropical oceans are studied: shallow cumulus, cumulus under stratocumulus, and well-mixed coastal stratus/stratocumulus. In the stratocumulus and coastal stratus regimes, SCMs without activated shallow convection generally simulated negative cloud feedbacks, while models with active shallow convection generally simulated positive cloud feedbacks. In the shallow cumulus alone regime, this relationship is less clear, likely due to the changes in cloud depth, lateral mixing, and precipitation or a combination of them. The majority of LES models simulated negative cloud feedback in the well-mixed coastal stratus/stratocumulus regime, and positive feedback in the shallow cumulus and stratocumulus regime. A general framework is provided to interpret SCM results: in a warmer climate, the moistening rate of the cloudy layer associated with the surface-based turbulence parameterization is enhanced; together with weaker large-scale subsidence, it causes negative cloud feedback. In contrast, in the warmer climate, the drying rate associated with the shallow convection scheme is enhanced. This causes positive cloud feedback. These mechanisms are summarized as the "NESTS" negative cloud feedback and the "SCOPE" positive cloud feedback (Negative feedback from Surface Turbulence under weaker Subsidence-Shallow Convection PositivE feedback) with the net cloud feedback depending on how the two opposing effects counteract each other. The LES results are consistent with these interpretations

Single Column Models↗

Interaction of the ABL with stratocumulus and cumulus cloud layers, appendix N

The role of the atmospheric boundary layer (ABL) over the oceans which in the general circulation of the atmosphere is to supply moisture to cumulus and stratus clouds is outlined. In extreme weather events, such as powerful storms and intense droughts, the primary role of the ABL is to supply or deny moisture to the weather system. Even for routine weather regimes, cloudiness and precipitation are key elements of any forecast. The premier problem for ABL parameterization is to formulate the physical coupling between the ABL turbulence and the clouds.

Randall, D. A.↗

Understanding Differences Between Co-Incident CloudSat, Aqua/MODIS and NOAA18 MHS Ice water Path Retrievals Over the Tropical Oceans

Accurate measurement of the physical and radiative properties of clouds and their representation in climate models continues to be a challe nge. Model parameterizations are still subject to a large number of t unable parameters; furthermore, accurate and representative in situ o bservations are very sparse, and satellite observations historically have significant quantitative uncertainties, particularly with respect to particle size distribution (PSD) and cloud phase. Ice Water Path (IWP), or amount of ice present in a cloud column, is an important cl oud property to accurately quantify, because it is an integral measur e of the microphysical properties of clouds and the cloud feedback pr ocesses in the climate system. This paper investigates near co-incident retrievals of IWP over tropical oceans using three diverse measurem ent systems: radar from CloudSat, Vis/IR from Aqua/MODIS, and microwa ve from NOAA-18IMHS. CloudSat 94 GHz radar measurements provide high resolution vertical and along-orbit structure of cloud reflectivity a nd enable IWP (and IWC) retrievals. Overlapping MODIS measurements of cloud optical thickness and phase allow estimates of IWP when cloud tops are identified as being ice. Periodically, NOAA18 becomes co-inci dent in space I time to enable comparison of A-Train measurements to IWP inferred from the 157 and 89 GHz channel radiances. This latter m easurement is effective only for thick convective anvil systems. We s tratify these co-incident data (less than 4 minutes separation) into cirrus only, cirrus overlying liquid water clouds, and precipitating d eep convective clouds. Substantial biases in IWP and ice effective ra dius are found. Systematic differences in these retrievals are consid ered in light of the uncertainties in a priori assumptions ofPSDs, sp ectral sensitivity and algorithm strategies, which have a direct impact on the IWP product.

Pittman, Jasna↗

Vertical Profile of Cloud Optical Parameters Derived from Airborne Measurements Above, Inside and Below Clouds

Past strategies for retrieving cloud optical properties from remote sensing assumed significant limits for desired parameters such as semi-infinite optical thickness, single scattering albedo equaling unity (non-absorbing scattering), absence of spectral dependence of the optical thickness, etc., and only one optical parameter could be retrieved (either optical thickness or single scattering albedo). Here, we demonstrate a new method based on asymptotic theory for thick atmospheres, and the presence of a diffusion domain within the clouds that does not put restrictions and makes it possible to get two or even three optical parameters (optical thickness, single scattering albedo and phase function asymmetry parameter) for every wavelength independently. We applied this method to measurements of angular distribution of solar radiation above, inside and below clouds, obtained with NASA's Cloud Absorption Radiometer (CAR) over two cases of marine stratocumulus clouds; first case, offshore of Namibia and the second case, offshore of California. The observational and retrieval errors are accounted for by regularization, which allows stable and smooth solutions. Results show good potential for parameterization of the shortwave radiative properties (reflection, transmission, radiative divergence and heating rate) of water clouds.

airborne observations↗