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At least 685 records · Page 38
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Speed of sound in methane under conditions of planetary interiors

We present direct observations of acoustic waves in warm dense matter. We analyze wave-number- and energy-resolved x-ray spectra taken from warm dense methane created by laser heating a cryogenic liquid jet. X-ray diffraction and inelastic free-electron scattering yield sample conditions of 0.3 ± 0.1 eV and 0.8 ± 0.1 g/ cm − 3 , corresponding to a pressure of ∼ 13 GPa. Inelastic x-ray scattering was used to observe the collective oscillations of the ions. With a highly improved energy resolution of ∼ 50 meV, we could clearly distinguish the Brillouin peaks from the quasielastic Rayleigh feature. Data at different wave numbers were utilized to derive a sound speed of 5.9 ± 0.5 km/s, marking a high-temperature data point for methane and demonstrating consistency with Birch's law in this parameter regime. Published by the American Physical Society 2024

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Measurement accuracy and spatial resolution of a distributed temperature sensor based on a two-pulse differential coherent reflectometer

We present a model and numerical simulation of a distributed temperature sensor based on a two-pulse differential coherent optical time-domain reflectometer (COTDR). The differential phase measured using a phase-sensitive Rayleigh reflectometer is shown to have a regular component, which is a linear function of temperature, and a random component, which is related to a random distribution of scattering centres in the fibre and restricts the accuracy of measurements of variations in temperature. Measurement accuracy can be improved by reducing the relative contribution of the random component via a decrease in pulse duration and/or an increase in the time delay between pulses. The spatial resolution of a differential two-pulse phase-sensitive reflectometer is shown to be determined by the time delay between pulses and to vary little with pulse duration. At a typical pulse duration (200 ns) and delay time (300 ns), the accuracy in measurements of variations in temperature in the 0.1-K range is 2 % and the spatial resolution is about 30 m. (fibre-optic sensors)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1989

Scattering by fluffy grains

There are indications (Greenberg et al., 1988), that fluffy (i.e., porous) particles are responsible for the observed 3.4 and 10 micron emissions of comet Halley. The absorption characteristics of small particles both solid and fluffy are needed in order to explain the Halley emissions. How isolated small solid particles react to an external radiation field is well known - the Rayleigh approximation. How these same small particles emit when assembled as fluffy aggregates in another question. To what degree are the emission spectra of isolated and aggregated particles comparable. In order to quantify the assertion that fluffy particles produce the observed Halley infrared emission features, the authors are performing calculations to determine the effect of porosity on the absorption characteristics of aggregates of interstellar grain-type particles. The calculations are based on an integral representation of the scattered electromagnetic field. Results are given with application to comet Halley.

Hage, J. I.↗
DOE OSTI2021

Engineering the beat phenomenon of quasi-Rayleigh waves for regions with minimal Surface Acoustic Wave (SAW) amplitude

Surface Acoustic Waves (SAW) are prevalent in a variety of scientific fields. Typically, the ability to manipulate these surface waves has a significant impact on the efficacy of any SAW-based device. In this paper, we present a simple method for designing localized regions that have minimal SAW amplitude. These localized regions have valley-like drops in SAW amplitude and are achieved by using the spatial beat phenomenon of quasi-Rayleigh waves. Controlling the beat phenomenon allows us to manipulate where and how these localized regions appear in the waveguide. In particular, the localized regions can be designed to have variable widths and can be positioned consecutively due to minimal wave scattering. The design methodology and physics are described in detail, and several supplementary simulations are provided to demonstrate the efficacy of the proposed method. Finally, we briefly discuss how the proposed approach could potentially be exploited to implement a localized high-pass filter and enables SAW wave propagation that avoids surface obstacles.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Discoveries in Blast-Driven Turbulence of Astrophysical Relevance

