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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 685 records · Page 38
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Infrared compatible rapid mixer to probe millisecond chemical kinetics

Fast microfluidic mixers are a valuable tool for studying solution-phase chemical reaction kinetics and molecular processes with spectroscopy. However, microfluidic mixers that are compatible with infrared vibrational spectroscopy have seen only limited development due to the poor infrared transparency of the current microfabrication material. We describe the design, fabrication, and characterization of CaF2-based continuous flow turbulent mixers, which are capable of measuring kinetics in the millisecond time window with infrared spectroscopy, when integrated into an infrared microscope. Kinetics measurements demonstrate the ability to resolve relaxation processes with 1 millisecond time resolution, and straightforward improvements are described that should result in sub-100 µs time-resolution.

Instruments & Instrumentation↗
DOE OSTI2015

Examining the infrared variable star population discovered in the Small Magellanic Cloud using the SAGE-SMC survey

We present our study on the infrared variability of point sources in the Small Magellanic Cloud (SMC). We use the data from the Spitzer Space Telescope Legacy Program “Surveying the Agents of Galaxy Evolution in the Tidally Stripped, Low Metallicity Small Magellanic Cloud” (SAGE-SMC) and the “Spitzer Survey of the Small Magellanic Cloud” (S{sup 3}MC) survey, over three different epochs, separated by several months to 3 years. Variability in the thermal infrared is identified using a combination of Spitzer’s InfraRed Array Camera 3.6, 4.5, 5.8, and 8.0 μm bands, and the Multiband Imaging Photometer for Spitzer 24 μm band. An error-weighted flux difference between each pair of three epochs (“variability index”) is used to assess the variability of each source. A visual source inspection is used to validate the photometry and image quality. Out of ∼2 million sources in the SAGE-SMC catalog, 814 meet our variability criteria. We matched the list of variable star candidates to the catalogs of SMC sources classified with other methods, available in the literature. Carbon-rich Asymptotic Giant Branch (AGB) stars make up the majority (61%) of our variable sources, with about a third of all of our sources being classified as extreme AGB stars. We find a small, but significant population of oxygen-rich (O-rich) AGB (8.6%), Red Supergiant (2.8%), and Red Giant Branch (<1%) stars. Other matches to the literature include Cepheid variable stars (8.6%), early type stars (2.8%), Young-stellar objects (5.8%), and background galaxies (1.2%). We found a candidate OH maser star, SSTISAGE1C J005212.88-730852.8, which is a variable O-rich AGB star, and would be the first OH/IR star in the SMC, if confirmed. We measured the infrared variability of a rare RV Tau variable (a post-AGB star) that has recently left the AGB phase. 59 variable stars from our list remain unclassified.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Main-belt asteroids with WISE/NEOWISE: Near-infrared albedos

We present revised near-infrared albedo fits of 2835 main-belt asteroids observed by WISE/NEOWISE over the course of its fully cryogenic survey in 2010. These fits are derived from reflected-light near-infrared images taken simultaneously with thermal emission measurements, allowing for more accurate measurements of the near-infrared albedos than is possible for visible albedo measurements. Because our sample requires reflected light measurements, it undersamples small, low-albedo asteroids, as well as those with blue spectral slopes across the wavelengths investigated. We find that the main belt separates into three distinct groups of 6%, 16%, and 40% reflectance at 3.4 μm. Conversely, the 4.6 μm albedo distribution spans the full range of possible values with no clear grouping. Asteroid families show a narrow distribution of 3.4 μm albedos within each family that map to one of the three observed groupings, with the (221) Eos family being the sole family associated with the 16% reflectance 3.4 μm albedo group. We show that near-infrared albedos derived from simultaneous thermal emission and reflected light measurements are important indicators of asteroid taxonomy and can identify interesting targets for spectroscopic follow-up.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

HIGH-SPEED IMAGING AND WAVEFRONT SENSING WITH AN INFRARED AVALANCHE PHOTODIODE ARRAY

Infrared avalanche photodiode (APD) arrays represent a panacea for many branches of astronomy by enabling extremely low-noise, high-speed, and even photon-counting measurements at near-infrared wavelengths. We recently demonstrated the use of an early engineering-grade infrared APD array that achieves a correlated double sampling read noise of 0.73 e{sup −} in the lab, and a total noise of 2.52 e{sup −} on sky, and supports simultaneous high-speed imaging and tip-tilt wavefront sensing with the Robo-AO visible-light laser adaptive optics (AO) system at the Palomar Observatory 1.5 m telescope. Here we report on the improved image quality simultaneously achieved at visible and infrared wavelengths by using the array as part of an image stabilization control loop with AO-sharpened guide stars. We also discuss a newly enabled survey of nearby late M-dwarf multiplicity, as well as future uses of this technology in other AO and high-contrast imaging applications.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2018

