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At least 667 records · Page 37

Optimizing observables with machine learning for better unfolding

Most measurements in particle and nuclear physics use matrix-based unfolding algorithms to correct for detector effects. In nearly all cases, the observable is defined analogously at the particle and detector level. We point out that while the particle-level observable needs to be physically motivated to link with theory, the detector-level need not be and can be optimized. We show that using deep learning to define detector-level observables has the capability to improve the measurement when combined with standard unfolding methods.

47 OTHER INSTRUMENTATION↗

Measurement of prompt D s + -meson production and azimuthal anisotropy in Pb–Pb collisions at s NN = 5.02 TeV

The production yield and angular anisotropy of prompt $D^{+}_{s}$ mesons were measured as a function of transverse momentum (p T ) in Pb–Pb collisions at a centre-of-mass energy per nucleon pair $\sqrt{s_{NN}}$ = 5.02 TeV collected with the ALICE detector at the LHC. $D^{+}_{s}$ mesons and their charge conjugates were reconstructed at midrapidity (|y| < 0.5) from their hadronic decay channel $D^{+}_{s}$ → φπ + , with φ → K - K + , in the p T intervals 2 < p T < 50 GeV/c and 2 < p T < 36 GeV/c for the 0–10% and 30–50% centrality intervals. For p T > 10 GeV/c, the measured $D^{+}_{s}$ -meson nuclear modification factor R AA is consistent with the one of non-strange D mesons within uncertainties, while at lower pT a hint for a $D^{+}_{s}$ -meson R AA larger than that of non-strange D mesons is seen. The enhanced production of $D^{+}_{s}$ relative to non- strange D mesons is also studied by comparing the pT-dependent $D^{+}_{s}$ /D 0 production yield ratios in Pb–Pb and in pp collisions. The ratio measured in Pb–Pb collisions is found to be on average higher than that in pp collisions in the interval 2 < p T < 8 GeV/c with a significance of 2.3σ and 2.4σ for the 0–10% and 30–50% centrality intervals. The azimuthal anisotropy coefficient v2 of prompt $D^{+}_{s}$ mesons was measured in Pb–Pb collisions in the 30–50% centrality interval and is found to be compatible with that of non-strange D mesons. The main features of the measured RAA, $D^{+}_{s}$ /D 0 ratio, and v 2 as a function of p T are described by theoretical calculations of charm-quark transport in a hydrodynamically expanding quark–gluon plasma including hadronisation via charm-quark recombination with light quarks from the medium. The p T -integrated production yield of $D^{+}_{s}$ mesons is compatible with the prediction of the statistical hadronisation model.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Excited-state dynamics of CH 2 I 2 and CH 2 IBr studied with UV-pump VUV-probe momentum-resolved photoion spectroscopy

We perform time-resolved ionization spectroscopy measurements of the excited state dynamics of CH 2 I 2 and CH 2 IBr following photoexcitation in the deep UV. The fragment ions produced by ionization with a vacuum-ultraviolet probe pulse are measured with velocity map imaging, and the momentum resolved yields are compared with trajectory surface hopping calculations of the measurement observable. Together with recent time-resolved photoelectron spectroscopy measurements of the same dynamics, these results provide a detailed picture of the coupled electronic and nuclear dynamics involved. Overall, our measurements highlight the non-adiabatic coupling between electronic states, which leads to notable differences in the dissociation dynamics for the two molecules.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Installation and Commissioning of the SBC-LAr10 Detector at Fermilab

This report describes the progress towards a scalable detector capable of quasi-background-free detection of sub-keV nuclear recoils under DOE award DE-SC0024254. Work supported by this award follows two distinct thrusts: (1) the first calibration of sensitivity to sub-keV nuclear recoils in a liquid-noble bubble chamber, based on data taken in a prototype liquid xenon bubble chamber run previously at Northwestern University, and (2) the successful assembly and installation of the 10-kg liquid argon bubble chamber SBC-LAr10 in the MINOS underground area at Fermilab. These accomplishments have paved the way for the precision calibration of SBC-LAr10 in the MINOS underground area at Fermilab in the coming year, which will use novel calibration techniques to measure the potential of the liquid noble bubble chamber technology for the detection of GeV-scale dark matter particles and the measurement of coherent elastic nuclear scattering by reactor anti-neutrinos (CEvNS).