The fluid mixing caused by variable-density instabilities is important in a wide variety of scenarios from ocean mixing and astrophysical phenomena to nuclear fusion techniques and atomic weapons. This thesis explores the mixing resulting from a specific instability known as the Blast Driven Instability (BDI). This work investigates the variable density mixing in an explosively driven environment due to the fluid instabilities at the material interfaces. Specifically, diverging Richtmyer-Meshkov (impulsive-acceleration environment) and Rayleigh-Taylor (variable-acceleration environment) instabilities (present in supernova and inertial confinement fusion) are studied using advanced high-speed diagnostics in carefully designed laboratory experiments. The BDI morphology is presented through a time development of Mie scattering images, and steps through the parameter space (varying density ratio and driver speed), highlighting the development of the structures that form during mixing. A scaling criterion is used to relate the two systems of vastly different spatiotemporal scales. Velocity fields in the BDI have been captured for the first time using the high temporal resolution PIV technique. Subsequent analysis of the dynamics of the instability from the velocity fields illustrates the distribution of kinetic energy, the transition to turbulence, and the characteristic growth of the instability are discussed. This study furthers understanding of how blast-driven instability pertains to supernova and inertial confinement fusion science. The morphology of the BDI has been characterized for the first time. This work steps through the parameter space covered in Mie scattering experiments, and how the different parameters contribute to development of structures and mixing. It also examines a scaling of the Atwood number for expanding predictive capabilities to other experimental conditions and simulations. The first collection of velocity fields acquired for the BDI are recorded, and subsequent analysis evaluating the distribution of kinetic energy throughout space and time for two density ratios from the overall parameter space, as well as the transition to turbulence, estimated from a Reynolds number calculated based on momentum mixing are all presented. This information is useful in advancing the development of models to predict physics of high energy density applications where experiments are not always readily available. This research has successfully demonstrated understanding for the time criteria defining regimes where the shock driven (Richtmyer-Meshkov instability) and the buoyancy driven (Rayleigh-Taylor instability) dominates through a parametric study of density variation (Atwood number) and driver speed (Mach number). All this furthers understanding of how the BDI pertains to SN and ICF.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1980

Investigation of numerical properties of Hovenier's exit function equation for multiple scattering of light

A technique of deriving Hovenier's exit function equation (1978) for multiple scattering, starting with a set of invariant imbedding equations, is presented. The feasibility of the exit function equation as a means to obtain reflection and transmission functions is investigated for isotropic, Rayleigh, and Henyey-Greenstein phase functions with emphasis on the numerical stability, accuracy and timing. It is possible to compute the reflection function rather accurately with an efficiency comparable to that of the standard doubling technique for the same phase functions with moderate anisotropy. The resulting transmission is slightly less accurate than the reflection function, but it may be acceptable for practical purposes.

Kawabata, K.↗
NASA NTRS1994

Intercomparison of density and temperature profiles obtained by lidar, ionizatoin gauges, falling spheres, datasondes and radiosondes during the DYANA campaign

During the course of the DYnamics Adapted Network for the Atmosphere (DYANA) campaign in early 1990, various techniques to measure densities and temperatures from the ground up to the lower thermosphere were employed. Some of these measurements were performed near simultaneously (maximum allowed time difference: 1 h) and at the same location, and therefore offered the unique chance of intercomparison of different techniques. In this study, we will report on intercomparisons of data from ground-based instruments (Rayleigh- and sodium-lidar), balloon-borne methods (datasondes and radiosondes) and rocket-borne techniques (falling spheres and ionization gauges). The main result is that there is good agreement between the various measurements when considering the error bars. Only occasionally did we notice small but systematic differences (e.g. for the datasondes above 65 km). The most extensive intercomparison was possible between the Rayleigh lidar and the falling sphere technique, both employed in Biscarrosse (44 deg N, 1 deg W). Concerning densities, excellent agreement was found below 63 km: the mean of the deviations is less than 1% and the root mean square (RMS) is approximately 3%. Systematic differences of the order of 5% were noticed around 67 km and above 80 km. The former can be accounted for by an instrumental effect of the falling sphere (Ma = 1 transition; Ma = Mach number), whereas the latter is tentatively explained by the presence of Mie scatterers in the upper mesosphere. Concerning temperatures, the agreement is excellent between 35 and 65 km: the mean of the deviations is less than +/- 3 K and the variability is +/- 5 K. The two systematic density differences mentioned above also affect the temperatures: between 65 and 80 km, the Rayleigh lidar temperatures are systematically lower than the falling sphere values by approximately 5 K.

Lubken, F.-J.↗
NASA NTRS1973

On the surface-to-bulk mode conversion of Rayleigh waves.

Surface-to-bulk wave conversion phenomena occurring at a discontinuity characterized by a surface contour deformation are shown to be usable as a means for tapping Rayleigh waves in a nonpiezoelectric solid. A boundary perturbation technique is used in the treatment of the mode conversion problem. A systematic procedure is presented for calculating not only the first-order scattered waves, which include the reflected surface wave and the converted bulk wave, but also the higher order terms.

