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At least 649 records · Page 36

Acoustic response of a rectangular waveguide with a strong transverse temperature gradient

An acoustic wave equation was developed for a perfect gas with spatially-variable temperature. The strong-gradient wave equation was used to analyze the response of a rectangular wave guide containing a thermally-stratified gas. It was assumed that the temperature gradient is constant, representing one-dimensional heat transfer with a constant coefficient of conductivity. The analysis of the waveguide shows that the resonant frequencies of the waveguide are shifted away from the values that would be expected from the average temperature of the waveguide. For small gradients, the frequency shift is proportional to the square of the gradient. The factor of proportionality is a quadratic function of the natural frequency of the waveguide with uniform temperature. An experiment is designed to verify the essential features of the strong-gradient theory.

Zorumski, William E.↗

Superconducting Films for Absorber-coupled MKID Detectors for Sub-millimeter and Far-infrared Astronomy

We describe measurements of the properties, at dc, gigahertz, and terahertz frequencies, of thin superconducting films with relatively high normal state sheet resistance. Such films can be applied to construct microwave kinetic inductance detector sensor arrays for submillimeter and far-infrared astronomical applications in which the incident power excites quasiparticles directly in a superconducting resonator that is configured to present a matched-impedance to the high frequency radiation being detected. For several materials, and a range of thicknesses down to 10 nm, we present measurements of normal state sheet resistance, resistance-temperature curves for the superconducting transition, quality factor and kinetic inductance fraction for microwave resonators made from patterned films, and terahertz measurements of the sheet impedance measured with a Fourier Transform Spectrometer.

Stevenson, T. R.↗

Probing Non-Equilibrium Pair-Breaking and Quasiparticle Dynamics in Nb Superconducting Resonators Under Magnetic Fields

We conducted a comprehensive study of the non-equilibrium dynamics of Cooper pair breaking, quasiparticle (QP) generation, and relaxation in niobium (Nb) cut from superconducting radio-frequency (SRF) cavities, as well as various Nb resonator films from transmon qubits. Using ultrafast pump–probe spectroscopy, we were able to isolate the superconducting coherence and pair-breaking responses. Our results reveal both similarities and notable differences in the temperature- and magnetic-field-dependent dynamics of the SRF cavity and thin-film resonator samples. Moreover, femtosecond-resolved QP generation and relaxation under an applied magnetic field reveals a clear correlation between non-equilibrium QPs and the quality factor of resonators fabricated by using different deposition methods, such as DC sputtering and high-power impulse magnetron sputtering. These findings highlight the pivotal influence of fabrication techniques on the coherence and performance of Nb-based quantum devices, which are vital for applications in superconducting qubits and high-energy superconducting radio-frequency applications.

43 PARTICLE ACCELERATORS↗

Energetics and dynamics of resonant and nonresonant scattering in strong magnetic fields

The energetics and the dynamics resulting from electron-photon resonant and nonresonant scattering in a plasma with magnetic field about 10 to the 12th G are studied in detail. Precise analytic results are obtained in the optically thin limit, and numerical results are presented for the optically thick case. For the latter, it is found that when the equilibrium temperature T(C) is determined by the cooling/heating balance due solely to cyclotron resonant scattering, the ratio of T(C) to the superstrong field B remains fairly constant for N(e) up to about 6 x 10 to the 21st electrons/sq cm. This line-dominated region comes to an end when the extra heating from the hard continuum photons becomes competitive with the line processes and drives T(C) well above the pure line value. For parameters characteristic of GB 880205, the thickness of the line-dominated region is determined to be between 10 to the 21st and 10 to the 22nd electrons/sq cm.

Lamb, Don Q.↗

Impact of microstructure on elastic properties in the alloy Ti-42Al-8.5 Nb

The microstructure of a γ-TiAl alloy containing niobium undergoes continuous transformations during annealing at 550 °C. These take place within the α 2 -phase of lamellar (α 2 +γ) colonies. We have characterized these changes by transmission electron microscopy and made a correlation to the elastic constants determined by resonant ultrasonic spectroscopy during in-situ annealing at the same temperature. Further, the results show a continuous increase of the E-modulus. This can be attributed to elastic strains acting within α 2 lamellae as a result of lattice transformations. After 5000h, a thermodynamic equilibrium was established with equal fractions of α 2 -phase and O-phase that differ only in lattice symmetry and Nb content. Generally, the presence of O-phase should contribute to lower elastic moduli, however in the present case the evolving microstructural characteristics were responsible for the observed increase in the E-modulus.

