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At least 685 records · Page 38

Electron–Phonon and Spin–Lattice Coupling in Atomically Thin Layers of MnBi 2 Te 4

MnBi 2 Te 4 represents a new class of magnetic topological insulators in which novel quantum phases emerge at temperatures higher than those found in magnetically doped thin films. Here in this paper, we investigate how couplings between electron, spin, and lattice are manifested in the phonon spectra of few-septuple-layer thick MnBi 2 Te 4 . After categorizing phonon modes by their symmetries, we study the systematic changes in frequency, line width, and line shape of a spectrally isolated A1g mode. The electron–phonon coupling increases in thinner flakes as manifested in a broader phonon line width, which is likely due to changes of the electron density of states. In 4- and 5-septuple thick samples, the onset of magnetic order below the Néel temperature is concurrent with a transition to an insulating state. We observe signatures of a reduced electron–phonon scattering across this transition as reflected in the reduced Fano parameter. Finally, spin–lattice coupling is measured and modeled from temperature-dependent phonon frequency.

36 MATERIALS SCIENCE↗

Electron-momentum dependence of electron-phonon coupling underlies dramatic phonon renormalization in YNi 2 B 2 C

Electron-phonon coupling, i.e., the scattering of lattice vibrations by electrons and vice versa, is ubiquitous in solids and can lead to emergent ground states such as superconductivity and charge-density wave order. A broad spectral phonon line shape is often interpreted as a marker of strong electron-phonon coupling associated with Fermi surface nesting, i.e., parallel sections of the Fermi surface connected by the phonon momentum. Alternatively broad phonons are known to arise from strong atomic lattice anharmonicity. Here, we show that strong phonon broadening can occur in the absence of both Fermi surface nesting and lattice anharmonicity, if electron-phonon coupling is strongly enhanced for specific values of electron-momentum, k. We use inelastic neutron scattering, soft x-ray angle-resolved photoemission spectroscopy measurements and ab-initio lattice dynamical and electronic band structure calculations to demonstrate this scenario in the highly anisotropic tetragonal electron-phonon superconductor YNi 2 B 2 C. This new scenario likely applies to a wide range of compounds.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Evidence of a distinct collective mode in Kagome superconductors

The collective modes of the superconducting order parameter fluctuation can provide key insights into the nature of the superconductor. Recently, a family of superconductors has emerged in non-magnetic kagome materials AV 3 Sb 5 (A = K, Rb, Cs), exhibiting fertile emergent phenomenology. However, the collective behaviors of Cooper pairs have not been studied. Here, we report a distinct collective mode in CsV 3-x Ta x Sb 5 using scanning tunneling microscope/spectroscopy. The spectral line-shape is well-described by one isotropic and one anisotropic superconducting gap, and a bosonic mode due to electron-mode coupling. With increasing x, the two gaps move closer in energy, merge into two isotropic gaps of equal amplitude, and then increase synchronously. The mode energy decreases monotonically to well below 2Δ and survives even after the charge density wave order is suppressed. We propose the interpretation of this collective mode as Leggett mode between different superconducting components or the Bardasis-Schrieffer mode due to a subleading superconducting component.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Control of electron recollision and molecular nonsequential double ionization

Abstract Intense laser pulses lasting a few optical cycles, are able to ionize molecules via different mechanisms. One such mechanism involves a process whereby within one optical period an electron tunnels away from the molecule, and is then accelerated and driven back as the laser field reverses its direction, colliding with the parent molecule and causing correlated non-sequential double ionization (NSDI). Here we report control over NSDI via spectral-phase pulse shaping of femtosecond laser pulses. The measurements are carried out on ethane molecules using shaped pulses. We find that the shaped pulses can enhance or suppress the yield of dications resulting from electron recollision by factors of 3 to 6. This type of shaped pulses is likely to impact all phenomena stemming from electron recollision processes induced by strong laser fields such as above threshold ionization, high harmonic generation, attosecond pulse generation, and laser-induced electron diffraction.

