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At least 685 records · Page 38

Bridging the length scales on mechanical property evaluation (Final Report)

The development of small-scale mechanical testing in combination with microstructural investigation is of great interest to the nuclear materials community for both materials development and monitoring applications. Dramatically reducing the sample sizes to reduce radioactivity and obtaining mechanical properties of irradiated samples is truly intriguing. Moreover, such studies promise a range of benefits including cost reduction, fundamental insight in structure-property relationships, increased statistics on less sample material, and reinvestigation of prior irradiated and tested reactor samples while simultaneously enabling the generation of mechanical test data on ion beam irradiated materials with limited penetration depths. Small scale materials testing on sub-sized samples has been studied for several decades, though it has only been after the development of micro-testing based on Focused Ion Beam (FIB) sample manufacturing in that orders of magnitude smaller samples could really be investigated in a quantitative manner. In recent years, small scale mechanical testing techniques at a number of length scales has been developed for both unirradiated and irradiated (ion and neutron) materials. Technological advances made in this field have enabled ex-situ and in-situ transmission electron microscopy (TEM) and scanning electron microscopy (SEM) examination, thus leading to more accurate measurements as well as additional mechanistic information. A recent review of the benefits of these techniques show that these techniques are at a stage to tackle multi-scale ranges of materials investigations and can be utilized to obtain fundamental science-based understanding of nuclear materials. Considering the tremendous advances made, one can see how small-scale mechanical testing techniques combined with modeling can enable true small scale to bulk scale mechanical property correlations. However, for the engineering community to adapt this approach fully, one needs to demonstrate that a) that these techniques can produce results with high fidelity and reproducibility, b) generate engineering stress-strain data that one can utilize to understand bulk behavior, and c) generate new insight into relevant phenomena fostering the true understanding of radiation damage and microstructure in materials for nuclear applications. It is the objective of this proposal to bridge the length scale between macro- and micro- scale mechanical testing of unirradiated and irradiated materials. This involves the development and demonstration of procedures for multi-scale mechanical testing that enable high fidelity reproducibility of data and the generation bulk property data from small-scale mechanical tests. Through this, the proposal aims to enhance the confidence in the obtained data at the smaller length scales and enhance the insight provided from these techniques for bulk scale applications on both unirradiated and irradiated materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Validation of the SCEPTRE Boltzmann-CSD Solver

A new Boltzmann-CSD solver has been developed within the SCEPTRE radiation-transport code, based on the 1st-order form of the transport equation, using discontinuous finite elements in space and energy and discrete ordinates in angle. The Boltzmann-CSD solver has been validated against experimental data for electron energy deposition distributions and for electron emission spectra. Comparison of the calculated results with experimental data shows excellent agreement for many of the test configurations and reasonable agreement for other test configurations. The tests have also been modeled with the ITS Monte Carlo code, which also shows excellent to reasonable agreement with the SCEPTRE results and experimental data. The SCEPTRE Boltzmann-CSD solver relies on electron cross sections generated by the legacy CEPXS code, which currently is limited to electron-only Boltzmann-CSD cross sections. Performing full electron-photon radiation transport with the Boltzmann-CSD solver will require further development in the cross section generating code. For the energy- deposition calculations, neglecting photon transport results in at most about 5% overprediction of the energy deposition for high-energy electrons on high-Z targets, and relatively insignificant difference for the other test configurations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Preliminary Procedures and Acceptance Criteria for in-situ Structural Materials Surveillance for MSR

This report describes the initial development of the technical basis for a materials surveillance technology that, when fully developed and validated, can be used by stakeholders to develop and implement a materials surveillance program to manage materials degradation during reactor operations. The procedures described in this report aim to bound the detrimental effects of the reactor environment on the creep-fatigue life of the reactor components through materials surveillance. Specifically, the report describes procedures for selecting critical locations within the reactor components for surrogate materials surveillance and the sizing and placements of passively-actuated materials surveillance test articles under development by the US Department of Energy, Advanced Reactor Technologies Program. These test articles apply cyclic thermomechanical load to a surrogate sample of the component structural material passively through thermal expansion mismatch within the articles, without requiring any penetrations in the reactor coolant boundary. The procedures can be used to size materials surveillance test articles so that they will fail before the corresponding structural component. These articles would be exposed to the component operating environment, located to experience a bounding radiation fluence and representative coolant exposure. They can be monitored during reactor operations to ensure that they have not failed under the combination of creep-fatigue damage and environmental degradation. The report describes the key technical decisions and the corresponding rational for using these procedures to provide advanced warning of any impending material failure. An appendix describes the technical basis and the procedure for sizing a family of passively-actuated test articles. Finally, the report describes future work needed to complete the technical basis underlying this materials surveillance technology.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

