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At least 667 records · Page 37

Evaluation of ASCE 4-16 and AISC 43-18 (Draft) for use in the Risk-Informed Performance-Based Seismic Design of Nuclear Power Plant Structures, Systems, and Components

This report describes the assessment of ASCE Standards 4-16 and 43-18 (Draft) for use in the Risk-Informed Performance-Based (RIPB) seismic design of structures, systems, and components (SSCs) at nuclear power plants. This work was performed for the U.S. Nuclear Regulatory Commission (NRC) Office of Regulatory Research (RES), to support potential endorsement of these industry standards for the design of nuclear power plants based on the RIPB approach. Currently, the NRC endorses a deterministic design approach for demonstrating the design adequacy of SSCs based on the Standard Review Plan (NUREG-0800) and NRC Regulatory Guides. In the RIPB approach, the design criteria are developed to achieve a target performance goal, which is defined by the annual frequency of occurrence of the design basis earthquake (i.e., Seismic Design Category) and the acceptable level of structural performance (i.e., Limit State) for the SSCs. ASCE 4-16 provides methods for performing a seismic analysis of structures to obtain the seismic response of these structures (e.g., building displacements, accelerations, in-structure response spectra) which are used in the design of the SSCs. It also provides methods for performing seismic analysis of SSCs to determine the seismic demands (e.g. member forces and displacements) needed to design individual SSCs. ASCE 43-18 (Draft) provides the criteria for the seismic design of SSCs using the seismic demands developed in ASCE 4-16. The use of ASCE Standard 43-18 (Draft), along with ASCE 4-16, provides the criteria for the seismic design of the SSCs. ASCE 43-18 (DRAFT) relies on other consensus codes and standards such as ACI 349 for reinforced concrete, AISC/N690 for steel structures, ASME Section III for pressure-retaining mechanical components and Containments, and IEEE-344 for Class 1E equipment. The goal of this technical review was to assess the adequacy of the provisions in these standards for use by the NRC in developing regulatory guidance for design of SSCs in nuclear power plants, based on the RIPB approach. The research reported herein describes the basis for acceptance of the new standards and identifies areas where additional staff guidance is needed for the seismic design of SSCs at nuclear power plants. This technical review has determined that ASCE 4-16 and ASCE 43-18 (Draft) provide an appropriate framework for the seismic design of SSCs at nuclear power plants using a Risk-Informed Performance-Based approach. However, some of the criteria therein warrant exceptions, qualifications, and/or clarifications.

42 ENGINEERING↗

End-to-End Simulations of a 3.4-Meter Detector Wall for Neutron-Diagnosed Subcritical Experiments

The Nevada National Security Site, together with Los Alamos National Laboratory and Lawrence Livermore National Laboratory, is developing a novel diagnostic to measure the reactivity of subcritical experiments. This capability is known as neutron-diagnosed subcritical experiments. The decay of the fission gamma rays from the neutron-interrogated subcritical experiment is measured as a function of time with a large (~3-meter diameter) detector wall consisting of 151 individual detector pixels. The data from this current mode measurement inform the neutron multiplication factor, keff, and thus the relative reactivity of the subcritical experiment. The Nevada National Security Site developed the Gamma Array Simulation Toolkit initially to help inform the design of the individual detector pixels and the 3.4-meter diameter detector wall to be fielded as part of neutron-diagnosed subcritical experiments. This toolkit is now being used to simulate and predict the performance of the final design of the individual detector pixels and the aggregate detector wall. Key detector characteristics evaluated from these simulations include impulse response, pulse height spectrum, number of photoelectrons per MeV, detector efficiency, and cross talk between detector pixels. Collectively, the results of these simulations inform how well the fission gamma ray die-off distribution from a neutron-diagnosed subcritical experiment measurement can be resolved. This is critical to determining the relative reactivity of the experiment. Furthermore, the Gamma Array Simulation Toolkit can be used to aid in the analysis of the experimental data from a neutrondiagnosed subcritical experiment measurement once the simulation has been benchmarked.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

End-to-End Simulations of a 3.4-Meter Detector Wall for Neutron-Diagnosed Subcritical Experiments