Carnegie Supernova Project-II: Extending the Near-infrared Hubble Diagram for Type Ia Supernovae to z ~0.1

The Carnegie Supernova Project-II (CSP-II) was an NSF-funded, four-year program to obtain optical and near-infrared observations of a "Cosmology" sample of ~100 Type Ia supernovae located in the smooth Hubble flow (0.03 $\lesssim$ z $\lesssim$ 0.10). Light curves were also obtained of a "Physics" sample composed of 90 nearby Type Ia supernovae at z ≤ 0.04 selected for near-infrared spectroscopic timeseries observations. The primary emphasis of the CSP-II is to use the combination of optical and near-infrared photometry to achieve a distance precision of better than 5%. Here in this paper, details of the supernova sample, the observational strategy, and the characteristics of the photometric data are provided. In a companion paper, the near-infrared spectroscopy component of the project is presented.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Ultraviolet to far-infrared dielectric function of n -doped cadmium oxide thin films

Spectroscopic ellipsometry and Fourier transform infrared spectroscopy were applied to extract the ultraviolet to far-infrared (150 – 33333 cm -1 ) complex dielectric functions of high-quality, sputtered indium-doped cadmium oxide (In:CdO) thin crystalline films on MgO substrates possessing carrier densities (N d ) ranging from 1.1 x 10 19 cm -1 to 4.1 x 10 20 cm -1 . A multiple oscillator fit model was used to identify and analyze the three major contributors to the dielectric function and their dependence on doping density: interband transitions in the visible, free-carrier excitations (Drude response) in the near- to far-infrared, and IR-active optic phonons in the far-infrared. More specifically, values pertinent to the complex dielectric function such as the optical band gap (E g ), are shown here to be dependent upon carrier density, increasing from approximately 2.5–3 eV, while the high-frequency permittivity (ε ∞ ) decreases from 5.6 to 5.1 with increasing carrier density. The plasma frequency (ω p ) scales as $\sqrt{N_d}$, resulting in ω p values occurring within the mid- to near-IR, and the effective mass (m *) was also observed to exhibit doping density-dependent changes, reaching a minimum of 0.11 m o in unintentionally doped films (1.1 x 10 19 cm -1 ). Good quantitative agreement with prior work on polycrystalline, higher-doped CdO films is also demonstrated, illustrating the generality of the results. The analysis presented here in this paper will aid in predictive calculations for CdO-based next-generation nanophotonic and optoelectronic devices, while also providing an underlying physical description of the key properties dictating the dielectric response in this atypical semiconductor system.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

From binary to quinary: The rationale and development of GaInAsSbBi for mid- and long-wave infrared sensing applications

Given the added complexity in flux calibration and composition evaluation inherent to quinary alloy growth, what motivates compounding the challenges of III–V-Bi growth with the goal of producing a quinary alloy of GaInAsSbBi for mid- and long-wave infrared sensing applications? Each elemental constituent provides some additional design freedom to achieve the ultimate goal of producing a lattice-matched, bulk random alloy mid-wave infrared III–V material with smooth surface morphology and high optoelectronic quality to enable high performance elevated operating temperatures. Here, this paper reviews the evolution of Bi-containing semiconductor research, focusing on mid- and long-wave infrared materials and highlighting key research findings that motivated the decisions to accept the added complexity in going from binaries like InAs or InSb, to InAsBi, to InAsSbBi, and, finally, to GaInAsSbBi to meet the performance demands of advanced infrared sensing applications.

Webster, Preston T. [Air Force Research Laboratory↗
DOE OSTI2022

Infrared plasmons propagate through a hyperbolic nodal metal

Metals are canonical plasmonic media at infrared and optical wavelengths, allowing one to guide and manipulate light at the nanoscale. A special form of optical waveguiding is afforded by highly anisotropic crystals revealing the opposite signs of the dielectric functions along orthogonal directions. These media are classified as hyperbolic and include crystalline insulators, semiconductors, and artificial metamaterials. Layered anisotropic metals are also anticipated to support hyperbolic waveguiding. However, this behavior remains elusive, primarily because interband losses arrest the propagation of infrared modes. Here, we report on the observation of propagating hyperbolic waves in a prototypical layered nodal-line semimetal ZrSiSe. The observed waveguiding originates from polaritonic hybridization between near-infrared light and nodal-line plasmons. Unique nodal electronic structures simultaneously suppress interband loss and boost the plasmonic response, ultimately enabling the propagation of infrared modes through the bulk of the crystal.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2022