74 ATOMIC AND MOLECULAR PHYSICS↗

Analysis of Liquids Using the Submerged Plasma for Isotopic Detection and Elemental Resolution (SPIDER)

We developed a sensor called the Submerged Plasma for Isotopic Detection and Elemental Resolution (SPIDER) probe, which uses an atmospheric pressure glow discharge below the surface of liquids to excite species in the liquid. Through emission spectroscopy of molten salts, liquid metals, and heavy water, we demonstrated the SPIDER probe’s high resolution, accuracy, and versatility. We successfully identified trace concentrations of transition and rare-earth metals in molten salts and detected the isotopic shift of the H β → D β emission line. Our analysis revealed unconventional spectral alkali line shapes, indicating two competing excitation modes: film explosion and droplet vaporization. The film explosion mode, characterized by dense plasma, exhibited self-reversal and broadband continuum emission, while the droplet vaporization mode, associated with diffusive plasma, produced narrow-line emissions. Furthermore, by analyzing circuit transients alongside individual plasma events, we observed that film explosions generate higher currents, likely due to a shorter plasma length as the current preferentially flows through the thin liquid layer. Altogether, our results highlight the SPIDER probe’s efficacy and flexibility, making it well-suited for online material quantification of liquids in extreme environments.

AES↗

Methods for measuring the loudness and noisiness of complex sounds

Physical and temporal aspects of sound which influence the rating of subjective noisiness are intensity, spectrum shape and bandwidth, spectral complexity, and duration. Objective rating methods include a graphic method, full octave and one-third octave methods, and methods that measure one value over all frequencies.

Kryter, K.↗

Temperature distribution in a stellar atmosphere diagnostic basis

A stellar chromosphere is considered a region where the temperature increases outward and where the temperature structure of the gas controls the shape of the spectral lines. It is shown that lines which have collision-dominated source sink terms, like the Ca(+) and Mg(+) H and K lines, can be used to obtain the distribution of temperature with height from observed line profiles. Intrinsic emission lines and geometrical emission lines are found in spectral regions where the continuum is depressed. In visual regions, where the continuum is not depressed, emission core in absorption lines are attributed to reflections of intrinsic emission lines.

Jefferies, J. T.↗

Turbulent transport measurements with a laser Doppler velocimeter

The power spectrum of phototube current from a laser Doppler velocimeter operating in the heterodyne mode has been computed. The spectrum is obtained in terms of the space time correlation function of the fluid. The spectral width and shape predicted by the theory are in agreement with experiment. For normal operating parameters the time average spectrum contains information only for times shorter than the Lagrangian integral time scale of the turbulence. To examine the long time behavior, one must use either extremely small scattering angles, much longer wavelength radiation or a different mode of signal analysis, e.g., FM detection.

Edwards, R. V.↗

Turbulent transport measurements with a laser Doppler velocimeter.

The power spectrum of phototube current from a laser Doppler velocimeter operating in the heterodyne mode has been computed. The spectral width and shape predicted by the theory are in agreement with experiment. For normal operating parameters the time-average spectrum contains information only for times shorter than the Lagrangian-integral time scale of the turbulence. To examine the long-time behavior, one must use either extremely small scattering angles, much-longer-wavelength radiation, or a different mode of signal analysis, e.g., FM detection.

