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At least 685 records · Page 38

SPACE CHARGE EFFECT IN LOW ENERGY MAGNETIZED ELECTRON BEAM

Magnetized electron cooling is one of the major approaches towards obtaining the required high luminosity in the proposed Electron-Ion Collider (EIC). In order to increase the cooling efficiency, a bunched electron beam with a high bunch charge and high repetition rate is required. At Jefferson Lab, we generated magnetized electron beams with high bunch charge using a new compact DC high voltage photogun biased at -300 kV with bialkali-antimonide photocathode and a commercial ultra-fast laser. This contribution discusses how magnetization affects space charge dominated beams as a function of magnetic field strength, gun high voltage, and laser pulse width, and spot size in comparison with simulations performed using General Particle Tracer.

Wijethunga, S.A.K.↗

Harmonic combiner and divider

The harmonic combiner and divider efficiently combines multiple harmonic signals onto a common transmission line. Combined harmonic signals can be used to generate fast, high-fidelity arbitrary waveforms by superimposing the harmonics described in their Fourier series. Fast arbitrary waveforms have applications in communications, radar, and can be used for manipulating and controlling charged particle beams. The harmonic combiner and divider also efficiently divides fast arbitrary waveforms into their constituent harmonics and provides an efficient mechanism for waveform analysis and for multi-channel communications.

Roberts, Brock Franklin↗

The nanoscale distribution of copper and its influence on charge collection in CdTe solar cells

For decades, Cu has been the primary dopant in CdTe photovoltaic absorbers. Typically, Cu acceptor concentrations in these devices are on the order of 1 1014 cm-3, which has made it notoriously difficult to directly correlate nanoscale Cu distributions to the local charge transport properties of these devices. To measure and correlate these properties, measurement techniques require high sensitivity to elemental concentration, large penetration depth, and operando compatibility. Techniques such as secondary-ion mass spectroscopy and X-ray energy dispersive spectroscopy are widely adopted to measure Cu concentrations, but they are limited by penetration depth, sensitivity, or spatial resolution. Additionally, they lack the operando capabilities required to correlate one-to-one Cu concentrations to electrical performance. In this work, correlative X-ray microscopy is used to investigate the spatial distribution of Cu and its impact on charge collection through the depth and breadth of CdTe photovoltaic devices. Plan-view, nanoscale X-ray fluorescence maps clearly demonstrate the spatial segregation of copper around regions thought to be CdTe grain boundaries. Complementary cross-section imaging unveils the transition of the maximum charge-collection efficiency from the ZnTe-CdTe interface to the CdS-CdTe interface as a function of Cu incorporation. The copper concentration through the depth of the CdTe layer is characterized by slow and fast diffusion components, and cross-section charge-transport modeling shows that the experimentally obtained charge collection can be explained by the modeled acceptor distribution through the depth of the CdTe layer.

14 SOLAR ENERGY↗

MIDAS prototype Multispectral Interactive Digital Analysis System for large area earth resources surveys. Volume 2: Charge coupled device investigation

MIDAS is a third-generation, fast, low cost, multispectral recognition system able to keep pace with the large quantity and high rates of data acquisition from large regions with present and projected sensors. MIDAS, for example, can process a complete ERTS frame in forty seconds and provide a color map of sixteen constituent categories in a few minutes. A principal objective of the MIDAS Program is to provide a system well interfaced with the human operator and thus to obtain large overall reductions in turn-around time and significant gains in throughput. The need for advanced onboard spacecraft processing of remotely sensed data is stated and approaches to this problem are described which are feasible through the use of charge coupled devices. Tentative mechanizations for the required processing operations are given in large block form. These initial designs can serve as a guide to circuit/system designers.