47 OTHER INSTRUMENTATION↗

Adiabatic fast passage spin manipulation measurements in solid polarized targets

Adiabatic fast passage (AFP) is a rapid method for reversing nuclear polarization and manipulating spin populations in polarized solid targets, avoiding the long repolarization times associated with dynamic nuclear polarization (DNP). We report AFP measurements in a 5 T, 1 K polarized-target system for irradiated 15 NH 3 , irradiated 14 ND 3 , and butanol-based materials prepared either with TEMPO doping or by irradiation. We also present a joint manipulated-lineshape analysis for spin-1 targets and demonstrate that vector and tensor polarizations can be extracted from AFP-manipulated deuteron NMR spectra even when the populations are not described by a single Boltzmann spin temperature. In conclusion, we report a reproducible polarization- and direction-dependent AFP response in a large irradiated 15 NH 3 sample. These ammonia results are presented as empirical observations under the specific sample–coil conditions of the experiment, with possible circuit-mediated mechanisms such as radiation damping or superradiant behavior discussed but not assigned as a definitive cause.

Adiabatic fast passage↗

Validation of MPACT BWR capabilities against critical experiments

Over the years, significant validation work for the neutronics code MPACT has been performed against zero-power critical benchmarks and measured data from operating nuclear power plants. As a part of the Modeling and Analysis of Exelon BWRs for Eigenvalue and Thermal Limits Predictability project, new validation efforts relevant to boiling water reactor (BWR) core applications have been performed. This paper presents the results of the critical experiment portion of the BWR validation efforts for MPACT. The Kritz-4 experiments and IPEN/MB-01 BWR-relevant configurations are modeled with MPACT. The Kritz-4 BWR critical experiments were performed at both cold and hot conditions, which is a unique feature among other critical experiment facilities. The MPACT results with linear source (LS) Method of Characteristics (MOC) have very good agreement with the measured criticality. When using the 60-group BWR library with LS and P2 scattering, the maximum k{sub eff} error is 109 pcm, and the average cold-hot bias is only -0.11 pcm/K. The fission rate distributions of MPACT are also verified with Serpent calculations. For the IPEN facility, two configurations are considered: one with a large central void, and one with a cruciform control rod. The MPACT k{sub eff} errors are less than 50 pcm for all IPEN problems. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Electropotential Verification for Nuclear Safeguards

The international safeguards regime desires methods to efficiently verify that facilities are only performing declared activities. Electropotential verification (EPV) is a newly proposed technique that was tested for its feasibility to perform facility design information verification (DIV) and verification of spent nuclear fuel while in a cooling pool. EPV works by passing a constant, low voltage current through a conductive system (facility infrastructure of nuclear fuel assembly) and measuring the resulting voltage at various places throughout the infrastructure in order to establish a baseline. Changes made to the system affect these voltage readings, which will deviate from the baseline and indicate that a change to the system was made. For facility DIV, it appears feasible that changes in configuration of the system’s grounding can be detected in real-time, and the location of the change can be inferred from the measured intensity of the change in voltage. Determination of whether or not spent fuel was present in a fuel rod, as well as the presence/absence of a fuel rod from an assembly using EPV, proved unsuccessful with the sensitivity of instrumentation used in this study.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Investigating Fission Reaction Rate Ratio Sensitivities [Abstract]

Reaction rate ratios are a measurable parameter for reactor and criticality applications. A number of foil irradiations and fission chamber measurements have been performed for critical assemblies at Los Alamos National Laboratory starting in the 1950’s including (i) Godiva, a bare HEU spherical assembly; (ii) Flattop-25, a spherical assembly consisting of an HEU core and a natural uranium reflector; (iii) Jezebel, a bare 239 Pu assembly; and (iv) Flattop-Pu, a spherical assembly consisting of a 239Pu core and a natural uranium reflector. Fission ratio data for 238 U(n,f)/ 235 U(n,f), 237 Np(n,f)/ 235 U(n,f), 233 U(n,f)/ 235 U(n,f) and 239 Pu(n,f)/ 235 U(n,f) were obtained and reported. The EUCLID (Experiments Underpinned by Computational Learning for Improvements in nuclear Data) project at Los Alamos National Laboratory (LANL) aims to constrain nuclear data by using a suite of measurement types beyond k-effective. Recent investigations include the use of pulsed spheres for nuclear data validation and other measurement methods of interest. One focus of the work is to determine if other methods are complimentary to the critical experiments utilized for nuclear data validation. It is anticipated the investigations will help inform methods that may be utilized in machine learning algorithms for nuclear validation. In order to use a measurement type for nuclear validation, it is necessary to obtain cross-section sensitivities for parameters. This work looks at reaction rate ratio sensitivities with SENSMG and Monte Carlo N-Particle R Code Version 6.21.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Accelerator-Based Studies of Heavy Ion Interactions Relevant to Space Biomedicine

