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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 667 records · Page 37
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Nuclear Astrophysics in the Storage Ring: Background Suppressed Simultaneous Measurement of (p,γ) and (p,n) Reactions

We report the application of the new elimination of Rutherford elastic scattering technique for the measurement of proton-induced reaction cross sections utilizing stored ions decelerated to astrophysical energies. This approach results in a background reduction factor of about 1 order of magnitude, enabling the first measurement of a (p, n) cross section in a storage ring. Here, the reaction channels 124 Xe⁢(p,n) and 124 Xe⁢(p,γ) have been studied just above the neutron threshold energy. The new data provide valuable constraints for Hauser-Feshbach theory and extrapolation of the (p,γ) cross section to lower energies. Most importantly, for nuclei of limited availability, the method represents a powerful improvement to efficiently study proton-induced reactions at energies within or close to the astrophysical Gamow window, bringing many reaction measurements within reach that were previously inaccessible in the laboratory.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Cross section measurements of deuteron electro-disintegration at very high recoil momenta and large 4-momentum transfers (Q^2)

The 2H(e,e'p)n cross sections have been measured at negative 4-momentum transfers of Q^2 = 4.5 +/- 0.5 (GeV/c)^2 and Q^2 = 3.5 +/- 0.5 (GeV/c)^2 reaching neutron recoil (missing) momenta up to p_r ?1.0 GeV/c. The data have been obtained at fixed neutron recoil angles 5 <= theta_nq <= 95 degrees with respect to the 3-momentum transfer q. The new data agree well with the previous data which reached p_r ?550 MeV/c. At theta_nq = 35 and 45 degrees, final state interactions (FSI), meson exchange currents (MEC) and isobar configurations (IC) are suppressed and the plane wave impulse approximation (PWIA) provides the dominant cross section contribution. The new data are compared to recent theoretical calculations, and a significant disagreement for recoil momenta p_r > 700 MeV/c is observed. The experiment was carried out in experimental Hall C at the Thomas Jefferson National Accelerator Facility (TJNAF) and formed part of a group of four experiments that were used to commission the new Super High Momentum Spectrometer (SHMS). The experiment consisted of a 10.6 GeV electron beam incident on a liquid deuterium target which resulted in the break-up of the deuteron into a proton and neutron. The scattered electrons were detected by the SHMS in coincidence with the knocked-out protons detected in the previously existing High Momentum Spectrometer (HMS) and the recoiling neutrons were reconstructed from energy-momentum conservation laws. To ensure that the 2H(e,e'p)n reaction channel was selected, we required the missing energy of the system to be the binding energy of the deuteron (?2.22 MeV). The spectrometers? central angles and momenta were set to measure three central missing momentum settings of the neutron corresponding to p_r = 80, 580 and 750 MeV/c, which required the SHMS central angle and momentum to be fixed and the HMS to be rotated from smaller to larger angles corresponding to the lower and higher missing momentum settings, respectively. The experiment was carried out in a time period of six days with typical electron beam currents of 45-60 uA at about 50% beam efficiency.

Yero, Carlos↗
DOE OSTI2024

Measurement of the 13 C(α, n 0 ) 16 O Differential Cross Section from 0.8 to 6.5 MeV

The cross section of the 13 C(α, n 0 ) 16 O reaction is needed for nuclear astrophysics and applications to a precision of 10% or better, yet inconsistencies among 50 years of experimental studies currently lead to an uncertainty of ≈15%. Here, using a state-of-the-art neutron detection array, we have performed a high resolution differential cross section study covering a broad energy range. These measurements result in a dramatic improvement in the extrapolation of the cross section to stellar energies potentially reducing the uncertainty to ≈5% and resolving long standing discrepancies in higher energy data.

