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NASA NTRS1995

Nearly sonic and transsonic convective motions in the solar atmosphere related to the solar wind origin

MHD equations are considered for the solar atmosphere. 15 different simplest MHD regimes are indicated for the momentum transport equation depending on the mutual binary interplay between 6 possible and locally dominant terms: non-stationarity and inhomogeneity of the flow, gas pressure, magnetic tensions, viscous and gravity forces. These regimes are delimited by five physically independent dimensionless parameters, for example, Strouhal, sonic Mach, alfvenic Mach, Reynolds and Froude numbers or their combinations. Another partially overlapping classification of the simplest regimes may be introduced based on the energy conservation equation. There are also 15 independent binary combinations between nonstationary and inhomogeneous convective terms, dissipative energy sinks and sources (viscous, heat-conductive, Joule and radiative ones) in the energy equation. More complicated regimes are considered with multiple dominated terms. All these MHD regimes play their important role somewhere in the solar atmosphere complicated by the tensor transport coefficients in the magnetically dominated regions of the upper atmosphere. Nearly sonic and transsonic nonstationary convective motions with ascending and descending flows are observed in the solar chromosphere. the transition region and the lower pans of the solar corona together with related horizontal velocity components. This convection represents a kind of the 'cocoonery' manufacturing nonstationary vortices generated here and partially connected to the photosphere and to the solar wind. The solar wind originates from this powerful transsonic muddle in the solar atmosphere as a tiny fraction of the streamlines which are temporarily getting detached from the 'cocoons; and going to the infinity. The topologically complicated instantaneous 'runaway surface' around the Sun, i.e., the surface which separates outgoing to the infinity streams from other finite flows in the solar atmosphere was not described in the literature and needs additional investigation. We conclude that a simple one-connected smooth and quasistationary 'critical surface' which is often supposed to be placed somewhere in the solar corona (say, at 4 solar radii) in reality does not exist. Observational and theoretical arguments favor instead of this a highly structured, disordered, patched and time-dependent sonic transition surface in the solar atmosphere permanently fluctuating at positional dependent heights starting sometimes from photospheric (and maybe subphotospheric) levels and more frequently from the chromosphenc network up to several solar radii in the solar corona.

Veselovsky, I. S.↗

DOE OSTI2023

Size-Resolved Elemental Composition of Respiratory Particles in Three Healthy Subjects

The chemical composition of respiratory particles is of interest because the viability of any viruses and bacteria in the particles has been shown to depend on this factor. Here, using computer controlled scanning electron microscopy/energy dispersive X-ray spectroscopy (CCSEM/EDX), we analyzed the size-resolved chemical composition of greater than 35,000 individual respiratory particles collected from three healthy human subjects, quantitatively at nanometer-scale spatial resolution. The desiccated particles ranged in size from 0.05 to 4.4 μm, and the mode of the size distribution was approximately 0.1 μm. Particles were heterogeneous in composition, with approximately 42% of them containing a carbon atomic percentage greater than 95% and approximately 53% of them containing a Na + P + K + Cl percentage greater than 5%. Based on the particles’ elemental composition, we classified them into five categories: 48%–56% of the total number were carbonaceous, mostly organic; 40%–50% Na-rich salt; 0.3%–0.5% P-rich salt; 0.1–0.8% K-rich salt; and 1%–2.5% mixed salt. The number ratio of Na-rich salt particles to carbonaceous particles increased with increasing particle size; particles larger than approximately 2 μm were dominated by Na-rich salt. Size-dependent differences in the chemical composition of respiratory particles may have important implications for the efficiency of airborne transmission of respiratory pathogens.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2020

Flue Gas CO 2 Capture via Electrochemically Mediated Amine Regeneration: Desorption Unit Design and Analysis