Information Content of a Synergy of Ground-Based and Space-Based Infrared Sounders. Part I: Clear-Sky Environments

Abstract Profiles of atmospheric temperature and water vapor from remotely sensed platforms provide critical observations within the temporal and spatial gaps of the radiosonde network. The 2017 National Academies of Science Decadal Survey highlighted that observations of the planetary boundary layer (PBL) from the current space-based observing system are not of the necessary accuracy or resolution for monitoring and predicting high-impact weather phenomena. One possible solution to improving observations of the PBL is supplementing the existing space-based observing system with a network of ground-based profilers. A synthetic information content study is developed utilizing profiles from the Atmospheric Radiation Measurement (ARM) program sites at the Southern Great Plains (SGP), east North Atlantic (ENA), and North Slope of Alaska (NSA) to assess the benefits, in terms of degrees of freedom (DOF), vertical resolution, and uncertainties, of a synergy between the ground-based Atmospheric Emitted Radiance Interferometer (AERI) with space-based hyperspectral infrared (IR) sounders. A combination of AERI with any of the three polar-orbiting IR sounders: the Atmospheric Infrared Sounder (AIRS), the Cross-track Infrared Sounder (CrIS), or the Infrared Atmospheric Sounding Interferometer (IASI), results in a DOF increase of 30%–40% in the surface-to-700-hPa layer compared to the space-based instrument alone. Introducing AERI measurements to the observing system also results in significant improvements to vertical resolution and uncertainties in the bottom 1000 m of the atmosphere compared to CrIS measurements alone. A synergy of CrIS and AERI exceeds the 1-km-vertical-resolution goal set by the Decadal Survey in the lowest 1000 m.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2015

Detection range enhancement using circularly polarized light in scattering environments for infrared wavelengths

We find for infrared wavelengths there are broad ranges of particle sizes and refractive indices that represent fog and rain where the use of circular polarization can persist to longer ranges than linear polarization. Using polarization tracking Monte Carlo simulations for varying particle size, wavelength, and refractive index, we show that for specific scene parameters circular polarization outperforms linear polarization in maintaining the intended polarization state for large optical depths. This enhancement with circular polarization can be exploited to improve range and target detection in obscurant environments that are important in many critical sensing applications. Specifically, circular polarization persists better than linear for radiation fog in the short-wave infrared, for advection fog in the short-wave infrared and the long-wave infrared, and large particle sizes of Sahara dust around the 4 micron wavelength.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Intense infrared lasers for strong-field science

The advent of chirped-pulse amplification in the 1980s and femtosecond Ti:sapphire lasers in the 1990s enabled transformative advances in intense laser–matter interaction physics. Whereas most of experiments have been conducted in the limited near-infrared range of 0.8–1 μm, theories predict that many physical phenomena such as high harmonic generation in gases favor long laser wavelengths in terms of extending the high-energy cutoff. Significant progress has been made in developing few-cycle, carrier-envelope phase-stabilized, high-peak-power lasers in the 1.6–2 μm range that has laid the foundation for attosecond X ray sources in the water window. Even longer wavelength lasers are becoming available that are suitable to study light filamentation, high harmonic generation, and laser–plasma interaction in the relativistic regime. Long-wavelength lasers are suitable for sub-bandgap strong-field excitation of a wide range of solid materials, including semiconductors. In the strong-field limit, bulk crystals also produce high-order harmonics. In this review, we first introduce several important wavelength scaling laws in strong-field physics, then describe recent breakthroughs in short- (1.4–3 μm), mid- (3–8 μm), and long-wave (8–15 μm) infrared laser technology, and finally provide examples of strong-field applications of these novel lasers. Furthermore, some of the broadband ultrafast infrared lasers will have profound effects on medicine, environmental protection, and national defense, because their wavelengths cover the water absorption band, the molecular fingerprint region, as well as the atmospheric infrared transparent window.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Ultra-broadband mid-infrared generation in dispersion-engineered thin-film lithium niobate

Thin-film lithium niobate (TFLN) is an emerging platform for compact, low-power nonlinear-optical devices, and has been used extensively for near-infrared frequency conversion. Recent work has extended these devices to mid-infrared wavelengths, where broadly tunable sources may be used for chemical sensing. To this end, we demonstrate efficient and broadband difference frequency generation between a fixed 1-µm pump and a tunable telecom source in uniformly-poled TFLN-on-sapphire by harnessing the dispersion-engineering available in tightly-confining waveguides. We show a simultaneous 1–2 order-of-magnitude improvement in conversion efficiency and ∼5-fold enhancement of operating bandwidth for mid-infrared generation when compared to equal-length conventional lithium niobate waveguides. We also examine the effects of mid-infrared loss from surface-adsorbed water on the performance of these devices.

