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At least 667 records · Page 37
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Realizing gapped surface states in the magnetic topological insulator Mn Bi 2 - x Sb x Te 4

The interplay between magnetism and nontrivial topology in magnetic topological insulators (MTIs) is expected to give rise to exotic topological quantum phenomena like the quantum anomalous Hall effect and the topological axion states. A key to assessing these novel properties is to realize gapped topological surface sates. MnBi 2 Te 4 possesses nontrivial band topology with an intrinsic antiferromagnetic state. However, the highly electron-doped nature of the MnBi 2 Te 4 crystals obstructs the exhibition of the surface band gap. Here, we tailor the material through Sb substitution to reveal the gapped surface states in MnBi 2-x Sb x Te 4 . By shifting the Fermi level into the bulk band gap, we access the surface states and show a band gap of 50 meV at the Dirac point from quasiparticle interference measured by scanning tunneling microscopy (STM). Surface-dominant conduction is confirmed through transport spectroscopy measured by multiprobe STM below the Néel temperature. The surface band gap is robust against the out-of-plane magnetic field despite the promotion of field-induced ferromagnetism. Finally, the realization of bulk-insulating MTIs with the large exchange gap offers a promising platform for exploring emergent topological phenomena.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Defect-driven ferrimagnetism and hidden magnetization in MnBi 2 Te 4

MnBi 2 Te 4 (MBT) materials are promising antiferromagnetic topological insulators in which field-driven ferromagnetism is predicted to cause a transition between axion insulator and Weyl semimetallic states. However, the presence of antiferromagnetic coupling between Mn/Bi antisite defects and the main Mn layer can reduce the low-field magnetization, and it has been shown that such defects are more prevalent in the structurally identical magnetic insulator MnSb 2 Te 4 (MST). We use high-field magnetization measurements to show that the magnetization of MBT and MST occur in stages and full saturation requires fields of ~60 T. As a consequence, the low-field magnetization plateau state in MBT, where many determinations of the quantum anomalous Hall state are studied, actually consists of ferrimagnetic septuple blocks containing both uniform and staggered magnetization components.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Engineering magnetic topological insulators in Eu 5 M 2 X 6 Zintl compounds

Magnetic topological insulators provide a prominent material platform for quantum anomalous Hall physics and axion electrodynamics. However, the lack of material realizations with cleanly gapped surfaces hinders technological utilization of these exotic quantum phenomena. Here, using the Zintl concept and the properties of nonsymmorphic space groups, we computationally engineer magnetic topological insulators. Specifically, we explore Eu 5 M 2 X 6 (M=metal, X=pnictide) Zintl compounds and find that Eu 5 Ga 2 Sb 6 , Eu 5 Tl 2 Sb 6 , and Eu 5 In 2 Bi 6 form stable structures with nontrivial Z 2 indices. We also show that epitaxial and uniaxial strain can be used to control the Z 2 index and the bulk energy gap. Lastly, we discuss experimental progress towards the synthesis of the proposed candidates and provide insights that can be used in the search for robust magnetic topological insulators in Zintl compounds.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Possible coexistence of magnetism and paramagnetic singularity in lightly Fe-doped WTe 2

Topological semimetals possess nodal or nodal-line phases where conduction and valence bands touch at points or lines in momentum space, respectively. Such band touching is symmetry protected and gives rise to exotic and interesting electronic properties. Coupling topological order with magnetism provides a platform for exploring time-reversal (TR) symmetry breaking topological physics, such as axion electrodynamics, inverse spin-galvanic effect, and the quantized anomalous Hall effect. The Weyl semimetal (WSM) requires breaking either TR symmetry or lattice inversion symmetry (I). By doping inversion-symmetry-broken WSM with magnetic dopants, one can expect to create a WSM with both symmetries breaking simultaneously. Here, structural, electrical, and magnetic properties of Fe x ⁢W 1–x Te 2 (x = 0 and 0.011) are reported. It is revealed that, with a small Fe doping concentration (x = 0.011), a ferromagnetism is induced at low temperature (<10 K). Scanning tunneling microscopy and spectroscopy measurements in Fe 0.011 ⁢W 0.989 ⁢Te 2 further reveal only substitution and no intercalated dopants being observed. The probabilities of the Fe substitutions at the two nonequivalent W sites are quantified with equal probability. The dl/dV point spectra indicates that the Fe substitution in WTe 2 manifests itself as electron doping regardless of doping sites. The results clearly reveal the possible coexistence of magnetism and Weyl points in the lightly Fe doped WTe2 at low temperature. Furthermore, this provides an ideal system for further study on the interplay between the topological Weyl points and the TR symmetry breaking.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Investigating the XENON1T low-energy electronic recoil excess using NEST