We analyzed the performance of an electrochemical desorption unit to be implemented in an electrochemically mediated amine regeneration (EMAR) process, which separates CO 2 and regenerates the amine upon modulation of a targeted species that complexes with the amine molecules. Using a simplified one-dimensional boundary layer model, we combined the kinetic expressions of the faradaic reactions with mass transfer effects to analyze the polarization behavior of the flow cell. Mass transfer limitations become dominant at high current densities, leading to increases in energy consumption. An understanding of scaling laws with key parameters, such as the Sherwood number, is required to achieve high power operation with minimal mass transfer losses. Because the EMAR chemistry is sensitive to temperature, heat distribution in the unit is also examined. Our results indicate that the desorption performance increases with addition of a high-temperature heat source. Additionally, incorporation of membrane crossover suggests energy losses because of diffusion and migration of active species. Furthermore, these findings inform on scaling laws for at-scale desorber design and provide a model for scaling up the EMAR system for larger scale operations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2023

Ageing and quenching through the ageing diagram: predictions from simulations and observational constraints

We study recent changes on the star-formation history (SFH) of galaxies by means of the ageing diagram (AD), tracing the fraction of stars formed during the last ∼20 Myr through the equivalent width of the Hα line and ∼1−3 Gyr through the dust-corrected optical colour ( g − r ) 0 or the Balmer break. We provide a physical characterization by using Pipe3Destimates of the SFH of Calar Alto Legacy Integral Field Area and Mapping Nearby Galaxies at Apache Point Observatory galaxies, in combination with the predictions from IllustrisTNG-100. Our results show that the AD may be divided into four domains that correlate with the stellar mass fractions formed in the last 20 Myr and 3 Gyr: ageing systems, whose star formation rate changes on scales of several Gyr, account for 70-80 per cent of the galaxy population. Objects whose SFH was abruptly truncated in the last ∼1 Gyr arrange along a detached quenched sequence that represents ∼5 - 10 per cent by (volume-corrected) number for 10 9 < M * /M ⊙ < 10 12 . Undetermined systems represent an intermediate population between the ageing and quenched regimes. Finally, Retired galaxies, dominated by old stellar populations, are located at the region in the AD where the ageing and quenched sequences converge. Defining different star formation activity levels in terms of the birth rate parameter $b\equiv \frac{SFR}{\langle SFR \rangle }$, we find that galaxies transit from the ageing to quenched sequences on scales ∼500 Myr. We conclude that the AD provides a useful tool to discern recently quenched galaxies from the dominant ageing population.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2021

Dislocation content of grain boundary phase junctions and its relation to grain boundary excess properties

In this work, we analyze the dislocation content of grain boundary (GB) phase junctions, i.e., line defects separating two different GB phases coexisting on the same GB plane. While regular GB disconnections have been characterized for a variety of interfaces, GB phase junctions formed by GBs with different structures and different numbers of excess atoms have not been previously studied. We apply a general Burgers circuit analysis to calculate the Burgers vectors b of junctions in two Σ5 Cu boundaries previously simulated with molecular dynamics. The Burgers vectors of these junctions cannot be described by the displacement shift complete (DSC) lattice alone. We show that, in general, the normal component of b is not equal to the difference in the GB excess volumes but contains another contribution from the numbers of GB atoms per unit area ΔN* required to transform one GB phase into another. In the boundaries studied, the latter component dominates and even changes the sign of b. We derive expressions for the normal and tangential components of b in terms of the DSC lattice vectors and the non-DSC part due to ΔN* and additional GB excess properties, including excess volume and shears. These expressions provide a connection between GB phase transformations driven by the GB free energy difference and the motion of GB junctions under applied normal and shear stresses. The proposed analysis quantifies b and therefore makes it possible to calculate the elastic part of the energy of these defects, evaluate their contribution to the nucleation barrier during GB phase transformations, and treat elastic interactions with other defects.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2022

Effect of Coaxial Electrode Geometry on the Electric Field Enhancement Factor for a High Voltage Vacuum Gap