Evaluation of the effects of space radiation on the crews of long duration space missions must take into account the interactions of high energy atomic nuclei in spacecraft and planetary habitat shielding and in the bodies of the astronauts. These heavy ions (i.e. heavier than hydrogen), while relatively small in number compared to the total galactic cosmic ray (GCR) charged particle flux, can produce disproportionately large effects by virtue of their high local energy deposition: a single traversal by a heavy charged particle can kill or, what may be worse, severely damage a cell. Research into the pertinent physics and biology of heavy ion interactions has consequently been assigned a high priority in a recent report by a task group of the National Research Council. Fragmentation of the incident heavy ions in shielding or in the human body will modify an initially well known radiation field and thereby complicate both spacecraft shielding design and the evaluation of potential radiation hazards. Since it is impractical to empirically test the radiation transport properties of each possible shielding material and configuration, a great deal of effort is going into the development of models of charged particle fragmentation and transport. Accurate nuclear fragmentation cross sections (probabilities), either in the form of measurements with thin targets or theoretical calculations, are needed for input to the transport models, and fluence measurements (numbers of fragments produced by interactions in thick targets) are needed both to validate the models and to test specific shielding materials and designs. Fluence data are also needed to characterize the incident radiation field in accelerator radiobiology experiments. For a number of years, nuclear fragmentation measurements at GCR-like energies have been carried out at heavy ion accelerators including the LBL Bevalac, Saturne (France), the Synchrophasotron and Nuklotron (Dubna, Russia), SIS-18 (GSI, Germany), the Alternating Gradient Synchrotron at Brookhaven National Laboratory (BNL AGS) and the Heavy Ion Medical Accelerator (HIMAC) in Chiba, Japan. Until fairly recently most of these experiments were done to investigate fundamental problems in nuclear physics, but with the increasing interest in heavy charged particles on the part of the space flight, radiobiology and radiotherapy communities, an increasing number of experiments are being directed at these areas. Some of these measurements are discussed in references therein. Over the past several years, our group has taken cross section and fluence data at the AGS and HIMAC for several incident beams with nuclear charge, Z, between 6 and 26 at energies between 290 and 1050 MeV/nucleon. Iron (Z = 26) has been studied most extensively, since it is the heaviest ion present in significant numbers in the GCR. Targets have included tissue-equivalent and proposed shielding materials, as well as a variety of elemental targets for cross section measurements. Most of the data were taken along the beam axis, but measurements have been made off-axis, as well. Here we present selected data and briefly discuss some implications for spacecraft and planetary habitat design.

Miller, J.↗

Investigation of B 11 and Ca 40 levels at 8–9 MeV by nuclear resonance fluorescence

Here, we report on the measurement of 11 B and 40 Ca levels between excitation energies of 8 and 9 MeV using nuclear resonance fluorescence (NRF). The experiment was carried out with nearly monoenergetic and linearly polarized photon beams provided by the High-Intensity γ-ray Source (HIγS) facility at the Triangle Universities Nuclear Laboratory (TUNL). States in 11 B are important for calibrations of NRF measurements, while the properties of 40 Ca levels impact potassium nucleosynthesis in globular clusters. For 40 Ca, we report on improved excitation energies and an unambiguous 2¯ assignment for the state at 8425 keV. For 11 B, we obtained improved values for γ-ray multipolarity mixing ratios and branching ratios of the 8920-keV level.

