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At least 685 records · Page 38

Design of a first-of-A-kind instrumented advanced test reactor irradiation Capsule experiment for In situ thermal conductivity measurements of metallic fuel

Metallic fuel undergoes dramatic microstructural changes early in life due to fission gas swelling until ~2–3 at% burnup which affects the conductivity of the material, however the evolution of metallic fuel thermal conductivity during this early phase burnup has never been successfully measured in situ. The Irradiated Material Properties Accelerated Characterization Test (IMPACT) experiment will be the first in a series of experiments to irradiate advanced nuclear metallic fuel specimens with novel embedded thermal conductivity probes in ATR. In the current work the IMPACT experiment final design and supporting analysis is reported in detail. Results are evaluated for various reactor operational conditions to meet the functional requirements of the experiment. Finally, the first iteration of this IMPACT experiment will provide data regarding thermal properties evolution in uranium-zirconium (U10Zr) fuel, but this experiment vehicle is envisioned for future advanced fuels and structural materials irradiations in ATR.

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Future TRISO fuel irradiations in the Advanced Test Reactor

AGR-5/6/7 was thought to be the last experiment in the AGR series and the last experiment directly sponsored by DOE. Over the last five years three developments have caused a reevaluation of that assumption. First is that interest in TRISO fueled reactors has spiked dramatically. Virtually all of the new reactor designs are for SMRs or micro-reactors . Some of these reactors use new fuel designs with higher concentrations of U235. This results in changes to the particle design and even fuel pellet design. Second, a design flaw in AGR-5/6/7 Capsule 1 produced a large number of particle failures which resulted in the loss of data from Capsule 1. An additional irradiation could fill in this lost data set. Thirdly, many reactor developers have decided to use AGR spec fuel but different irradiation goals have been identified.

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Bench-Scale Monolith Autothermal Reformer Catalyst Screening Evaluations in a Micro-Reactor With Jet-A Fuel

Solid oxide fuel cell systems used in the aerospace or commercial aviation environment require a compact, light-weight and highly durable catalytic fuel processor. The fuel processing method considered here is an autothermal reforming (ATR) step. The ATR converts Jet-A fuel by a reaction with steam and air forming hydrogen (H2) and carbon monoxide (CO) to be used for production of electrical power in the fuel cell. This paper addresses the first phase of an experimental catalyst screening study, looking at the relative effectiveness of several monolith catalyst types when operating with untreated Jet-A fuel. Six monolith catalyst materials were selected for preliminary evaluation and experimental bench-scale screening in a small 0.05 kWe micro-reactor test apparatus. These tests were conducted to assess relative catalyst performance under atmospheric pressure ATR conditions and processing Jet-A fuel at a steam-to-carbon ratio of 3.5, a value higher than anticipated to be run in an optimized system. The average reformer efficiencies for the six catalysts tested ranged from 75 to 83 percent at a constant gas-hourly space velocity of 12,000 hr 1. The corresponding hydrocarbon conversion efficiency varied from 86 to 95 percent during experiments run at reaction temperatures between 750 to 830 C. Based on the results of the short-duration 100 hr tests reported herein, two of the highest performing catalysts were selected for further evaluation in a follow-on 1000 hr life durability study in Phase II.

Tomsik, Thomas M.↗

Ferritic Alloys as Accident Tolerant Fuel Cladding Material for Light Water Reactors