6 ≤ A ≤ 19↗
DOE OSTI2021

Modeling of the Molten Salt Reactor Experiment with SCALE

A SCALE model was developed for the Molten Salt Reactor Experiment (MSRE) benchmark that was recently added to the International Handbook of Evaluated Reactor Physics Benchmark Experiments. This SCALE model served as a basis for criticality calculations and nuclear data sensitivity and uncertainty analyses with the Monte Carlo code Shift and the TSUNAMI computational capabilities in the SCALE code system. The focus of this work is the assessment of the impact of nuclear data on the calculated eigenvalue results in support of the discussion of differences between the calculated and the experimental eigenvalue result. The differences in the eigenvalues obtained using the ENDF/B-VII.0, ENDF/B-VII.1, and ENDF/B-VIII.0 nuclear data libraries cover a relatively small range of ~230 pcm. Since eigenvalue sensitivity of the MSRE is dominated by the neutron multiplicity and neutron capture of 235 U and elastic scattering in graphite, relevant changes in the ENDF/B libraries for nuclear reactions (such as carbon capture) that caused large differences in other graphite-moderated systems did not have a significant impact. Propagation of nuclear data uncertainty results in an eigenvalue uncertainty of ~700 pcm with the major contributors being 235 U neutron multiplicity, graphite elastic scattering, and 7Li neutron capture. All calculations resulted in large differences of ~2000 pcm in eigenvalue compared to the benchmark experimental value. Several potential contributors to this difference—including uncertainties and gaps in the knowledge of the material, geometry, and nuclear data—were identified. Simplified models of the full MSRE core were developed, and similarity assessments were conduced with the full MSRE core model. It was found that simplified models can serve as adequate surrogates of the full-core model such that they can be used for performing selected nuclear data performance assessments with a lower computational burden.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2022

Improvements to the 115g/115m Cd Nuclear Data

Repeated measurements of the isotope 115m Cd by Los Alamos National Laboratory (LANL), Pacific Northwest National Laboratory (PNNL), and Atomic Weapons Establishment (AWE) have revealed a consistent discrepancy between beta and gamma counting. This suggests that a significant disparity exists between the true value of the isotope’s gamma-ray branching ratios and the values reported by the National Nuclear Data Center (NNDC). Enriched 114 Cd was irradiated using thermal neutrons to produce a high-purity 115m/g Cd source for counting and analysis using traditional singles gamma-ray spectroscopy, liquid scintillation counting, gas-proportional counting, and analysis using the new Gamma-Alpha-Beta-Gamma (GABγ) and Gamma-Alpha-Beta Radio-Isotope EvaLuator (GABRIEL) coincidence detection systems. Using the D-T fusion generated neutrons, reduces the wait time required to let the short-lived 115Cd ground state decay away by leveraging the 1:1 production ratio of the ground and metastable state of 115 Cd from the 115 In (n,p) reaction relative to the 10:1 production ratio of the ground and metastable isotopes of 115 Cd by thermal neutron capture on 114 Cd. However, the much higher flux in from the Washington State University TRIGA reactor is a more rapid method of production of 115m/gCd but requires access to enriched 114 Cd. High purity 115m/g Cd samples were analyzed on regular intervals over a period of 140-days. The activity of 115m Cd measured by beta and gamma show a clear discrepancy using the current best known gamma-ray decay branching ratios. Based on these observations and measurements, a set of new branching ratio recommendations have been produced using conventional counting techniques and the advanced GAB? and GABRIEL instruments.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2021

