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At least 649 records · Page 36

Development of a Research Reactor Protocol for Neutron Multiplication Measurements

Establishing a protocol for measurements on research reactors is the next step in advanced subcritical neutron multiplication inference measurements. Such measurements can help identify deficiencies and quantify uncertainties in nuclear data and validate predictive Monte Carlo radiation transport simulation capabilities related to subcritical neutron multiplication inference techniques. This work expands on previous benchmark-quality efforts performed at the National Criticality Experiments Research Center (NCERC) located in Nevada, including subcritical experiments with a 4.5-kg {alpha}-phase plutonium sphere surrounded by copper, tungsten and nickel. Evaluations of the nickel and tungsten measurements have both been accepted into the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Handbook. The nickel benchmark was the first ICSBEP-accepted evaluation of measurements using the Feynman Variance-to-Mean method based on the Hage-Cifarelli formulism, and was the culmination of many years of subcritical experiment research. To help establish a protocol for research reactor-based subcritical measurements, a series of Critical and Subcritical {Phi}-Power Experiments at Rensselaer (CaSPER) have been designed. This neutron multiplication measurement series will be executed at the Rensselaer Polytechnic Institute Walthousen Reactor Critical Facility (RPI-RCF) in upstate New York. The RPI reactor facility can provide benchmark-quality integral experimental configurations where different reactivity states can be achieved by varying the control rod height/water height in the reactor. The diversity of achievable configurations are also unique in contrast to previous subcritical benchmark measurements in that they are spatially complex, involve different materials (fuel, moderator), and are characterized by system-specific neutron cross section sensitivities (various energy ranges and neutron reaction contributions). It is worth noting that previous proof-of-concept subcritical measurements have been performed on thermal systems at NCERC, at a variety of reactivity states by separation distance, yet it was not possible to know the reactivity of various configurations accurately for benchmarking (there are no control rod worth curves as there are no control rods). (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Assembling Multiple Models Within the RAVEN Framework

RAVEN (Risk Analysis Virtual Environment) is an INL-developed software tool that can be used to identify and increase the safety margin in complex systems. As a generic software framework, RAVEN is designed to perform parametric and probabilistic analysis based on the response of complex system codes. RAVEN is capable of investigating the system response as well as the input space using Monte Carlo, Grid, or Latin Hyper Cube sampling schemes, but its strength is focused toward system feature discovery, such as limit surfaces, separating regions of the input space leading to system failure, using dynamic supervised learning techniques. RAVEN is currently able to construct multi-targets Reduced Order Models (ROMs), which are aimed to represent the response of a system (in a fixed configuration) for multiple Figures of Merits (FOMs) and time-dependent ROMs. These capabilities represent the initial steps for a larger implementation about the interaction of multiple models. In fact, in several cases, multiple models need to interface with each other since the initial conditions of one are dependent on the outcomes of another. To better understand the problem that here is solved, it is useful to consider a simple example: The following problem is considered: a weather forecast simulation code 'a' is used to compute the external (i.e. ambient) temperature in a certain location. A second model 'b' is inquired to compute the average temperature in a room having as boundary condition, among several others, the external ambient temperature. The response of the model 'b' depends on the outcome of the model 'a'. The reported example is only aimed to illustrate the reason why the creation of a framework to make interact different models is a key development for the advancement of RAVEN as a comprehensive calculation flow driver. Before reporting how the ensemble-models have been implemented, it is necessary to briefly describe the representative Model 'entities' that are available in RAVEN.

42 ENGINEERING↗

Design of Nuclear Criticality Safety Framework for Hands-on Construction of Fast Systems Over Ranges of Multiplication

Since 1945, Los Alamos National Laboratory (LANL) has performed critical experiments, primarily at the Los Alamos Critical Experiments Facility (LACEF) at Technical Area 18 (TA-18). Since 2011, these experiments have been conducted by the National Criticality Experiments Research Center (NCERC), operated by LANL, at the Device Assembly Facility (DAF) in the Nevada National Security Site (NNSS). These experiments utilize various types of Special Nuclear Material (SNM). Some of these experiments utilize what is referred to as the Rocky Flat Shells, which are called such as they came from the Rocky Flats Plant. These concentric hemi-shells are made of Highly Enriched Uranium (HEU), which is 93 w/o 235U. Fig. 1. Subset of the Rocky Flat Shells LANL is designing a new subcritical hands-on experiment with the goal of achieving a neutron multiplication in the range of 50 to 200, which correlates to Keff values of 0.98 to 0.995. ANSI/ANS-1 is the standard for Conduct of Critical Experiments which governs critical operations at NCERC. Section 3.9 of ANSI/ANS-1 states that when manipulating a critical assembly by hand, the predicted k eff of a known configuration should not exceed 0.95 (a neutron multiplication of 20). This presents a challenge, as this system would have a higher multiplication than 20 and the assembly would have to remain subcritical in normal and credible accident scenarios. To ensure the safety of such an assembly, the different normal and abnormal conditions that could alter the criticality 1 MCNP® and Monte Carlo N-Particle® are registered trademarks owned by Triad National Security, LLC, manager and operator of Los Alamos National Laboratory. Any third party use of such registered marks should be properly of the system must be considered and analyzed. If such a condition is deemed to be credible, it will be further investigated using the Monte Carlo N-Particle (MCNP) transport code. If the results of these simulations show that a k eff larger than one could be possible, modifications to the assembly will be made until such an event is deemed no longer possible.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Vortex-Controlled Quasiparticle Multiplication and Self-Growth Dynamics in Superconducting Resonators