First full Dalitz plot measurement in neutron 𝛽 decay using the Nab spectrometer and implications for new physics

Precision measurements of observables in neutron 𝛽 decay are used to test the standard model description of the weak interaction and search for evidence of new physics. The Nab experiment at the Fundamental Neutron Physics Beamline at the Spallation Neutron Source was constructed to measure correlations in neutron decay by utilizing an asymmetric spectrometer and novel detection system to accurately reconstruct the proton momentum and electron energy for each 𝛽 decay. This work describes the detection of neutron 𝛽-decay products in the Nab spectrometer and presents the first full Dalitz plot representation of the phase space of neutron 𝛽 decay for all electrons >100 keV. In addition, new constraints are placed on a possible excited neutron state, hypothesized to explain the disagreement between the appearance and disappearance neutron lifetime techniques.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

3D radiated power analysis of JET SPI discharges using the Emis3D forward modeling tool

Abstract Precise values for radiated energy in tokamak disruption experiments are needed to validate disruption mitigation techniques for burning plasma tokamaks like ITER and SPARC. Control room analysis of radiated power ( P rad ) on JET assumes axisymmetry, since fitting 3D radiation structures with limited bolometry coverage is an under-determined problem. In mitigated disruptions, radiation is toroidally asymmetric and 3D, due to fast-growing 3D MHD modes and localized impurity sources. To address this problem, Emis3D adopts a physics motivated forward modeling (‘guess and check’) approach, comparing experimental bolometry data to synthetic data from user-defined radiation structures. Synthetic structures are observed with the Cherab modeling framework and a best fit chosen using a reduced χ 2 statistic. 2D tomographic inversion models are tested, as well as helical flux tubes and 3D MHD simulated structures from JOREK. Two nominally identical pure neon shattered pellet injection (SPI) mitigated discharges in JET are analyzed. 2D tomographic inversions with added toroidal freedom are the best fits in the thermal quench (TQ) and current quench (CQ). In the pre-TQ, 2D reconstructions are statistically the best fits, but are likely over-optimized and do not capture the 3D radiation structure seen in fast camera images. The next-best pre-TQ fits are helical structures that extend towards the high-field side, consistent with an impurity flow under the magnetic nozzle effect also observed in JOREK simulations. Whole-disruption radiated fractions of 0.98 + 0.03 / − 0.29 and 1.01 + 0.02 / − 0.17 are found, suggesting that the stored energy may have been fully mitigated by each SPI, although mitigation efficiencies well below ITER and SPARC requirements for high energy pulses are still within the large uncertainties. Emis3D is also used to validate JOREK SPI simulations, and confirms improvements in matching experiment from changes to impurity modeling. Time-dependent toroidal peaking factors are calculated and discussed.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Complete time-resolved X-ray shape capability for a 10 MJ implosion: Milestone Report for MRT 8818

