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At least 685 records · Page 38
All sourcesNASA NTRSDOE OSTI
DOE OSTI2017

Strong size-dependent stress relaxation in electrospun polymer nanofibers

Here, electrospun polymer nanofibers have garnered significant interest due to their strong size-dependent material properties, such as tensile moduli, strength, toughness, and glass transition temperatures. These properties are closely correlated with polymer chain dynamics. In most applications, polymers usually exhibit viscoelastic behaviors such as stress relaxation and creep, which are also determined by the motion of polymer chains. However, the size-dependent viscoelasticity has not been studied previously in polymer nanofibers. Here, we report the first experimental evidence of significant size-dependent stress relaxation in electrospun Nylon-11 nanofibers as well as size-dependent viscosity of the confined amorphous regions. In conjunction with the dramatically increasing stiffness of nano-scaled fibers, this strong relaxation enables size-tunable properties which break the traditional damping-stiffness tradeoff, qualifying electrospun nanofibers as a promising set of size-tunable materials with an unusual and highly desirable combination of simultaneously high stiffness and large mechanical energy dissipation.

42 ENGINEERING↗
DOE OSTI2020

Wettability of ultra-small pores of carbon electrodes by size-asymmetric ionic fluids

Recently, we studied the phase behavior of ionic fluids under confinement using the classical density functional theory within the framework of the restricted primitive model. Additionally, the theoretical results indicate that narrowing the pore size may lead to a drastic reduction in the electric double layer capacitance, while increasing the surface electrical potential would improve the ionic accessibility of micropores. In this work, we extend the theoretical investigation to systems containing size-asymmetric electrolytes that may exhibit a vapor-liquid like phase transition in the bulk phase. The effects of pore size and surface electric potential on the phase diagram and microscopic structures of the confined electrolytes were studied over a broad range of parameters. We found that decreasing the pore size or increasing the surface potential could destabilize the liquid phase in micropores, and capillary evaporation could occur regardless of the size asymmetry between cations and anions. Compared to that in a symmetric ionic system, the vapor-liquid phase separation is more likely to take place as the size asymmetry becomes more pronounced. The phase transition would alter the “accessibility” of ions to micropores and lead to coexisting micropores with different surface charge densities as identified by Monte Carlo simulation.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Effect of grain size on damage and failure in two-phase materials: Homogenized CuPb

It is well known that spall failure strongly depends on the microstructure of a material. There have been numerous studies to study the effect of grain size on the overall spall strength and the total amount of damage in single element metals like copper. However, such systematic studies remain rare in two-phase materials and alloys. In this work, two incipient spall experiments were performed on a Cu–1%Pb alloy to understand the effect of grain size on the damage and failure in a two-phase material. Overall, these results showed that even though the spall strength did not change as a function of grain size, there were significant differences in the total amount of damage as a function of grain size. A clear increase in the total damage present in the material was seen as the grain size was increased from 32 to either 70 or 75 μm in either of the experiments. Furthermore, this difference was attributed to variations in the void growth rate as the grain size was increased.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Spot size measurement of a deuterium–tritium dense plasma focus using neutron radiography

Neutron radiography is a technique uniquely suited to applications in nuclear diagnostics, non-destructive testing, and subcritical experiments. The spatial resolution of neutron radiographs is degraded by optical blur in the imaging system and the neutron source size, where the ideal source is point-like to optimize the point-spread function. A potential neutron source for radiography is the dense plasma focus (DPF), a coaxial Z-pinch that produces thermonuclear and beam-target neutrons. To assess if the source size is suitable for radiography, a neutron imaging system was used to measure the source size of the 4 MA Sodium DPF at the Nevada National Security Site operating with deuterium–tritium gas-fill. The source size was measured using the edge-spread function of tungsten objects, each having a rolled (convex) edge. The spot size was found to be 7–12 mm full-width at half-max (FWHM) assuming a Gaussian source, though comparison is presented for Lorentzian and Bennett distributions. The average FWHM was found to be 8.6 ± 1.2 mm vertically and 10.8 ± 1.2 mm horizontally with respect to the image plane, averaging over varied edges and alignments. The results were sensitive to source alignment and edge metrology, which introduced notable uncertainties. These results are consistent with separate experimental measurements as well as magnetohydrodynamics simulations of this DPF, which suggest that neutron production can originate from pinches ∼5–7 mm off-axis. These results suggest that the DPF should be used for radiography at low magnification (M < 1) where spot size does not dominate spatial blur.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Repartitioning the Hamiltonian in many-body second-order Brillouin–Wigner perturbation theory: Uncovering new size-consistent models