The search for dark matter, the missing mass of the Universe, is one of the most active fields of study within particle physics. The XENON1T experiment recently observed a 3.5⁢𝜎 excess potentially consistent with dark matter, or with solar axions. Here, we will use the Noble Element Simulation Technique (NEST) software to simulate the XENON1T detector, reproducing the excess. We utilize different detector efficiency and energy reconstruction models, but they primarily impact sub-keV energies and cannot explain the XENON1T excess. However, using NEST, we can reproduce their excess in multiple, unique ways, most easily via the addition of 31 ± 11 37 Ar decays. Furthermore, this results in new, modified background models, reducing the significance of the excess to ≤2.2⁢𝜎 at least using non-Profile Likelihood Ratio (PLR) methods. This is independent confirmation that the excess is a real effect, but potentially explicable by known physics. Many cross-checks of our 37 Ar hypothesis are presented.

particle dark matter↗
DOE OSTI2021

Growth of accretion driven scalar hair around Kerr black holes

We report that Scalar fields around compact objects are of interest for scalar-tensor theories of gravity and dark matter models consisting of a massive scalar, e.g., axions. We study the behavior of a scalar field around a Kerr black hole with nontrivial asymptotic boundary conditions - both nonzero density and nonzero angular momentum. Starting from an initial radially homogeneous configuration, a scalar cloud is accreted, which asymptotes to known stationary configurations over time. We study the cloud growth for different parameters including black hole spin, scalar field mass, and the scalar field density and angular momentum far from the black hole. We characterize the transient growth of the mass and angular momentum in the cloud, and the spatial profile of the scalar around the black hole, and relate the results of fully nonlinear simulations to an analytic perturbative expansion. We also highlight the potential for these accreted clouds to create monochromatic gravitational wave signals - similar to the signals from superradiant clouds, although significantly weaker in amplitude.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Dynamical friction in self-interacting ultralight dark matter

Here, we explore how dynamical friction in an ultralight dark matter (ULDM) background is affected by dark matter self-interactions. We calculate the force of dynamical friction on a point mass moving through a uniform ULDM background with self-interactions, finding that the force of dynamical friction vanishes for sufficiently strong repulsive self-interactions. Using the pseudospectral solver ultraDark.jl, we show with simulations that reasonable values of the ULDM self-interaction strength and particle mass cause $\mathcal{O}$(1) differences in the acceleration of an object like a supermassive black hole (SMBH) traveling near the center of a soliton, relative to the case with no self-interactions. For example, repulsive self-interactions with λ=10 -90 yield a deceleration due to dynamical friction ≈ 70% smaller than a model with no self-interactions. We discuss the observational implications of our results for SMBHs near soliton centers and for massive satellite galaxies falling into ultralight axion halos and show that outcomes are dependent on whether a self-interaction is present or not.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Search for a scalar or pseudoscalar dilepton resonance produced in association with a massive vector boson or top quark-antiquark pair in multilepton events at s = 13 TeV

A search for beyond the standard model spin-0 bosons, ϕ , that decay into pairs of electrons, muons, or tau leptons is presented. The search targets the associated production of such bosons with a W or Z gauge boson, or a top quark-antiquark pair, and uses events with three or four charged leptons, including hadronically decaying tau leptons. The proton-proton collision data set used in the analysis was collected at the LHC from 2016 to 2018 at a center-of-mass energy of 13 TeV, and corresponds to an integrated luminosity of 138 fb - 1 . The observations are consistent with the predictions from standard model processes. Upper limits are placed on the product of cross sections and branching fractions of such new particles over the mass range of 15 to 350 GeV with scalar, pseudoscalar, or Higgs-boson-like couplings, as well as on the product of coupling parameters and branching fractions. Several model-dependent exclusion limits are also presented. For a Higgs-boson-like ϕ model, limits are set on the mixing angle of the Higgs boson with the ϕ boson. For the associated production of a ϕ boson with a top quark-antiquark pair, limits are set on the coupling to top quarks. Finally, limits are set for the first time on a fermiophilic dilaton-like model with scalar couplings and a fermiophilic axion-like model with pseudoscalar couplings.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Detecting dark matter substructures on small scales with fast radio bursts