36 MATERIALS SCIENCE↗

Tuning Hybrid exciton–Photon Fano Resonances in Two-Dimensional Organic–Inorganic Perovskite Thin Films

As easy-to-grow quantum wells with narrow excitonic features at room temperature, two-dimensional (2D) Ruddleson–Popper perovskites are promising for realizing novel nanophotonic devices based on exciton–photon interactions. Here, we demonstrate a distinct hybrid exciton–photon Fano resonance in (C 4 H 9 NH 3 ) 2 PbI 4 thin films prepared via spin coating. Using a classical coupled-oscillator model and finite-difference time-domain simulations, we link the Fano interference to the coupling of the exciton with the Rayleigh-like scattering of the film microstructure. Combining colloidal plasmonic cavities with the 2D perovskite films, we demonstrate tuning of the Fano resonance. In combination with silver nanoparticles, the exciton–photon Fano interference couples to the in-plane plasmonic modes with indications of Rabi splitting. By creating a nanoparticle on mirror geometry, we address the out-of-plane excitonic component, reaching an intermediate coupling regime. Furthermore, these structures suggest possible photonic targets for biomolecular self-assembly applications.

2D perovskites↗

Mass loss from red giants - Results from ultraviolet spectroscopy

New instrumentation in space, primarily the IUE spacecraft, has enabled the application of ultraviolet spectroscopic techniques to the determination of physical properties and reliable mass loss rates for red giant winds. One important result is the determination of where in the H-R diagram are found stars with hot outer atmospheres and with cool winds. So far it appears that single cool stars, except perhaps the so-called hybrid stars, have either hot outer atmospheres or cool winds but not both. The C II resonance (1335 A) and intersystem (2325 A) multiplets have been used to derive temperatures, densities, and geometrical extents for the chromospheric portions of red giant winds, with the result that the red giants and the earlier giants with hot coronae have qualitatively different chromospheres. Mass loss rates can now be derived accurately from the analysis of asymmetric emission lines, such as the Mg II resonance lines, and from P Cygni profile lines of atoms in the dominant ionization stage when a hot star is available to probe the wind of a red giant. The Zeta Aur systems, consisting of a K-M supergiant and a main sequence B star are important systems for reliable mass loss rates for the red supergiant components are becoming available.

Linsky, J. L.↗

In situ electric-field control of ferromagnetic resonance in the low-loss organic-based ferrimagnet V[TCNE] x ∼2

We demonstrate indirect electric-field control of ferromagnetic resonance (FMR) in devices that integrate the low-loss, molecule-based, room-temperature ferrimagnet vanadium tetracyanoethylene (V[TCNE]x∼2) mechanically coupled to PMN-PT piezoelectric transducers. Upon straining the V[TCNE]x films, the FMR frequency is tuned by more than 6 times the resonant linewidth with no change in Gilbert damping for samples with α = 6.5 × 10−5. We show this tuning effect is due to a strain-dependent magnetic anisotropy in the films and find the magnetoelastic coefficient |λs| ∼ (1–4.4) ppm, backed by theoretical predictions from density-functional theory calculations and magnetoelastic theory. Noting the rapidly expanding application space for strain-tuned FMR, we define a new metric for magnetostrictive materials, magnetostrictive agility, given by the ratio of the magnetoelastic coefficient to the FMR linewidth. This agility allows for a direct comparison between magnetostrictive materials in terms of their comparative efficacy for magnetoelectric applications requiring ultra-low loss magnetic resonance modulated by strain. With this metric, we show V[TCNE]x is competitive with other magnetostrictive materials, including YIG and Terfenol-D. This combination of ultra-narrow linewidth and magnetostriction, in a system that can be directly integrated into functional devices without requiring heterogeneous integration in a thin film geometry, promises unprecedented functionality for electric-field tuned microwave devices ranging from low-power, compact filters and circulators to emerging applications in quantum information science and technology.

