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At least 685 records · Page 38

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DOE OSTI2022

Field Emission Mitigation in CEBAF SRF Cavities Using Deep Learning

The Continuous Electron Beam Accelerator Facility (CEBAF) operates hundreds of superconducting radio frequency (SRF) cavities in its two main linear accelerators. Field emission can occur when the cavities are set to high operating RF gradients and is an ongoing operational challenge. This is especially true in newer, higher gradient SRF cavities. Field emission results in damage to accelerator hardware, generates high levels of neutron and gamma radiation, and has deleterious effects on CEBAF operations. So, field emission reduction is imperative for the reliable, high gradient operation of CEBAF that is required by experimenters. Here we explore the use of deep learning architectures via multilayer perceptron to simultaneously model radiation measurements at multiple detectors in response to arbitrary gradient distributions. These models are trained on collected data and could be used to minimize the radiation production through gradient redistribution. This work builds on previous efforts in developing machine learning (ML) models, and is able to produce similar model performance as our previous ML model without requiring knowledge of the field emission onset for each cavity.

Ahammed, K.↗

NASA NTRS1980

Large volume multiple path nuclear lasing of /He-3/-Ar

Output power of 550 W has been achieved from a nuclear-pumped multiple path laser system containing (He-3)-Ar by using the (He-3)(n, p)3(H) nuclear reaction for power deposition. Lasing was achieved in Ar at 1790 nm. The complex beam profile was resolved by an InAs array detector. Laser output was directly proportional to thermal neutron flux, and also increased proportionally with increasing (He-3) pressure up to 292.6 kPa. The variation of the laser output power with the number of passes through the excited medium was found to peak at 5-7 passes.

De Young, R. J.↗

NASA NTRS2004

Central Avra Valley Storage and Recovery Project (CAVSARP) Site, Tucson, Arizona: Floodwater and Soil Moisture Investigations with Extraterrestrial Applications

Planetary geologists, geomorphologists, and hydrologists have hypothesized that Mars is a dynamic, water-enriched planet since the Mariner and Viking missions based on geologic, geomorphic, and topographic information. Recent acquisition of Gamma Ray and Neutron Spectrometer information has added further credence to this hypothesis. A unique investigation is underway to work towards being able to successfully map the extent and depth of water on Mars. Researchers from the University of Arizona and members of the Autonomous Sciencecraft Experiment (ASE) have been compiling multiple layers of information in time and space at the Central Avra Valley Storage and Recovery Project (CAVSARP) site, Tucson, Arizona, for eventual comparative analysis. This information has been acquired from a variety of observational/scientific platforms in controlled conditions. CAVSARP facility:

Rucker, D. F.↗

NASA NTRS2002

Pathology effects at radiation doses below those causing increased mortality

Mortality data from experiments conducted at the Argonne National Laboratory (ANL) on the long-term effects of external whole-body irradiation on B6CF(1) mice were used to investigate radiation-induced effects at intermediate doses of (60)Co gamma rays or fission-spectrum neutrons either delivered as a single exposure or protracted over 60 once-weekly exposures. Kaplan-Meier analyses were used to identify the lowest dose in the ANL data (within radiation quality, pattern of exposure, and sex) at which radiation-induced mortality caused by primary tumors could be detected (approximately 1-2 Gy for gamma rays and 10-15 cGy for neutrons). Doses at and below these levels were then examined for radiation-induced shifts in the spectrum of pathology detected at death. To do this, specific pathology events were pooled into larger assemblages based on whether they were cancer, cardiovascular disease or non-neoplastic diseases detected within the lungs and pleura, liver and biliary tract, reproductive organs, or urinary tract. Cancer and cardiovascular disease were further subdivided into categories based on whether they caused death, contributed to death, or were simply observed at death. Counts of how often events falling within each of these combined pathology categories occurred within a mouse were then used as predictor variables in logistic regression to determine whether irradiated mice could be distinguished from control mice. Increased pathology burdens were detected in irradiated mice at doses lower than those causing detectable shifts in mortality-22 cGy for gamma rays and 2 cGy for neutrons. These findings suggest that (1) models based on mortality data alone may underestimate radiation effects, (2) radiation may have adverse health consequences (i.e. elevated health risks) even when mortality risks are not detected, and (3) radiation-induced pathologies other than cancer do occur, and they involve multiple organ systems.