We present an experimental analysis of the change in the electric field enhancement factor with varying gap size and penetration depth (P.D) of cathode into anode for a coaxial vacuum gap, diagnosed using Fowler–Nordheim analysis and optical imaging via scanning electron microscope (SEM) and time integrated Digital single lens reflex camera (DSLR). Data were collected on the Coaxial Gap Breakdown Machine (240 A, 25 kV, 150 ns, 0.1 Hz). Experiments using five different gap sizes at nine different P.Ds are compared over runs comprising 50 shots for each case. The results show a strong link between enhancement factor and gap size, with P.D and surface topology. For large gap sizes, 150, 330, and 700 μm, the average enhancement factor value increases with increasing P.D. For smaller gap sizes, 50 and 100 μm, the average enhancement factor decreases with P.D. SEM imaging before and after plasma formation for each gap size allows for quantifying surface finish, microprotrusion growth, average blast diameter, and an estimation of the surface area breakdowns occupy. Time integrated DSLR imaging analysis of the gap at each shot allows for a determination of the distribution of breakdowns about the circumference of the gap for each case tested. Here, the Fowler–Nordheim analysis allows for a quantitative analysis of the surface roughness of all gap sizes tested. Results show that for large gap sizes, the gap geometry and increasing area of breakdown is the main cause for increasing average enhancement factor. For small gap sizes, the dominant driving factor for small average enhancement factors—that subsequently decrease with P.D—is significant changes in surface topology due to an increased number of breakdowns.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2021

Aircraft measurements of aerosol and trace gas chemistry in the eastern North Atlantic

The Aerosol and Cloud Experiment in the Eastern North Atlantic (ACE-ENA) investigated properties of aerosols and subtropical marine boundary layer (MBL) clouds. Low subtropical marine clouds can have a large effect on Earth's radiative budget, but they are poorly represented in global climate models. In order to understand their radiative effects, it is imperative to understand the composition and sources of the MBL cloud condensation nuclei (CCN). The campaign consisted of two intensive operation periods (IOPs) (June–July 2017 and January–February 2018) during which an instrumented G-1 aircraft was deployed from Lajes Field on Terceira Island in the Azores, Portugal. The G-1 conducted research flights in the vicinity of the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic (ENA) atmospheric observatory on Graciosa Island. An Aerodyne high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) and Ionicon proton-transfer-reaction mass spectrometer (PTR-MS) were deployed aboard the aircraft, characterizing chemistry of non-refractory aerosol and trace gases, respectively. The eastern North Atlantic region was found to be very clean, with an average non-refractory submicrometer aerosol mass loading of 0.6 µg m −3 in the summer and 0.1 µg m −3 in the winter, measured by the AMS. Average concentrations of the trace reactive gases methanol and acetone were 1–2 ppb; benzene, toluene and isoprene were even lower, <1 ppb. Mass fractions of sulfate, organics, ammonium and nitrate in the boundary layer were 69 %, 23 %, 7 % and 1 % and remained largely similar between seasons. The aerosol chemical composition was dominated by sulfate and highly processed organics. Particulate methanesulfonic acid (MSA), a well-known secondary biogenic marine species, was detected, with an average boundary layer concentration of 0.021 µg m −3 , along with its gas-phase precursor, dimethyl sulfide (DMS). MSA accounted for no more than 3 % of the submicron, non-refractory aerosol in the boundary layer. Examination of vertical profiles of aerosol and gas chemistry during ACE-ENA reveals an interplay of local marine emissions and long-range-transported aged aerosol. A case of transport of biomass burning emissions from North American fires has been identified using back-trajectory analysis. In the summer, the non-refractory portion of the background CCN budget was heavily influenced by aerosol associated with ocean productivity, in particular sulfate formed from DMS oxidation. Episodic transport from the continents, particularly of biomass burning aerosol, periodically increased CCN concentrations in the free troposphere. In the winter, with ocean productivity lower, CCN concentrations were overall much lower and dominated by remote transport. These results show that anthropogenic emissions perturb CCN concentrations in remote regions that are sensitive to changes in CCN number and illustrate that accurate predictions of both transport and regional aerosol formation from the oceans are critical to accurately modeling clouds in these regions.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1972

Lee-side vortices on delta wings at hypersonic speeds.