This report documents completion of MRT 8818, which established an upgraded equatorial time-resolved X-ray imaging capability for high-yield inertial confinement fusion experiments at the National Ignition Facility (NIF) using the equatorial Dilation X-ray Imager (DIXI). The need for this work arose from the sustained increase in fusion yield at NIF, which progressively intensified the neutron and gamma-ray environment experienced by target diagnostics. Although the existing polar imaging capability, particularly the Polar Dilation X-ray Imager (PDIXI), remained viable at high yields, the equatorial capability became inadequate because of radiation-induced failure of electronic readout hardware and increasing background levels that degraded image quality and ultimately caused saturation. The work performed under MRT 8818 addressed this limitation through a combination of hardware replacement, background characterization, and targeted mitigation. The DIXI backend was converted from CCD-based electronic readout to photographic film, and the principal sources of internally generated background were investigated using prior analyses, dedicated tests, and comparison with PDIXI performance on high-yield shots. This effort led to implementation of two principal improvements: a multilayer optical coating to suppress broadband radiation-induced background generated in the fiber-optic extension cylinder, and replacement of Kodak TMAX 400 film with Agfa Copex Rapid to reduce background generated directly in the film. These upgrades were completed in 2025 and performance assessment based on DT shot data since then, comparing with Polar DIXI and scaling of these experiments to 10 MJ indicates an expected signal-to-background ratio of approximately 34 for a single pinhole image, substantially exceeding the MRT 8818 completion criterion of SNR > 5.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Trigger-System Development for the HGCAL Cassette Testing (Final Report, Summer Internship 2023)

The Large Hadron Collider (LHC) will be upgraded to increase the instantaneous luminosity, which will result in an increase in the number of collisions from the 15 pile-up events of the first run of phase 1 to the 150-200 pile-up events of phase 2. Increasing the number of collisions means increasing the amount of radiation that the experiments will absorb. To meet these challenging conditions, the CMS calorimeters need to be upgraded. The new version of the hadronic HGCAL (High Granularity CALorimeters) in the endcaps will be assembled and tested in Fermilab’s laboratory. This report describes the new trigger system for testing the HGCAL’s cassettes.

42 ENGINEERING↗

Multi-frequency General Relativistic Radiation-hydrodynamics with M 1 Closure

We report on recent upgrades to our general relativistic radiation-magnetohydrodynamics code, Cosmos++ , which expands the two-moment, M 1 , radiation treatment from gray to multi-frequency transport, including Doppler and gravitational frequency shifts. The solver accommodates either photon (Bose–Einstein) or neutrino (Fermi–Dirac) statistical distribution functions with absorption, emission, and elastic scattering processes. An implicit scheme is implemented to simultaneously solve the primitive inversion problem together with the radiation–matter coupling source terms, providing stability over a broad range of opacities and optical depths where the interaction terms can be stiff. We discuss our formulations and numerical methods, and validate our methods against a wide variety of test problems spanning optically thin to thick regimes in flat, weakly curved, and strongly curved spacetimes.

79 ASTRONOMY AND ASTROPHYSICS↗

Modeling of ATR fuel in DOE Standard Canisters with Helium Backfilled Condition

Road-ready and final disposition packaging configurations for the advanced test reactor (ATR) fuel dictates storage within helium backfilled sealed DOE standard canisters. These sealed canisters are intended for extened (>50 year) dry storage). The typical packaging configuration for the 15-foot DOE canisters places 10 ATR elements within a Type 1a basket, and three baskets are loaded within each DOE canister. During in-reactor operations and cooling pond storage conditions, oxyhydroxide layers form on the surface of the aluminum clad fuel. These layers produce hydrogen gas over time due to the fuel’s radiation field. As part of the packing procedure, the ATR fuel should be dried to remove any residual physio-/chemi- sorbed water from the surface. As testing to the effectiveness of the drying procedure is still underway, this modeling will include results at fully saturated and fully dried conditions. In previous modeling efforts, the G-value for the production of hydrogen from the oxyhydroxide layers was assumed to be in argon environments as measured by Task 2 - Oxyhydroxide Layer Radiolytic Gas Generation Resolution. Previous experimental testing showed differences in the hydrogen generated based on the gaseous environment. In the associated experimental work, Task 2 - Oxyhydroxide Layer Radiolytic Gas Generation Resolution, additional tests were completed in a helium environment, and updated G-values for the radiolytic production of hydrogen from the oxyhydroxide layers were provided. These values are 28% and 58% higher than values for argon. In addition, a change to the modeling of the oxyhydroxide radiolysis has been made from previous reports. This change assumes the dependency of the dose rate on the overall reaction rate is applied to the total weight of the sample, rather than to just the weight of the oxyhydroxide layer. This decreases the dependency of the radiolytic reaction on the thickness of the oxyhydroxide layer. For a nominal scenario of stored ATR fuel, assuming the chemi-/physio- sorbed water have been fully removed, the internal canister pressure increases to 1.61 atm over a 50 year period, with a hydrogen mole percentage of 21%. As in previous modeling, any oxygen present is in negligible amounts (<1 ppt). If a small amount residual air is present, nitric acid can form up to 1300 ppm. For a scenario with high fuel decay heat, the model shows internal pressure increasing to 2.1 atm, with 39.3 mole percentage of hydrogen. In a scenario where significant chemi-/physio- sorbed water is present within the corrosion layer, the nominal scenario shows a pressure increase to 2.54 atm, with 21.1 mole percent hydrogen. The high decay heat case shows a pressure increase to 3.18 atm with 39.9 mole percent hydrogen.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Thermodynamic assessment of the quaternary WTaCrV refractory high entropy alloy as a means to guide experimental approaches