The Nevada National Security Site, together with Los Alamos National Laboratory and Lawrence Livermore National Laboratory, is developing a novel diagnostic to measure the reactivity of subcritical experiments. This capability is known as neutron-diagnosed subcritical experiments. The decay of the fission gamma rays from the neutron-interrogated subcritical experiment is measured as a function of time with a large (~3-meter diameter) detector wall consisting of 151 individual detector pixels. The data from this current mode measurement inform the neutron multiplication factor, keff, and thus the relative reactivity of the subcritical experiment. The Nevada National Security Site developed the Gamma Array Simulation Toolkit initially to help inform the design of the individual detector pixels and the 3.4-meter diameter detector wall to be fielded as part of neutron-diagnosed subcritical experiments. This toolkit is now being used to simulate and predict the performance of the final design of the individual detector pixels and the aggregate detector wall. Key detector characteristics evaluated from these simulations include impulse response, pulse height spectrum, number of photoelectrons per MeV, detector efficiency, and cross talk between detector pixels. Collectively, the results of these simulations inform how well the fission gamma ray die-off distribution from a neutron-diagnosed subcritical experiment measurement can be resolved. This is critical to determining the relative reactivity of the experiment. Furthermore, the Gamma Array Simulation Toolkit can be used to aid in the analysis of the experimental data from a neutron-diagnosed subcritical experiment measurement once the simulation has been benchmarked.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

ASNF Dry Storage Pilot with HFIR Fuel: Concept Plan

The U.S. Department of Energy (DOE) currently manages a large inventory of aluminum-clad spent nuclear fuel (ASNF) from U.S. High Performance Research Reactors and also some fuel from foreign research reactors. A transition to new dry storage configurations is desired to facilitate decisions related to potential storage of future ASNF and transitioning current ASNF out of aging storage facilities. DOE has developed designs for a set of DOE Standard Canisters (DSCs) to provide sealed, road-ready dry storage suitable for interim storage, transportation, and potentially disposition in a future repository. Extensive experiments and modeling activities have been carried out to develop the technical basis for such storage, with results to date indicating this storage approach should be safe and viable following suitable drying processes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Impulse response measurements of fast scintillator-based current mode detectors

In this study, experimental measurements were performed to characterize the impulse response of seven different gamma ray detector prototypes being considered to be fielded as a current mode diagnostic for neutron-diagnosed subcritical experiments at the Nevada National Security Site (NNSS). For such experiments, the impulse response of the fielded detector is required to have a full-width half-maximum (FWHM) of approximately 5 ns or less and a low amplitude tail. Each of the detector prototypes evaluated in this work were selected based on the potential to meet this performance requirement. An impulse of bremsstrahlung x-rays created from 2 MeV electrons from the NNSS’s Transformational Diagnostics and Imaging, Los Alamos, linear accelerator was measured with each detector. The measured impulse response was evaluated for each detector configuration. A comparison of these impulse responses revealed a relationship between fast timing performance and scintillator material, geometry, surface reflectivity conditions, and photomultiplier tube (PMT) selection. The detector configuration yielding an impulse response with the shortest FWHM of 3.82 ± 0.11 ns and possessing a low amplitude tail was a 5-inch (12.7-cm) diameter, 5-inch (12.7-cm) height cylindrical EJ-399-17-VI liquid scintillator in a black-painted housing coupled to an Adit D798B 5-inch (12.7-cm) PMT by means of a 0.079-inch (0.2-cm) EJ-560 optical coupling pad.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

5G Communications in Nuclear: Potential Use Cases and Security Considerations

As fifth-generation (5G) communications continues to revolutionize the future of wireless technology, there is growing demand to utilize its benefits for critical infrastructures such as nuclear power plants (NPPs). In regard to achieving full automation and control in the operation of existing and future nuclear reactors, the unique capabilities of 5G can bring several potential advantages over other wireless technologies. However, a deep investigation is needed for the availability and security of 5G communications under various NPP operational scenarios. This article examines how 5G security capabilities can be architecturally deployed in nuclear applications so as to replace existing communication infrastructures. We discuss the current use of all wireless technologies in NPPs with their key features. Consequently, we investigated several NPP use cases in which 5G offers potential advantages but entails specific security considerations. The present article covers the characteristics of 5G communications, general challenges to its application in nuclear, and the security gaps that need to be addressed. We also highlight certain 5G security-by-design features that can help addressing current stringent NPP requirements. In addition, we discuss some future research direction that can facilitate the implementation of 5G in a nuclear facility. The findings presented herein can help foster 5G deployment in NPPs, thus enabling secured data transmission, cost savings, and increased operational efficiency with enhanced reliability.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Safety and Regulatory Research R&D [Slides]

