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At least 667 records · Page 37
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

The Liquid Jet Endstation for Hard X-ray Scattering and Spectroscopy at the Linac Coherent Light Source

The ability to study chemical dynamics on ultrafast timescales has greatly advanced with the introduction of X-ray free electron lasers (XFELs) providing short pulses of intense X-rays tailored to probe atomic structure and electronic configuration. Fully exploiting the full potential of XFELs requires specialized experimental endstations along with the development of techniques and methods to successfully carry out experiments. The liquid jet endstation (LJE) at the Linac Coherent Light Source (LCLS) has been developed to study photochemistry and biochemistry in solution systems using a combination of X-ray solution scattering (XSS), X-ray absorption spectroscopy (XAS), and X-ray emission spectroscopy (XES). The pump–probe setup utilizes an optical laser to excite the sample, which is subsequently probed by a hard X-ray pulse to resolve structural and electronic dynamics at their intrinsic femtosecond timescales. The LJE ensures reliable sample delivery to the X-ray interaction point via various liquid jets, enabling rapid replenishment of thin samples with millimolar concentrations and low sample volumes at the 120 Hz repetition rate of the LCLS beam. This paper provides a detailed description of the LJE design and of the techniques it enables, with an emphasis on the diagnostics required for real-time monitoring of the liquid jet and on the spatiotemporal overlap methods used to optimize the signal. Additionally, various scientific examples are discussed, highlighting the versatility of the LJE.

EXAFS↗
DOE OSTI2022

A Tunable Resolution Grating Monochromator and the Quest for Transform Limited Pulses

A variable resolution, transform limited monochromator is designed for the Free Electron Laser (FEL) source of LCLS. It provides monochromatic beam in the 250–1500 eV range, delivering the beam on the second floor of the LCLS experimental Hall. One major requirement for this monochromator is to provide, as close as possible, monochromatic transform limited pulses for time-resolved experiments. The theory and the limit of using classical diffraction scheme to monochromatize Soft X-ray beam, while preserving the pulse length, will be presented, together with the optical scheme of this versatile monochromator design.

47 OTHER INSTRUMENTATION↗
DOE OSTI2011

Second and Third Harmonic Measurements at the Linac Coherent Light Source

The Linac Coherent Light Source (LCLS) started user commissioning in October of 2009, producing Free Electron Laser (FEL) radiation between 800 eV and 8 keV [1]. The fundamental wavelength of the FEL dominates radiation in the beamlines, but the beam also produces nonnegligible levels of radiation at higher harmonics. The harmonics may be desirable as a source of harder X-rays, but may also contribute backgrounds to user experiments. In this paper we present preliminary measurements of the second and third harmonic content in the FEL. We also measure the photon energy cutoff of the soft X-ray mirrors to determine the extent to which higher harmonics reach the experimental stations. We present preliminary second and third harmonic measurements for LCLS. At low energies (below 1 keV fundamental) we measure less than 0.1% second harmonic content. The second harmonic will be present in the soft X-ray beam line for fundamental photon energies below approximately 1.1 keV. At low and high energies, we measure third harmonic content ranging from 0.5% to 3%, which is consistent with expectations. For both second and third harmonics, experimental work is ongoing. More rigorous analysis of the data will be completed soon.

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

ESTB: A New Beam Test Facility at SLAC

End Station A Test Beam (ESTB) is a beam line at SLAC using a small fraction of the bunches of the 13.6 GeV electron beam from the Linac Coherent Light Source (LCLS), restoring test beam capabilities in the large End Station A (ESA) experimental hall. ESTB will provide one of a kind test beam essential for developing accelerator instrumentation and accelerator R&D, performing particle and particle astrophysics detector research, linear collider machine and detector interface (MDI) R&D studies, development of radiation-hard detectors, and material damage studies with several distinctive features. In the past, 18 institutions participated in the ESA program at SLAC. In stage I, 4 new kicker magnets will be added to divert 5 Hz of the LCLS beam to the A-line. A new beam dump will be installed and a new Personnel Protection System (PPS) is being built in ESA. In stage II, a secondary hadron target will be installed, able to produce pions up to about 12 GeV/c at 1 particle/pulse.