A fluid-dynamic investigation was carried out to determine the cause of intense heating observed on the lee meridian of hypersonic delta wings and also to derive means for its suppression. Several experimental techniques were combined with analysis of extensive heat-transfer measurements at a freestream Mach number of six in a range of Reynolds number to acquire a general description of the lee-flow structure. With attached leading-edge flow on the delta wings, the dominant feature is a pair of embedded vortices on the lee meridian whose interaction with the boundary-layer is responsible for the observed local heating. On the basis of flow visualization results and heat-transfer correlations, a qualitative vortex flow model is proposed which differs essentially from the conventional inboard separation vortex model.

Rao, D. M.↗

NASA NTRS1981

Some anomalies between wind tunnel and flight transition results

A review of environmental disturbance influence and boundary layer transition measurements on a large collection of reference sharp cone tests in wind tunnels and of recent transonic-supersonic cone flight results have previously demonstrated the dominance of free-stream disturbance level on the transition process from the beginning to end. Variation of the ratio of transition Reynolds number at onset-to-end with Mach number has been shown to be consistently different between flight and wind tunnels. Previous correlations of the end of transition with disturbance level give good results for flight and large number of tunnels, however, anomalies occur for similar correlation based on transition onset. Present cone results with a tunnel sonic throat reduced the disturbance level by an order of magnitude with transition values comparable to flight.

Harvey, W. D.↗

NASA NTRS1988

New insights in the numerical reliability properties of existing Kalman filter implementations

The convergence properties of Kalman filter algorithms are investigated analytically. A theoretical error analysis is performed on four types of algorithms, as defined by Anderson and Moore (1979): (1) a conventional Kalman filter, (2) a square-root (SR) covariance filter, (3) the Chandrasekhar SR filter, and (4) an SR information filter. The derivations are given in detail, and numerical results for the flight-path reconstruction problem studied by Verhaegen (1987) are presented in tables and graphs. It is shown that error propagation in algorithms (1) and (2) is sensitive to the condition number of the innovation-signal covariance matrix and the spectral norm of the filter state-transition matrix, whereas other parameters are dominant in (3) and (4). Filter (2) is found to be the most reliable for the class of problems studied.

Verhaegen, M. H.↗

NASA NTRS1990

Modern developments in shear flow control with swirl

Passive and active control of swirling turbulent jets is experimentally investigated. Initial swirl distribution is shown to dominate the free jet evolution in the passive mode. Vortex breakdown, a manifestation of high intensity swirl, was achieved at below critical swirl number (S = 0.48) by reducing the vortex core diameter. The response of a swirling turbulent jet to single frequency, plane wave acoustic excitation was shown to depend strongly on the swirl number, excitation Strouhal number, amplitude of the excitation wave, and core turbulence in a low speed cold jet. A 10 percent reduction of the mean centerline velocity at x/D = 9.0 (and a corresponding increase in the shear layer momentum thickness) was achieved by large amplitude internal plane wave acoustic excitation. Helical instability waves of negative azimuthal wave numbers exhibit larger amplification rates than the plane waves in swirling free jets, according to hydrodynamic stability theory. Consequently, an active swirling shear layer control is proposed to include the generation of helical instability waves of arbitrary helicity and the promotion of modal interaction, through multifrequency forcing.

