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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 685 records · Page 38
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

A statistical search for a population of exo-Trojans in the Kepler data set

Trojans are small bodies in planetary Lagrangian points. In our solar system, Jupiter has the largest number of such companions. Their existence is assumed for exoplanetary systems as well, but none have been found so far. We present an analysis by super-stacking ∼4 × 10{sup 3} Kepler planets with a total of ∼9 × 10{sup 4} transits, searching for an average Trojan transit dip. Our results give an upper limit to the average Trojan transiting area (per planet) that corresponds to one body of radius <460 km with 2σ confidence. We find a significant Trojan-like signal in a sub-sample for planets with more (or larger) Trojans for periods >60 days. Our tentative results can and should be checked with improved data from future missions like PLATO 2.0, and can guide planetary formation theories.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Instability of flux flow and production of vortex-antivortex pairs by current-driven Josephson vortices in layered superconductors

We report numerical simulations of the nonlinear dynamics of Josephson vortices driven by strong dc currents in layered superconductors. Dynamic equations for interlayer phase differences in a stack of coupled superconducting layers were solved to calculate a drag coefficient η(J) of the vortex as a function of the perpendicular dc current density J. It is shown that Cherenkov radiation produced by a moving vortex causes significant radiation drag increasing η(v) at high vortex velocities v and striking instabilities of driven Josephson vortices moving faster than a terminal velocity v c . The steady-state flux flow breaks down at v > v c as the vortex starts producing a cascade of expanding vortex-antivortex pairs evolving into either planar macrovortex structures or branching flux patterns propagating both along and across the layers. This vortex-antivortex pair production triggered by a rapidly moving vortex is most pronounced in a stack of underdamped planar junctions where it can occur at J > J s well below the interlayer Josephson critical current density. Both v c and J s were calculated as functions of the quasiparticle damping parameter, and the dc magnetic field was applied parallel to the layers. The effects of vortex interaction on the Cherenkov instability of moving vortex chains and lattices in annular stacks of Josephson junctions were considered. It is shown that a vortex driven by a current density J > J s in a multilayer of finite length excites self-sustained large-amplitude standing waves of magnetic flux, resulting in temporal oscillations of the total magnetic moment. We evaluated a contribution of this effect to the power W radiated by the sample and showed that W increases strongly as the number of layers increases. Furthermore, these mechanisms can result in nonlinearity of the c-axis electromagnetic response and contribute to THz radiation from the layered cuprates at high dc current densities flowing perpendicular to the ab planes.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Evidence of TeV halos around millisecond pulsars

Using data from the HAWC gamma-ray Telescope, we have studied a sample of 37 millisecond pulsars (MSPs), selected for their spindown power and proximity. From among these MSP, we have identified four which favor the presence of very high-energy gamma-ray emission at a level of (2Δ ln L) 1/2 ≥ 2.5. Adopting a correlation between the spindown power and gamma-ray luminosity of each pulsar, we performed a stacked likelihood analysis of these 37 MSPs, finding that the data supports the conclusion that these sources emit very high-energy gamma-rays at a level of (2Δ ln L) 1/2 = 4.24. Among sets of randomly selected sky locations within HAWC’s field-of-view, less than 1% of such realizations yielded such high statistical significance. Our analysis suggests that MSPs produce very high-energy gamma-ray emission with a similar efficiency to that observed from the Geminga TeV-halo, η MSP = (0.39 - 1.08) x η Geminga . So this conclusion poses a significant challenge for pulsar interpretations of the Galactic Center gamma-ray excess, as it suggests that any population of MSPs potentially capable of producing the GeV excess would also produce TeV-scale emission in excess of that observed by HESS from this region. Future observations by CTA will be able to substantially clarify this situation

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2012

Hard X-ray Fluorescence Measurements of Heteroepitaxial Solid Oxide Fuel Cell Cathode Materials