The deployment of fusion energy poses challenges for materials in plasma facing components to withstand high temperatures and thermal gradients, particle implantation and neutron damage. The current material of choice is tungsten, although property degradation limits its consideration in future fusion reactors. Hence, materials with better resistance to harsh environments need to be developed for fusion energy to become a reality. High entropy alloys are being explored as potential candidates with some compositions showing good radiation resistance to defect cluster formation. One of these materials is the WTaCrV system, although only one composition has been tested under ion irradiation. In this work, we study the thermodynamic properties of the entire quaternary alloy composition range. Coupling first principles calculations, cluster expansion approaches, and Monte Carlo methods, we access the free energy functionals, short-range ordering as a function of temperature, and atomic configurations that can be compared to experimental observations. We use this data to inform experiments into compositions with higher propensity to form solid solutions, instead of phase separating. With this formalism we have developed thermodynamic database (TDB) files that can be used to plot quaternary phase diagrams.

Cluster Expansion↗

Fracturing process of micro-concrete under uniaxial and triaxial compression: Insights from in-situ X-ray mechanical tests

This paper presents an experimental study of concrete at meso-scale (aggregates, macro-pores and mortar matrix) in order to get a better understanding of the local failure mechanisms known to drive the macroscopic mechanical behaviour of the material. The main originality comes from conducting in-situ X-ray mechanical tests on micro-concrete samples of realistic composition (including cement, sand, aggregates and water), under uniaxial compression and, for the first time, under triaxial compression at 5 MPa, 10 MPa and 15 MPa confining pressures. A timeseries analysis of the set of 3D images coming from each test allows for the measurement of the 3D kinematic fields (displacement and strain fields) throughout the experiments. The different failure patterns observed for each loading path are discussed, along with a quantification of the 3D fracturing processes at the scale of the largest heterogeneities (aggregates and macro-pores). With an increasing level of confinement, the transition from brittle to ductile response is observed, as well as an increase of the strength of the material. The pronounced impact of the meso-scale heterogeneities of concrete on their local failure mechanisms is highlighted. It is shown that strain localisation mainly originates between aggregates and mortar matrix, with the shape and location of the largest aggregates and macro-pores essentially driving the propagation of the cracking network.

36 MATERIALS SCIENCE↗

A comparison of surrogate constitutive models for viscoplastic creep simulation of HT-9 steel

Mechanistic microstructure-informed constitutive models for the mechanical response of polycrystals are a cornerstone of computational materials science. However, as these models become increasingly more complex – often involving coupled differential equations describing the effect of specific deformation modes – their associated computational costs can become prohibitive, particularly in optimization or uncertainty quantification tasks that require numerous model evaluations. To address this challenge, surrogate constitutive models that balance accuracy and computational efficiency are highly desirable. Data-driven surrogate models, that learn the constitutive relation directly from data, have emerged as a promising solution. In this work, we develop two local surrogate models for the viscoplastic response of a steel: a piecewise response surface method and a mixture of experts model. These surrogates are designed to adapt to complex material behavior, which may vary with material parameters or operating conditions. The surrogate constitutive models are applied to creep simulations of HT-9 steel, an alloy of considerable interest to the nuclear energy sector due to its high tolerance to radiation damage, using training data generated from viscoplastic self-consistent (VPSC) simulations. In conclusion, we define a set of test metrics to numerically assess the accuracy of our surrogate models for predicting viscoplastic material behavior, and show that the mixture of experts model outperforms the piecewise response surface method in terms of accuracy.