Second-order Møller-Plesset perturbation theory is well-known as a computationally inexpensive approach to the electron correlation problem that is size-consistent with a size-consistent reference but fails to be regular. On the other hand, the less well-known many-body version of Brillouin-Wigner perturbation theory has the reverse properties: it is regular but fails to be size-consistent when used with the standard MP partitioning. Consequently, its widespread use remains limited. In this work, we analyze the ways in which it is possible to use alternative non-MP partitions of the Hamiltonian to yield variants of BW2 that are size-consistent as well as regular. We show that there is a vast space of such BW2 theories and also show that it is possible to define a repartitioned BW2 theory from the ground state density alone, which regenerates the exact correlation energy. We also provide a general recipe for deriving regular, size-consistent, and size-extensive partitions from physically meaningful components, and we apply the result to small model systems. The scope of these results appears to further set the stage for a revival of BW2 in quantum chemistry.

Ab initio perturbation↗
DOE OSTI2012

SIZES AND SURFACE BRIGHTNESS PROFILES OF QUIESCENT GALAXIES AT z {approx} 2

We use deep Hubble Space Telescope Wide Field Camera 3 near-infrared imaging obtained of the GOODS-South field as part of the CANDELS survey to investigate a stellar mass-limited sample of quiescent galaxies at 1.5 < z < 2.5. We measure surface brightness profiles for these galaxies using a method that properly measures low surface brightness flux at large radii. We find that quiescent galaxies at z {approx} 2 very closely follow Sersic profiles, with n{sub median} = 3.7, and have no excess flux at large radii. Their effective radii are a factor of {approx}4 smaller than those of low-redshift quiescent galaxies of similar mass. However, there is a significant spread in sizes ({sigma}{sub log{sub 1{sub 0r{sub e}}}}= 0.24), with the largest z {approx} 2 galaxies lying close to the z = 0 mass-size relation. We compare the stellar mass surface density profiles with those of massive elliptical galaxies in the Virgo Cluster and confirm that most of the mass growth which occurs between z {approx} 2 and z = 0 must be due to accretion of material onto the outer regions of the galaxies. Additionally, we investigate the evolution in the size distribution of massive quiescent galaxies. We find that the minimum size growth required for z {approx} 2 quiescent galaxies to fall within the z = 0 size distribution is a factor of {approx}2 smaller than the total median size growth between z {approx} 2 and z = 0.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

Size dependence of the radio-luminosity-mechanical-power correlation in radio galaxies

We examine the relationship between source radio luminosity and kinetic power in active galactic nucleus jets. We show that neglecting various loss processes can introduce a systematic bias in the jet powers inferred from radio luminosities for a sample of radio galaxies. This bias can be corrected for by considering source size as well as radio luminosity; effectively the source size acts as a proxy for source age. Based on a sample of Fanaroff-Riley Type II radio sources with jet powers derived from the measured hotspot parameters, we empirically determine a new expression for jet power that accounts for the source size, (Q{sub jet}/10{sup 36} W)=1.5{sub −0.8}{sup +1.8}(L{sub 151}/10{sup 27} W Hz{sup −1}){sup 0.8}(1+z){sup 1.0}(D/kpc){sup 0.58±0.17}, where D is source size and L {sub 151} the 151 MHz radio luminosity. By comparing a flux-limited and volume-limited sample, we show that any derived radio-luminosity-jet-power relation depends sensitively on sample properties, in particular the source size distribution and the size-luminosity correlation inherent in the sample. Such bias will affect the accuracy of the kinetic luminosity function derived from lobe radio luminosities and should be treated with caution.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