Kriegler, F.↗

Solar wind ion composition and charge states

The solar wind, a highly tenuous plasma streaming from the Sun into interplanetary space at supersonic speed, is roughly composed of 95% hydrogen and 5% helium by number. All other, heavy elements contribute less than 0.1% by number and thus are truly test particles Nevertheless, these particles provide valuable information not present in the main components. We first discuss the importance of the heavy ions as tracers for processes in the solar atmosphere. Specifically, their relative abundances are found to be different in the solar wind as compared to the photosphere. This fractionation, which is best organized as a function of the first ionization time (FIT) of the elements under solar surface conditions, provides information on the structure of the chromosphere. where it is imparted on the partially ionized material by an atom-ion separation mechanism. Moreover, the charge states of the heavy ions can be used to infer the coronal temperature, since they are frozen-in near the altitude where the expansion time scale overcomes the ionization/recombination time scales. Next, we review the published values of ion abundances in the solar wind, concentrating on the recent results of the SWICS instrument on Ulysses. About 8 elements and more than 20 charge states can be routinely analyzed by this sensor. There is clear evidence that both the composition and the charge state distribution is significantly different in the fast solar wind from the south polar coronal hole, traversed by Ulysses in 1993/94, as compared to the solar wind normally encountered near the ecliptic plane. The fractionation between low- and high-FIT elements is reduced, and the charge states indicate a lower, more uniform coronal temperature in the hole. Finally, we discuss these results in the framework of existing theoretical models of the chromosphere and corona, attempting to identify differences between the low- and high-latitude regions of the solar atmosphere.

vonSteiger, R.↗

Self‐Assembled Membranes for High Ion Selectivity and Proton Blocking in Electrochemical Applications

Anion-exchange membranes (AEMs) with high anion/cation selectivity and exceptional proton-blocking ability are critical for applications such as bipolar membrane electrodialysis and electrochemical acid recovery. However, existing AEMs are constrained by a trade-off between ionic conductivity and selectivity, largely due to the intrinsic coupling between charge density and water content, and they suffer from excessive proton leakage facilitated by the Grotthuss hopping mechanism. In this work, poly(vinylimidazolium) membranes functionalized with long alkyl side chains that self-assemble into well-defined microphase-separated morphologies stabilized by hydrophobic and electrostatic interactions are reported. These unique structures localize the charge density along the polymer backbone to promote fast and selective ion transport. As a result, these membranes exhibit ionic conductivities and counter-ion diffusivities surpassing those of conventional homogeneous membranes, along with unprecedented counter-ion/co-ion selectivity and proton-blocking ability. These results establish a new design paradigm for high-performance, phase separated charged polymer membranes that overcome the limitations of homogeneous membranes, with broad implications for advanced electrochemical technologies.

36 MATERIALS SCIENCE↗

Modeling of pickup ion distributions in the Halley cometosheath: Empirical limits on rates of ionization, diffusion, loss and creation of fast neutral atoms

The shape of the velocity distribution of water group ions observed by the Giotto ion mass spectrometer on its approach to comet Halley is modeled to derive empirical values for the rates of ionization, energy diffusion, and loss in the midcometosheath. The model includes the effect of rapid pitch angle scattering into a bispherical shell distribution as well as the effect of the magnetization of the plasma on the charge exchange loss rate. It is found that the average rate of ionization of cometary neutrals in this region of the cometosheath appears to be of the order of a factor 3 faster than the `standard' rates approx. 1 x 10(exp -6)/s that are generally assumed to model the observations in most regions of the comet environment. For the region of the coma studied in the present work (approx. 1 - 2 x 10(exp 5) km from the nucleus), the inferred energy diffusion coefficient is D(sub 0) approx. equals 0.0002 to 0.0005 sq km/cu s, which is generally lower than values used in other models. The empirically obtained loss rate appears to be about an order of magnitude greater than can be explained by charge exchange with the `standard' cross section of approx. 2 x 10(exp -15)sq cm. However such cross sections are not well known and for water group ion/water group neutral interactions, rates as high as 8 x 10(exp -15) sq cm have previously been suggested in the literature. Assuming the entire loss rate is due to charge exchange yields a rate of creation of fast neutral atoms of the order of approx. 10(exp -4)/s or higher, depending on the level of velocity diffusion. The fast neutrals may, in turn, be partly responsible for the higher-than-expected ionization rate.