Commonly, SOFCs are operated at high temperatures (above 800°C). At these temperatures expensive housing is needed to contain an operating stack as well as coatings to contain the oxidation of the metallic interconnects. Lowering the temperature of an operating device would allow for more conventional materials to be used, thus lowering overall cost. Understanding the surface chemical states of cations in the surface of the SOFC cathode is vital to designing a system that will perform well at lower temperatures. The samples studied were grown by pulsed laser deposition (PLD) at the Environmental Molecular Sciences Laboratory (EMSL) at Pacific Northwest National Laboratory (PNNL). 20% strontium doped lanthanum manganite (LSM-20) was grown on YSZ and NGO (neodymium gallate). The films on YSZ have a fiber texture. LSM-20 on NGO is heteroepitaxial. Lanthanum strontium cobalt ferrite (LSCF-6428) films were grown on LAO and YSZ with a GDC barrier layer. Total X-ray Reflection Fluorescence (TXRF) was used to depth profile the samples. In a typical experiment, the angle of the incident beam is varied though the critical angle. Below the critical angle, the x-ray decays as an evanescent wave and will only penetrate the top few nanometers. TXRF experiments done on LSM films have suggested strontium segregates to the surface and form strontium enriched nanoparticles (1). It should be pointed out that past studies have focused on 30% strontium A-site doping, but this project uses 20% strontium doped lanthanum manganite. XANES and EXAFS data were taken as a function of incoming angle to probe composition as a function of depth. XANES spectra can be difficult to analyze fully. For other materials density functional theory calculations compared to near edge measurements have been a good way to understand the 3d valence electrons (2).

Environmental Molecular Sciences Laboratory↗
DOE OSTI2023

Field Laboratory for Emerging Stacked Unconventional Plays in Central Appalachia

The goal of the Field Laboratory for Emerging Stacked Unconventional Plays (ESUP) in Central Appalachia project was to investigate and characterize the resource potential for multi-play production of emerging unconventional reservoirs in Central Appalachia. Project activities included drilling, logging and coring of a vertical characterization well drilled to basement to approximately 15,000 feet in depth. The data from drilling and well logs as well recovered core samples were used by the research team to support characterization of the geology and potential pay zones within the Nora Gas Field of southwestern Virginia and the greater Central Appalachian Basin. This project was led by Dr. Nino Ripepi of the Virginia Center for Coal and Energy Research (VCCER) in close collaboration with EnerVest Operating LLC (EnerVest). VCCER is housed in the Department of Mining and Minerals Engineering at Virginia Tech and was created by an Act of the Virginia General Assembly on March 30, 1977, as an interdisciplinary study, research, information, and resource facility for the Commonwealth of Virginia. EnerVest is a top tier, low-cost oil and natural gas company with a long history of traditional operating relationships with institutional investors as well as public and private companies. This report summarizes two major research activities: 1) Log and Core Analysis and 2) Numerical Modeling. Core analysis comprises the characterization efforts of the ESUP Field Laboratory and includes a discussion of the well logs run in the deep characterization wells, an initial analysis of those, the number, size and location of cores recovered, core testing and analysis done to date as well as plans for future analysis. Numerical modeling is comprised of seven major modeling efforts, including (1) Multiphysics shale transport modeling work, (2) the developed in-house compositional simulator studies, (3) reservoir modeling studies using GEM software, (4) fracture modeling work using EFRAC3D software and (5) numerical modeling efforts with ABAQUS software, (6) Numerical modeling efforts using FLAC3D and PFC3D, and (7) Automatic Machine Learning (AutoML) Studies.

02 PETROLEUM↗
DOE OSTI2012

Single crystalline and rare earth substituted La{sub 2}RuO{sub 5} investigated by x-ray diffraction and EXAFS spectroscopy

Single crystals of La{sub 2}RuO{sub 5} were obtained from a BaCl{sub 2} flux. The structure was determined by single crystal x-ray diffraction and compared to earlier x-ray and neutron powder diffraction results. The local structures of Ru and La/Ln in pure La{sub 2}RuO{sub 5} and the rare earth substituted La{sub 2-x}Ln{sub x}RuO{sub 5} (Ln=Pr, Nd, Sm, Gd, Dy) polycrystalline samples were determined from the extended x-ray absorption fine structures (EXAFS) of the K- and L{sub III}-edges of Ru, La, and Ln, respectively. A four shell model was developed to reduce the number of refinable parameters in the fit of the EXAFS spectra. The distribution of the Ln-ions in the layered crystal structure was determined by a comparison of the coordination spheres obtained from the Ln-edges with the unsubstituted La{sub 2}RuO{sub 5}. Interatomic distances were compared to the values obtained from the single crystal diffraction and were found to agree very well. - Graphical abstract: The crystal structure of La{sub 2-x}Ln{sub x}RuO{sub 5} (Ln=Pr, Nd, Sm, Gd, Dy) is shown viewed along the c-axis. The alternating stacking of LaRuO{sub 4} and LnO layers leads to the formation of zig-zag layers of corner sharing RuO{sub 6} octahedra. The La sites in the LaRuO{sub 4} layers are represented by light blue spheres, while the La/Ln sites in the LnO layers are colored dark blue. EXAFS investigations reveal a cationic ordering with roughly 65% of the substituting Ln ions occupying the LnO layers. Highlights: Black-Right-Pointing-Pointer Structure determination of La{sub 2}RuO{sub 5} by single crystal x-ray diffraction. Black-Right-Pointing-Pointer Ru-K EXAFS investigations of La{sub 2-x}Ln{sub x}RuO{sub 5} powder samples. Black-Right-Pointing-Pointer EXAFS of La and Ln in La{sub 2-x}Ln{sub x}RuO{sub 5} powder samples using K- and L{sub III}-absorption edges. Black-Right-Pointing-Pointer Good agreement of EXAFS results and crystal structure data despite low symmetry space group. Black-Right-Pointing-Pointer Observed partial cationic ordering of the inserted Ln on the two La sites.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Anisotropic Ferromagnetism in CrAu 3 Sb 6