Included are slides for a MIT nuclear engineering department invited seminar. The talking points are: (1) Current R&D at INL in safety, risk, and reliability; (2) Technical focus; and (3) Future directions.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

High Radiation Resistance in the Binary W‐Ta System Through Small V Additions: A New Paradigm for Nuclear Fusion Materials

Abstract Refractory High‐Entropy Alloys (RHEAs) are promising candidates for structural materials in nuclear fusion reactors, where W‐based alloys are currently leading. Fusion materials must withstand extreme conditions, including i) severe radiation damage from energetic neutrons, ii) embrittlement due to H and He ion implantation, and iii) exposure to high temperatures and thermal gradients. Recent RHEAs, such as WTaCrV and WTaCrVHf, have shown superior radiation tolerance and microstructural stability compared to pure W, but their multi‐element compositions complicate bulk fabrication and limit practical use. In this study, it is demonstrated that reducing alloying elements in RHEAs is feasible without compromising radiation tolerance. Herein, two Highly Concentrated Refractory Alloys (HCRAs) − W 53 Ta 44 V 3 and W 53 Ta 42 V 5 (at.%) − were synthesized and investigated. We found that small V additions significantly influence the radiation response of the binary W–Ta system. Experimental results, supported by ab‐initio Monte Carlo simulations and machine‐learning‐driven molecular dynamics, reveal that minor variations in V content enhance Ta–V chemical short‐range order (CSRO), improving radiation resistance in the W 53 Ta 42 V 5 HCRA. By focusing on reducing chemical complexity and the number of alloying elements, the conventional high‐entropy alloy paradigm is challenged, suggesting a new approach to designing simplified multi‐component alloys with refractory properties for thermonuclear fusion applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Decontamination of urban surfaces contaminated with radioactive materials and consequent onsite recycling of the waste water

Enhancing rapid remediation strategies is paramount for recovery after a large-scale nuclear contamination event in an urban environment. Some current strategies recommend use of readily available equipment, materials, and facilities to expedite recovery. For example, applying pressurized water to contaminated surfaces may effectively remove radioactive contamination. In this study, a commercial power washer removes soluble forms of 152 Eu 3 + , 85 Sr 2 + , and 137 Cs + contamination from common porous building materials, and computer simulations characterize the recycling of the resultant contaminated wash water. Pressure washing the porous building materials under spray conditions typical with do-it-yourself units improved decontamination factors (DFs) for 152 Eu compared to low-pressure application of tap water (majority of two-tailed t-test p-values < 0.1), but pressure did not improve DFs for 137 Cs or 85 Sr. For both pressurized and low-pressure applications, adding potassium ions (K + ) to promote ion exchange reactions produced significantly higher DFs for tested radionuclides on asphalt, brick, and concrete. The resultant contaminated wash water can be processed through self-prepared chemical filtration beds of clay and sand. Modeled in a prior study, the beds yielded linear trends (R 2 > 0.98) in sensitivity analyses between most bed configuration variables and bed performance variables, permitting flexible ad-hoc bed design. The experimental and simulation results led to estimates of the remediation rate and waste generated after cleaning 250 m 2 of cesium-contaminated concrete from the combined deployment of a power washer and two different mobile treatment beds. Furthermore, the first treatment bed was designed to reduce treatment time and processed 1900 L of wash solution in 70 min using 880 kg of clay/sand infill material. Designed to reduce the solid waste generated, the second bed processed the same solution volume in 1040 min (17 h) using 170 kg of clay/sand infill material. The results of this analysis warrant further investigation of power washing with recycled salt solution as an effective rapid decontamination method with manageable waste.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

The current status of inelastic and capture Gamma-ray production evaluations in translated ENDF-VIII.0 GNDS files and recommended remediation actions

This report provides the status of discrete nuclear levels and inelastic gamma-ray production for neutron induced reactions in current ENDF-VIII.0 evaluations for the isotopes in the GRIN project. Different categories of issues are identified after a comparison with information from “adopted” ENSDF files. Improvement strategies are given and recommendations are described. We have included a similar, but more limited, analysis for thermal capture data where EGAF and ENSDF thermal libraries are considered. In addition, we provide a validation plan to employ different transport code simulations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Part 1: Nuclear Mis- and Disinformation and Impacts to the American Public

Russia’s nuclear saber rattling throughout the war in Ukraine, reports of China’s increasing nuclear modernization, and the 2023 release of Oppenheimer has reignited in the public talk of nuclear weapons. With the increasing prevalence of conversation around nuclear weapons comes increasing opportunity for mis- or disinformation to spread about them and the nuclear enterprise (NE). Mis- and disinformation are not new phenomena. However, the speed and reach offered by current digital communications technology is novel. What are the impacts of misinformation or disinformation about nuclear weapons to the American public?