The objective of the GE project is to demonstrate that advanced steels such as iron-chromium-aluminum (FeCrAl) alloys could be used as accident tolerant fuel cladding material in commercial light water reactors. The GE project does not include fuel development. Current findings support the concept that a FeCrAl alloy could be used for the cladding of commercial nuclear fuel. The use of this alloy will benefit the public since it is going to make the power generating light water reactors safer. In the Phase 1A of this cost shared project, GE (GRC + GNF) teamed with the University of Michigan, Los Alamos National Laboratory, Brookhaven National Laboratory, Idaho National Laboratory, and Oak Ridge National Laboratory to study the environmental and mechanical behavior of more than eight candidate cladding materials both under normal operation conditions of commercial nuclear reactors and under accident conditions in superheated steam (loss of coolant condition). The main findings are as follows: (1) Under normal operation conditions the candidate alloys (e.g. APMT, Alloy 33) showed excellent resistance to general corrosion, shadow corrosion and to environmentally assisted cracking. APMT also showed resistance to proton irradiation up to 5 dpa. (2) Under accident conditions the selected candidate materials showed several orders of magnitude improvement in the reaction with superheated steam as compared with the current zirconium based alloys. (3) Tube fabrication feasibility studies of FeCrAl alloys are underway. The aim is to obtain a wall thickness that is below 400 µm. (4) A strategy is outlined for the regulatory path approval and for the insertion of a lead fuel assembly in a commercial reactor by 2022. (5) The GE team worked closely with INL to have four rodlets tested in the ATR. GE provided the raw stock for the alloys, the fuel for the rodlets and the cost for fabrication/welding of the rodlets. INL fabricated the rodlets and the caps and welded them to provide hermetic seal. The replacement of a zirconium alloy using a ferritic material containing chromium and aluminum appears to be the most near term implementation for accident tolerant nuclear fuels.

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Accelerating Nuclear-Integrated Data Centers in the USA: SWOT Analysis, Power-Thermal Management Strategies, and Industrial-Scale Demonstration and Potential Deployment

Driven by the growth in digital services, cloud computing, AI, and manufacturing, data centers face rising energy demands that challenge traditional power sources and cooling efficiency. This study explores using nuclear power to meet these demands, focusing on accelerated reactor technology deployment and highlighting needs such as N+1/N+2 power supplies and integrated power-thermal management. A SWOT analysis addresses grid connectivity, reactors, and site selection, particularly DOE sites. Reactor technology demonstration and deployment could be accelerated by leveraging test facilities such as MARVEL, MAGNET, TED, FAS, DOME, LOTUS, ATR, Energy System Proving Grounds, and upcoming Energy Launch Pads, along with modeling and simulation tools such as RELAP5, MOOSE, VERA, RAVEN, and FORCE. The potential power and thermal management options, including various cooling technologies, waste-heat utilization, and an industrial-scale demonstration plan, aim to accelerate the integration of nuclear power and data centers in the USA, while emphasizing community and stakeholder engagement and synergistic efforts.

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As-run thermal-hydraulics analysis of the EPRI-2 experiment

The EPRI-2 experiment was designed to irradiate various types of reactor pressure vessel steels at a temperature of 288°C (PLN-3934). The specimens were irradiated in a non-instrumented test train inside a pressurized water loop in the center lobe of the ATR during PALM cycle 153B. Temperature was indicated by post-irradiation examination of melt wires placed within the test train. The purpose of this analysis is to calculate specimen temperature using measured data on reactor power and as-run calculations of heating rates of the test train. The experiment contains several melt wires spanning the temperature range 239°C to 327°C. The accuracy of the model is assessed by comparing the measured and calculated in-pile tube inlet to outlet temperature difference, and comparing the calculated specimen temperature to the temperature range indicated by examination of the melt wires.

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As-run thermal-hydraulic analysis of the EPRI-3 experiment

The EPRI-3 experiment was designed to irradiate various types of reactor internal component steels at a temperature of 288°C. The specimens were irradiated in an instrumented test train inside a pressurized water loop in the center lobe of the ATR during cycles 155B and 158B. Temperature was monitored using thermocouples placed at the top of the test train and melt wires placed within the test train. The purpose of this analysis is to calculate specimen temperature using measured data on reactor power and as-run calculations of heating rates of the test train. The experiment contains four thermocouples and several melt wires spanning the temperature range 239°C to 327°C. The accuracy of the model is assessed by comparing the measured and calculated in-pile tube inlet to outlet temperature difference, comparing the measured and calculated thermocouple temperatures, and comparing the calculated melt wire temperature to the temperature range indicated by examination of the melt wires.