The crystal structure and properties of CrAu 3 Sb 6 are presented, determined by measurements on single crystal and polycrystalline samples and first-principles calculations. The trigonal structure (space group P$\overline{3}$1m) comprises a CdI 2 -like sublattice of AuSb 2 with Cr occupying octahedral holes in a fully ordered triangular array. It can be viewed as a variation of the interesting and well-known families of partially intercalated transition metal dichalcogenides, but with stronger interactions along the stacking direction evidenced by short Cr–Au distances. The compound is metallic and ferromagnetic with a Curie temperature of 164 K. A strong anomalous contribution to the Hall effect is seen in the ferromagnetic state, and quantum oscillations are observed in magnetization at 2 K. Magnetization measurements show that the ordered moments of 1.5 μ B per Cr are oriented along the c-axis with relatively strong magnetocrystalline anisotropy. Electronic structure calculations confirm this uniaxial anisotropy and the important role of spin–orbit coupling in CrAu 3 Sb 6 and reveal strongly favored ferromagnetic ground state consistent with the measured Curie temperature. Through combined experiment and theory, this work provides a detailed picture of the basic properties and behaviors of this uniquely structured, Cr-based, anisotropic ferromagnet.

Crystal structure↗
DOE OSTI2022

Understanding Solution State Conformation and Aggregate Structure of Conjugated Polymers via Small Angle X-ray Scattering

Donor-acceptor (D-A) conjugated polymers are high-performance organic electronic materials that exhibit complex aggregation behavior. Understanding the solution state conformation and aggregation of conjugated polymers is crucial for controlling morphology during thin-film deposition and the subsequent electronic performance. However, a precise multiscale structure of solution state aggregates is lacking. Here, we present an in-depth small-angle X-ray scattering (SAXS) analysis of the solution state structure of an isoindigo-bithiophene-based D-A polymer (PII-2T) in chlorobenzene and decane as our primary system. Modeling the system as a combination of hierarchical fibrillar aggregates mixed with dispersed polymers, we extract information about conformation and multiscale aggregation and also clarify the physical origin of features often observed but unaddressed or misinterpreted in small-angle scattering patterns of conjugated polymers. The persistence length of the D-A polymer extracted from SAXS agrees well with a theoretical model based on the dihedral potentials. Additionally, we show that the broad high q structure factor peak seen in scattering profiles can be attributed to lamellar stacking occurring within the fibril aggregates and that the low q aggregate scattering is strongly influenced by the polymer molecular weight. Overall, the SAXS profiles of D-A polymers in general exhibit a sensitive dependence on the co-existence of fibrillar aggregate and dispersed polymer chain populations. We corroborate our findings from SAXS with electron microscopy of freeze-dried samples for direct imaging of fibrillar aggregates. Finally, we demonstrate the generality of our approach by fitting the scattering profiles of a variety of D-A polymers based on thieno-isoindigo (PTII-2T), diketopyrrolopyrrole (DPP2T-TT, DPP-BTZ, PDPP2FT-C- 16 ), naphthalenediimide (P(NDI2OD-T2)), and a conjugated block copolymer P3HT-b-DPPT-T. The results presented here establish a picture of the D-A polymer solution state structure and provide a general method of interpreting and analyzing their scattering profiles.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Non-proportionality of magnetic anisotropy and damping in CoFeB/MgO-based systems