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

The influence of nitrogen and nitrides on the structure and properties of proton irradiated ferritic/martensitic steel

The 12Cr1MoWV (wt%) ferritic/martensitic steel HT9 is a candidate material for fuel cladding in advanced nuclear reactors, such as the Versatile Test Reactor currently under development. As such, understanding the relationship between microstructure and mechanical properties in the context of irradiation environments for these steels is critical. N content, and more specifically interstitial N, has been hypothesized to be detrimental to irradiated properties at lower temperatures (less than 0.3T m ) to a total of 6 dpa; however, in this work at a dose of 1 dpa the irradiated microstructure was improved with added N, leading to less irradiation hardening. Three variants of HT9 were irradiated with 1.5 MeV protons to a dose of 1 dpa at 300°C. The HT9 variants included Low (10 ppm), Mid (190 ppm), and High (440 ppm) N alloys that were otherwise nearly identical. Changing the N content had a variety of effects on the irradiated defect structures. As N content increased, the average dislocation loop diameter decreased, while the number density of loops increased. Additionally, extensive Ni clustering was observed on dislocations and interfaces. The Mid and High N specimens exhibited significantly less hardening (ΔHV≃100) relative to the Low N specimen (ΔHV≃160). The decrease in hardening is attributed to vanadium carbonitride acting as a sink for Ni clusters that would otherwise form on dislocations. Under the irradiation conditions used, these results suggest increasing the N content in HT9 may have a desirable effect on the irradiated structure and properties at the dose studied, as well as the swelling resistance at higher doses. In other words, N content appears to be a powerful tool for tailoring the self-interstitial atom cluster mobility in F/M steels for different temperature and dose applications.

36 MATERIALS SCIENCE↗

On the physics potential to study the gluon content of proton and deuteron at NICA SPD

The Spin Physics Detector (SPD) is a future multipurpose experiment foreseen to run at the NICA collider, which is currently under construction at the Joint Institute for Nuclear Research (JINR, Dubna, Russia). The physics program of the experiment is based on collisions of longitudinally and transversely polarized protons and deuterons at √s up to 27 GeV and luminosity up to 10 32 cm –2 s –1 . SPD will operate as a universal facility for the comprehensive study of the unpolarized and polarized gluon content of the nucleon, using complementary probes such as: charmonia, open-charm, and prompt-photon production processes. Furthermore, the aim of this work is to provide a thorough review of the physics objectives that can potentially be addressed at SPD, underlining related theoretical aspects and discussing relevant experimental results when available. Among different pertinent phenomena particular attention is drawn to the study of the gluon helicity, gluon Sivers and Boer-Mulders functions in the nucleon, as well as the gluon transversity distribution in the deuteron, via the measurement of single and double spin asymmetries.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Tolerance of Perovskite Solar Cells to Targeted Proton Irradiation and Electronic Ionization Induced Healing

Mixed organic–inorganic halide perovskite solar cells (PSCs) are of interest for space photovoltaic applications due to their apparent tolerance to high-energy proton radiation. Here, the use of a more stable wide-bandgap FA0.8Cs0.2PbI2.4Br0.6Cl0.02 perovskite with thin encapsulation enables, for the first time, the detailed dependence of fluence and energy of energetic protons on device performance. Energies were chosen to provide the highest concentration of displacements within the active region, and therefore the highest amount of degradation. Not only are these devices tolerant when compared to conventional technologies, but an unexpected increase in open circuit voltage and power density is observed for increased electronic ionization when the proton energy is increased. This study aims to expand the description of the proton radiation tolerance to include not only nonionizing nuclear energy losses that are most detrimental to current technologies, but electronic ionization, which is shown to yield benefits in PSCs.

device performance↗

First identification of resonant states in the {sup 45}V(p, {gamma}){sup 46}Cr reaction and their influence on the production of {sup 44}Ti in Core Collapse Supernovae