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

A Compact X-Band Linac for an X-Ray FEL

With the growing demand for FEL light sources, cost issues are being reevaluated. To make the machines more compact, higher frequency room temperature linacs are being considered, specifically ones using C-band (5.7 GHz) rf technology, for which 40 MV/m gradients are achievable. In this paper, we show that an X-band (11.4 GHz) linac using the technology developed for NLC/GLC can provide an even lower cost solution. In particular, stable operation is possible at gradients of 100 MV/m for single bunch operation and 70 MV/m for multibunch operation. The concern, of course, is whether the stronger wakefields will lead to unacceptable emittance dilution. However, we show that the small emittances produced in a 250 MeV, low bunch charge, LCLS-like S-band injector and bunch compressor can be preserved in a multi-GeV X-band linac with reasonable alignment tolerances. The successful lasing and operation of the LCLS [1] has generated world-wide interest in X-ray FELs. The demand for access to such a light source by researchers eager to harness the capabilities of this new tool far exceeds the numbers that can be accommodated, spurring plans for additional facilities. Along with cost, spatial considerations become increasingly important for a hard X-ray machine driven by a multi-GeV linac. The consequent need for high acceleration gradient focuses attention on higher frequency normal conducting accelerator technology, rather than the superconducting technology of a soft X-ray facility like FLASH. C-band technology, such as used by Spring-8, is a popular option, capable of providing 40 MV/m. However, more than a decade of R&D toward an X-band linear collider, centered at SLAC and KEK, has demonstrated that this frequency option can extend the gradient reach to the 70-100 MV/m range. The following design and beam dynamics calculations show an X-band linac to be an attractive choice on which to base an X-ray FEL.

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

Facility for Advanced Accelerator Experimental Tests (FACET) at SLAC and its Radiological Considerations

Facility for Advanced Accelerator Experimental Tests (FACET) in SLAC will be used to study plasma wakefield acceleration. FLUKA Monte Carlo code was used to design a maze wall to separate FACET project and LCLS project to allow persons working in FACET side during LCLS operation. Also FLUKA Monte Carlo code was used to design the shielding for FACET dump to get optimum design for shielding both prompt and residual doses, as well as reducing environmental impact. FACET will be an experimental facility that provides short, intense pulses of electrons and positrons to excite plasma wakefields and study a variety of critical issues associated with plasma wakefield acceleration [1]. This paper describes the FACET beam parameters, the lay-out and its radiological issues.

43 PARTICLE ACCELERATORS↗
DOE OSTI2011

First Beam to FACET

The SLAC 3km linear electron accelerator has been reconfigured to provide a beam of electrons to the new Facility for Advanced Accelerator Experimental Tests (FACET) while simultaneously providing an electron beam to the Linac Coherent Light Source (LCLS). On June 23, 2011, the first electron beam was transported through this new facility. Commissioning of FACET is in progress. On June 23, 2011, an electron beam was successfully transported through the new FACET system to a dump in Sector 20 in the linac tunnel. This was achieved while the last third of the linac, operating from the same control room, but with a separate injector system, was providing an electron beam to the Linac Coherent Light Source (LCLS), demonstrating that concurrent operation of the two facilities is practical. With the initial checkout of the new transport line essentially complete, attention is now turning toward compressing the electron bunches longitudinally and focusing them transversely to support a variety of accelerator science experiments.

43 PARTICLE ACCELERATORS↗
DOE OSTI2012

A New Control Room for SLAC Accelerators

We are planning to construct a new control room at SLAC to unify and improve the operation of the LCLS, SPEAR3, and FACET accelerator facilities, and to provide the space and flexibility needed to support the LCLS-II and proposed new test beam facilities. The existing control rooms for the linac and SPEAR3 have been upgraded in various ways over the last decade, but their basic features have remained unchanged. We propose to build a larger modern Accelerator Control Room (ACR) in the new Research Support Building (RSB) which is currently under construction at SLAC. Shifting the center of control for the accelerator facilities entails both technical and administrative challenges. In this paper, we describe the history, concept, and status of this project.

43 PARTICLE ACCELERATORS↗
DOE OSTI2012

Breaking the Attosecond, Angstrom and TV/M Field Barriers with Ultra-Fast Electron Beams

Recent initiatives at UCLA concerning ultra-short, GeV electron beam generation have been aimed at achieving sub-fs pulses capable of driving X-ray free-electron lasers (FELs) in single-spike mode. This use of very low Q beams may allow existing FEL injectors to produce few-100 attosecond pulses, with very high brightness. Towards this end, recent experiments at the LCLS have produced {approx}2 fs, 20 pC electron pulses. We discuss here extensions of this work, in which we seek to exploit the beam brightness in FELs, in tandem with new developments in cryogenic undulator technology, to create compact accelerator-undulator systems that can lase below 0.15 {angstrom}, or be used to permit 1.5 {angstrom} operation at 4.5 GeV. In addition, we are now developing experiments which use the present LCLS fs pulses to excite plasma wakefields exceeding 1 TV/m, permitting a table-top TeV accelerator for frontier high energy physics applications.