Non-NASA Center↗

NASA NTRS2007

Ground-Based Testing of TiB2 and Al2O3/TiB2 Response to Space Environment

Two materials, titanium diboride and an alumina/titanium diboride composite, exhibit characteristics favorable for use in multiple space applications. These characteristics include low mass (4.52 gm/cc), high strain rate impact resistance, high temperature use (3000oC M.P.), thermal and electrical conductivity, thermal shock resistance, and high visible-range reflectivity. Additionally, the presence of boron in these materials gives them the potential to shield against neutron radiation as well as charged radiation. These materials are flying on MISSE 6 to assess material changes resulting from exposure to the space environment. This study provides a preliminary, ground-based examination of these materials' interactions with individual components of the space environment, in particular atomic oxygen (AO) and neutron radiation, in order to better predict and understand post-flight results. Individual specimens are exposed to ground state AO and surface oxidation is measured. Equivalent exposures of up to 13 months show no rapid oxidation, however evidence indicates some surface oxidation occurring. Other samples are placed near a polyethylene moderated, one Ci Am/Be neutron source to determine their shielding capability. Comparisons between exposed and shielded indium foil, which is activated by transmitted neutrons, measure each material's ability to shield neutrons. Preliminary results indicate a significant shielding benefit provided by both materials.

Jefferies, Sharon A.↗

NASA NTRS2016

Electromagnetic Dissociation Cross Sections for High LET Fragments

Nuclear interaction cross sections are used in space radiation transport codes to calculate the probability of fragment emission in high energy nucleus-nucleus collisions. Strong interactions usually dominate in these collisions, but electromagnetic (EM) interactions can also sometimes be important. Strong interactions typically occur when the projectile nucleus hits a target nucleus, with a small impact parameter. For impact parameters larger than the sum of the nuclear radii, EM reactions dominate and the process is called electromagnetic dissociation (EMD) if one of the nuclei undergo fragmentation. Previous models of EMD have been used to calculate single proton (p) production, single neutron (n) production or light ion production, where a light ion is defined as an isotope of hydrogen (H) or helium (He), such as a deuteron (2H), a triton (3H), a helion (3He) or an alpha particle (4He). A new model is described which can also account for multiple nucleon production, such as 2p, 2n, 1p1n, 2p1n, 2p2n, etc. in addition to light ion production. Such processes are important to include for the following reasons. Consider, for example, the EMD reaction 56Fe + Al --> 52Cr + X + Al, for a 56Fe projectile impacting Al, which produces the high linear energy transfer (LET) fragment 52Cr. In this reaction, the most probable particles representing X are either 2p2n or 4He. Therefore, production of the high LET fragment 52Cr, must include the multiple nucleon production of 2p2n in addition to the light ion production of 4He. Previous models, such as the NUCFRG3 model, could only account for the 4He production process in this reaction and could not account for 2p2n. The new EMD model presented in this work accounts for both the light ion and multiple nucleon processes, and is therefore able to correctly account for the production of high LET products such as 52Cr. The model will be described and calculations will be presented that show the importance of light ion and multiple nucleon production. The work will also show that EMD reactions contribute most to those fragments with the highest LET.

Norbury, John↗

DOE OSTI2026

A Bayesian desmearing algorithm for Bonse–Hart USANS with anisotropic scattering

Ultra-small-angle neutron scattering (USANS) using Bonse–Hart optics provides micrometer-scale structural insights but suffers from severe slit-geometry smearing. While well-established for isotropic systems, quantitative desmearing of anisotropic data remains a challenge because conventional corrections break down for non-radial scattering. In this work, we address this by developing a resolution-aware Bayesian framework that explicitly incorporates anisotropy via an affine deformation to the scattering pattern, guided by the principle of parsimony. This results in orientation-resolved point-spread functions that enable a self-consistent determination of both the resolution and deformation parameters. Using Gaussian process regression with uncertainty quantification and a probabilistic correction for multiple scattering, we demonstrate the framework’s effectiveness through numerical benchmarks and experimental studies of a stretched polymer melt. Our approach enables the seamless integration of SANS and USANS data, facilitating quantitative structural analysis of deformed materials at nanometer to micrometer scales.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Structural Insights into Low and High Recalcitrance Natural Poplar Variants Using Neutron and X-ray Scattering

Here, we used small-angle neutron scattering (SANS) and wide-angle X-ray scattering (WAXS) to study two Populus trichocarpa variants, GW-11012 and BESC-316, with lignin contents of 17.8 and 23.2%, respectively, to understand why the low lignin variant has increased sugar release during liquid hot water (LHW) pretreatment. SANS showed differences in cell wall polymer arrangement in the variants. In GW-11012, the cellulose microfibrils were similar in size to BESC-316 but were not equally spaced and lignin was aggregated rather than homogenously interspersed with other matrix co-polymers. However, after LHW pretreatments, the SANS profiles of the pretreated variants were almost indistinguishable, indicating that the nanoscale structural features could not adequately explain the increased sugar release observed in GW-11012. WAXS analysis revealed higher cellulose crystallinity and larger crystallite size in native and pretreated GW-11012. However, the most significant difference was that the crystallite orientation was approximately 2-fold higher in GW-11012. This suggests that higher crystallite orientation may be favorable for the action of processive cellulases leading to increased sugar release from GW-11012. Our study shows that there is a complex interplay between cell wall polymers during their deposition resulting in changes in lignin distribution and cellulose structure, highlighting the importance of investigating plant cell wall architecture across multiple length scales.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2025