Farokhi, Saeed↗

NASA NTRS1990

Modern developments in shear flow control with swirl

Farokhi, S.↗

NASA NTRS1992

Infrared weak quasars

Examples of quasars with anomalously weak IR emission are presented, and the effects of starlight subtraction on estimates of the UV and IR component strengths are discussed. Inferred model parameters are very sensitive to the position of the peak of the UV energy distribution. In many low redshift objects the peak is not seen; even in those objects where the turnover is clear, the turnover may not be intrinsic but instead due to reddening within the quasar host galaxy. The small number of unusual quasars with weak IR emission will be of utility as a probe of the quasar phenomenon in the absence of dominant dust reprocessing.

Mcdowell, J. C.↗

NASA NTRS2003

Cool Flames in Propane-Oxygen Premixtures at Low and Intermediate Temperatures at Reduced-Gravity

The Cool Flame Experiment aims to address the role of diffusive transport on the structure and the stability of gas-phase, non-isothermal, hydrocarbon oxidation reactions, cool flames and auto-ignition fronts in an unstirred, static reactor. These reactions cannot be studied on Earth where natural convection due to self-heating during the course of slow reaction dominates diffusive transport and produces spatio-temporal variations in the thermal and thus species concentration profiles. On Earth, reactions with associated Rayleigh numbers (Ra) less than the critical Ra for onset of convection (Ra(sub cr) approx. 600) cannot be achieved in laboratory-scale vessels for conditions representative of nearly all low-temperature reactions. In fact, the Ra at 1g ranges from 10(exp 4) - 10(exp 5) (or larger), while at reduced-gravity, these values can be reduced two to six orders of magnitude (below Ra(sub cr)), depending on the reduced-gravity test facility. Currently, laboratory (1g) and NASA s KC-135 reduced-gravity (g) aircraft studies are being conducted in parallel with the development of a detailed chemical kinetic model that includes thermal and species diffusion. Select experiments have also been conducted at partial gravity (Martian, 0.3gearth) aboard the KC-135 aircraft. This paper discusses these preliminary results for propane-oxygen premixtures in the low to intermediate temperature range (310- 350 C) at reduced-gravity.

Pearlman, Howard↗

NASA NTRS2016

Phased Acoustic Array Measurements of a 5.75 Percent Hybrid Wing Body Aircraft

Detailed acoustic measurements of the noise from the leading-edge Krueger flap of a 5.75 percent Hybrid Wing Body (HWB) aircraft model were recently acquired with a traversing phased microphone array in the AEDC NFAC (Arnold Engineering Development Complex, National Full Scale Aerodynamics Complex) 40- by 80-Foot Wind Tunnel at NASA Ames Research Center. The spatial resolution of the array was sufficient to distinguish between individual support brackets over the full-scale frequency range of 100 to 2875 Hertz. For conditions representative of landing and take-off configuration, the noise from the brackets dominated other sources near the leading edge. Inclusion of flight-like brackets for select conditions highlights the importance of including the correct number of leading-edge high-lift device brackets with sufficient scale and fidelity. These measurements will support the development of new predictive models.

Krueger noise↗

NASA NTRS2012

Stability Analysis for HIFiRE Experiments

The HIFiRE-1 flight experiment provided a valuable database pertaining to boundary layer transition over a 7-degree half-angle, circular cone model from supersonic to hypersonic Mach numbers, and a range of Reynolds numbers and angles of attack. This paper reports selected findings from the ongoing computational analysis of the measured in-flight transition behavior. Transition during the ascent phase at nearly zero degree angle of attack is dominated by second mode instabilities except in the vicinity of the cone meridian where a roughness element was placed midway along the length of the cone. The growth of first mode instabilities is found to be weak at all trajectory points analyzed from the ascent phase. For times less than approximately 18.5 seconds into the flight, the peak amplification ratio for second mode disturbances is sufficiently small because of the lower Mach numbers at earlier times, so that the transition behavior inferred from the measurements is attributed to an unknown physical mechanism, potentially related to step discontinuities in surface height near the locations of a change in the surface material. Based on the time histories of temperature and/or heat flux at transducer locations within the aft portion of the cone, the onset of transition correlated with a linear N-factor, based on parabolized stability equations, of approximately 13.5. Due to the large angles of attack during the re-entry phase, crossflow instability may play a significant role in transition. Computations also indicate the presence of pronounced crossflow separation over a significant portion of the trajectory segment that is relevant to transition analysis. The transition behavior during this re-entry segment of HIFiRE-1 flight shares some common features with the predicted transition front along the elliptic cone shaped HIFiRE-5 flight article, which was designed to provide hypersonic transition data for a fully 3D geometric configuration. To compare and contrast the crossflow dominated transition over the HIFiRE-1 and HIFiRE-5 configurations, this paper also analyzes boundary layer instabilities over a subscale model of the HIFiRE-5 flight configuration that was tested in the Mach 6 quiet tunnel facility at Purdue University.