Materials Science↗

Resonance scattering of Fe XVII - A density diagnostic

Resonance scattering of the 15.01 A Fe XVII line, found to be important by Rugge & McKenzie, provides a new density diagnostic for solar active regions that is not subject to the lower density limit of the competing diagnostic. For a 'typical' active region, over 50 percent of the photons for this resonance line could be scattered out of the line of sight. The effect is much stronger for this line than for any other line in the soft X-ray part of the spectrum used routinely to determine active region electron temperatures, emission measures, or densities. Once understood and accounted for in the analysis, the resonance scattering of the 15.01 A Fe XVII line leads to a direct measurement of the density of the active region plasma. In the four active regions studied here, the derived densities range is 1-4 x 10 exp 9/cu cm.

Schmelz, J. T.↗

Magnetism and spin dynamics in room-temperature van der Waals magnet Fe 5 GeTe 2

Two-dimensional van der Waals (vdWs) materials have gathered a lot of attention recently. However, the majority of these materials have Curie temperatures that are well below room temperature, making it challenging to incorporate them into device applications. In this work, we synthesized a room-temperature vdW magnetic crystal Fe 5 GeTe 2 with a Curie temperature T c = 332 K, and studied its magnetic properties by vibrating sample magnetometry (VSM) and broadband ferromagnetic resonance (FMR) spectroscopy. The experiments were performed with external magnetic fields applied along the c -axis (H∥ c ) and the ab -plane (H∥ ab ), with temperatures ranging from 300 to 10 K. We have found a sizable Landé g -factor difference between the H∥ c and H∥ ab cases. In both cases, the Landé g -factor values deviated from g = 2. This indicates contribution of orbital angular momentum to the magnetic moment. The FMR measurements reveal that Fe 5 GeTe 2 has a damping constant comparable to Permalloy. With reducing temperature, the linewidth was broadened. Together with the VSM data, our measurements indicate that Fe 5 GeTe 2 transitions from ferromagnetic to ferrimagnetic at lower temperatures. Our experiments highlight key information regarding the magnetic state and spin scattering processes in Fe 5 GeTe 2 , which promote the understanding of magnetism in Fe 5 GeTe 2 , leading to implementations of Fe 5 GeTe 2 based room-temperature spintronic devices.

36 MATERIALS SCIENCE↗

Detecting rare earth elements via optically detected magnetic resonance (ODMR) and spin-relaxometry using nitrogen vacancy centers in nanodiamonds

Nanodiamonds embedded with nitrogen-vacancy (NV) centers are emerging as powerful tools in quantum sensing due to their remarkable sensitivity to local variations in electromagnetic fields, temperature, and pressure. These point defects in the diamond lattice can be probed using optically detected magnetic resonance (ODMR) and spin relaxometry techniques, allowing for the detection and characterization of magnetic nanoparticles and ions. The sensing mechanism relies on laser-induced excitation of the NV center's non-degenerate triplet ground state, which promotes electrons to an excited state. Subsequent photoluminescence (PL) emission, which is spin-state dependent, is then measured. These spin states are highly responsive to magnetic perturbations in the surrounding environment. By analyzing changes in the ODMR spectra and spin relaxation times, we can effectively monitor how magnetic species influence the NV center's spin dynamics, thus enabling sensitive and selective characterization of nanoscale magnetic materials. These techniques have been applied for the characterization of transition metals and rare earth elements which shows natural ferromagnetic properties.

magnetic nanopartgicles and ions↗

Kinetics of the reaction O + ClO yields Cl + O2

The bimolecular rate constant for the reaction O + ClO yields Cl + O2 has been measured over the temperature range 236-422 K in a discharge flow system using atomic oxygen resonance fluorescence at 130 nm to monitor the decay of O in an excess of ClO. The results are found to be independent of the method used to produce the ClO radical. At 296 K, the rate constant is given by (3.6 + or - 0.7) x 10 to the -11th cu cm/sec and the temperature dependence expressed in Arrhenius form by k2 = (5.0 + or - 1.0) x 10 to the -11th exp-(96 + or - 20)/T cu cm/sec. The results are compared with earlier values, and the implications for stratospheric chemistry are discussed briefly.

