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At least 685 records · Page 38

Anisotropic magnetic and transport properties of orthorhombic o-Pr 2 Co 3 Ge 5

Abstract The crystal structure, electron energy-loss spectroscopy (EELS), heat capacity, and anisotropic magnetic and resistivity measurements are reported for Sn flux grown single crystals of orthorhombic Pr 2 Co 3 Ge 5 (U 2 Co 3 Si 5 -type, Ibam ). Our findings show that o -Pr 2 Co 3 Ge 5 hosts nearly trivalent Pr ions, as evidenced by EELS and fits to temperature dependent magnetic susceptibility measurements. Complex magnetic ordering with a partially spin-polarized state emerges near T sp = 32 K, with a spin reconfiguration transition near T M = 15 K. Heat capacity measurements show that the phase transitions appear as broad peaks in the vicinity of T sp and T M . The magnetic entropy further reveals that crystal electric field splitting lifts the Hund’s rule degeneracy at low temperatures. Taken together, these measurements show that Pr 2 Co 3 Ge 5 is an environment for complex f state magnetism with potential strongly correlated electron states.

36 MATERIALS SCIENCE↗

Formation of short-range magnetic order and avoided ferromagnetic quantum criticality in pressurized LaCrGe 3

LaCrGe 3 has attracted attention as a paradigm example of the avoidance of ferromagnetic (FM) quantum criticality in an itinerant magnet. In this work, we combined thermodynamic (specific heat and thermal expansion), transport, x-ray, and neutron scattering as well as μSR measurements to obtain insights on the temperature-pressure phase diagram of LaCrGe 3 . Consistent with previous studies of the phase diagram by transport measurements, our thermodynamic data shows clearly that the FM transition at T FM changes its character from second order to first order when it is suppressed to low temperatures by pressure. In addition, previous studies demonstrated that for high pressures a new phase occurs below T 2 , which was proposed to be a long-wavelength antiferromagnetic state (AFM q ). In this paper, we provide evidence from our thermodynamic data that this phase transition is preceded by yet another phase transition at T 1 >T 2 . Our μSR data indicate that full magnetic volume fraction is only established below T 2 , but that this magnetism is characterized by a short correlation length. Within the experimental resolution, our neutron-scattering data is not able to identify any magnetic Bragg peaks. Overall, the microscopic magnetic data is therefore consistent with the formation of FM clusters in the proximity of the avoided FM quantum critical point in LaCrGe 3 . This conclusion is at odds with the previous proposal of AFM q order and raises questions on the role of disorder in this stochiometric compound.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Evidence for electronic signature of a magnetic transition in the topological magnet HoSbTe

Topological insulators with intrinsic magnetic order are emerging as an exciting platform to realize fundamentally new excitations from topological quantum states of matter. To study these systems and their physics, people have proposed a variety of magnetic topological insulator systems, including HoSbTe, an antiferromagnetic weak topological insulator candidate. Here, in this work, we use scanning tunneling microscopy to probe the electronic structure of HoSbTe with antiferromagnetic and ferromagnetic orders that are tuned by applying an external magnetic field. Although around the Fermi energy we find minor differences between the quasiparticle interferences under the ferromagnetic and antiferromagnetic orders, deep inside the valance region, a quasiparticle interference signal emerges with ferromagnetism. This observation is consistent with our first-principles calculations indicating the magnetism-driven transition of the electronic states in this spin-orbit coupled topological magnet.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic properties of Sr 3 NiIrO 6 and Sr 3 CoIrO 6 : Magnetic hysteresis with coercive fields of up to 55 T

Here, we report extraordinarily large magnetic hysteresis loops in the iridates Sr 3 NiIrO 5 and Sr 3 CoIrO 6 . We find coercive magnetic fields of up to 55 T with switched magnetic moments ≈1μ B per formula unit in Sr 3 NiIrO 6 and coercive fields of up to 52 T with switched moments ≈3μ B per formula unit in Sr 3 CoIrO 6 . We propose that the magnetic hysteresis involves the field-induced evolution of quasi-one-dimensional chains in a frustrated triangular configuration. In conclusion, the striking magnetic behavior is likely to be linked to the unusual spin-orbit-entangled local state of the Ir 4+ ion and its potential for anisotropic exchange interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Coupling of structure to magnetic and superconducting orders in quasi-one-dimensional K 2 Cr 3 As 3

Here, quasi-one-dimensional A 2 Cr 3 As 3 (with A = K, Cs, Rb) is an intriguing new family of superconductors which exhibit many similar features to the cuprate and iron-based unconventional superconductor families. Yet, in contrast to these systems, no charge or magnetic ordering has been observed which could provide the electronic correlations presumed necessary for an unconventional superconducting pairing mechanism—an absence which defies predictions of first-principles models. We report the results of neutron scattering experiments on polycrystalline K 2 Cr 3 As 3 (T c ~ 7) which probed the low-temperature dynamics near T c . Neutron diffraction data evidence a subtle response of the nuclear lattice to the onset of superconductivity while inelastic scattering reveals a highly dispersive column of intensity at the commensurate wave vector q = (001/2) which loses intensity beneath T c -indicative of short-range magnetic fluctuations. Using linear spin-wave theory, we model the observed scattering and suggest a possible structure to the short-range magnetic order. These observations suggest that K 2 Cr 3 As 3 is in close proximity to a magnetic instability and that the incipient magnetic order both couples strongly to the lattice and competes with superconductivity, in direct analogy with the iron-based superconductors.