Huddleston, D. E.↗

The Psyche Gamma-Ray and Neutron Spectrometer

A Gamma-Ray and Neutron Spectrometer (GRNS) instrument has been developed as part of the science payload for NASA’s Discovery Program Psyche mission to the M-class asteroid (16) Psyche. The GRNS instrument is designed to measure the elemental composition of Psyche with the goal to understand the origin of this mysterious, potentially metal-rich planetary body. The GRNS will measure the near-surface abundances for the elements Ni, Fe, Si, K, S, Al, and Ca, as well as the spatial distribution of Psyche’s metal-to-silicate fraction (or metal fraction). These measurements address three of the five Psyche mission science objectives: determine if Psyche is a core; determine whether small metal bodies incorporate light elements into the metal phase; and determine whether Psyche was formed under reducing conditions. The Gamma-Ray Spectrometer (GRS) uses a cryocooled, high-purity Ge (HPGe) sensor to detect cosmic-ray generated gamma rays in the 60 to 9000-keV energy range. The HPGe sensor is surrounded by a borated plastic anticoincidence shield that provides three functions: active background rejection from charged particle interactions in the HPGe sensor; fast neutron measurements; and direct measurements of the incident galactic cosmic ray flux. The Neutron Spectrometer (NS) uses three 3 He gas proportional sensors, each with different material wraps to measure thermal (<0.4 eV), low-energy epithermal (0.4 eV to 1 keV), and high-energy epithermal (up to 100 keV) neutrons. This paper provides an overview of the Psyche GRNS, including: its science and measurement objectives; the design of the instrument hardware, software, and operation; pre-launch performance measurements and its initial performance in space; and an overview of its data products and expected operation for different Psyche mission phases.

Engineering - Instrumentation related to nuclear s↗

Scintillation properties of diamond powders and feasibility of using them in thermal neutron detectors

Diamond offers unique properties for radiation detection, including high radiation hardness, very low gamma sensitivity, and fast response. Conventional diamond detectors rely on charge collection, but this approach requires ultra-pure single crystals and suffers from radiation-induced degradation. Here, in this work, we demonstrate an alternative approach using diamonds as scintillators for detection of charged particles and thermal neutrons. Prototypes were fabricated from commercially available diamond powders bonded to glass substrates and coupled with 6 LiF converters and silicon photomultipliers (SiPMs) and conventional PMTs. We characterized their scintillation properties under alpha particle excitation, x-ray photoluminescence, and thermal neutrons. The tryout detectors exhibit strong scintillation light signals, nanosecond-scale response times, and neutron detection efficiencies up to approximately 14 %, evaluated by comparison to conventional 3 He detector with known efficiency. These results demonstrate the feasibility of cost-effective, lightweight and robust diamond scintillation detectors for applications in space and planetary science, nuclear security, safeguards and environmental monitoring requiring efficient, robust, gamma-blind neutron detectors.

47 OTHER INSTRUMENTATION↗

Time-resolved RIXS experiment with pulse-by-pulse parallel readout data collection using X-ray free electron laser

Abstract Time-resolved resonant inelastic X-ray scattering (RIXS) is one of the developing techniques enabled by the advent of X-ray free electron laser (FEL). It is important to evaluate how the FEL jitter, which is inherent in the self-amplified spontaneous emission process, influences the RIXS measurement. Here, we use a microchannel plate (MCP) based Timepix soft X-ray detector to conduct a time-resolved RIXS measurement at the Ti L 3 -edge on a charge-density-wave material TiSe 2 . The fast parallel Timepix readout and single photon sensitivity enable pulse-by-pulse data acquisition and analysis. Due to the FEL jitter, low detection efficiency of spectrometer, and low quantum yield of RIXS process, we find that less than 2% of the X-ray FEL pulses produce signals, preventing acquiring sufficient data statistics while maintaining temporal and energy resolution in this measurement. These limitations can be mitigated by using future X-ray FELs with high repetition rates, approaching MHz such as the European XFEL in Germany and LCLS-II in the USA, as well as by utilizing advanced detectors, such as the prototype used in this study.