We study the relationship between anisotropy K and damping α in MgO/CoFeB/Ta/CoFeB/MgO/cap films using vector network analyzer ferromagnetic resonance. Capping the stack with Ta and changing the thickness of the top MgO layer allow us to create significant variations in anisotropy while keeping the thickness and process conditions of the magnetic layer constant. The change in anisotropy can be attributed to the degradation of the CoFeB/MgO interface due to Ta intermixing with MgO upon deposition. This hypothesis is supported by measurements of similar samples with the bottom MgO thickness varied instead, which exhibit no significant change in anisotropy. This method of varying K allows identifying a regime where a spin reorientation transition occurs while α remains constant, proving the non-proportionality of K and α in perpendicular CoFeB/MgO systems. The effects of changing the capping layer material, notably Ru, are also discussed.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Epitaxial Ni-Mn-Ga-Co thin films on PMN-PT substrates for multicaloric applications

Multicaloric stacks consisting of a magnetocaloric film on a piezoelectric substrate promise improved caloric properties as the transition temperature can be controlled by both magnetic and electric fields. We present epitaxially grown magnetocaloric Ni-Mn-Ga-Co thin films on ferroelectric Pb(Mg{sub 1/3}Nb{sub 2/3}){sub 0.72}Ti{sub 0.28}O{sub 3} substrates. Structure and microstructure of two samples, being in the austenitic and martensitic state at room temperature, are investigated by X-ray diffraction in two- and four-circle geometry and by atomic force microscopy. In addition, high temperature magnetometry was performed on the latter sample. The combination of these methods allows separating the influence of epitaxial growth and martensitic transformation. A preferential alignment of twin boundaries is observed already in the as-deposited state, which indicates the presence of prestress, without applying an electric field to the substrate. A temperature-magnetic field phase diagram is presented, which demonstrates the inverse magnetocaloric effect of the epitaxial Ni-Mn-Ga-Co film.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2012

X-RAY CONSTRAINTS ON THE Ly{alpha} ESCAPE FRACTION

We have co-added the X-ray flux of all known Ly{alpha} emitters (LAEs) in the 4 Ms Chandra Deep Field South (CDF-S) region, achieving the tightest upper limits yet on the X-ray to Ly{alpha} ratio. We use the X-ray data to place sensitive upper limits on the average unobscured star formation rate (SFR{sub X}) in these galaxies. A very small fraction of Ly{alpha} galaxies in the field are individually detected in the X-rays, implying a low fraction of active galactic nucleus activity. After excluding the few X-ray-detected LAEs, we stack the undetected LAEs located in the 4 Ms CDF-S data and 250 ks Extended CDF-S (ECDF-S) data, and compute a 1{sigma} upper limit on SFR{sub X} < 1.6, 14, 28, 28, 140, 440, 880 M{sub Sun} yr{sup -1} for LAEs located at z {approx} 0.3 and z = 2.1, 3.1, 3.2, 4.5, 5.7, and 6.5, respectively. The upper limit of SFR{sub X} in LAEs can be then compared to SFR{sub Ly{alpha}} derived from Ly{alpha} line and thus can constrain on the Ly{alpha} escape fraction (f{sup Esc}{sub Ly{alpha}}). The f{sup Esc}{sub Ly{alpha}} from X-ray at z {approx} 0.3 is substantially larger than that from UV or H{alpha}. Three X-ray-detected LAE galaxies at z {approx} 0.3 show f{sup Esc}{sub Ly{alpha}} {approx} 3%-22%, and the average Ly{alpha} escape fraction from stacking the X-ray-undetected LAEs show f{sup Esc}{sub Ly{alpha}} > 28% at 3{sigma} significance level at the same redshift. We derive a lower limit on f{sup Esc}{sub Ly{alpha}} > 14% (84% confidence level, 1{sigma} lower limit) for LAEs at redshift z {approx} 2.1 and z {approx} 3.1-3.2. At z > 4, the current LAE samples are not of sufficient size to constrain SFR{sub X} well. By averaging all the LAEs at z > 2, the X-ray non-detection constrains f{sup Esc}{sub Ly{alpha}} > 17% (84% confidence level, 1{sigma} lower limit), and rejects f{sup Esc}{sub Ly{alpha}} < 5.7% at the 99.87% confidence level from 2.1 < z < 6.5.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Coexistence of Weyl physics and planar defects in the semimetals TaP and TaAs