1-dimensional systems↗

Quench Protection Performance Measurements in the First MQXF Magnet Models

The European Organization for Nuclear Research (CERN) and U.S. LHC Accelerator Research Program (LARP) are jointly developing Nb3Sn quadrupole magnets to be installed in the LHC for its upgrade to higher luminosity. These magnets' quench protection system will include a combination of quench heaters attached to the coil surfaces and coupling-loss-induced quench (CLIQ) units electrically connected to the magnets. Different protection elements have been characterized separately and simultaneously by implementing them on two 1.2-m-long model quadrupole magnets, tested at Fermi National Acceleration Laboratory and CERN, and one 4-m-long mirror magnet tested at Brookhaven Nation Laboratory. After analyzing the test data, their performances have been positively evaluated. Furthermore, the electrothermal transients occurring after a quench have been simulated with the LEDET software and the results are compared to experimental results. The preferred quench protection system configuration relies both on heaters and CLIQ. This solution is based on electrically robust components, achieves an effective reduction of the coils hot spot temperature after a quench, and offers increased redundancy against component failures.

43 PARTICLE ACCELERATORS↗

Quench Protection of the First 4-m-Long Prototype of the HL-LHC Nb$_3$Sn Quadrupole Magnet

The quadrupole magnets for the LHC upgrade to higher luminosity are jointly developed by CERN and US-LARP (LHC Accelerator Research Program). These Nb3Sn magnets will be protected against overheating after a quench by a combination of heaters bonded to the coil outer surface and CLIQ (Coupling-Loss Induced Quench) units. The first 4 meter long prototype magnet, called MQXFAP1, was tested at the Brookhaven National Laboratory in stand-alone configuration. The magnet training campaign, consisting of 18 quenches, was interrupted due to the development of a short circuit between one heater strip and the coil. During the campaign, different quench protection schemes were implemented, including heaters attached to outer and inner layers, one CLIQ unit, and the energy-extraction system. The configuration including outer-layer heaters and CLIQ achieved the fastest current discharge, hence the lowest hot-spot temperature. The electro-magnetic and thermal transients after a quench were simulated with the program STEAM-LEDET and found in good agreement.

43 PARTICLE ACCELERATORS↗

Magnetic State of Quasiordered Fe–Al Alloys Doped with Ga and B: Magnetic Phase Separation and Spin Order

Results of structural, magnetic, and Mössbauer studies of quasi ordered alloys Fe{sub 65}Al{sub 35−} {sub x}M{sub x} (M{sub x} = Ga, B; x = 0, 5 at %) are presented. The magnetic state of examined structurally–single-phase alloys at low temperatures is interpreted from the viewpoint of magnetic phase separation. An explanation is proposed for the observed behavior of magnetic characteristics of Fe{sub 65}Al{sub 35} and Fe{sub 65}Al{sub 30}Ga{sub 5} in the framework of the model of two magnetic phases, a ferromagnetic-type one and a spin density wave. The boron-doped alloy Fe{sub 65}Al{sub 30}B{sub 5} is shown to demonstrate behavior that is typical of materials with the ferromagnetic type of ordering.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Effect of Longitudinal Magnetic Field on the Spread of Erosion Laser Plasma in Vacuum and Generation of Plasma Magnetic Fields

Dynamics of erosion laser plasma in vacuum and generation of magnetic field by moving plasma (in particular, in the presence of external static magnetic field oriented along the direction of plasma motion) are experimentally studied. Radial confinement of the spread of plasma, a decrease in the electrification of target upon plasma formation, and an increase in the induction of the plasma magnetic field by a factor of 10–15 are revealed at an induction of the external magnetic field of about 0.35 T. Dependences of the induction of the plasma magnetic field on the power density of the laser radiation are determined for the above regimes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

High magnetic field magnetization of a new triangular lattice antiferromagnet

In CsV(MoO 4 ) 2 , the magnetic V 3+ ions with octahedral oxygen-coordination form a geometrically frustrated triangular lattice. So fare, there is no magnetic properties reported on it. Recently, we successfully grew single crystals of CsV(MoO 4 ) 2 by using flux method. The susceptibility shows a sharp drop around 24 K, representing a long range magnetic ordering. To understand the physical properties of this new triangular lattice antiferromagnet (TLAF), we pursued high field magnetization measurements to answer two questions: (i) what is the saturation field, which will be very useful to calculate the exchange interaction of the system? (ii) Will it exhibit spin state transition, such as the up up down phase with 1/3-saturation moment as other TLAFs? Recently, we performed VSM measurements in Cell 8, Tallahassee, NHMFL, the results show that the magnetization reaches 0.38 MuB at 34 T, which is just 19% of the full moment of 2 MuB for V 3+ (3d 2 ) ions. Apparently we need higher field to reach 1/3 value or full moment.