Tritiated Sulfur Hexafluoride Disposition Strategies

Tritium (T 2 ) is a radioactive isotope of hydrogen that is produced in nuclear fission reactions and is often used in nuclear fusion reactions and accelerator-based applications for medical isotope production. As a hydrogen isotope, tritium can readily bind to hydroxyl radicals (OH), forming tritiated water (HTO or T 2 0), and to carbon atoms. Tritium decays to helium-3 ( 3 He) via beta-decay with max decay energy of 18.6 keV. While it is not an external radiation hazard, it can be an internal radiation hazard if tritium is inhaled, ingested, or absorbed through the skin. In applications where tritium is handled, tritium confinement is performed using different barriers to minimize releases to the environment. For gaseous (elemental), liquid (oxide), and metal (hydride) tritium, process piping and components provide the primary confinement function. Secondary tritium confinement is typically provided by inert (i.e. non-flammable gases such as nitrogen, argon, or helium) gloveboxes which are connected to a tritium stripper system. Primary tritium confinement barriers typically produce low volumes of high tritium concentrations of tritiated methane from carbon in steels or organic materials along with tritiated water/tritium oxide (e.g. HTO) and tritiated ammonia from reactions with oxygen and nitrogen. Tritium escaping primary confinement into secondary confinement atmospheres (e.g. gloveboxes) produce higher volumes of lower activity contamination than found in process piping. Tritium contamination also occurs by leaks or tritium permeation/diffusion through confinement materials. Tritium from inside primary confinement barriers will diffuse or leak out of the primary confinement barrier and usually into the air, if the system is inside an air hood or ventilated hot cell, or into the secondary confinement (e.g. glovebox) atmosphere which is either exhausted or stripped based on the function of the secondary confinement (glovebox) system. Accelerator based processes for medical isotope production represent an atypical tritium contamination challenge. In medical isotope production, deuterium supply gas is ionized and accelerated to a tritium gas target to produce neutrons that are then used to produce the medical isotopes through additional nuclear fission reactions. To create large voltage differentials for accelerator operations, an electrical insulation medium is needed to prevent or rapidly quench electric discharges. A common electrical insulation medium utilized in accelerator applications is sulfur hexafluoride (SF 6 ) gas. SF 6 has a high dielectric strength and allows for the construction of smaller accelerator systems compared to other electrical insulation mediums such as air or dry nitrogen. Due to tritium permeation/diffusion through accelerator process and confinement materials, there is the possibility that tritium can contaminate the electrical insulation medium of the accelerator. Tritium contaminated SF 6 creates a material without any obvious processes for managing the contamination, reuse, or disposal of the used SF 6 . This document will discuss possible management strategies for tritium contaminated SF 6 for accelerator-based processes for Molybdenum-99 (Mo-99) production.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2025

Ultra-fast single-crystal CVD diamonds in the particle time-of-flight (PTOF) detector for low yield burn-history measurements on the NIF (invited)

The Particle Time of Flight (PTOF) diagnostic is a chemical vapor deposition diamond-based detector and is the only diagnostic for measuring nuclear bang times of low yield (<1013) shots on the National Ignition Facility. Recently, a comprehensive study of detector impulse responses revealed certain detectors with very fast and consistent impulse responses with a rise time of <50 ps, enabling low yield burn history measurements. At the current standoff of 50 cm, this measurement is possible with fast 14 MeV neutrons from deuterium–tritium (DT) fusion plasmas. PTOF-inferred DT burn width numbers compare well with widths inferred from the gamma reaction history diagnostic on mid-yield (1013–1015) shots, where both systems are capable of making this measurement. These new capabilities could be extended to 2.5 MeV deuterium–deuterium neutrons from D plasmas and to even lower yield by reducing the detector standoff distance to 10 cm; a design for this is also presented.

42 ENGINEERING↗
DOE OSTI2022

Single neutron transfer on 23 Ne and its relevance for the pathway of nucleosynthesis in astrophysical X-ray bursts

We present new experimental measurements of resonance strengths in the astrophysical 23 Al($p, γ$) 24 Si reaction, constraining the pathway of nucleosynthesis beyond 22 Mg in X-ray burster scenarios. Specifically, we have performed the first measurement of the ($d, p$) reaction using a radioactive beam of 23 Ne to explore levels in 24 Ne, the mirror analog of 24 Si. Four strong single-particle states were observed and corresponding neutron spectroscopic factors were extracted with a precision of ~20%. Using these spectroscopic factors, together with mirror state identifications, we have reduced uncertainties in the strength of the key ℓ = 0 resonance at $E_r$ = 157 keV, in the astrophysical 23 Al($p, γ$) reaction, by a factor of 4. Our results show that the 22 Mg($p, γ$) 23 Al($p, γ$) pathway dominates over the competing 22 Mg($α, γ$) reaction in all but the most energetic X-ray burster events (T > 0.85 GK), significantly affecting energy production and the preservation of hydrogen fuel.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Mirror-symmetry violation in bound nuclear ground states

Conservation laws are deeply related to any symmetry present in a physical system. Analogously to electrons in atoms exhibiting spin symmetries, it is possible to consider neutrons and protons in the atomic nucleus as projections of a single fermion with an isobaric spin (isospin) of t = 1/2. Every nuclear state is thus characterized by a total isobaric spin T and a projection T z —two quantities that are largely conserved in nuclear reactions and decays. A mirror symmetry emerges from this isobaric-spin formalism: nuclei with exchanged numbers of neutrons and protons, known as mirror nuclei, should have an identical set of states, including their ground state, labelled by their total angular momentum J and parity π. In this work, we report evidence of mirror-symmetry violation in bound nuclear ground states within the mirror partners strontium-73 and bromine-73. We find that a J π = 5/2 - spin assignment is needed to explain the proton-emission pattern observed from the T = 3/2 isobaric-analogue state in rubidium-73, which is identical to the ground state of strontium-73. Therefore the ground state of strontium-73 must differ from its J π = 1/2 - mirror bromine-73. This observation offers insights into charge-symmetry-breaking forces acting in atomic nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Constraining explosive nucleosynthesis by indirect reaction methods at storage rings using unstable beams in batch mode