The matter power spectrum is only weakly constrained on subgalactic scales, while physics beyond the Standard Model can leave unique imprints, especially on sub-parsec scales. We propose measuring the arrival-time difference of fast radio bursts (FRBs) along two adjacent sightlines as a new probe to dark matter substructures on scales down to ∼ 1 AU . We discuss two observational scenarios in which it may be possible to place interesting constraints on such models through the monitoring of repeating FRB sources: (i) By sending radio receivers to space to form a baseline of tens of AU or more and measuring the temporal variation of the arrival-time difference between receivers. (ii) By measuring the temporal variation of the arrival-time difference between two lensed images of one strongly lensed repeater. In both scenarios, obtaining interesting constraints requires correlating the voltage time series to measure the radio signal arrival time to sub-nanosecond precision. We find that two radio dishes separated by 20 AU may be sensitive to the enhancement of small-scale structures at ∼ 10 - 8 M ⊙ masses in the QCD axion dark matter scenario, or from an early epoch of matter domination with a reheating temperature up to 60 MeV. Other dark matter models, such as those composed of ∼ 10 - 13 M ⊙ primordial black holes produced during inflation, would also be probed by this method. We further show that a strong lensing situation of multiple images provides an equivalent ∼ 2000 AU ( σ v / 10 3 km s - 1 ) ( δ t / 10 yr ) baseline, for a typical velocity of dark matter substructures σ v and an observational time span δ . This is much more sensitive, but with the uncertainty that intervening decoherence from the interstellar medium may degrade the timing precision, and that spatial variation in the FRB emission spot may result in confounding signals. We show that the lensing magnifications of Type Ia supernovae constrain a similar quantity to such FRB timing, with present limits being equivalent to ruling out the same parameter space that would be probed by a 0.14 AU baseline.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Deepest sensitivity to wavelike dark photon dark matter with superconducting radio frequency cavities

Wavelike, bosonic dark matter candidates like axions and dark photons can be detected using microwave cavities known as haloscopes. Traditionally, haloscopes consist of tunable copper cavities operating in the TM 010 mode, but ohmic losses have limited their performance. In contrast, superconducting radio frequency (SRF) cavities can achieve quality factors of ∼ 10 10 , perhaps 5 orders of magnitude better than copper cavities, leading to more sensitive dark matter detectors. In this paper, we first derive that the scan rate of a haloscope experiment is proportional to the loaded quality factor Q L , even if the cavity bandwidth is much narrower than the dark matter halo line shape. We then present a proof-of-concept search for dark photon dark matter using a nontunable ultrahigh-quality SRF cavity. We exclude dark photon dark matter with kinetic mixing strengths of χ > 1.5 × 10 − 16 for a dark photon mass of m A ′ = 5.35 μ eV , achieving the deepest exclusion to wavelike dark photons by almost an order of magnitude. Published by the American Physical Society 2024

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Constraints on dark matter from dynamical heating of stars in ultrafaint dwarfs. II. Substructure and the primordial power spectrum

There is a large and growing interest in observations of small-scale structure in dark matter. We propose a new way to probe dark matter structures in the ∼ 10 – 10 8 M ⊙ range. This allows us to constrain the primordial power spectrum over shorter distances scales than possible with direct observations from the CMB. For k in the range ∼ 10 – 1000 Mpc − 1 our constraints on the power spectrum are orders of magnitude stronger than previous bounds. We also set some of the strongest constraints on dark matter isocurvature perturbations. Our method relies on the heating effect such dark matter substructures would have on the distribution of stars in an ultrafaint dwarf galaxy. Many models of inflation produce enhanced power at these short distance scales and can thus be constrained by our observation. Further, many dark matter models such as axion dark matter, self-interacting dark matter and dissipative dark matter, produce dense structures which could be constrained this way. Published by the American Physical Society 2024