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The Fission Accelerated Steady State Test (FAST) -- A Revised Capsule Design for the Accelerated Testing of Advanced Reactor Fuels

In an effort to improve the development and testing of novel nuclear fuels, a detailed evaluation on reducing the size of fuel specimens for irradiation has been performed. Theoretically speaking, reducing the fuels diameter and incorporating an inner capsule while maintaining the original outside diameter of the experiment significantly reduces the experiment’s sensitivity to fabrication tolerances and drastically reduces the time necessary to reach a desired fuel burnup; both of which improve the cost and schedule associated with the fuel testing. Simulations of this reduced diameter, double encapsulated concept have been performed using Abaqus, MCNP, and ORIGEN. The results of the Abaqus simulations are beyond the scope of this summary and will not be presented herein. For results of these Abaqus simulations, see Beausoleil [2]. The models were tested using various parameters and design deviations which were then compared to the original Advanced Fuels Campaign (AFC) designs. The results of these simulations confirmed that the introduction of a second capsule coupled to a reduction in the fuel pin diameter significantly reduces the experiment’s sensitivity to fabrication tolerances and reduces the time to reach a desired burnup by nearly an order of magnitude. The original AFC design requires approximately 11.7 years to reach 30 Atom % Heavy Metal (at% HM) burnup. A burnup of 30 at% HM can be reached in approximately 2.5 to 3.5 years (irradiation position dependent) with a fuel diameter ½ (~0.097 in. diameter) that of the original AFC design. An added benefit to the fuel pin diameter reduction is that more specimens can be irradiated in any given cycle. Essentially, significantly more specimens can be tested and incur more burnup over a given operating cycle relative to the AFC design. This allows the development of a large test matrix of samples with rapid throughput in ATR.

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Projection Analysis for ATR Irradiation of the AFC-FAST Experiment

Analyses of the Advanced Fuels Campaign Fission Accelerated Steady-state Test (AFC-FAST) in the Advanced Test Reactor are presented. A detailed methodology was employed to better account for uncertainties in the planned power and duration of sequential reactor loading cycles. By performing coupled depletion analyses at multiple power levels and durations, the differences in experiment heating outputs can be found. The effects of these uncertainties upon multiple experiment configurations were assessed in an effort to streamline the process of planning for and documenting future irradiations. In conclusion, the data generated from this work have been used to help inform assumptions on subsequent projections to perform only a nominal case depletion.

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Challenges and Solutions for Fast Neutron Irradiation of Bulk Material Specimens

Reactor developers continue to recognize opportunities for further enhancing fast spectrum reactor designs with advanced core materials, but all the material test reactors currently available to the United States are thermal spectrum designs. Fortunately, the Advanced Test Reactor and High Flux Isotope Reactor are versatile high flux facilities where spectral modification strategies can be used to reduce undesirable thermal neutron capture transmutation damage and augment fast flux delivered to specimens. New opportunities to leverage high flux regions and specially designed fast flux boosting experiment configurations can be used to achieve meaningful fast fluences on large specimens in ATR. New optimization potentials can be employed to achieve even higher fluences, albeit for smaller specimens, using thermal neutron filters in HFIR test positions. These capabilities, while not true fast reactors, can provide highly relevant environments for researchers needing to study the effects of fast neutron damage in bulk material specimens.