39 ≤ A ≤ 58↗

YAHFC: A Code Framework to Model Nuclear Reactions and Estimate Correlated Uncertainties

Reaction modeling is a key ingredient in designing experiments and interpreting their results, and is an essential component in the process of evaluating nuclear data and assembling nuclear data libraries used in nuclear technology applications. Typically, experimental data are available only for a handful of reaction channels and theory models are used to fill in the gaps. In addition, theory is often called upon as the arbitrator between discrepant data. Most importantly, theory and modeling are required for an accurate determination of uncertainties in the evaluated data and the correlations between the multiple channels. A fast, accurate, and flexible modeling capability has been developed at LLNL with the code system YAHFC (Yet Another Hauser-Feshbach Code). YAHFC is a Monte Carlo, Hauser-Feshbach code framework, making full use of dynamic memory allocation, derived types, and parallel computing. YAHFC can generate events to simulate experiments and is guiding experiments designed to measure inelastic neutron scattering from actinide targets. YAHFC is also being used to analyze decays from surrogate experiments, thereby enabling the inference of reaction cross sections inaccessible by direct measurement. Finally, by modeling nuclear reactions with constraints from experimental data, YAHFC can deliver complete nuclear data libraries, with evaluated uncertainties, using the modernized Generalized Nuclear Data Structure (GNDS).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Astromers in the Radioactive Decay of r-process Nuclei

Certain nuclear isomers are well known to affect nucleosynthesis with important observable consequences (e.g., 26 Al and 180 Ta). We study the impact of nuclear isomers in the context of rapid neutron capture process (r-process) nucleosynthesis. Here we demonstrate that nuclear isomers are dynamically populated in the r process and that some are populated far from thermal equilibrium; this makes them astrophysical isomers, or "astromers." We compute thermally mediated transition rates between long-lived isomers and the corresponding ground states in neutron-rich nuclei. We calculate the temperature-dependent β-decay feeding factors, which represent the fraction of material going to each of the isomer and ground state daughter species from the β-decay parent species. We simulate nucleosynthesis following the decay of a solar-like r-process composition and include as separate species nuclear excited states with measured terrestrial half-lives greater than 100 μs. We introduce a new metric to identify those astromers most likely to be influential and summarize them in a table. Notable entries include many second peak nuclei (e.g., the Te isotopic chain) and previously overlooked isomers in stable nuclei (e.g., 119 Sn, 131 Xe, and 195 Pt). Finally, we comment on the capacity of isomer production to alter radioactive heating in an r-process environment.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Absence of spin susceptibility decrease in a bulk organic superconductor with triangular lattice

The study of non-s-wave unconventional superconductivities in strongly correlated electron systems has been a central issue in condensed matter physics for more than 30 years. In such unconventional superconductivities, d-wave Cooper pairing with antiparallel spins has been often observed in various quasi-two-dimensional (quasi-2D) bulk systems. Interestingly, many theories predicted that the triangular lattice causes the d-wave pairing to be unstable and may lead to more exotic pairing such as parallel spin (spin-triplet) pairing. Here we focus on a bulk organic triangular-lattice system in which superconductivity emerges near a nonmagnetic Mott insulating phase. We demonstrate, by using low-power nuclear magnetic resonance (NMR) measurements, that the spin susceptibility of the superconducting state retains the normal state value even deep in the superconducting state. This result indicates the possibility that the material exhibits spin-triplet superconductivity. Our finding will bring insights also into understanding the 2D materials with triangular moiré superlattices that are considered also to show unconventional superconductivities near Mott-like insulating states.

36 MATERIALS SCIENCE↗

Summary of LET spectra and dose measurements on ten STS missions

A comparison of linear energy transfer (LET) spectra measurements made with plastic nuclear track detectors (PNTD's) from area passive dosimeters (APD's), was made for ten different STS missions under similar shielding. The results show that integral flux, dose rate and equivalent dose rate values follow a general increase with respect to increasing orbital inclination and altitude but that there are large variations from a simple relationship. This is to be expected since it has been shown that Shuttle attitude variations, combined with the anisotropic particle flux at the South Atlantic Anomaly (SAA), can result in differences of a factor of 2 in dose rate inside the Shuttle (Badhwar et al., 1995). Solar cycle and shielding differences also result in variations in radiation dose between STS missions. Spaceflight dosimeters from the STS missions are also being used in the development of a method for increasing LET spectra measurement accuracy by extending LET measurements to particle tracks of ranges 10-80 microns. Refinements in processing and measurement techniques for the flight PNTD's have yielded increased detection efficiencies for the short tracks when LET spectra determined by using the standard and refined methods were intercompared.