Nuclear reaction studies on unstable isotopes can strongly help in improving our understanding of nucleosynthesis in stars. Indirect approaches to determining astrophysical reaction rates are increasingly common-place and undergoing continuous refinement. Of particular interest is the use of such indirect techniques at storage rings, which, among other aspects, allow to recycle rare unstable beams. Here, we propose to investigate the reaction rates of astrophysical interest using indirect methods (surrogate, Trojan horse, etc.) in reverse kinematics at the IMP-CAS storage ring. Long lived radioactive ion beams, produced remotely, can be accelerated, and made to interact with light targets. The proposed reactions are 85 Kr(p, p’γ), 85 Kr(d, pγ), constraining the neutron flux in an s-process branching point, 79 Se(p, p’γ), 79 Se(d, pγ), constraining the temperature in s-process nucleosyntheses, and 59 Fe(d, pγ), constraining core collapse supernovae.

Angelis, G. de [National Inst. of Nuclear Physics ↗
DOE OSTI2024

A Multiscale Investigation of the Mechanisms Controlling Materials Degradation in the Fusion Energy Environment (DE-SC0006661: Final Report)

Realizing the promise of fusion as a commercially attractive energy source requires the development of advanced structural materials capable of sustained operation in an incredibly hostile environment. The fusion environment presents many challenges associated with high cyclic thermal-mechanical loadings, welding and joining disparate materials, and achieving chemical compatibility with coolants and tritium breeders. Yet, the overarching concern is the degradation of physical and mechanical properties, resulting from a neutron energy spectrum peaked at 14 MeV. The high-energy fusion neutron irradiation produces both displacement damage and high levels of hydrogen and helium through transmutation reactions. Advanced materials development for use in such a hostile environment is predicated on understanding the underlying mechanisms responsible for physical and material property degradation. This project has closely combined computational, theoretical and experimental techniques within a multiscale materials science paradigm to determine the mechanisms controlling material degradation in the fusion environment.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Optical Test Bench (SYSM 5620 Final Report)

The National Ignition Facility (NIF) is a research facility that focuses on High Energy Density Science and Inertial Confinement Fusion. In the NIF, 192 laser beams are directed into a miniscule Target Capsule to generate an implosion – this is called a NIF Shot. Many NIF Users conduct experiments using different Targets and laser inputs to generate reactions that are of interest to the scientific community. Those reactions are monitored using various Target Diagnostic instruments, including Shot Time Photography – which provides crucial images of the Target as the implosion occurs. A subset of these NIF Users is less interested in the reaction itself and more interested in subjecting materials or devices to the intense environment that these reactions can create. Using the Target as a source of x-rays, neutrons, or blast loading for particular materials has been significant to the shock physics community and to those who work in extreme design spaces. However, the Material and Radiation Effects team – that performs these experiments on behalf of the NIF Users – has not been able to make good use of the existing Shot Time Photography Diagnostics. The STP cameras are focused on the Targets rather than the MRE Customers’ materials, the current system is not oriented to have a good view of the MRE Customers’ materials, and the cameras are limited in their capabilities (black and white, poor resolution, etc.). As MRE experiments increase in quantity and importance to the scientific community, the desire for visual monitoring of the experiments to substantiate models and inform other data is also rising.