First observation of antiproton annihilation at rest on argon in the LArIAT experiment

We report the first observation and measurement of antiproton annihilation at rest on argon track and shower multiplicities and particle identification conducted with the LArIAT experiment. Stopping antiprotons from the Fermilab Test Beam Facility’s charged particle test beam are identified using beamline instrumentation and LArIAT’s liquid argon time projection chamber (LArTPC). The charged particle multiplicity from the annihilation vertex is manually evaluated via hand scanning, yielding a mean of 3.2 ± 0.4 tracks and a standard deviation of 1.3 tracks, consistent with a semiautomated reconstruction resulting in 2.8 ± 0.4 tracks and a standard deviation of 1.2 tracks. Both methods are consistent with Monte Carlo simulations within statistical uncertainty. The shower multiplicities and particle identification for outgoing tracks are also consistent with eant4 model predictions. These results, obtained from a low-statistics sample, provide a foundation for higher-statistics studies in larger LArTPCs, which could refine modeling of intranuclear annihilation on argon and inform scenarios such as neutron-antineutron oscillations. Published by the American Physical Society 2025

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Comparison of mechanical properties measured on multiple scales

FeCrAl alloys are being developed for accident tolerant fuels for current light water reactors. Specifically as fuel claddings with enhanced safety. These alloys are being developed to have excellent corrosion resistance in light water reactor coolant environments and structural integrity for longer durations in the case of a loss of coolant scenario where time is critical for safety. Tensile, shear punch, and Vickers hardness testing was performed on neutron irradiated FeCrAl alloys with three variations in composition. Testing was done at room temperature for comparison of the three techniques. FeCrAl alloys in this report were irradiated at Oak Ridge National Laboratory (ORNL) in the High Flux Isotope Reactor (HFIR) to 7 dpa and at 320 °C.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

NASA NTRS1980

The Eddington limit and supercritical accretion. I - Time-independent calculations

Spherically symmetric, steady state accretion of an ionized hydrogen plasma onto a neutron star is considered for accretion rates which exceed a critical rate at which the Eddington limiting luminosity is produced. The coupled hydrodynamic and frequency integrated, radiative transfer equations are solved for accretion rates up to 10 times the nominal limit. Steady state solutions are presented that imply a multiplicity of different luminosity solutions for a single accretion rate in this 'supercritical' regime.

Burger, H. L.↗

DOE OSTI2023

Spin wave Hamiltonian and anomalous scattering in NiPS 3

Here, we report a comprehensive spin wave analysis of the semiconducting honeycomb van der Waal antiferromagnet NiPS 3 . Using single-crystal inelastic neutron scattering, we map out the full Brillouin zone and fit the observed modes to a spin wave model with rigorously defined uncertainty. We find that the third-nearest-neighbor exchange J 3 dominates the Hamiltonian, a feature which we fully account for by ab initio density functional theory calculations. We also quantify the degree to which the threefold rotation symmetry is broken and account for the Q = 0 excitations observed in other measurements, yielding a spin exchange model which is consistent across multiple experimental probes. We also identify a strongly reduced static ordered moment and reduced low-energy intensity relative to the linear spin wave calculations, signaling unexplained features in the magnetism which requires going beyond the linear spin wave approximation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

A database of synthetic inelastic neutron scattering spectra from molecules and crystals

Abstract Inelastic neutron scattering (INS) is a powerful tool to study the vibrational dynamics in a material. The analysis and interpretation of the INS spectra, however, are often nontrivial. Unlike diffraction, for which one can quickly calculate the scattering pattern from the structure, the calculation of INS spectra from the structure involves multiple steps requiring significant experience and computational resources. To overcome this barrier, a database of INS spectra consisting of commonly seen materials will be a valuable reference, and it will also lay the foundation of advanced data-driven analysis and interpretation of INS spectra. Here we report such a database compiled for over 20,000 organic molecules and over 10,000 inorganic crystals. The INS spectra are obtained from a streamlined workflow, and the synthetic INS spectra are also verified by available experimental data. The database is expected to greatly facilitate INS data analysis, and it can also enable the utilization of advanced analytics such as data mining and machine learning. Notice: This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan ( http://energy.gov/downloads/doe-public-access-plan ).