36 MATERIALS SCIENCE↗

Energetic Electron Transport in Magnetized Plasma with Magnetic Islands (Final Technical Report)

The main scientific goal of this project was to investigate the interactions between energetic electrons and magnetic islands in magnetized plasmas from lab to space. The proposed plan of addressed the following specific objectives: (1) Determine if energetic electrons are trapped by magnetic islands. Specifically, test the hypothesis that energetic electrons are trapped near island O-points due to stable orbits and de-confined near island X-points due to X-point tangles. (2) Determine how electron transport changes with island width and location. Specifically, test the hypothesis that electrons are accelerated by contracting magnetic islands through a Fermi acceleration process. (3) Assess how electron transport is affected by island dynamics, including island rotation, bifurcation, and/or island overlap. Specifically, test the hypothesis that electrons are deconfined and possibly accelerated during island rotations, bifurcations, and overlap due to stochastization of the magnetic field lines.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Modulation of Magnetic Heating via Dipolar Magnetic Interactions in Monodisperse and Crystalline Iron Oxide Nanoparticles

Here, we report on the study of heat dissipation power in monodisperse and crystalline magnetite nanoparticles as function of particle and aggregate sizes, magnetic field frequencies (up to 435 kHz) and amplitudes (up to 50 mT), media viscosity and particle concentration. These nanoparticles display specific absorption rate values of few hundreds of Wg Fe -1 at moderate frequencies (~100 kHz), increasing up to 3632 Wg Fe -1 at more extreme field conditions (430 kHz and 40 mT) for the largest size. We have found that Néelian relaxation processes are dominant for all nanoparticle sizes, whereas Brownian contribution dominates only for the largest size (22 nm) at high particle concentrations when dipolar interactions enhance the effective magnetic anisotropy. Besides, the particle concentration dependence of the specific absorption rate reflects the importance of magnetic dipolar interactions which strongly depend on aggregate and particle size. Our results show that dipolar interactions tune the effective magnetic anisotropy determining the Néelian and Brownian contributions into SAR values. The possibility of switching between heating mechanisms via dipolar interactions is of great importance towards controlling the heat exposure supplied by IONP as intracellular heating mediators.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Radiofrequency hydrogen ion source with permanent magnets providing axial magnetic field

Uniform axial magnetic field of about 70 G is applied to a radiofrequency (rf) hydrogen ion source by arrays of permanent magnets. The plasma density and electron temperature downstream of the source and near the magnetic filter are compared with those in the previously described ion source, where the axial field has been applied by two solenoids. The source is operated at ∼350 kHz and above 10 kW rf power with a field-effect-transistor-based invertor power supply in 1.5 Pa hydrogen. The results show that the plasma density of ∼10{sup 19} m{sup −3} near the source exit and ∼10{sup 18} m{sup −3} near the magnetic filter can be obtained, which are higher than those with the solenoids.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Probes for investigating the effect of magnetic field, field orientation, temperature and strain on the critical current density of anisotropic high-temperature superconducting tapes in a split-pair 15 T horizontal magnet