36 MATERIALS SCIENCE↗

Improved limits on Fierz interference using asymmetry measurements from the Ultracold Neutron Asymmetry (UCNA) experiment

The Ultracold Neutron Asymmetry (UCNA) experiment was designed to measure the β-decay asymmetry parameter, A 0 , for free neutron decay. In the experiment, polarized ultracold neutrons are transported into a decay trap, and their β-decay electrons are detected with ≈4π acceptance into two detector packages which provide position and energy reconstruction. The experiment also has sensitivity to b n , the Fierz interference term in the neutron β-decay rate. In this work, we determine bn from the energy dependence of A 0 using the data taken during the UCNA 2011–2013 run. In addition, we present the same type of analysis using the earlier 2010 A dataset. Furthermore, motivated by improved statistics and comparable systematic errors compared to the 2010 data-taking run, we present a new b n measurement using the weighted average of our asymmetry dataset fits, to obtain b n = 0.066 ± 0.041 stat ± 0.024 syst which corresponds to a limit of -0.012 < b n < 0.144 at the 90% confidence level.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Pseudo-neutrino versus recoil formalism for 4-body phase space and applications to nuclear decay

It is well known that the traditional treatment of radiative corrections that utilizes the “true” neutrino momentum$\overrightarrow{p}_v$ in the differential decay rate formula could lead to a ~α/π systematic error in certain observables due to the mistreatment of 4-body kinematics. Here, I investigate the theory structure of one of the proposed solutions, the “v'-formalism”, in the nonrecoil limit appropriate for neutron and nuclear β decays. I derive an elegant master formula for the 4-body phase space and use it to reanalyze the spectrum-dependent “outer” radiative corrections to the β decay of a polarized spin-half nucleus; a complete set of analytic expressions is provided for readers to straightforwardly obtain the final numerical results. Furthermore, I compare it to the “recoil formalism” where the energy of the recoil nucleus is fixed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

SPC-70646 Specification for Reactor Supplemental Shielding for Use in DOME

NRIC is developing the Demonstration of Microreactor Experiments (DOME) test bed at the Idaho National Laboratory (INL) Materials and Fuels Complex (MFC): to allow for testing of advanced reactors in support of future licensing and commercial operations. One such need is a neutron and photon radiation shielding system to protect personnel and equipment from harsh neutron and photon fluxes during reactor operations and post shut down operations, disassembly, and decommissioning.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

CMS Outer Tracker Module QA

The High Luminosity Large Hadron Collider is a planned upgrade to the LHC that will allow it to take up to 7 times as much data. Upgrades to all detector systems, including the Outer Tracker, are necessary to allow them to handle the increased radiation and pileup. Fermilab has been tasked with assembling modules for the Outer Tracker system. This presentation discusses the QA tests performed on these modules and the integration procedure required to ensure all modules work in sync. The QA tests include sensor IV curves, MaPSA testing, visual inspection, skeleton testing, and module testing. There are additional tests that can only be performed on integrated modules that are working in sync, and developing an understanding of the timing and latency of the modules is necessary to perform this synchronization.

Hobbeheydar, Samuel [Fermilab; Carnegie Mellon U. ↗

CMS Outer Tracker Module QA

The High Luminosity Large Hadron Collider is a planned upgrade to the LHC that will allow it to take up to 7 times as much data. Upgrades to all detector systems, including the Outer Tracker, are necessary to allow them to handle the increased radiation and pileup. Fermilab has been tasked with assembling modules for the Outer Tracker system. This presentation discusses the QA tests performed on these modules and the integration procedure required to ensure all modules work in sync. The QA tests include sensor IV curves, MaPSA testing, visual inspection, skeleton testing, and module testing. There are additional tests that can only be performed on integrated modules that are working in sync, and developing an understanding of the timing and latency of the modules is necessary to perform this synchronization.

Hobbeheydar, Samuel [Fermilab; Carnegie Mellon U. ↗