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Optimal Control for the Quantum Simulation of Nuclear Dynamics

We propose a method for enacting the unitary time propagation of two interacting neutrons at leading order of chiral effective-field theory by efficiently encoding the nuclear dynamics into a single multilevel quantum device. The emulated output of the quantum simulation shows that, by applying a single gate that draws on the underlying characteristics of the device, it is possible to observe multiple cycles of the nuclear dynamics before the onset of decoherence. Owing to the signal's longevity, we can then extract spectroscopic properties of the simulated nuclear system. This allows us to validate the encoding of the nuclear Hamiltonian and the robustness of the simulation in the presence of quantum-hardware noise by comparing the extracted spectroscopic information to exact calculations. This work paves the way for transformative calculations of the dynamical properties of nuclei on near-term quantum devices.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2022

Revised 207 Pb Thermal Capture Gamma-ray Spectrum Evaluation

This report details the revision of the JENDL-4.0 thermal capture gamma-ray spectrum evaluation for 207 Pb and the comparison of the current evaluations and the revised spectrum. The history of the available reaction evaluations is described and the deficiencies are identified. The modified spectrum has an average energy of 7.329 MeV and an average multiplicity of 1.005, leading to a total energy released value of 7.366 MeV, just 0.03% off from the Q-value of the reaction, 7.368 MeV. Based on comparison to the measurements and structure libraries considered, the revised evaluation is closer to reality and should provide more accurate coupled neutron-gamma ray calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1996

Light ion components of the galactic cosmic rays: Nuclear interactions and transport theory

Light nuclei are present in the primary galactic cosmic rays (GCR) and are produced in thick targets due to projectile or target fragmentation from both nucleon and heavy induced reactions. In the primary GCR, He-4 is the most abundant nucleus after H-1. However, there are also a substantial fluxes of H-2 and He-3. In this paper we describe theoretical models based on quantum multiple scattering theory for the description of light ion nuclear interactions. The energy dependence of the light ion fragmentation cross section is considered with comparisons of inclusive yields and secondary momentum distributions to experiments described. We also analyze the importance of a fast component of lights ions from proton and neutron induced target fragementation. These theoretical models have been incorporated into the cosmic ray transport code HZETRN and will be used to analyze the role of shielding materials in modulating the production and the energy spectrum of light ions.

Cucinotta, F. A.↗

NASA NTRSDate not supplied

Toughening of Boron Carbide Composites by Hierarchical Microstructuring

Due to a unique combination of properties including high hardness, low density, chemical and thermal stability, semi-conductivity, and high neutron absorption, boron carbide (B4C) is a potential candidate for various applications involving extreme environment. However, B4C’s current application is limited because of its low fracture toughness. In this study, a hierarchical microstructure design with features including TiB2 grains and graphite platelets was used to toughen B4C by simultaneously utilizing multiple toughening mechanisms including crack deflection, bridging, and micro-crack toughening. Using field-assisted sintering technology (FAST), B4C composites with dense and hierarchical microstructure were fabricated. Previously, the fracture toughness of fabricated B4C composites was measured at micro-scale using micro-indentation to have up to 56% improvement. In this work, the B4C composites’ fracture toughness was characterized at macro-scale using four-point bending methods and compared with previous results obtained at micro-scale. Micromechanics modeling of fracture behaviors for B4C-TiB2 composites was also performed to evaluate the contributions from experimentally observed toughening mechanisms. From four-point bending tests, B4C composites reinforced with both TiB2 grains (~15 vol%) and graphite platelets (~8.7 vol%) exhibited the highest fracture toughness enhancement from 2.38 to 3.65 MPa∙m^(1/2). The measured values were lower than those obtained using micro-indentation but maintained the general trends. The discrepancy between the indentation and four-point bending test results originated from the complex deformation behaviors triggered by the high contact load during indentation tests. Through micromechanics modeling, introduced thermal residual stress due to thermal expansion mismatch between B4C and TiB2, and weak interphases at B4C-TiB2 boundaries were identified as the main causes for experimentally observed toughness enhancement. These results proved the effectiveness of hierarchical microstructure designs for B4C toughening and can provide reference for the future design of B4C composites with optimized microstructures for further fracture toughness enhancement.

composites↗

DOE OSTI2022

Development of the MCNP-ORIGEN activation automation tool

This paper introduces the MCNP-ORIGEN activation automation tool for streamlining the calculation of experiment source terms. This tool couples the Monte-Carlo radiation-transport solver, MCNP to the depletion tool, ORIGEN-S. To showcase its current capabilities, this paper presents an activation analysis exercise, which is conducted with Serpent, and the results are com- pared. The experiment consists in a 90%-enriched uranium sphere surrounded by light water. A non-fissile cylinder is placed in the water, representing an irradiation experiment. We conducted simulations for 2 different cylinder materials: iron and cobalt at two different temperatures: 300 K and 900 K. The exercise consists of an irradiation of 50 days at a constant power of 5 MW, followed by a decay of 50 days. These studies highlight the discrepancies between how the different tools handle nuclear data. Finally, the results underscore multiple areas of possible improvement.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