Leu, M.-T.↗

Fabrication and Preliminary Demonstration of Microwave Resonant Cavity Transducer Performance

We are investigating a microwave cavity-based transducer for in-core high-temperature fluid flow sensing in molten salt cooled reactors (MSCR) and sodium fast reactors (SFR). This sensor is a hollow metallic cylindrical cavity, which can be fabricated from stainless steel, and as such is expected to be resilient to radiation, high temperature and corrosive environment of MSCR and SFR. The principle of sensing consists of making one wall of the cylindrical cavity flexible enough so that dynamic pressure, which is proportional to fluid velocity, will cause membrane deflection. Membrane deflection causes cavity volume change, which leads to a shift in the resonant frequency. We have developed an initial design for proof-of-principle testing of the flow sensor performance in microwave K-band. A cylindrical resonator prototype was fabricated from brass for initial tests in water. The cavity size is matched to the flange of a standard WR-42 waveguide. Microwave field is coupled into the resonant cavity through a subwavelength-size aperture. A test article was developed, consisting of a piping Tee with bulkhead WR-42 microwave waveguide installed in leak-proof design. In the test article, the cylindrical cavity is positioned in the center of the pipe. A microwave waveguide circulator was installed in the setup to suppress microwave reflections at the cavity entrance. Preliminary spectral characterization of cavity spectral response was performed with microwave VNA. Applying mechanical pressure to cavity membrane showed a measurable shift in the microwave resonant frequency. We also investigate mechanical integrity of the flowmeter’s membrane through computer simulations. By calculating the stress on the plate due to deflection and, comparing the stress to the material ultimate tensile strength and yield strength, it can be estimated if the plate will fail. The stress on the plate was calculated with an analytic closed form solution model, and with COMSOL Structural Mechanics Module which does not involve any approximations. Both the analytic model and COMSOL model showed that maximum stresses on the plate, which are at the radial boundary of the plate, are three orders of magnitude smaller than the yield strength and ultimate tensile strength. This indicates that the sensor is at a low risk of mechanical failure.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Stabilizing Microwave Frequency of a Photonic Oscillator

A scheme for stabilizing the frequency of a microwave signal is proposed that exploits the operational characteristics of a coupled optoelectronic oscillator (COEO) and related optoelectronic equipment. An essential element in the scheme is a fiber mode-locked laser (MLL), the optical frequency of which is locked to an atomic transition. In this scheme, the optical frequency stability of the mode-locked laser is transferred to that of the microwave in the same device. Relative to prior schemes for using wideband optical frequency comb to stabilize microwave signals, this scheme is simpler and lends itself more readily to implementation in relatively compact, rugged equipment. The anticipated development of small, low-power, lightweight, highly stable microwave oscillators based on this scheme would afford great benefits in communication, navigation, metrology, and fundamental sciences. COEOs of various designs, at various stages of development, in some cases called by different names, have been described in a number of prior NASA Tech Briefs articles. A COEO is an optoelectronic apparatus that generates both short (picosecond) optical pulses and a steady microwave signal having an ultrahigh degree of spectral purity. The term "coupled optoelectronic" in the full name of such an apparatus signifies that its optical and electronic oscillations are coupled to each other in a single device. The present frequency-stabilization scheme is best described indirectly by describing the laboratory apparatus used to demonstrate it. The apparatus (see figure) includes a COEO that generates a comb-like optical spectrum, the various frequency components of which interfere, producing short optical pulses. This spectrum is centered at a nominal wavelength of 1,560 nm. The spectrum separation of this comb is about 10 GHz, as determined primarily by the length of an optical loop and the bandpass filter in the microwave feedback loop. The optical loop serves as microwave resonator having a very high value of the resonance quality factor (Q). The optical frequency of MLL is then stabilized by locking it to an atomic transition as described below. The COEO contains a tunable 1-nm band-pass optical filter and a piezoelectric-transducer (PZT) drum over which a stretch of fiber is wound. The 1-nm-wide pass band of the filter provides coarse tuning to overlap the frequency comb with the atomic transition frequency. Controlled stretching of the fiber by means of the PZT drum can be used in conjunction with temperature control for locking the laser frequency. To reference to an atomic resonance at 780 nm in this demonstration setup, the optical output of the COEO at 1,560 nm is fed through an erbium-doped-fiber amplifier (EDFA) to a frequency doubler in the form of a periodically poled lithium niobate (PPLN) crystal. The frequency-doubled output is combined with the output of a separate frequency-stabilized diode laser at a photodetector. As described thus far, the two 780-nm laser subsystems are nominally independent of each other and can, therefore, operate at different frequencies. Hence, at the photodetector, the two laser beams interfere, so that the output of the photodetector includes a beat note (a component at the difference between the two laser frequencies).