WITNESSING THE DIFFERENTIAL EVOLUTION OF DISK GALAXIES IN LUMINOSITY AND SIZE VIA GRAVITATIONAL LENSING

We take advantage of the magnification in size and flux of a galaxy provided by gravitational lensing to analyze the properties of 62 strongly lensed galaxies from the Sloan Lens ACS (SLACS) Survey. The sample of lensed galaxies spans a redshift range of 0.20 ≤ z ≤ 1.20 with a median redshift of z = 0.61. We use the lens modeling code LENSFIT to derive the luminosities, sizes, and Sérsic indices of the lensed galaxies. The measured properties of the lensed galaxies show a primarily compact, {sup d}isk{sup -}like population with the peaks of the size and Sérsic index distributions corresponding to ∼1.50 kpc and n ∼ 1, respectively. Comparison of the SLACS galaxies to a non-lensing, broadband imaging survey shows that a lensing survey allows us to probe a galaxy population that reaches ∼2 mag fainter. Our analysis allows us to compare the (z) = 0.61 disk galaxy sample (n ≤ 2.5) to an unprecedented local galaxy sample of ∼670, 000 SDSS galaxies at z ∼ 0.1; this analysis indicates that the evolution of the luminosity-size relation since z ∼ 1 may not be fully explained by a pure-size or pure-luminosity evolution but may instead require a combination of both. Our observations are also in agreement with recent numerical simulations of disk galaxies that show evidence of a mass-dependent evolution since z ∼ 1, where high-mass disk galaxies (M{sub *} > 10{sup 9} M{sub ☉}) evolve more in size and low-mass disk galaxies (M{sub *} ≤ 10{sup 9} M{sub ☉}) evolve more in luminosity.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

A spectroscopic sample of massive, quiescent z ∼ 2 galaxies: implications for the evolution of the mass-size relation

We present deep, near-infrared Hubble Space Telescope/Wide Field Camera 3 grism spectroscopy and imaging for a sample of 14 galaxies at z ≈ 2 selected from a mass-complete photometric catalog in the COSMOS field. By combining the grism observations with photometry in 30 bands, we derive accurate constraints on their redshifts, stellar masses, ages, dust extinction, and formation redshifts. We show that the slope and scatter of the z ∼ 2 mass-size relation of quiescent galaxies is consistent with the local relation, and confirm previous findings that the sizes for a given mass are smaller by a factor of two to three. Finally, we show that the observed evolution of the mass-size relation of quiescent galaxies between z = 2 and 0 can be explained by the quenching of increasingly larger star forming galaxies at a rate dictated by the increase in the number density of quiescent galaxies with decreasing redshift. However, we find that the scatter in the mass-size relation should increase in the quenching-driven scenario in contrast to what is seen in the data. This suggests that merging is not needed to explain the evolution of the median mass-size relation of massive galaxies, but may still be required to tighten its scatter, and explain the size growth of individual z = 2 galaxies quiescent galaxies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

PREDICTION OF SOLAR FLARE SIZE AND TIME-TO-FLARE USING SUPPORT VECTOR MACHINE REGRESSION

We study the prediction of solar flare size and time-to-flare using 38 features describing magnetic complexity of the photospheric magnetic field. This work uses support vector regression to formulate a mapping from the 38-dimensional feature space to a continuous-valued label vector representing flare size or time-to-flare. When we consider flaring regions only, we find an average error in estimating flare size of approximately half a geostationary operational environmental satellite (GOES) class. When we additionally consider non-flaring regions, we find an increased average error of approximately three-fourths a GOES class. We also consider thresholding the regressed flare size for the experiment containing both flaring and non-flaring regions and find a true positive rate of 0.69 and a true negative rate of 0.86 for flare prediction. The results for both of these size regression experiments are consistent across a wide range of predictive time windows, indicating that the magnetic complexity features may be persistent in appearance long before flare activity. This is supported by our larger error rates of some 40 hr in the time-to-flare regression problem. The 38 magnetic complexity features considered here appear to have discriminative potential for flare size, but their persistence in time makes them less discriminative for the time-to-flare problem.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

SILICATE DUST SIZE DISTRIBUTION FROM HYPERVELOCITY COLLISIONS: IMPLICATIONS FOR DUST PRODUCTION IN DEBRIS DISKS

Fragments generated by high-velocity collisions between solid planetary bodies are one of the main sources of new interplanetary dust particles. However, only limited ranges of collision velocity, ejecta size, and target materials have been studied in previous laboratory experiments, and the collision condition that enables the production of dust-sized particles remains unclear. We conducted hypervelocity impact experiments on silicate rocks at relative velocities of 9 to 61 km s{sup -1}, which is beyond the upper limit of previous laboratory studies. Sub-millimeter-diameter aluminum and gold spheres were accelerated by laser ablation and were shot into dunite and basalt targets. We analyzed the surfaces of aerogel blocks deployed near the targets using an electron probe micro analyzer and counted the number of particles that contained the target material. The size distributions of ejecta ranged from five to tens of microns in diameter. The total cross-sectional area of dust-sized ejecta monotonically increased with the projectile kinetic energy, independent of impact velocity, projectile diameter, and projectile and target material compositions. The slopes of the cumulative ejecta-size distributions ranged from -2 to -5. Most of the slopes were steeper than the -2.5 or -2.7 that is expected for a collisional equilibrium distribution in a collision cascade with mass-independent or mass-dependent catastrophic disruption thresholds, respectively. This suggests that the steep dust size-distribution proposed for the debris disk around HD172555 (an A5V star) could be due to a hypervelocity collision.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