47 OTHER INSTRUMENTATION↗
DOE OSTI2023

Mid-infrared spectroscopy with a broadly tunable thin-film lithium niobate optical parametric oscillator

Mid-infrared spectroscopy, an important technique for sensing molecules, has encountered barriers from sources either limited in tuning range or excessively bulky for widespread use. We present a compact, efficient, and broadly tunable optical parametric oscillator surmounting these challenges. Leveraging dispersion-engineered thin-film lithium niobate-on-sapphire photonics and a singly resonant cavity allows broad, controlled tuning over an octave from 1.5–3.3 µm. The device generates >25mW of mid-infrared light at 3.2 µm with 15% conversion efficiency. The ability to precisely control the device’s mid-infrared emission enables spectroscopy of methane and ammonia, demonstrating our approach’s relevance for sensing. Our work signifies an important advance in nonlinear photonics miniaturization, bringing practical field applications of high-speed, broadband mid-infrared spectroscopy closer to reality.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Solar Infrared Radiation Station (SIRS), Sky Radiation (SKYRAD), Ground Radiation (GNDRAD), and Broadband Radiometer Station (BRS) Instrument Handbook

The solar infrared radiation station (SIRS), ground radiometers on stand for upwelling radiation (GNDRAD), and sky radiometers on stand for downwelling radiation (SKYRAD) provide continuous measurements of broadband shortwave (solar) and longwave (atmospheric or infrared) irradiances for downwelling and upwelling components. The following six irradiance measurements are collected from a network of stations to help determine the total radiative flux exchange at each of the primary U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) field research sites—(Southern Great Plains [SGP], North Slope of Alaska [NSA)]and Eastern North Atlantic [ENA])—as well as the ARM mobile facilities (AMF): Direct normal shortwave (solar beam), Diffuse horizontal shortwave (sky), Global horizontal shortwave (total hemispheric), Upwelling shortwave (reflected), Downwelling longwave (atmospheric infrared), Upwelling longwave (surface infrared).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Infrared Thermometer Instrument Handbook

The infrared thermometer (IRT) is a ground-based radiation pyrometer that provides measurements of the brightness temperature of the scene in its field of view. The ground IRT (sometimes referred to as the upwelling instrument) lens has a wide field of view for measuring the radiating temperature of the ground surface. It measures in a narrow range of the infrared band, details of which can be found in Table 2. It provides data to the user averaged to 1-minute resolution. The infrared thermometer for sea-surface temperature (IRTSST) is a ship-based radiation pyrometer that provides measurements of the temperature of the sea surface. The upwelling infrared emission is determined with two different IRTs for over-ocean field campaigns and the data is at 1-second temporal resolution. The IRTs are mounted at heights varying between 2 and 42 m above the ground, oriented so the mounting platform and other human made objects are not in the field of view, and also to ensure that the ground and vegetation cover are representative of the local area. The Heitronics IRT is generally mounted inside a small enclosure, and the Apogee IRT is shielded by a cylindrical enclosure that is part of the design from the manufacturer.

47 OTHER INSTRUMENTATION↗
DOE OSTI2016

The contribution of host galaxies to the infrared energy output of z ≳ 5.0 quasars