Graham, Peter W. (ORCID:0000000216001601)↗
DOE OSTI2024

Lepton-flavor-violating ALP signals with TeV-scale muon beams

We explore the feasibility of using TeV-energy muons to probe lepton-flavor-violating (LFV) processes mediated by an axion-like particle (ALP) a with mass O(10 GeV). We focus on µτ LFV interactions and assume that the ALP is coupled to a dark state χ, which can be either less or more massive than a. Such a setup is demonstrated to be consistent with χ being a candidate for dark matter, in the experimentally relevant regime of parameters. We consider the currently operating NA64-µ experiment and proposed FASERν2 detector as both the target and the detector for the process µA → τA a, where A is the target nucleus. We also show that a possible future active muon fixed-target experiment operating at a 3 TeV muon collider or in its preparatory phase can provide an impressive reach for the LFV process considered, with future FASERν2 data providing a pilot study towards that goal. The implications of the muon anomalous magnetic moment (g - 2) µ measurements for the underlying model, in case of a positive signal, are also examined, and a sample UV completion is outlined.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2025

Connecting pseudo-Nambu-Goldstone dark matter with pseudo-Dirac neutrinos in a left-right symmetry model

Stringent constraints from the dark matter (DM) direct detection experiments can be naturally evaded for a pseudo-Nambu-Goldstone boson (pNGB) DM. We propose a realization of pNGB DM in the context of a left-right symmetric model, wherein the neutrinos are pseudo-Dirac in nature. The Dirac mass term for neutrinos arises from two-loop quantum corrections, whereas the Majorana mass terms are generated from Planck-induced corrections. This class of model also provides a parity solution to the strong C P problem without the need for an axion. We show an interesting correlation between the lifetime of the DM and the mass-squared differences between active and sterile neutrinos while maintaining a solution to the strong C P problem. Published by the American Physical Society 2025

Biswas, Sumit (ORCID:0009000561143501)↗
DOE OSTI2025

First Search for Dark Photon Dark Matter with a madmax Prototype

We report the first result from a dark photon dark matter search in the mass range from 78.62 to 83.95 μ eV / c 2 with a dielectric haloscope prototype for (Magnetized Disc and Mirror Axion eXperiment). Putative dark photons would convert to detectable photons within a stack consisting of three sapphire disks and a mirror. The emitted power of this system is received by an antenna and successively digitized using a low-noise receiver. No significant signal attributable to dark photons has been observed above the expected background. Assuming unpolarized dark photon dark matter with a local density of ρ χ = 0.3 G eV cm 3 we exclude a dark photon to photon mixing parameter χ > 2.7 × 10 − 12 over the full mass range and χ > 1.1 × 10 − 13 at a mass of 80.57 μ eV / c 2 with a 95% confidence level. This is the first physics result from a prototype and exceeds previous constraints on χ in this mass range by up to almost three orders of magnitude. Published by the American Physical Society 2025

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Metamagnetism of few-layer topological antiferromagnets

MnBi 2 Te 4 (MBT) materials are a promising class of antiferromagnetic topological insulators whose films provide access to novel and technologically important topological phases, including quantum anomalous Hall states and axion insulators. MBT device behavior is expected to be sensitive to the various collinear and noncollinear magnetic phases that are accessible in applied magnetic fields. Here, we use classical Monte Carlo simulations and electronic structure models to calculate the ground state magnetic phase diagram as well as topological and optical properties for few-layer films with up to six septuple layers. Using magnetic interaction parameters appropriate for MBT, we find that it is possible to prepare a variety of different magnetic stacking sequences, some of which have sufficient symmetry to disallow nonreciprocal optical response and Hall transport coefficients. Other stacking arrangements do yield large Faraday and Kerr signals, even when the ground state Chern number vanishes.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Ferromagnetic MnBi 4 Te 7 obtained with low-concentration Sb doping: A promising platform for exploring topological quantum states