36 MATERIALS SCIENCE↗

Kinetic equilibrium reconstruction and the impact on stability analysis of KSTAR plasmas

High fidelity kinetic plasma equilibrium reconstructions are an essential requirement for accurate stability and disruption prediction analyses to support continuous operation of high beta tokamak plasmas. The present kinetic equilibrium reconstructions of plasmas in the KSTAR device include plasma density and temperature profiles from Thomson scattering and ion temperature from charge exchange spectroscopy diagnostics, and allowance for fast particle pressure. In addition, up to 25 channels of motional Stark effect diagnostic data are used to constrain the magnetic field pitch angle profile in the plasma to produce a reliable computation of the safety factor, q, profile. In this work, H-mode plasmas exhibit clear pedestal characteristics in the reconstructed pressure profile compared to internal transport barrier or L-mode plasmas. The plasma configuration and vertical position of inner strike points are validated by CCD and infrared camera images. Ideal and resistive magnetohydrodynamic (MHD) stability analyses using the DCON and resistive DCON codes utilize these kinetic equilibrium reconstructions to compare to experimental plasma stability. Equilibria with sufficiently low convergence error can provide reliable computation of ideal and resistive MHD stability analysis.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Comparison of Feschenko BSM and Fast Faraday Cup with Low Energy Ion Beams

A comparison between Fast Faraday Cup and Feschenko longitudinal bunch shape detectors was recently performed at HELIAC Advanced Demonstrator beamline at GSI. Feschenko bunch shape monitor (BSM) uses the time to space conversion by means of secondary electrons emitted from a wire correlated to a rf deflector, while the fast Faraday cup (FFC) measures the deposited charge in a cup geometry matched to 50 Ohm. The FFC design aims to minimize the bunch shape dilution due to field polarization and secondary electrons produced on irradiation. An He¹⁺ with 100 µA average current and 1.4 MeV/u kinetic energy is utilized for this comparison. A buncher upstream of the detectors was operated to focus the beam longitudinally. The results are discussed in this contribution.

43 PARTICLE ACCELERATORS↗

Development of an Advanced Hydrogen Energy Storage System using Aerogel in a Cryogenic Flux Capacitor (CFC)

The Cryogenic Flux Capacitor (CFC) is a cold, dense fluid storage core with integrated design features that afford the designer flexibility and provide new possibilities for the storage and discharge of energy. The stored energy, in this case, is represented by hydrogen physically bonded within the nanoscale pores within the aerogel composite blanket material, and the process of bonding or debonding is governed by principles of physical adsorption (physisorption) and thermodynamics. The large surface area afforded by the nanoporous aerogel (~1,000 m2/g) allows for storage densities close to, or in some cases exceeding, that of normal boiling point liquids. Its performance easily exceeds what can be achieved via ambient temperature, high-pressure gas storage for an equivalent volume. CFC storage is predicted to be easily scalable, is constructed from readily available commercial materials, lends itself to a range of pressure applications, and is geometry insensitive. They can also be used in modular designs, affording even more flexibility for potential deployment. In addition to the aerogel adsorbent within the blanket material, a CFC includes thermally-conductive membrane layered with the aerogel, which acts as a large-area, quick-response thermal management system. The system conducts heat throughout the volume to discharge the unit quickly. This same thermal management system can also be connected to a refrigeration system, or cold fluid such as liquid nitrogen (LN2), to facilitate the charging up of the CFC. The charging and discharging can be performed as fast or as slow as desired by controlling the cooling or heating supplied to the CFC.