Chang, C.-P.↗
NASA NTRS1978

Forwardscattering corrections for optical extinction measurements in aerosol media. II - Polydispersions

The paper presents a parametric study of the forwardscattering corrections for experimentally measured optical extinction coefficients in polydisperse particulate media, since some forward scattered light invariably enters, along with the direct beam, into the finite aperture of the detector. Forwardscattering corrections are computed by two methods: (1) using the exact Mie theory, and (2) the approximate Rayleigh diffraction formula for spherical particles. A parametric study of the dependence of the corrections on mode radii, real and imaginary parts of the complex refractive index, and half-angle of the detector's view cone has been carried out for three different size distribution functions of the modified gamma type. In addition, a study has been carried out to investigate the range of these parameters in which the approximate formulation is valid. The agreement is especially good for small-view cone angles and large particles, which improves significantly for slightly absorbing aerosol particles. Also discussed is the dependence of these corrections on the experimental design of the transmissometer systems.

Deepak, A.↗
NASA NTRS1974

Observations of He I 584 A nighttime radiation - Evidence for an interstellar source of neutral helium

The intensity and spatial variations of the He I 584 A radiation in the night sky were measured to an altitude of 264 km from a sounding rocket launched from Thumba, India. The flux varied in intensity with look angle from a high of 16 plus or minus 5 rayleighs to a low of less than 1 rayleigh. The data obtained are presented in the form of an all-sky map. Since the peak flux levels observed are approximately two orders of magnitude larger than that expected from geocoronal resonant scattering, we have compared our results with those expected from two interplanetary sources of neutral helium: the penetration of the local interstellar medium into the solar neighborhood and the dust deionization of solar-wind alpha particles. The dust deionization-model predictions using currently accepted input parameters appear to be inconsistent with the observations. The interstellar helium source is compatible with the data to within the uncertainties of the models.

Paresce, F.↗
NASA NTRS1988

IUE observations of Neptune for H Lyman-alpha emission

Study of seven IUE observations has not resulted in the detection of H Ly-alpha emission from Neptune, with 1-sigma upper limits to the planet-averaged surface brightness as low as 180 Rayleighs. The intrinsic brightness is found to be less than the 400-1500 R that would be expected from scaling arguments, and it is noted that this upper limit excludes neither the possibility of scattered solar H Ly-alpha emission from a Jupiter-like atmosphere, nor auroral emission from an active magnetosphere. The results suggest that Neptune has a lower upper atmospheric temperature than Uranus.

Clarke, John T.↗
NASA NTRS1992

Measurements of Stratospheric Pinatubo Aerosol Extinction Profiles by a Raman Lidar

The Raman lidar has been used for remote measurements of water vapor, ozone and atmospheric temperature in the lower troposphere because the Raman cross section is three orders smaller than the Rayleigh cross section. We estimated the extinction coefficients of the Pinatubo volcanic aerosol in the stratosphere using a Raman lidar. If the precise aerosol extinction coefficients are derived, the backscatter coefficient of a Mie scattering lidar will be more accurately estimated. The Raman lidar has performed to measure density profiles of some species using Raman scattering. Here we used a frequency-doubled Nd:YAG laser for transmitter and received nitrogen vibrational Q-branch Raman scattering signal. Ansmann et al. (1990) derived tropospherical aerosol extinction profiles with a Raman lidar. We think that this method can apply to dense stratospheric aerosols such as Pinatubo volcanic aerosols. As dense aerosols are now accumulated in the stratosphere by Pinatubo volcanic eruption, the error of Ramen lidar signal regarding the fluctuation of air density can be ignored.

Abo, Makoto↗
NASA NTRS1992

Wind Measurements from 15 to 50 Km with a Doppler Rayleigh Lidar

The possibility to measure the mean wind in the high stratosphere using a Doppler Rayleigh lidar was demonstrated in 1989, and the Observatory of Haute Province (44 deg N, 6 deg E). It was originally developed to cover the height range 25-60 km, a region where the radars cannot operate; therefore, the system was designed to cover altitudes where the signal is only due to the Rayleigh backscattering. The instrument is currently set up at the Center d'Essais des Landes (44 deg N, 1 deg W) where it operated during the Dynamic Adapted Network for the Atmosphere Campaign in 1990. As the contribution of the Mie scattering was very low during this period above southern France, we have obtained vertical wind profiles in the stratosphere down to 15 km. Since the eruption of the Pinatubo volcano in Jun. 1991, the contribution of Mie scattering has increased between 15 and 30 km and it was very difficult with the original system to obtain wind measurements below 30 km. We will show that by using the same method with slightly different characteristics of the system, it is possible to measure the wind in the presence of Mie scattering. The first experimental results are presented.