Edwards, R. V.↗

The temperature of thermal X-ray and gamma-ray sources

The temperature of a source can be accurately measured, assuming that it is optically thin and exhibits a bremsstrahlung, on the basis of the shape of its spectral distribution. An explicit relation is derived for the temperature in terms of this slope, and as a sum of correction terms to the limiting form of the bremsstrahlung formula. The corrections can be evaluated easily in terms of simple, accurate asymptotic formulae. For the case where there is a distribution of temperatures in the plasma, an additional correction is derived in terms of the rms variation in the plasma temperature. Corrections due to a modified Bessel function, the Born approximation, plasma electron energy distribution and electron-electron bremsstrahlung are discussed

Gould, R. J.↗

On the maximum-entropy/autoregressive modeling of time series

The autoregressive (AR) model of a random process is interpreted in the light of the Prony's relation which relates a complex conjugate pair of poles of the AR process in the z-plane (or the z domain) on the one hand, to the complex frequency of one complex harmonic function in the time domain on the other. Thus the AR model of a time series is one that models the time series as a linear combination of complex harmonic functions, which include pure sinusoids and real exponentials as special cases. An AR model is completely determined by its z-domain pole configuration. The maximum-entropy/autogressive (ME/AR) spectrum, defined on the unit circle of the z-plane (or the frequency domain), is nothing but a convenient, but ambiguous visual representation. It is asserted that the position and shape of a spectral peak is determined by the corresponding complex frequency, and the height of the spectral peak contains little information about the complex amplitude of the complex harmonic functions.

Chao, B. F.↗

Angle-resolved Auger electron spectra induced by neon ion impact on aluminum

Auger electron emission from aluminum bombarded with 1 to 5 keV neon ions was studied by angle-resolved electron spectroscopy. The position and shape of the spectral features depended on the incident ion energy, angle of ion incidence, and electron take-off angle with respect to the aluminum surface. These spectral dependencies were interpreted in terms of the Doppler shift given to the Auger electron velocity by the excited atom ejected into the vacuum. For oblique ion incidence it is concluded that a flux of high energy atoms are ejected in a direction close to the projection of the ion beam on the target surface. In addition, a new spectral feature was found and identified as due to Auger emission from excited neon in the aluminum matrix.

Pepper, S. V.↗

A study of native oxides of beta-SiC using Auger electron spectroscopy

Thermal and anodic oxide films of beta-SiC are analyzed using Auger electron spectroscopy. Auger depth-composition profiles are obtained in order to determine the chemical composition of the oxide films. The position and shape of silicon spectral peaks are used to estimate the chemical bonding of the oxide constituents. It is found that the wet thermal oxide is almost stoichiometric but contains about 14 pct C. Dry oxide, on the other hand, has less than 3 pct C but is highly nonstoichiometric. The C content in the anodic oxide is 12 pct. Anodic oxide films, like dry-oxide films, are nonstoichiometric. A model of the SiC oxidation process is presented.

Chaudhry, M. Iqbal↗

(C-12)O emission from the envelopes of cool stars in the solar neighborhood

Results are presented on observations of the CO J = 1-0 line emission from all M giants, S stars, and C stars listed in the Two-Micron Sky Survey having strong FIR emission and lying north of delta = -10 deg. The data from this survey and other data for C and S stars show that the line profiles of these stars look like flattened parabolas and have roughly the same shape for different stars. In contrast, the shapes of the spectral lines from giant M stars are diverse, ranging from triangular to spiked and asymmetric, suggesting that the envelopes of M stars have complex kinematics and structure. The outflow velocities inferred from the line profiles of the stars surveyed span a range of more than an order of magnitude, with the velocities of C stars correlating with IR color.

Margulis, M.↗

IRAS observations of young stellar objects in the Corona Australis dark cloud

The young stellar object (YSO) population associated with the dark cloud complex in Corona Australis is studied by synthesizing IRAS data with newly obtained near-IR and mid-IR photometry and previously published optical/IR data. Twenty-four YSOs in the Cr A complex are identified. The observed range of spectral energy distribution shapes and bolometric luminosities are consistent with those observed in other dark clouds. The duration and efficiency of star formation are found to be similar to the Rho Ophiuchi IR cluster. The low number of YSOs compared to other dark clouds is understood by a reevaluation of the molecular mass of the R Cr A cloud which shows it to be much less massive than previously assumed.