The infrared spectral energy distributions of z ≳ 5 quasars can be reproduced by combining a low-metallicity galaxy template with a standard active galactic nucleus (AGN) template. The host galaxy is represented by Haro 11, a compact, moderately low metallicity, starbursting galaxy that shares typical features of high-z galaxies. For the vast majority of z ≳ 5 quasars, the AGN contribution is well modeled by a standard empirical template with the contamination of star formation in the infrared subtracted. Together, these two templates can separate the contributions from the host galaxy and the AGN even in the case of limited data points, given that this model has only two free parameters. Using this method, we reanalyze 69 z ≳ 5 quasars with extensive Herschel observations and derive their AGN luminosities [L{sub AGN} = (0.78--27.4)×10{sup 13} L{sub ⊙}], infrared luminosities from star formation [L{sub SF,IR} ≲ (1.5--25.7)×10{sup 12} L{sub ⊙}], and corresponding star formation rates (SFR ≲290--2650M{sub ⊙} yr{sup −1}). The average infrared luminosity from star formation and the average total AGN luminosity of the z ≳ 5 quasar sample follow the correlation defined by quasars at z < 2.6. We assume that these quasar host galaxies maintain a constant average SFR (∼620 M{sub ⊙} yr{sup −1}) during their mass assembly and estimate the stellar mass that could form prior to z ∼ 5−6 to be 〈M{sub ∗}〉∼(3--5)×10{sup 11}M{sub ⊙}. Combining with the black hole (BH) mass measurements, this stellar mass is adequate to establish a BH–galaxy mass ratio M{sub BH}/M{sub ∗} at 0.1%–1%, consistent with the local relation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

NuSTAR unveils a heavily obscured low-luminosity active galactic nucleus in the luminous infrared galaxy NGC 6286

We report the detection of a heavily obscured active galactic nucleus (AGN) in the luminous infrared galaxy (LIRG) NGC 6286 identified in a 17.5 ks Nuclear Spectroscopic Telescope Array observation. The source is in an early merging stage and was targeted as part of our ongoing NuSTAR campaign observing local luminous and ultra-luminous infrared galaxies in different merger stages. NGC 6286 is clearly detected above 10 keV and by including the quasi-simultaneous Swift/XRT and archival XMM-Newton and Chandra data, we find that the source is heavily obscured (N{sub H} ≃(0.95−1.32) × 10{sup 24} cm{sup −2}) with a column density consistent with being Compton-thick (CT, log(N{sub H}/cm{sup −2})⩾24). The AGN in NGC 6286 has a low absorption-corrected luminosity (L{sub 2−10 keV} ∼ 3−20 × 10{sup 41} erg s{sup −1}) and contributes ≲1% to the energetics of the system. Because of its low luminosity, previous observations carried out in the soft X-ray band (<10 keV) and in the infrared did not notice the presence of a buried AGN. NGC 6286 has multiwavelength characteristics typical of objects with the same infrared luminosity and in the same merger stage, which might imply that there is a significant population of obscured low-luminosity AGNs in LIRGs that can only be detected by sensitive hard X-ray observations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

The [N ii] 205 μm emission in local luminous infrared galaxies

In this paper, we present the measurements of the [N ii] 205 μm line for a flux-limited sample of 122 (ultra-)luminous infrared galaxies [(U)LIRGs] and 20 additional normal galaxies, obtained with the Herschel Space Observatory (Herschel). We explore the far-infrared (FIR) color dependence of the [N ii] 205 μm (L{sub [N ii]205 μm}) to the total infrared (L{sub IR}) luminosity ratio, and find that L{sub [N ii]205 μm}/L{sub IR} only depends modestly on the 70–160 μm flux density ratio (f{sub 70}/f{sub 160}) when f{sub 70}/f{sub 160}≲0.6, whereas such dependence becomes much steeper for f{sub 70}/f{sub 160}>0.6. We also investigate the relation between L{sub [N ii]205 μm} and star formation rate (SFR), and show that L{sub [N ii]205 μm} has a nearly linear correlation with SFR, albeit the intercept of such a relation varies somewhat with f{sub 60}/f{sub 100}, consistent with our previous conclusion that [N ii] 205 μm emission can serve as an SFR indicator with an accuracy of ∼0.4 dex, or ∼0.2 dex if f{sub 60}/f{sub 100} is known independently. Furthermore, together with the Infrared Space Observatory measurements of [N ii], we use a total of ∼200 galaxies to derive the local [N ii] 205 μm luminosity function (LF) by tying it to the known IR LF with a bivariate method. As a practical application, we also compute the local SFR volume density ( ρ-dot {sub SFR}) using the newly derived SFR calibrator and LF. The resulting log ρ-dot {sub SFR}=−1.96±0.11 M{sub ⊙} yr{sup −1} Mpc{sup −3} agrees well with previous studies. Finally, we determine the electron densities (n{sub e}) of the ionized medium for a subsample of 12 (U)LIRGs with both [N ii] 205 μm and [N ii] 122 μm data, and find that n{sub e} is in the range of ∼1–100 cm{sup −3}, with a median value of 22 cm{sup −3}.

79 ASTRONOMY AND ASTROPHYSICS↗