The observation of active 44Ti in supernova remnants offers the potential to solve one of the most debated questions in modern astrophysics, the exact underlying explosion mechanism of core collapse supernovae (CCSNe). In particular, a comparison between the predicted synthesized yield of 44Ti and the ejected flux is expected to allow for a determination of the mass cut of the star. Unfortunately, such comparisons are currently severely hindered by large uncertainties in the nuclear reactions governing the production and destruction of 44Ti. On this note, the astrophysical 45Vðp; γÞ46Cr reaction is expected to play a decisive role. We present the first experimental information on resonant states in the 45Vðp; γÞ46Cr reaction. Excitation energies have been measured with high precision for ten previously unknown, low-spin, proton-unbound states in 46Cr, and spin-parity-assignment constraints have been made using observed γ-decay patterns and shell-model calculations. We find that an l ¼ 1 resonance at 714 keV dominates the 45Vðp; γÞ46Cr reaction for the entire temperature range of α-rich freezeout. Moreover, the nominal rate is found to be ∼25–50% of previous estimates for T > 1.2 GK, indicating an increase in 44Ti production in CCSNe of ∼20–35%.

Cousins, C↗

Measurement and modeling of proton-induced reactions on arsenic from 35 to 200 MeV

72 As is a promising positron emitter for diagnostic imaging that can be employed locally using a 72 Se generator. However, current reaction pathways to 72 Se have insufficient nuclear data for efficient production using regional 100–200 MeV high-intensity proton accelerators. In order to address this deficiency, stacked-target irradiations were performed at LBNL, LANL, and BNL to measure the production of the 72 Se/ 72 As positron emission tomography (PET) generator system via 75 As (p, x) between 35 and 200 MeV. This work provides the most well-characterized excitation function for 75 As ( p , 4 n ) 72 Se starting from threshold. Additional focus was given to report the first measurements of 75 As (p, x) 68 Ge and bolster an already robust production capability for the highly valuable 68 Ge/ 68 Ga PET generator. Thick target yield comparisons with prior established formation routes to both generators are made. In total, high-energy proton-induced cross sections are reported for 55 measured residual products from 75 As, nat Cu , and nat Ti targets, where the latter two materials were present as monitor foils. These results were compared with literature data as well as the default theoretical calculations of the nuclear model codes TALYS, COH, EMPIRE, and ALICE. Reaction modeling at these energies is typically unsatisfactory due to few prior published data and many interacting physics models. Therefore, a detailed assessment of the talys code was performed with simultaneous parameter adjustments applied according to a standardized procedure. Particular attention was paid to the formulation of the two-component exciton model in the transition between the compound and preequilibrium regions, with a linked investigation of level density models for nuclei off of stability and their impact on modeling predictive power. This paper merges experimental work and evaluation techniques for high-energy charged-particle isotope production in an extension to an earlier study of this kind.

43 PARTICLE ACCELERATORS↗

Influence of Nanoconfinement and Elevated Temperatures on Geocolloid-Facilitated Transport of Energy related Contaminants

Fossil fuels obtained using hydraulic fracturing and nuclear energy are deemed crucial for meeting the current and future energy demands of the United States. The utilization of these resources, especially fossil fuels from hydraulic fracturing, has increased rapidly within the last decade. However, with the increasing levels of hydraulic fracturing activities, the occurrence and fate of chemicals used in these processes in the geosystem, as well as the potential consequences of their interactions with environment and geosystems (e.g. mineral-based geocolloids and geosurfaces), have been increasingly recognized as issues warranting consideration owing to the toxic nature of these chemicals. Scientific results originated from this project has brought better understandings on how such contaminants can preferentially or adversely interact with geosystems and how geocolloids can facilitate their transport by realistically mimicking geological conditions and environments in the laboratory level for the first time. Based on such knowledge, it may eventually lead to the development of mitigation strategies for reducing and minimizing the transport and wide distribution of contaminants and pollutants. This aspect is important for the society to ensure that energy-related contaminants do not find their way to waterbodies that are used as drinking water or irrigation. The project is also anticipated to increase public awareness about potential adverse effects of energy systems on the geosphere and environment and may motivate society to consider better mitigation strategies to prevent such occurrences.

(Nano)Confinement↗

Routine Beryllium-10 analysis from post-detonation debris and geologic materials [Slides]

Beryllium (Be) isotope measurements provide insight into weapon design, yield, etc. Sample preparation nor measurement capability currently existed at LANL. Potential capability directly benefits nuclear forensics venture. PI Goehring has nearly 20 years of Be chemistry experience, including method implementation with difficult samples.

07 ISOTOPE AND RADIATION SOURCES↗