The tuning of the magnetic phase, chemical potential, and structure is crucial to observe diverse exotic topological quantum states in Mn Bi 2 Te 4 (Bi 2 Te 3 ) m (m = 0–3). Here we show a ferromagnetic (FM) phase with a chiral crystal structure in Mn (Bi 1–x Sb x ) 4 Te 7 , obtained via tuning the growth conditions and Sb concentration. Unlike previously reported Mn (Bi 1–x Sb x ) 4 Te 7 , which exhibits FM transitions only at high Sb doping levels, our samples show FM transitions (T C = 13.5 K) at 15%–27% doping levels. Furthermore, our single-crystal x-ray-diffraction structure refinements find Sb doping leads to a chiral structure with the space group of P3, contrasted with the centrosymmetric $P\bar{3}m1$ crystal structure of the parent compound MnBi 4 Te 7 . Through angle-resolved photoemission spectroscopy measurements, we also demonstrated that the nontrivial band topology is preserved in the Sb-doped FM samples. Given that the nontrivial band topology of this system remains robust for low Sb doping levels, our success in making FM Mn(Bi 1–x Sb x ) 4 Te 7 with x = 0.15, 0.175, 0.2, and 0.27 paves the way for realizing the predicted topological quantum states, such as the axion insulator and Weyl semimetals. Additionally, we also observed magnetic glassy behavior in both antiferromagnetic MnBi 4 Te 7 and FM Mn (Bi 1–x Sb x )4 Te 7 samples, which we believe originates from cluster spin-glass phases coexisting with long-range antiferromagnetic/FM orders. Further, we have also discussed how the antisite Mn ions impact the interlayer magnetic coupling and how FM interlayer coupling is stabilized in this system.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Site Mixing for Engineering Magnetic Topological Insulators

The van der Waals compound, MnBi 2 Te 4 , is the first intrinsic magnetic topological insulator, providing a materials platform for exploring exotic quantum phenomena such as the axion insulator state and the quantum anomalous Hall effect. However, intrinsic structural imperfections lead to bulk conductivity, and the roles of magnetic defects are still unknown. With higher concentrations of the same types of magnetic defects, the isostructural compound MnSb 2 Te 4 is a better model system for a systematic investigation of the connections among magnetism, topology, and lattice defects. In this work, the impact of antisite defects on the magnetism and electronic structure is studied in MnSb 2 Te 4 . Mn-Sb site mixing leads to complex magnetic structures and tunes the interlayer magnetic coupling between antiferromagnetic and ferromagnetic. The detailed nonstoichiometry and site mixing of MnSb2Te4 crystals depend on the growth parameters, which can lead to ≈40% of Mn sites occupied by Sb and ≈15% of Sb sites by Mn in as-grown crystals. Single-crystal neutron diffraction and electron microscopy studies show nearly random distribution of the antisite defects. Band structure calculations suggest that the Mn-Sb site mixing favors a ferromagnetic interlayer coupling, consistent with experimental observation, but is detrimental to the band inversion required for a nontrivial topology. Overall, our results suggest a long-range magnetic order of Mn ions sitting on Bi sites in MnBi 2 Te 4 . The effects of site mixing should be considered in all layered heterostructures that consist of alternating magnetic and topological layers, including the entire family of MnTe(Bi 2 Te 3 )n, its Sb analogs, and their solid solution.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

Defect-induced displacement of topological surface state in quantum magnet MnBi2Te4

The topological magnet MnBi2⁢Te4 (MBT), with gapped topological surface state, is an attractive platform for realizing quantum anomalous Hall and axion insulator states. However, the experimentally observed surface state gaps fail to meet theoretical predictions, although the exact mechanism behind the gap suppression has been debated. Recent theoretical studies suggest that intrinsic antisite defects push the topological surface state away from the MBT surface, closing its gap and making it less accessible to scanning probe experiments. Here, we report on the local effect of defects on the MBT surface states and demonstrate that high defect concentrations lead to a displacement of the surface states well into the MBT crystal, validating the theorized mechanism. The local and global influence of antisite defects on the topological surface states are studied with samples of varying defect densities by combining scanning tunneling microscopy, angle-resolved photoemission spectroscopy, and density functional theory. Our findings identify a combination of increased defect density and reduced defect spacing as the primary factors underlying the displacement of the surface states and suppression of surface gap, guiding further development of topological quantum materials.

Lupke, Felix [Carnegie Mellon University (CMU)]↗