08 HYDROGEN↗

The electric fields and “lightning jets” of the Sun and solar wind

A model of electric energization of the solar wind and corona is developed, including electro-magnetic particle effects precluded by traditional magneto-hydro (MHD) assumptions. Using standard 1D radial solar models for particle density and temperature, the core gravito-electric field is calculated; and the range of possible photospheric photo-electric fields is estimated. The extant DC field apparently arises from about 460 C of charge displacement, mainly caused by the immense solar energy flux pushing electrons outward. Energetically, this electric field can accelerate surface protons out of the 2 keV gravity well and up to the 4 keV energies observed in the fast solar wind. The electrical energy is released in pervasive, persistent “proton lightning jets,” which are proton beams, charge-neutralized by co-propagating electrons. The jets are formed by pinched “avalanche breakdown” of the weakly ionized photosphere, probably initiated on the down-welling edges of solar surface granulations. These energetic jets will glow as discrete filamentary surface spicules and will be observed in reflected solar light as the diffuse K-corona. Significantly, the total charge displacement and observed fast wind speed are quantitatively predicted by a novel “virial limit”: the (positive) electrical potential energy at r = 0 is limited in magnitude to the 10 keV gravitational well at r = 0.

Physics↗

Proton discrimination in CLYC for fast neutron spectroscopy

The Cs 2 LiYCl 6 :Ce (CLYC) elpasolite scintillator is known for its response to fast and thermal neutrons along with good γ-ray energy resolution. While the 35 Cl(n,p) reaction has been identified as a potential means for CLYC-based fast neutron spectroscopy in the absence of time-of-flight (TOF), previous efforts to functionalize CLYC as a fast neutron spectrometer have been thwarted by the inability to isolate proton interactions from 6 Li(n,α) and 35 Cl(n,α) signals. This work introduces a new approach to particle discrimination in CLYC for fission spectrum neutrons using a multi-gate charge integration algorithm that provides excellent separation between protons and heavier charged particles. Neutron TOF data were collected using a 252 Cf source, an array of EJ-309 organic liquid scintillators, and a 6 Li-enriched CLYC scintillator outfitted with fast electronics. Modal waveforms were constructed corresponding to the different reaction channels, revealing significant differences in the pulse characteristics of protons and heavier charged particles at ultrafast, fast, and intermediate time scales. These findings informed the design of a pulse shape discrimination algorithm, which was validated using the TOF data. This study also proposes an iterative subtraction method to mitigate contributions from confounding reaction channels in proton and heavier charged particle pulse height spectra, opening the door for CLYC-based fast neutron and γ-ray spectroscopy while preserving sensitivity to thermal neutron capture signals.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Laser pulse driven control of charge and spin order in the two-dimensional Kondo lattice

Fast and dynamical control of quantum phases is highly desired in the application of quantum phenomena in devices. On the experimental side, ultrafast laser pulses provide an ideal platform to induce femtosecond dynamics in a variety of materials. Here we show that a laser pulse driven heavy fermion system can be tuned to dynamically evolve into a phase, which is not present in equilibrium. Using the state-of-the-art time-dependent variational Monte Carlo method, we perform numerical simulations of realistic laser pulses applied to the Kondo lattice model. By tracking spin and charge degrees of freedom we identify a dynamical phase transition, within the partially Kondo screened phase, from a charge ordered into a metallic state, while preserving the spin order of the system. Furthermore, we propose using high-harmonic generation and nonequilibrium optical conductivity to identify the dynamical phase transition in an ultrafast experiment.

36 MATERIALS SCIENCE↗

Space-charge effects in ionization beam profile monitors

Ionization profile monitors (IPMs) are widely used in accelerators for non-destructive and fast diagnostics of high energy particle beams. At high beam intensities, the space-charge forces make the measured IPM profiles significantly different from those of the beams. We analyze dynamics of the secondaries in IPMs and develop an effective algorithm to reconstruct the beam sizes from the measured IPM profiles. Efficiency of the developed theory is illustrated in application to the Fermilab 8 GeV proton Booster IPMs.

43 PARTICLE ACCELERATORS↗

Space-Charge Effects in Ionization Beam Profile Monitors

Ionization profile monitors (IPMs) are widely used in accelerators for non-destructive and fast diagnostics of high energy particle beams. At high beam intensities, the space-charge forces make the measured IPM profiles significantly different from those of the beams. We analyze dynamics of the secondaries in IPMs and develop an effective algorithm to reconstruct the beam sizes from the measured IPM profiles. Efficiency of the developed theory is illustrated in application to the Fermilab 8 GeV proton Booster IPMs.

Shiltsev, Vladimir D.↗