Li, Fei↗

NASA NTRS1991

Naturally occurring and forced azimuthal modes in a turbulent jet

Naturally occurring instability modes in an axisymmetric jet were studied using the modal frequency technique. The evolution of the modal spectrum was obtained for a jet with a Reynolds number based on a diameter of 400,000 for both laminar and turbulent nozzle boundary layers. In the early evolution of the jet the axisymmetric mode was predominant, with the azimuthal modes growing rapidly but dominating only the end of the potential core. The growth of the azimuthal was observed closer to the nozzle exit for the jet in the laminar boundary layer case than for the turbulent. Target modes for efficient excitation of the jet were determined and two cases of excitation were studied. First, a jet was excited simultaneously by two helical modes, m equals plus 1 and m equals minus 1 at a Strouhal number based on jet diameter of 0.15 and the axisymmetric mode, m equals 0 at a jet diameter of 0.6. Second, m equals plus one and m equals minus 1 at jet diameter equals 0.3 and m equals 0 at jet diameter equals 0.6 were excited simultaneously. The downstream evolution of the hydrodynamic modes and the spreading rate of the jet were documented for each case. Higher jet spreading rates, accompanied by distorted jet cross sections were observed for the cases where combinations of axisymmetric and helical forcings were applied.

Raman, Ganesh↗

DOE OSTI2025

Concentration-Driven Slowdown of Chain-Exchange Kinetics in Block Copolymer Micelle Solutions

Here, we investigate the dependence of chain-exchange kinetics on polymer concentration for spherical micelles prepared from a polystyrene-b-poly(ethylene-alt-propylene) (SEP) diblock copolymer ( M n = 75 kDa, Ð = 1.05, and f PS = 0.18) in the PEP-selective solvent squalane. Solutions with concentrations of 15 vol% or more adopt a body-centered-cubic (BCC) packing of micelles, or a dense liquid-like packing (LLP), as confirmed by small-angle X-ray scattering. Concurrently, the mean aggregation number of the micelles grows steadily from about 60 in dilute solution to nearly 200 by 50 vol%. Time-resolved small-angle neutron scattering (TR-SANS) analysis reveals a monotonic and substantial (i.e., more than four orders of magnitude) decrease in the rate of chain exchange as the polymer concentration increases from 1 to 50 vol%. The TR-SANS relaxation functions are analyzed, taking into account both changes in contrast (due to chain exchange) and evolution in the structure factor (due to refinement of micelle packing). The activation energy for chain pullout is extracted using an established model and can be expressed as a linear function of polymer concentration, indicating that, in addition to the enthalpic barrier for extracting the core block, the evolution of micelle characteristics with increasing concentration imposes further constraints on chain exchange. Consistent with a theory of Halperin, these results suggest that the dominant factor reflects steric penalties during core block pullout arising from a reduced interfacial area per chain and associated increased corona crowding, due to the increase in aggregation number. The rate of exchange is independent of whether the micelles adopt a BCC or LLP arrangement, confirming that the rate-limiting step is extraction of the core block.

chemical structure↗