43 PARTICLE ACCELERATORS↗
DOE OSTI2012

RF Gun Photocathode Research at SLAC

LCLS is presently operating with a third copper photocathode in the original rf gun, with a quantum efficiency (QE) of {approx}1 x 10{sup -4} and projected emittance {gamma}{var_epsilon}{sub x,y} = 0.45 {micro}m at 250 pC bunch charge. The spare LCLS gun is installed in the SLAC Accelerator Structure Test Area (ASTA), fully processed to high rf power. As part of a wider photocathode R and D program, a UV laser system and additional gun diagnostics are being installed at ASTA to measure QE, QE lifetime, and electron beam emittance under a variety of operating conditions. The near-term goals are to test and verify the spare photocathode production/installation sequence, including transfer from the final holding chamber to the rf gun. Mid- and longer-term goals include development of a rigorous understanding of plasma and laser-assisted surface conditioning and investigation of new, high-QE photocathode materials. In parallel, an x-ray photoemission spectroscopy station is nearing completion, to analyze Cu photocathode surface chemistry. In this paper we review the status and anticipated operating parameters of ASTA and the spectroscopy test chamber.

43 PARTICLE ACCELERATORS↗
DOE OSTI2012

LLRF System Upgrade for the SLAC Linac

The Linac Coherent Light Source (LCLS) at SLAC is in full user operation and has met the stability goals for stable lasing. The 250pC bunch can be compressed to below 100fS before passing through an undulator. In a new mode of operation a 20pC bunch is compressed to about 10fS. Experimenters are regularly using this shorter X-ray pulse and getting pristine data. The 10fS bunch has timing jitter on the order of 100fS. Physicists are requesting that the RF system achieve better stability to reduce timing jitter. Drifts in the RF system require longitudinal feedbacks to work over large ranges and errors result in reduced performance of the LCLS. A new RF system is being designed to help diagnose and reduce jitter and drift in the SLAC linac.

43 PARTICLE ACCELERATORS↗
DOE OSTI2012

Fast Beam-Based BPM Calibration

The Alignment Diagnostic System (ADS) of the LCLS undulator system indicates that the 33 undulator quadrupoles have extremely high position stability over many weeks. However, beam trajectory straightness and lasing efficiency degrade more quickly than this. A lengthy Beam Based Alignment (BBA) procedure must be executed every two to four weeks to re-optimize the X-ray beam parameters. The undulator system includes RF cavity Beam Position Monitors (RFBPMs), several of which are utilized by an automatic feedback system to align the incoming electron-beam trajectory to the undulator axis. The beam trajectory straightness degradation has been traced to electronic drifts of the gain and offset of the BPMs used in the beam feedback system. To quickly recover the trajectory straightness, we have developed a fast beam-based procedure to recalibrate the BPMs. This procedure takes advantage of the high-precision monitoring capability of the ADS, which allows highly repeatable positioning of undulator quadrupoles. This report describes the ADS, the position stability of the LCLS undulator quadrupoles, and some results of the new recovery procedure.

43 PARTICLE ACCELERATORS↗
DOE OSTI2014

Analysis of New High-Q0 SRF Cavity Tests by Nitrogen Gas Doping at Jefferson Lab

In order to refine systematic understanding and establish confident process control, Jefferson Lab has joined with partners to investigate and thoroughly characterize the dramatically higher Q0 of 1.3 GHz niobium cavities first reported by FNAL in 2013[1]. With partial support from the LCLS-II project, JLab has undertaken a parametric study of nitrogen doping in vacuum furnace at 800 °C followed by variable depth surface removal in the 5 - 20 μm range. Q0 above 3×1010 are typical at 2.0 K and 16 MV/m accelerating field. We report observations from the single cell study and current interpretations. In addition to the parametric single cell study, we also report on the ongoing serial testing of six nitrogen-doped 9-cell cavities as baseline prototypes for LCLS-II.

Palczewski, Ari D.↗
DOE OSTI2019

Fluorescence intensity monitors as intensity and beam-position diagnostics for X-ray free-electron lasers

For LCLS-II, a fluorescence intensity monitor for the non-invasive, pulse-by-pulse normalization of experiments has been developed. A prototype diagnostic was constructed with a microchannel plate assembly and two photodiodes. The diagnostic was then installed in the LCLS SXR instrument Kirkpatrick–Baez mirror chamber with the detectors located above the vertically reflecting mirror. The linearity, noise and position sensitivity of the detectors have been characterized. The photodiode responsivity is suitable for high pulse energies. The microchannel plate detector shows sufficient responsivity over a wide range of pulse energies. The relative signal from the two photodiodes provides a sensitive measure of the X-ray beam position. The fluorescence intensity monitor provides intensity normalization while being compatible with high incident power, a 0.93 MHz repetition rate and ultra-high vacuum.