42 ENGINEERING↗
DOE OSTI2026

Impact of in situ nuclear networks and atomic opacities on neutron star merger ejecta dynamics, nucleosynthesis, and kilonovae

Context. Binary neutron star merger (BNSM) ejecta are key sites of rapid neutron capture (r-process) nucleosynthesis and they produce kilonovae powered by the radioactive decay of freshly synthesized nuclei. Modeling their evolution requires multi-physics simulations involving hydrodynamics, nuclear reactions, and radiative processes. The impact of nuclear burning and atomic opacity is poorly understood and often treated with simplified prescriptions. Aims. We systematically investigate different treatments of nuclear heating, particle thermalization, and atomic opacities in radiation-hydrodynamics simulations of BNSM ejecta and kilonova light curves. Methods. Ejecta profiles from long-term numerical-relativity simulations of asymmetric neutron star binaries with a massive neutron star remnant were evolved to ∼30 days using a 2D ray-by-ray approach. We compared simplified heating-rate and thermalization prescriptions with in situ Nuclear reaction Network (NN) calculations that track nuclear energy deposition and include a composition-dependent thermalization scheme. We also contrasted various gray opacity models with a frequency-dependent treatment based on atomic calculations. Results. Coupling NN and hydrodynamics significantly affects nucleosynthesis and kilonova emission. Assuming homologous expansion alters abundance evolution and produces a narrower, less populated second r-process peak and a third peak shifted to higher mass numbers. The back-reaction of nuclear heating affects the temperature evolution enough to delay and redden the early (t∼ hours) kilonova peaks. A constant thermalization efficiency underestimates and reddens the early emission while overestimating the late-time luminosity compared to the composition-dependent treatment. Analytical opacity prescriptions yield a more extended, colder photosphere, resulting in dimmer, redder kilonovae at early times (t≲ hour), while the delayed recession of the photosphere prolongs the red emission at t ≳ 5 days. Conclusions. Coupling hydrodynamics to an in situ NN is crucial for reliable nucleosynthesis and kilonova predictions. Resolving the first several hundred milliseconds of the hydrodynamics is essential for robust nucleosynthesis calculations. Composition-dependent thermalization and frequency-dependent, atomic-physics-based opacities are needed to accurately capture the temperature evolution of the ejecta and the brightness and color evolution of the kilonova. Calibrated analytic nuclear-power fits with simplified thermalization and opacity prescriptions can still reproduce the density and temperature evolution of the ejecta.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2025

Let There Be Neutrons! Hadronic Photoproduction from a Large Flux of High-energy Photons

We propose that neutrons may be generated in high-energy, high-flux photon environments via photo-induced reactions on pre-existing baryons. These photohadronic interactions are expected to occur in astrophysical jets and surrounding material. Historically, these reactions have been attributed to the production of high-energy cosmic rays and neutrinos. We estimate the photoproduction off of protons in the context of gamma-ray bursts, where it is expected there will be sufficient baryonic material that may be encompassing or entrained in the jet. We show that typical stellar baryonic material, even material completely devoid of neutrons, can become inundated with neutrons in situ via hadronic photoproduction. Consequently, this mechanism provides a means for collapsars and other astrophysical sites containing substantial flux of high-energy photons to be favorable for neutron-capture nucleosynthesis.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

The Nuclear Reaction Network WinNet

Abstract We present the state-of-the-art single-zone nuclear reaction network WinNet , which is capable of calculating the nucleosynthetic yields of a large variety of astrophysical environments and conditions. This ranges from the calculation of the primordial nucleosynthesis, where only a few nuclei are considered, to the ejecta of neutron star mergers with several thousands of involved nuclei. Here we describe the underlying physics and implementation details of the reaction network. We additionally present the numerical implementation of two different integration methods, the implicit Euler method and Gears method, along with their advantages and disadvantages. We furthermore describe basic example cases of thermodynamic conditions that we provide together with the network and demonstrate the reliability of the code by using simple test cases. With this publication, WinNet will be publicly available and open source at GitHub and Zenodo.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Quantifying Burst Repeatability for Godiva IV

The minimum resolvable relative change in the neutron source emission of Godiva IV between bursts, i.e., burst repeatability, was quantified using a combination of activation monitors and a resistance temperature detector (RTD). Measurements support changes in the neutron source emission between bursts can be determined with a precision of 2.7%. The measurements were performed during a series of twelve Godiva IV bursts and were a collaborative effort between Los Alamos National Laboratory, Sandia National Laboratories, and Pacific Northwest National Laboratory. Gold, iron, nickel, and sulfur activation monitors were positioned in a sample holder in the central cavity of Godiva IV for each burst. The RTD is part of the Godiva burst diagnostic system and is in a fixed location in the safety block of Godiva IV. It is used to determine the temperature rise of the burst, i.e., the difference between the maximum temperature recorded during the burst and the initial temperature prior to the burst. Differences in either the specific activity of the activation monitor reactions, or the temperature rise can be used to determine the relative change in the neutron source emission for separate bursts, but historic results have proven that each method is susceptible to various sources of biases which generally cannot be isolated using a single method. We address this issue by applying both measurement methods and analyzing the correlation between them. The results presented in this work will be used to support future experiments with Godiva IV at the National Criticality Experiments Research Center (NCERC).