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Property analysis and advanced manufacturing technique development for light water reactor annular composite fuel

The University of Florida (UF) has been developing a composite UO{sub 2}-Diamond Fuel design for water-cooled reactors that offers greatly increased thermal conductivity as measured at BOL. Currently, Diamond composite fuel pellets are being irradiated in the ATR to determine whether the thermal conductivity increase is maintained as a function of burnup. UF has further increased the benefits of this increased thermal conductivity of the additive UO{sub 2} fuel by implementing an annular pellet design. The central core material for our annular fuel design must have a high thermal conductivity, a high melting point, a low absorption cross section, a low coefficient of thermal expansion and a neutron thermal moderating capability, which will enhanced the reactivity and performance of the cored pellet. The chosen ZrC core material has a very high melting temperature of 3,700 Celsius degrees, a high thermal conductivity, a good moderating effect, and a low value of thermal expansion. UF has successfully manufactured UO{sub 2} annular pellets. The University of Florida (UF) team believes such an annular pellet can eliminate pellet cracking, reduce fission gas release by over 50% and reduce the maximum pellet temperature by between 300 to 600 Celsius degrees. It is believed that such a pellet design would tolerate a loss of coolant accident (LOCA). (authors)

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Ultrasonic Transducer Irradiation Test Results

Ultrasonic technologies offer the potential for high-accuracy and -resolution in-pile measurement of a range of parameters, including geometry changes, temperature, crack initiation and growth, gas pressure and composition, and microstructural changes. Many Department of Energy-Office of Nuclear Energy (DOE-NE) programs are exploring the use of ultrasonic technologies to provide enhanced sensors for in-pile instrumentation during irradiation testing. For example, the ability of small diameter ultrasonic thermometers (UTs) to provide a temperature profile in candidate metallic and oxide fuel would provide much needed data for validating new fuel performance models. Other ongoing efforts include an ultrasonic technique to detect morphology changes (such as crack initiation and growth) and acoustic techniques to evaluate fission gas composition and pressure. These efforts are limited by the lack of identified ultrasonic transducer materials capable of long term performance under irradiation test conditions. For this reason, the Pennsylvania State University (PSU) was awarded an ATR NSUF project to evaluate the performance of promising magnetostrictive and piezoelectric transducers in the Massachusetts Institute of Technology Research Reactor (MITR) up to a fast fluence of at least 10 21 n/cm 2 . The goal of this research is to characterize and demonstrate magnetostrictive and piezoelectric transducer operation during irradiation, enabling the development of novel radiation-tolerant ultrasonic sensors for use in Material Testing Reactors (MTRs). As such, this test is an instrumented lead test and real-time transducer performance data is collected along with temperature and neutron and gamma flux data. The current work bridges the gap between proven out-of-pile ultrasonic techniques and in-pile deployment of ultrasonic sensors by acquiring the data necessary to demonstrate the performance of ultrasonic transducers. To date, one piezoelectric transducer and two magnetostrictive transducers have demonstrated reliable operation under irradiation. The irradiation is ongoing.

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ECAR-3386 AS-RUN THERMAL ANALYSIS OF THE AGC-3 EXPERIMENT

The third Advanced Graphite Creep (AGC-3) experiment was designed to irradiate various types of graphite specimens at a temperature of 900°C. The specimens were irradiated in an instrumented leadout capsule experiment in the east flux trap of the ATR during cycles 152B, 154B, 155A, and 155B. Temperature was monitored using twelve thermocouples located at various elevations in the reactor core, and a helium-argon gas mixture was used for gas gap temperature control of the specimens. The purpose of this analysis is to calculate specimen temperature using measured data on reactor power and helium-argon gas flows, and as-run calculations of heating rates and displacement per atom (DPA) in graphite. The accuracy of the model is assessed by comparing measured and calculated thermocouple temperatures. Uncertainty in gas gaps may preclude an accurate temperature calculation. In these cases, adjustments are made to the thermal model in order to reconcile the measured and calculated thermocouple temperature and to ensure the accuracy of the calculated specimen temperature.