SIZING UP Ly{alpha} AND LYMAN BREAK GALAXIES

We measure the sizes for a sample of 174 Ly{alpha}-selected galaxies with broadband imaging with the Hubble Space Telescope. Over the redshift range 2.25 < z < 6, Ly{alpha}-selected galaxies have a characteristic, constant, small size in rest-frame ultraviolet (UV) light. Coupled with a characteristic star formation intensity (i.e., UV luminosity per unit area), this can explain their non-evolving ultraviolet continuum luminosity function. This is in contrast to Lyman break galaxies (LBGs) over the same redshift range, which have been previously shown to increase in linear size as H(z){sup -1}. The compact physical size seems to be a critical determining factor in whether a galaxy will show Ly{alpha} emission or not. The L{sub *} of LBGs and its evolution with redshift can be derived from a simple model where the star formation intensity has an upper limit set by feedback processes, independent of redshift. The increase in L{sub *} of LBGs is mainly driven by the increase in linear size over redshifts for z = 2-7. Since Ly{alpha} galaxies do not grow in linear size, they do not show an increase in L{sub *}.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Source size measurement options for low-emittance light sources

Radiation-based techniques for measuring electron source sizes are widely used as emittance diagnostics at existing synchrotron sources. Three of these techniques, namely, pinhole imaging, double-slit interferometry, and a K-edge filter-based beam position and size monitor system (ps-BPM), are evaluated for measuring source sizes at low-emittance storage rings. Each technique is reviewed with a detailed system description, design optimization, and practical considerations targeted for small source sizes. Pinhole imaging has the simplest setup and gives the beam profile in both transverse dimensions but with limited resolution. Double-slit interferometry has the highest resolution but with a limited detectable size range. The ps-BPM system shows reasonable resolution for monitoring small source sizes and divergence and can give real-time information of the source position and angle. New facilities may consider an integrated system that combines some or all of these techniques.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Size Effects in the Thermal Conductivity of Amorphous Polymers

Manipulating thermal conductivity through nanoengineering is of critical importance to advance technologies, such as soft robotics, artificial skin, wearable electronics, batteries, thermal insulation, and thermoelectrics. Here, by examining amorphous polymers, including polystyrene, polypropylene, polyethylene, and ethylene vinyl alcohol, using molecular dynamics simulations, we find that the thermal conductivities of amorphous polymers can be reduced below their amorphous limit by size effects. Size-dependent thermal transport in amorphous materials is decomposed into crystalline, crystalline-to-amorphous, and amorphous regimes. In the amorphous regime, the mean free path of propagating heat carriers can range from tens of nanometers to more than 100 nm, contributing 16%–36% of the total thermal conductivity. A two-channel model that combines no size effect (i.e., difusons and locons) and size effect (i.e., propagons) is proposed to account for size-dependent thermal conductivity. We also find that the presence of charged molecules in polymers can significantly affect the thermal conductivity and its size effects due to electrostatic interactions. Overall, this work provides insights into the thermal conductivity of amorphous polymers that will have a broad impact on the nano- and chemical engineering of polymers for various energy-related applications.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Chemical control of the Rashba spin splitting size of α-GeTe(111) surface states by adjusting the potential at the topmost atomic layer

As control of the Rashba spin splitting size is highly desirable for spintronic devices, intensive studies have been performed to vary the splitting size by, for example, applying an electric field or designing novel heterostructures. However, direct observation of Rashba spin splitting size change via spectroscopic measurements has not been done so far. Here, we report results of angle-resolved photoemission studies on ferroelectric α-GeTe(111). We observe that the Rashba splitting size of α-GeTe(111) surface states is reduced upon dosing with potassium (K) which has a very low electron affinity. Based on density functional theory calculations, we find that the electric potential energy at the topmost atomic layer and the surface potential energy barrier is reduced upon K dosing. Furthermore, this change in the surface potential induces both delocalization of the surface states and reduction of the splitting size. We expect to increase the splitting size by dosing other elements or molecules with high electron affinity.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Understanding Strong Scaling on GPUs Using Empirical Performance Saturation Size