We present the designs of probes for making critical current density (J{sub c}) measurements on anisotropic high-temperature superconducting tapes as a function of field, field orientation, temperature and strain in our 40 mm bore, split-pair 15 T horizontal magnet. Emphasis is placed on the design of three components: the vapour-cooled current leads, the variable temperature enclosure, and the springboard-shaped bending beam sample holder. The vapour-cooled brass critical-current leads used superconducting tapes and in operation ran hot with a duty cycle (D) of ∼0.2. This work provides formulae for optimising cryogenic consumption and calculating cryogenic boil-off, associated with current leads used to make J{sub c} measurements, made by uniformly ramping the current up to a maximum current (I{sub max}) and then reducing the current very quickly to zero. They include consideration of the effects of duty cycle, static helium boil-off from the magnet and Dewar (b{sup ′}), and the maximum safe temperature for the critical-current leads (T{sub max}). Our optimized critical-current leads have a boil-off that is about 30% less than leads optimized for magnet operation at the same maximum current. Numerical calculations show that the optimum cross-sectional area (A) for each current lead can be parameterized by LI{sub max}/A=[1.46D{sup −0.18}L{sup 0.4}(T{sub max}−300){sup 0.25D{sup −{sup 0{sup .{sup 0{sup 9}}}}}}+750(b{sup ′}/I{sub max})D{sup 10{sup −{sup 3I{sub m}{sub a}{sub x}−2.87b{sup ′}}}}]× 10{sup 6}A m{sup −1} where L is the current lead's length and the current lead is operated in liquid helium. An optimum A of 132 mm{sup 2} is obtained when I{sub max} = 1000 A, T{sub max} = 400 K, D = 0.2, b{sup ′} = 0.3 l h{sup −1} and L = 1.0 m. The optimized helium consumption was found to be 0.7 l h{sup −1}. When the static boil-off is small, optimized leads have a boil-off that can be roughly parameterized by: b/I{sub max } ≈ (1.35 × 10{sup −3})D{sup 0.41} l h{sup ‑1} A{sup −1}. A split-current-lead design is employed to minimize the rotation of the probes during the high current measurements in our high-field horizontal magnet. The variable-temperature system is based on the use of an inverted insulating cup that operates above 4.2 K in liquid helium and above 77.4 K in liquid nitrogen, with a stability of ±80 mK to ±150 mK. Uniaxial strains of −1.4% to 1.0% can be applied to the sample, with a total uncertainty of better than ±0.02%, using a modified bending beam apparatus which includes a copper beryllium springboard-shaped sample holder.

43 PARTICLE ACCELERATORS↗

Improvement of charged particles transport across a transverse magnetic filter field by electrostatic trapping of magnetized electrons

A study on the transport of charged particles across a magnetic filter field has been carried out in a double plasma device (DPD) and presented in this manuscript. The DPD is virtually divided into two parts viz. source and target regions by a transverse magnetic field (TMF) which is constructed by inserting strontium ferrite magnets into two stainless steel rectangular tubes. Plasma electrons are magnetized but ions are unmagnetized inside the TMF region. Negative voltages are applied to the TMF tubes in order to reduce the loss of electrons towards them. Plasma is produced in the source region by filament discharge method and allowed to flow towards the target region through this negatively biased TMF. It is observed that in the target region, plasma density can be increased and electron temperature decreased with the help of negatively biased TMF. This observation is beneficial for negative ion source development. Plasma diffusion across the negatively biased TMF follows Bohm or anomalous diffusion process when negative bias voltage is very less. At higher negative bias, diffusion coefficient starts deviating from the Bohm diffusion value, associated with enhanced plasma flow in the target region.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Direct observation of ferromagnetism in grain boundary phase of Nd-Fe-B sintered magnet using soft x-ray magnetic circular dichroism

We have investigated the magnetism of the grain boundary (GB) phase in a Nd{sub 14.0}Fe{sub 79.7}Cu{sub 0.1}B{sub 6.2} sintered magnet using soft x-ray magnetic circular dichroism (XMCD) at the Fe L{sub 2,3}-edges. Soft XMCD spectra were measured from the fractured surface that was confirmed to be covered with a thin GB phase by Auger electron spectroscopy. The magnetic moment of Fe in the GB phase was estimated to be m{sub GB}=1.4 μ{sub B} at 30 °C using the sum rule analysis for XMCD spectra, which is 60% of that of Fe in the Nd{sub 2}Fe{sub 14}B compound. The temperature dependence of m{sub GB} evaluated with reference to Fe in the Nd{sub 2}Fe{sub 14}B phase indicated that the Curie temperature of the GB phase is more than 50 °C lower compared to that of Nd{sub 2}Fe{sub 14}B.

36 MATERIALS SCIENCE↗

The structural and magnetic properties of Pr{sub 1−x}Er{sub x}Al{sub 2}

We report on the effect of Er addition to PrAl{sub 2} on the lattice parameters, magnetic behavior, heat capacity, and magnetocaloric effect by using x-ray diffraction, magnetization, and heat capacity measurements. Unlike Pr{sub 0.6}Er{sub 0.4}Al{sub 2}, other alloys we studied in the pseudobinary (Pr{sub 1−x}Er{sub x})Al{sub 2} system do not exhibit a sharp peak in heat capacity with the application of magnetic field. Both the cubic lattice parameter and the Curie temperature decrease with increasing Er concentration. The nuclear specific heat coefficient decreases from 660 mJ K mol{sup −1} for x = 0.05 to a nearly negligible value for x = 0.95. The magnetic entropy and adiabatic temperature change varies from 2 to 4 J mol{sup −1} K{sup −1} and 2.5 to 5 K at ΔH = 20 kOe for x = 0.05 to 0.95, respectively. These values of the magnetocaloric effect are comparable to those of the other rare-earth dialuminides systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