Wilking, Bruce A.↗

Radar Observations of Asteroid 10115 (1992 SK)

The approach of 1992 SK to within 0.056 AU of Earth on 1999 March 26 provided an excellent opportunity for radar observations. We observed it daily between March 22-26 at Goldstone at a transmitter frequency of 8560 MHz (3.50 cm). Weighted, optimally smoothed sums of cw (Doppler-only) echoes achieve a signal-to-noise ratio of about 300. Our highest resolution cw setup places up to approx. 30 0.5-Hz Doppler cells on the target at echo powers exceeding two standard deviations of the noise. Our highest resolution imaging setup places about 20 0.25-us (37.5 m) x 2.0 Hz pixels on 1992 SK at echo powers above the same threshold. We completed nearly 300 runs with each setup and obtained thorough rotational phase coverage (period = 7.320 h, P. Pravec, pers. comm.). The dispersion of the echoes in time delay indicates a lower bound on 1992 SK's maximum pole-on breadth of approx. 0.4 km that is consistent with the echo bandwidth and rotation period. Variations in the cw spectral bandwidths and shapes and in the delay-Doppler images as a function of rotation phase are evident on each day, are consistent in bandwidth with each other and with the rotation period, and indicate that the asteroid is asymmetric and modesty elongated.

Benner, L. A. M.↗

The Kepler Mission: A Photometric Search for Earthlike Planets

If Earth lies in or near the orbital plane of an extrasolar planet, that planet passes in front of the disk of its star once each orbit as viewed from Earth. Precise photometry can reveal such transits, which can be distinguished from rotationally-modulated starspots and intrinsic stellar variability by their periodicity, square-well shapes and relative spectral neutrality. Transit observations would provide the size and orbital period of the detected planet. Although geometrical considerations limit the fraction of planets detectable by this technique, many stars can be surveyed within the field of view of one telescope, so transit photometry is quite efficient. Scintillation in and variability of Earth's atmosphere limit photometric precision to roughly one-thousandth of a magnitude, allowing detection of transits by Jupiter-sized planets but not by Earth-sized planets from the ground. The COROT spacecraft will be able to detect Uranus-sized planets orbiting near stars. The Kepler Mission, which is being proposed to NASA's Discovery Program this year, will have a photometer with a larger aperture (1 meter) than will COROT, so it will be able to detect transits by planets as small as Earth. Moreover, the Kepler mission will examine the same star field for four years, allowing confirmation of planets with orbital periods of a year. If the Sun's planetary system is typical for single stars, Kepler should detect approximately 480 terrestrial planets. Assuming the statistics from radial velocity surveys are typical, Kepler should also detect transits of 150 inner giant planets and reflected light variations of 1400 giant planets with orbital periods of less than one week.

Lissauer, Jack J.↗

Athermal Energy Loss from X-rays Deposited in Thin Superconducting Films on Solid Substrates

When energy is deposited in a thin-film cryogenic detector, such as from the absorption of an X-ray, an important feature that determines the energy resolution is the amount of athermal energy that can be lost to the heat bath prior to the elementary excitation systems coming into thermal equilibrium. This form of energy loss will be position-dependent and therefore can limit the detector energy resolution. An understanding of the physical processes that occur when elementary excitations are generated in metal films on dielectric substrates is important for the design and optimization of a number of different types of low temperature detector. We have measured the total energy loss in one relatively simple geometry that allows us to study these processes and compare measurements with calculation based upon a model for the various di.erent processes. We have modeled the athermal phonon energy loss in this device by finding an evolving phonon distribution function that solves the system of kinetic equations for the interacting system of electrons and phonons. Using measurements of device parameters such as the Debye energy and the thermal di.usivity we have calculated the expected energy loss from this detector geometry, and also the position-dependent variation of this loss. We have also calculated the predicted impact on measured spectral line-shapes, and shown that they agree well with measurements. In addition, we have tested this model by using it to predict the performance of a number of other types of detector with di.erent geometries, where good agreement is also found.

Kozorezov, Alexander G.↗