The roofline model provides a concise overview of the maximum performance capabilities of a given computer system through a combination of peak memory bandwidth and compute performance rates. The increasing complexity of scheduling and cache in recent GPUs, however, has introduced complicated performance variability that is not captured by arithmetic intensity alone. This work examines the effect of problem size and GPU launch configurations on roofline performance for V100, A100, MI100, and MI250X graphics processing units. We introduce an extended roofline model that takes problem size into account, and find that strong scaling on GPUs can be characterized by saturation problem sizes as additional key metrics. Saturation problem sizes break up a plot of GPU performance vs. problem size into three distinct performance regimes– size-limited, cache-bound, and DRAM-bound. With our extended roofline model, we are able to provide a robust view of these performance regimes across recent GPU architectures.

Eberius, David↗
DOE OSTI2016

Uniform deposition of size-selected clusters using Lissajous scanning

Size-selected clusters can be deposited on the surface using size-selected cluster ion beams. However, because of the cross-sectional intensity distribution of the ion beam, it is difficult to define the coverage of the deposited clusters. The aggregation probability of the cluster depends on coverage, whereas cluster size on the surface depends on the position, despite the size-selected clusters are deposited. It is crucial, therefore, to deposit clusters uniformly on the surface. In this study, size-selected clusters were deposited uniformly on surfaces by scanning the cluster ions in the form of Lissajous pattern. Two sets of deflector electrodes set in orthogonal directions were placed in front of the sample surface. Triangular waves were applied to the electrodes with an irrational frequency ratio to ensure that the ion trajectory filled the sample surface. The advantages of this method are simplicity and low cost of setup compared with raster scanning method. The authors further investigated CO adsorption on size-selected Pt{sub n} (n = 7, 15, 20) clusters uniformly deposited on the Al{sub 2}O{sub 3}/NiAl(110) surface and demonstrated the importance of uniform deposition.

42 ENGINEERING↗
DOE OSTI2012

Automated size-specific CT dose monitoring program: Assessing variability in CT dose

Purpose: The potential health risks associated with low levels of ionizing radiation have created a movement in the radiology community to optimize computed tomography (CT) imaging protocols to use the lowest radiation dose possible without compromising the diagnostic usefulness of the images. Despite efforts to use appropriate and consistent radiation doses, studies suggest that a great deal of variability in radiation dose exists both within and between institutions for CT imaging. In this context, the authors have developed an automated size-specific radiation dose monitoring program for CT and used this program to assess variability in size-adjusted effective dose from CT imaging. Methods: The authors radiation dose monitoring program operates on an independent health insurance portability and accountability act compliant dosimetry server. Digital imaging and communication in medicine routing software is used to isolate dose report screen captures and scout images for all incoming CT studies. Effective dose conversion factors (k-factors) are determined based on the protocol and optical character recognition is used to extract the CT dose index and dose-length product. The patient's thickness is obtained by applying an adaptive thresholding algorithm to the scout images and is used to calculate the size-adjusted effective dose (ED{sub adj}). The radiation dose monitoring program was used to collect data on 6351 CT studies from three scanner models (GE Lightspeed Pro 16, GE Lightspeed VCT, and GE Definition CT750 HD) and two institutions over a one-month period and to analyze the variability in ED{sub adj} between scanner models and across institutions. Results: No significant difference was found between computer measurements of patient thickness and observer measurements (p= 0.17), and the average difference between the two methods was less than 4%. Applying the size correction resulted in ED{sub adj} that differed by up to 44% from effective dose estimates that were not adjusted by patient size. Additionally, considerable differences were noted in ED{sub adj} distributions between scanners, with scanners employing iterative reconstruction exhibiting significantly lower ED{sub adj} (range: 9%-64%). Finally, a significant difference (up to 59%) in ED{sub adj} distributions was observed between institutions, indicating the potential for dose reduction. Conclusions: The authors developed a robust automated size-specific radiation dose monitoring program for CT. Using this program, significant differences in ED{sub adj} were observed between scanner models and across institutions. This new dose monitoring program offers a unique tool for improving quality assurance and standardization both within and across institutions.

60 APPLIED LIFE SCIENCES↗