Heimann, Philip↗
DOE OSTI2019

Industrial Cavity Production: Lessons Learned to Push the Boundaries of Nitrogen-Doping

Nitrogen doping has been proven now in several labs to enhance Q0 values of 1.3 GHz cavities in the gradient domain favored by CW operation. The choice of doping for the LCLS-II project has given the community a wealth of statistics and experience on the challenge of transferring the doping technology to industry. Overall, industry-produced nitrogen-doped cavities have shown excellent performance, however some technical issues have arisen. This talk focuses on lessons learned from the production of over 300 nitrogen-doped cavities for LCLS-II and how issues were mitigated to further improve performance. Finally, I will discuss pushing the boundaries of nitrogen-doping further by exploring different doping regimes in order to maintain excellent Q0 performance, while reaching higher quench fields.

Gonnella, D.↗
DOE OSTI2025

LLRF System Analysis for the Fermilab PIP-II Superconducting LINAC

PIP-II is a superconducting linac that is in the initial acceleration chain for the Fermilab accelerator complex. The RF system consists of a warm front-end with an RFQ and buncher cavities along with 25 superconducting cryo-modules comprised of cavities with five different acceleration \(β\). The LLRF system for the linac has to provide field and resonance control for a total of 125 RF cavities. Various components of the LLRF system have been tested with and without beam at the PIP-II test stands. The LLRF system design is derived from the LCLS-II project with its self-excited loop architecture used in the majority of the cryo-modules. The PIP-II beam loading at 2 mA is much higher than the LCLS-II linac. The control system architecture is analyzed and evaluated for the operational limits of feedback gains and their ability to meet the project regulation requirements for cavity field amplitude and phase regulation.

Varghese, P. [Fermilab] (ORCID:0009000925131983)↗
DOE OSTI2010

Monte Carlo Studies of the Radiation Fields in the Linac Coherent Light Source Undulators and of the Corresponding Signals in the Cerenkov Beam Loss Monitors

In 2009 the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Center started free electron laser (FEL) operation. In order to continue to produce the bright and short-pulsed x-ray laser demanded by FEL scientists, this pioneer hard x-ray FEL requires a perfectly tailored magnetic field at the undulators, so that the photons generated at the electron wiggling path interact at the right phase with the electron beam. In such a precise system, small (>0.01%) radiation-induced alterations of the magnetic field in the permanent magnets could affect FEL performance. This paper describes the simulation studies of radiation fields in permanent magnets and the expected signal in the detectors. The transport of particles from the radiation sources (i.e. diagnostic insert) to the undulator magnets and to the beam loss monitors (BLM) was simulated with the intra nuclear cascade codes FLUKA and MARS15. In order to accurately reproduce the optics of LCLS, lattice capabilities and magnetic fields were enabled in FLUKA and betatron oscillations were validated against reference data. All electron events entering the BLMs were printed in data files. The paper also introduces the Radioactive Ion Beam Optimizer (RIBO) Monte Carlo 3-D code, which was used to read from the event files, to compute Cerenkov production and then to simulate the optical coupling of the BLM detectors, accounting for the transmission of light through the quartz.

COMP, SAFETY, XFEL, OTHER↗
DOE OSTI2022

The time-resolved atomic, molecular and optical science instrument at the Linac Coherent Light Source

The newly constructed time-resolved atomic, molecular and optical science instrument (TMO) is configured to take full advantage of both linear accelerators at SLAC National Accelerator Laboratory, the copper accelerator operating at a repetition rate of 120 Hz providing high per-pulse energy as well as the superconducting accelerator operating at a repetition rate of about 1 MHz providing high average intensity. Both accelerators power a soft X-ray free-electron laser with the new variable-gap undulator section. With this flexible light source, TMO supports many experimental techniques not previously available at LCLS and will have two X-ray beam focus spots in line. Thereby, TMO supports atomic, molecular and optical, strong-field and nonlinear science and will also host a designated new dynamic reaction microscope with a sub-micrometer X-ray focus spot. The flexible instrument design is optimized for studying ultrafast electronic and molecular phenomena and can take full advantage of the sub-femtosecond soft X-ray pulse generation program.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