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As-run thermal hydraulics analysis of the EPRI-1 Experiment

The EPRI-1 experiment was designed to irradiate various types of reactor pressure vessel steels at a temperature of 288°C (PLN-3934). The specimens were irradiated in an instrumented test train inside a pressurized water loop in the center lobe of the ATR during cycle 157C. Temperature was monitored using thermocouples placed at the top of the test train. Additional temperature indications were obtained by post-irradiation examination of melt wires placed within the test train and spanning the temperature range 239°C to 327°C. The purpose of this analysis is to calculate specimen temperature using measured data on reactor power and as-run calculations of heating rates of the test train. The accuracy of the model is assessed by comparing the measured and calculated in-pile tube inlet to outlet temperature difference, comparing the measured and calculated thermocouple temperatures, and comparing the calculated specimen temperature to the temperature range indicated by the melt wires.

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ECAR-2322 As-Run Thermal Analysis Of The AGC-2 Experiment

The second Advanced Graphite Creep (AGC-2) experiment was designed to irradiate various types of graphite specimens at a temperature of 600°C. The specimens were irradiated in an instrumented leadout capsule experiment in the south flux trap of the ATR during cycles 149A, 1498, 1508, 151A, and 1518. Temperature was monitored using twelve thermocouples located at various elevations in the reactor core, and a helium-argon gas mixture was used for gas gap temperature control of the specimens. The purpose of this analysis is to calculate specimen temperature using measured data on reactor power and helium-argon gas flows, and as-run calculations of heating rates and displacement per atom (DPA) in graphite. The accuracy of the model is assessed by comparing measured and calculated thermocouple temperatures. Uncertainty in gas gaps may preclude an accurate temperature calculation. In these cases, adjustments are made to the thermal model in order to reconcile the measured and calculated thermocouple temperature and to ensure the accuracy of the calculated specimen temperature.

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Autothermal reforming of aliphatic and aromatic hydrocarbon liquids

Results are presented from a study of the autothermal reforming of paraffins and aromatics over nickel catalysts. The trials were performed to examine the carbon products that appear when steam is passed over hydrocarbon liquids to form H2-rich gases, i.e., the autothermal process (ATR). Attention was given to n-hexane, n-tetradecane, benzene, and benzene solutions of naphthalene with reactant preheat to 1000-1150 F. The carbon-formation limit was sought as a function of the steam-to-carbon and oxygen to carbon molar ratios at constant pressure and the preheat temperatures. The catalyst bed was examined after each trial to identify the locations and types of carbon formed using SEM, thermal gravimetric analysis, and X ray diffraction techniques. The hydrocarbon fuels each had a separate temperature and reaction profile, as well as carbon formation characteristics. No carbon formation was observed in the upper layer of the reactor bed, while both gas phase and surface-grown deposits were present in the lower part. The results are concluded of use in the study of No. 2 fuel oil for ATR feedstock.

Flytzani-Stephanopoulos, M.↗

Development of the generation III (ATR generation I) Plutonium-238 production target design

A domestic supply chain to produce 238 Pu fuel for radioisotope thermoelectric generators is critical for enabling future space exploration. A multi-laboratory effort has worked to establish a common target design to efficiently produce 238 Pu in two research reactors. This approach ensures that the annual production goals set forth by NASA are met, while also establishing redundant production capabilities. Here, this paper describes the effort to develop the common target design as well as considerations for future applications for the irradiation platform.

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A Variable Load LVDT-Based Creep Test Rig for Use in ATR Loop 2A

Understanding the creep behavior of materials in a radiation environment is essential in evaluating safety issues associated with nuclear power plant operation, especially for plants applying for life extension. In US materials testing reactors (MTRs), this understanding has been achieved through a “cook and look” approach (where specimens are irradiated under load for some period of time and then removed from an MTR for post-irradiation examination). A number of “cook and look” cycles can be required for each evaluated material, which makes this approach expensive. In addition, examinations are limited to end-state conditions, which may or may not be sufficient to reveal all phenomena of interest (because examinations are not performed at prototypic conditions relative to temperature, pressure, stress, etc.).

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