Garnier, A.↗
NASA NTRS1986

Methods for the solution of radiative transfer equation

To obtain an exact solution of the radiative-transfer equation in media where both absorption and scattering are significant, the usual approach is to use a numerical method. Three methods are known in the literature: invariant imbedding, eigenvalue-eigenfunction, and matrix doubling. This paper examines the practical application of these methods to the problem of emission from an inhomogeneous (Rayleigh) layer, the effects of layer parameters on the stability. It is found that invariant imbedding is most suitable for computing emission from an inhomogeneous layer with a temperature profile but tends to be unstable as the optical thickness of the layer increases beyond 0.5. On the other hand, the matrix-doubling method is stable for arbitrary optical thickness but is not suitable for handling multilayers. The eigenvalue-eigenfunction method is more stable than the invariant imbedding as optical thickness increases up to 2.0. It also permits temperature profile in the layer, but the computation is much more complicated. It is less stable than the matrix-doubling method when optical thickness is larger than 2.0. In general, the choice of a method is dependent on the nature of the problem.

Chen, M. F.↗
NASA NTRS1990

Experimental flaw detection by scattering of plate waves

The surface displacements of elastic waves scattered from a surface-breaking crack are measured with a capacitive transducer on a 2D plate, and comparisons with theoretical predictions are reported. The noncontacting detector has a wide and flat frequency response which measures the response of a glass plate to the propagation of Rayleigh-Lamb waves. A theoretical simulation of the surface displacements is generated by multiplying experimental traces with a cosine window, and Green's function is used to compute the source function. Power spectra are also recorded from the experiment to compare the results with a finite-element model of the crack, and good agreement is reported for results in both the time and frequency domains. The crack can be detected in the far field when the spacing of the receiver locations is small, and the transducer/probe appears to be a practical flaw-detection instrument.

Spetzler, Hartmut↗
NASA NTRS1973

Development of an experiment for visible radiation measurements from a satellite

The inversion problem, I.E., determining the atmospheric turbidity from polarimetry of radiation emerging from the earth's atmosphere, is presented. A major theoretical advance was made by finding a successful approximation for the forward peak scattering of aerosols together with a simplified characterization of particle size distributions. An engineering model of a multibarreled photopolarimeter suitable for operation from a satellite was evaluated in laboratory and high altitude jet aircraft tests. Comparison of the data from flights over the Mexican desert with theoretical curves for a Rayleigh atmosphere with negligible turbidity is in agreement.

Sekera, Z.↗
DOE OSTI2024

Surface-mediated spontaneous emulsification of the acylated peptide, semaglutide

Acylated peptides composed of glucagon-like peptide-1 receptor agonists modified with a fatty acid side chain are an important class of therapeutics for type 2 diabetes and obesity but are susceptible to an unusual physical instability in the presence of hydrophobic surfaces, i.e., spontaneous emulsification, also known as ouzo formation in practice. In this work, light scattering, small-angle X-ray scattering, and circular dichroism measurements are used to characterize the physical properties of the semaglutide colloidal phase, including size distribution, shape, secondary structure, internal structure, and internal composition, as a function of solution physico-chemical conditions. The existence and size of the colloids formed are successfully predicted by a classical Rayleigh model, which identifies the parameters controlling their size and formation. Colloid formation is found to be catalyzed by hydrophobic surfaces, and formation rates are modeled as an autocatalytic reaction, enabling the formation of a master curve for various surfaces that elucidates the mechanism. Surfaces differ due to differences in surface wettability, which can be correlated with Hansen solubility parameters. This work provides insights into this unusual colloidal phenomenon and guides the peptide synthesis process and drug product formulation in the pharmaceutical industry.

59 BASIC BIOLOGICAL SCIENCES↗
NASA NTRS1986

Detection of scattering in the 2175 A interstellar band

Spectrophotometric observations of two reflection nebulae and their illuminating stars obtained with the International Ultraviolet Explorer Satellite have provided the first evidence for the presence of a scattering contribution to the 2175 A interstellar extinction band. Lower than normal far-UV extinction for the stars embedded in the nebulae indicates that the nebulae have a dust particle size distribution that is dominated by larger particles. The strength of the 2175 A band is larger than normal in both cases. The scattering is found to dominate the long-wavelength wing of the band, without shifting the central wavelength of the band by more than 20 A toward longer wavelengths. These observations are taken to indicate that the solid particles responsible for the 2175 A band can be considerably larger than the Rayleigh limit in some interstellar locations. The absence of a notable shift in the central wavelength of the band in such large particles presents a new severe constraint for models of interstellar grains.

Witt, A. N.↗