We report a structural study of the Weyl semimetals TaAs and TaP, utilizing diffraction and imaging techniques, where we show that they contain a high density of defects, leading to nonstoichiometric single crystals of both semimetals. Despite the observed defects and nonstoichiometry on samples grown using techniques already reported in the literature, de Haas–van Alphen measurements on TaP reveal quantum oscillations and a high carrier mobility, an indication that the crystals are of quality comparable to those reported elsewhere. Electronic structure calculations on TaAs reveal that the position of the Weyl points relative to the Fermi level shift with the introduction of vacancies and stacking faults. In the case of vacancies the Fermi surface becomes considerably altered, while the effect of stacking faults on the electronic structure is to allow the Weyl pockets to remain close to the Fermi surface. The observation of quantum oscillations in a nonstoichiometric crystal and the persistence of Weyl fermion pockets near the Fermi surface in a crystal with stacking faults point to the robustness of these quantum phenomena in these materials.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Effect of Microstructure Refinement on Hardness Homogeneity of Aluminum Alloy 1100 Processed by Accumulative Roll Bonding

This work examines the effect of grain refinement via accumulative roll bonding (ARB) on the homogeneity of microstructure and hardness through the thickness of commercially pure aluminum AA1100 sheets. The use of 7 cycles of ARB was shown to produce homogeneous ultrafine-grained microstructure, reducing the grain size to 0.46 and 1.03 µm in normal direction and rolling direction, respectively. Examination by electron backscattered diffraction indicates that continuous dynamic recrystallization was the main mechanism for the formation of submicron equiaxed grains bounded with high-angle grain boundaries (HAGBs). The fraction of HAGBs increased gradually reaching a maximum of 71.6% after 7 cycles. Through-thickness hardness measurements using Vickers and nanoindentation tests show an increase from 43.5 Hv (0.85 GPa) for as-received sample to 63 Hv (1.1 GPa) after 7 cycles. The heterogeneity in hardness through the thickness of the as-received material was shown to restrain the evolution of uniform hardness across the sheet thickness with increasing ARB cycles. Tensile tests showed that the tensile strength is increased to 250 MPa, which is about 2 times its initial value. Owing to the high stacking fault energy of AA1100, strong dynamic recovery occurred with increasing ARB strain which was balanced with the strain hardening property of the material. This resulted in plastic instability at small strains and thus early necking during the tensile test.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Fingerprinting shock-induced deformations via diffraction

Abstract During the various stages of shock loading, many transient modes of deformation can activate and deactivate to affect the final state of a material. In order to fundamentally understand and optimize a shock response, researchers seek the ability to probe these modes in real-time and measure the microstructural evolutions with nanoscale resolution. Neither post-mortem analysis on recovered samples nor continuum-based methods during shock testing meet both requirements. High-speed diffraction offers a solution, but the interpretation of diffractograms suffers numerous debates and uncertainties. By atomistically simulating the shock, X-ray diffraction, and electron diffraction of three representative BCC and FCC metallic systems, we systematically isolated the characteristic fingerprints of salient deformation modes, such as dislocation slip (stacking faults), deformation twinning, and phase transformation as observed in experimental diffractograms. This study demonstrates how to use simulated diffractograms to connect the contributions from concurrent deformation modes to the evolutions of both 1D line profiles and 2D patterns for diffractograms from single crystals. Harnessing these fingerprints alongside information on local pressures and plasticity contributions facilitate the interpretation of shock experiments with cutting-edge resolution in both space and time.