Maleki, Lute↗

Terahertz magneto-nanoscopy of encapsulated monolayer graphene

This study investigates the nanoscale conductivity of encapsulated monolayer graphene at temperatures down to 5 K and magnetic fields of up to 1 T. We use the scattering-type scanning near-field optical microscopy technique to probe magnetic-field-dependent responses from graphene close to charge neutrality in the terahertz spectral region. We observe the near-perfect high-q reflector behavior of graphene but with subtle changes by the presence of magnetic fields. Measurements align with calculations of the magneto-optical conductivity and the near-field spectroscopic contrast that describes the field-tunable cyclotron resonance of Dirac fermions. Our result provides an initial step toward understanding temperature and magnetic field effects on nanoscale terahertz transport in two-dimensional quantum materials.

Kim, Richard H. J. [Ames Laboratory (AMES), Ames, ↗

Backscatter of solar resonance radiation. I.

Calculation of the angular dependence of the intensity of solar Lyman alpha resonantly scattered from neutral interstellar hydrogen which has penetrated the solar system. A simple model which essentially neglects temperature effects, but which includes gravity, radiation pressure, photoionization and charge exchange is used for this calculation. The results are then compared with the observations. The resonant scattering of He I 584 A is also treated.

Johnson, H. E.↗

Magnetostrictive Ultrasonic Waveguide Transducer for In-Pile Thermometry

Real-time and reliable temperature measurement on nuclear fuels is crucial for the safe operation of existing pressurized-water reactors and future advanced nuclear reactors. Magnetostrictive materials deform when subjected to a magnetic field or exhibit magnetization variation when stressed. Here, based on these properties, this study prototyped an ultrasonic thermometer (UT) consisting of a magnetostrictive waveguide, a dc coil providing appropriate magnetic biasing, and an ac coil generating an acoustic impulse and detecting the resulting acoustic echoes. By tracking the time of flight between the excitation pulse and the echoes, the UT can potentially detect nuclear fuel cladding temperature from a long distance. In this study, magnetostrictive iron–gallium alloys, or Galfenol, were selected as the waveguide due to their large magnetostriction, superior temperature survivability, excellent radiation resilience, and high mechanical robustness. A multiphysics finite-element model considering electrical, magnetic, and mechanical dynamics in the magnetostrictive UT was then developed. The model exhibited an error of 0.24% in time-of-flight simulation and, therefore, enabled computer-aided design and guided signal processing. Between room temperature and 120 °C, the new Galfenol-based UT exhibits a linear sensitivity of 162.8×10 ₋6 °C ₋1 , which is 51.7% higher than a previous magnetostrictive UT based on iron–cobalt–vanadium alloys.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Measurements of the dielectric properties of sea water at 1.43 GHz

Salinity and temperature of water surfaces of estuaries and bay regions are determined to accuracies of 1 ppt salinity and 0.3 kelvin surface temperature. L-band and S-band radiometers are used in combination as brightness temperature detectors. The determination of the brightness temperature versus salinity, with the water surface temperature as a parameter for 1.4 GHz, is performed with a capillary tube inserted into a resonance cavity. Detailed analysis of the results indicates that the measured values are accurate to better than 0.2 percent in the electric property epsilon' and 0.4 percent in epsilon''. The calculated brightness temperature as a function of temperature and salinity is better than 0.2 kelvin. Thus it is possible to reduce the measured data obtained with the two-frequency radiometer system with 1 ppt accuracy to values in the salinity range 5 to 40 ppt.

Ho, W. W.↗