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2024

Proton and neutron density distributions at supranormal density in low- and medium-energy heavy-ion collisions. II. Central Pb + Pb collisions

This paper represents a continuation of our investigation into the limitations on total, proton, and neutron particle number densities, as well as the asymmetry of proton and neutron density distributions achievable in central heavy-ion collisions. We explore these aspects at low and medium energies within the framework of the Boltzmann-Uhlenbeck-Uehling (pBUU) transport and time-dependent Hartree-Fock (TDHF) models. Previous studies, focusing on symmetric and asymmetric collisions of Ca and Sn nuclei [1], and initial results on Pb-nuclei collisions [2], emphasized the role of the Coulomb interaction in these events. Our findings indicated that: (i) the highest total densities predicted at 𝐸 beam = 800 MeV/nucleon were on the order of ≈ 2.5⁢𝜌 0 (𝜌 0 = 0.16 fm −3 ), (ii) the proton-neutron asymmetry for maximal densities, 𝛿=(𝜌$^{max}_{n}$− 𝜌$^{max}_{p}$)/(𝜌$^{max}_{n}$+𝜌$^{max}_{p}$), did not generally exceed the asymmetry in the initial state of the collision at all beam energies and tended to decrease during the reaction, and (iii) a significant portion of this asymmetry had its microscopic origin in Coulomb forces, masking the pure nuclear contribution. These new findings, particularly relevant in the astrophysical context, are further examined in this work, focusing on the heaviest target-projectile combination 212,208 Pb accessible in an experiment. We introduce the SkT3 Skyrme force model, not previously used for the Pb system, and compare it to the SV-bas and SV-sym34 models to explore the symmetry-energy dependence of the results. Contour plots of nucleonic densities are presented, contrasting the time evolution of the density distributions in low (TDHF) and high (pBUU) models. We also present the evolution of normalized maximal proton, neutron, and total nucleon number density with increasing beam energy in the full pBUU model and the Vlasov approximation, aiming to explore the impact of correlations in the reaction. The time evolution of the proton and neutron density distributions in the plane transverse to the beam direction is illustrated at both low and high beam energy. In conclusion, our detailed examination of the Pb system in this work provides further essential evidence that the aforementioned findings (i)–(iii) are only weakly dependent on system size and a symmetry-energy model, and thus, they are of more general importance.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

C 13 ( n , 2 n γ ) C 12 γ -ray production in the 14–16 MeV incident neutron energy range

We report γ-ray emission from 12 C and 13 C samples irradiated with deuterium-tritium fusion neutrons was experimentally measured at the Omega Laser Facility and at the Ohio University Edwards Accelerator Laboratory. The intent of these measurements was to determine the feasibility of using 13 C-based plastic ablators with embedded 12 C layers for “dark mix” diagnosis of inertial confinement fusion implosions. Spectrally resolved measurements at Ohio University identified significant 4.44-MeV γ-ray emission from the 13 C(n, 2nγ) 12 C-L1 reaction channel. The recorded 4.44-MeV 13 C signal was compared against emission from an identically irradiated 12 C target with known 12 C(n, n'γ) 12 C-L1 cross section, which resulted in an average 13 C(n, 2nγ) 12 C-L1 cross section of 117 ± 17 mb over the incident neutron energy distribution range from 14.4 to 15.8 MeV. Integrated 13C γ -ray signals above 2.9 MeV recorded with the Gas Cherenkov Detector at Omega exceeded MCNP6.1 predictions by a factor of 3. The additional signal was attributed to 4.44-MeV γs resulting in an inferred 13 C(n, 2nγ) 12 C-L1 cross section of 95 ± 11 mb at 14.1-MeV average incident neutron energy. As a result, the 13 C-based “dark mix” diagnostic concept was deemed infeasible.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