36 MATERIALS SCIENCE↗
DOE OSTI2013

MID-INFRARED DETERMINATION OF TOTAL INFRARED LUMINOSITY AND STAR FORMATION RATES OF LOCAL AND HIGH-REDSHIFT GALAXIES

We demonstrate estimating the total infrared luminosity, L(TIR), and star formation rates (SFRs) of star-forming galaxies at redshift 0 < z < 2.8 from single-band 24 {mu}m observations, using local spectral energy distribution (SED) templates without introducing additional free parameters. Our method is based on characterizing the SEDs of galaxies as a function of their L(TIR) surface density, which is motivated by the indications that the majority of IR luminous star-forming galaxies at 1 < z < 3 have extended star-forming regions, in contrast to the strongly nuclear concentrated, merger-induced starbursts in local luminous and ultraluminous IR galaxies. We validate our procedure for estimating L(TIR) by comparing the resulting L(TIR) with those measured from far-IR observations, such as those from Herschel in the Extended Chandra Deep Field South (ECDFS) and Hubble Deep Field North (HDFN), as well as L(TIR) measured from stacked far-IR observations at redshift 0 < z < 2.8. Active galactic nuclei were excluded using X-ray and 3.6-8.0 {mu}m observations, which are generally available in deep cosmological survey fields. The Gaussian fits to the distribution of the discrepancies between the L(TIR) measurements from single-band 24 {mu}m and Herschel observations in the ECDFS and HDFN samples have {sigma} < 0.1 dex, with {approx}10% of objects disagreeing by more than 0.2 dex. Since the 24 {mu}m estimates are based on SEDs for extended galaxies, this agreement suggests that {approx}90% of IR galaxies at high z are indeed much more physically extended than local counterparts of similar L(TIR), consistent with recent independent studies of the fractions of galaxies forming stars in the main-sequence and starburst modes, respectively. Because we have not introduced empirical corrections to enhance these estimates, in principle, our method should be applicable to lower luminosity galaxies. This will enable use of the 21 {mu}m band of the Mid-Infrared Instrument on board the James Webb Space Telescope to provide an extremely sensitive tracer of obscured SFR in individual star-forming galaxies across the peak of the cosmic star formation history.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Tunable electronic structure in gallium chalcogenide van der Waals compounds

Transition-metal monochalcogenides comprise a class of two-dimensional materials with electronic band gaps that are highly sensitive to material thickness and chemical composition. Here, we explore the tunability of the electronic excitation spectrum in GaSe by using angle-resolved photoemission spectroscopy. The electronic structure of the material is modified by in situ potassium deposition as well as by forming GaS x Se 1- x alloy compounds. We find that potassium-dosed samples exhibit a substantial change of the dispersion around the valence-band maximum (VBM). The observed band dispersion resembles that of a single tetralayer and is consistent with a transition from the direct-gap character of the bulk to the indirect-gap character expected for monolayer GaSe. Upon alloying with sulfur, we observe a phase transition from AB to AA' stacking. Alloying also results in a rigid energy shift of the VBM towards higher binding energies, which correlates with a blueshift in the luminescence. The increase of the band gap upon sulfur alloying does not appear to change the dispersion or character of the VBM appreciably, implying that it is possible to engineer the gap of these materials while maintaining their salient electronic properties.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

SU-E-J-46: Development of a Compton Camera Prototype for Online Range Verification of Laser-Accelerated Proton Beams

Purpose: Development of a photon detection system designed for online range verification of laser-accelerated proton beams via prompt-gamma imaging of nuclear reactions. Methods: We develop a Compton camera for the position-sensitive detection of prompt photons emitted from nuclear reactions between the proton beam and biological samples. The detector is designed to be capable to reconstruct the photon source origin not only from the Compton scattering kinematics of the primary photon, but also to allow for tracking of the Compton-scattered electrons. Results: Simulation studies resulted in the design of the Compton camera based on a LaBr{sub 3}(Ce) scintillation crystal acting as absorber, preceded by a stacked array of 6 double-sided silicon strip detectors as scatterers. From the design simulations, an angular resolution of ≤ 2° and an image reconstruction efficiency of 10{sup −3} −10{sup −5} (at 2–6 MeV) can be expected. The LaBr{sub 3} crystal has been characterized with calibration sources, resulting in a time resolution of 273 ps (FWHM) and an energy resolution of about 3.8% (FWHM). Using a collimated (1 mm diameter) {sup 137}Cs calibration source, the light distribution was measured for each of 64 pixels (6×6 mm{sup 2}). Data were also taken with 0.5 mm collimation and 0.5 mm step size to generate a reference library of light distributions that allows for reconstructing the interaction position of the initial photon using a k-nearest neighbor (k-NN) algorithm developed by the Delft group. Conclusion: The Compton-camera approach for prompt-gamma detection offers promising perspectives for ion beam range verification. A Compton camera prototype is presently being developed and characterized in Garching. Furthermore, an arrangement of, e.g., 4 camera modules could even be used in a ‘gamma-PET’ mode to detect delayed annihilation radiation from positron emitters in the irradiation interrupts (with improved performance in the presence of an additional third (prompt) photon (as in 10C and 14O). This work was supported by the DFG Cluster of Excellence MAP (Munich-Centre for Advanced Photonics)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