Source record↗

Use of Machine Learning for Signature Development in a Multi-Sensor Environment for Safeguard Applications of Solvent Extraction Processes

Idaho National Laboratory is constructing the Special Nuclear Material test bed (Beartooth) for research and development pertaining to nuclear fuel processing operations using centrifugal contactors. Beartooth will enable give researchers the opportunity to study the dissolution, separation, and conversion of special nuclear materials (e.g., plutonium, enriched uranium, and thorium). As a lead-in to Beartooth, this project constructed a test bed to study the process and equipment behavior with real time series data collection using a variety of non-traditional sensors, in order to identify process failures and label them as either accidental or purposeful, thus enhancing nuclear nonproliferation stewardship. The measurement sources in this test bed include vibration, acoustic, current, flow, colorimetric, and thermal data. These measurements vary in terms of magnitude, frequency, and location. This information will be combined and used within data-driven machine-learning methods to detect operation condition changes that are either intentional (i.e., changes in operating set points) or malicious (i.e., flow diversion) in nature. This presentation covers the data processing and signature development activities necessary for utilizing this heterogeneous dataset to classify process anomalies.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Connecting Activation Calculations with Gamma Spectroscopy

For many years Lawrence Livermore National Laboratory (LLNL) has used gamma spectroscopy to determine quantities of radioactive nuclides created by irradiation of stable species with neutrons and light charged particles. LLNL has also maintained activation codes and nuclear cross sections for the purpose of modeling activations under the experimental conditions, and the cross section sets used in those calculations typically include nuclear isomers. Connecting the measurements to activation calculations that include isomers is a non-trivial matter because an activation calculation must be followed by a procedure for bookkeeping of calculated isomer populations after the irradiation to simulate what radiochemists would infer about isotope populations from gamma spectroscopy performed days or weeks after the irradiation. Traditionally we have used the method of “isomer sums” for this bookkeeping. This report explains our formulation of isomer sums and application to specific cross section sets for different nuclides that were detected.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

NMR study of Ni 50+x ⁢Ti 50-x strain glasses

Here, we studied Ni 50+x ⁢Ti 50-x with compositions up to x = 2, performing 47 Ti and 49 Ti nuclear magnetic resonance (NMR) measurements from 4 to 400 K. For large x in this system, a strain glass appears in which frozen ferroelastic nanodomains replace the displacive martensite structural transition. Here, we demonstrate that NMR can provide an extremely effective probe of the strain-glass freezing process, with large changes in NMR line shape due to the effects of random strains which become motionally narrowed at high temperatures. At the same time with high-resolution x-ray diffraction we confirm the lack of structural changes in x ≥ 1.2 samples, while we show that there is little change in the electronic behavior across the strain-glass freezing temperature. NMR spin-lattice relaxation time (T 1 ) measurements provide a further measure of the dynamics of the freezing process, and indicate a predominantly thermally activated behavior both above and below the strain-glass freezing temperature. We show that the strain-glass results are consistent with a very small density of critically divergent domains undergoing a Vogel-Fulcher-type freezing process, coexisting with domains exhibiting faster dynamics and stronger pinning.

36 MATERIALS SCIENCE↗

CERBERUS: A Multi-Purpose Spectrometer and Alignment Station at SNS

In order to maximally utilize the existing beam ports at the Spallation Neutron Source, development and installation of a new neutron instrument is proposed at beam port 16a within building 8700 at Oakridge National Laboratory. Said instrument will provide nominally equal neutron beam access for three main science purposes; (1) as an alignment station for proposed single-crystal spectrometer samples to be run across the facility, (2) as a Near-Infrared (>100meV) filter analyzer spectrometer, nearly identical to that which was previously housed at the Lujan Center in Los Alamos, and (3) as a high-throughput nuclear cross-section measurement station. These three experimental applications would require no substantial technical developments, are complimentary in their technical requirements, and provide a worth-while capability that is infinitely beyond the current use of the 16a beam port at the First Target Station within the SNS complex. All three methods would enhance the facility’s science contributions, while accommodating two niche experiment methods that may not be strong enough to stand on their own.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