Even in the quantum limit, non-equilibrium quasiparticle (QP) populations induce QP poisoning that irreversibly relaxes the quantum state and significantly degrades the coherence of transmon qubits. A particularly detrimental yet previously unexplored mechanism arises from QP multiplication facilitated by vortex trapping in superconducting quantum circuits, where a high-energy QP relaxes by breaking additional Cooper pairs and amplifying the QP population due to the locally reduced excitation gap and enhanced quantum confinement within the vortex core. Here we directly resolve this elusive QP multiplication process by revealing vortex-controlled QP self-generation in a highly nonequilibrium regime preceding the phonon bottleneck of QP relaxation. At sufficiently low fluence, femtosecond-resolved magneto-reflection spectroscopy directly reveals a continuously increasing QP population that is strongly dependent on magnetic-field-tuned vortex density and absent at higher excitation fluences. Quantitative analysis of the emergent QP pre-bottleneck dynamics further reveals that, although the phonon population saturates within $\simeq$10~ps, both free and trapped QPs continue to grow in a self-sustained manner--hallmarks of the long-anticipated QP-vortex interactions in nonequilibrium superconductivity. We estimate a substantial increase of $\sim$34% in QP density at vortex densities of $\sim$ 100 magnetic flux quanta per $\mathrm{μm^{2}}$. Our findings establish a powerful spectroscopic tool for uncovering QP multiplication and reveal vortex-assisted QP relaxation as a critical materials bottleneck whose mitigation will be essential for resolving QP poisoning and enhancing coherence in superconducting qubits.

Park, Joong M. [Ames Lab]↗

Method for measuring multiple scattering corrections between liquid scintillators

In this study, a time-of-flight method is proposed to experimentally quantify the fractions of neutrons scattering between scintillators. An array of scintillators is characterized in terms of crosstalk with this method by measuring a californium source, for different neutron energy thresholds. The spectral information recorded by the scintillators can be used to estimate the fractions of neutrons multiple scattering. With the help of a correction to Feynman's point model theory to account for multiple scattering, these fractions can in turn improve the mass reconstruction of fissile materials under investigation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Contribution of higher multiplicity collisions to elastic p{sup 6,8}He and p{sup 8,9}Li scattering within Glauber theory

Differential cross sections for elastic p{sup 6,8}He and p{sup 8,9}Li scattering at energies between 60 and 70 MeV per nucleon and at the energy of 700 MeV per nucleon were calculated. The calculations in question were performed with the wave functions found on the basis of the α–n–n (for {sup 6}He), α–t–n (for {sup 8}Li), and α–t–2n (for {sup 9}Li) three-body models and with the density from the large-scale shell model for the {sup 8}He nucleus. The respective matrix elements were derived either upon taking fully into account the multiple-scattering operator or in the optical-limit approximation. A comparison of the results of the precise and approximate calculations made it possible to estimate reliably the contribution of higher multiplicity collisions to the differential cross sections.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multiple‐Repeated Plasma Surface Treatments for Significantly Improving Bonding Performance of Metal‐Carbon‐Fiber‐Reinforced Thermoplastic Polymer Dissimilar Adhesive Joints

This work investigates how multiple‐repeated plasma surface treatments can significantly enhance adhesively bonded metal‐carbon‐fiber‐reinforced thermoplastic polymer (CFRTP) dissimilar joints, a topic that has been rarely investigated compared to other parameters during the plasma treatment process. By conducting double cantilever beam tests on adhesively bonded AA6061‐carbon‐fiber‐reinforced polyphthalamide (CFRPPA) dissimilar joints, it is shown that the average Mode I specific fracture energy after 20 repetitions of the same plasma treatment, using processing parameters without noticeably changing surface roughness, can be improved and saturated up to almost 2000% compared to non‐treated joints and almost 240% compared to a single plasma treatment commonly used in the literature. The improvement can be attributed to the enhanced chemical bonding at the CFRPPA‐adhesive interface. This study is important for achieving strong bonding performance of CFRTP‐related structural joints using multiple plasma treatments, a simple and effective method.

36 MATERIALS SCIENCE↗

Topology property analysis and application of stable time-delay regions for linear multiple time-delay systems

This study examines the relationship between the topology of stable time-delay regions and the stability analysis of an linear multiple time delay system. To analyze the topology of stable time-delay regions, we construct a function with a value equal to zero for the time-delay points on the boundaries of stable time-delay regions. The function is continuous and differentiable in the whole defining field with a global minimum of zero so that we can locate the boundaries by minimizing the value of the function. Based on the topology analysis, we proposed a performance validation approach for controllers that are designed to stabilize the system using feedback signals with time delays. The method based on the topology analysis is simple and reliable so that can deal with a linear time-invariant system with high order and multiple time delays (more than 3). The example case study shows that the above method is reliable and enables ultra-low latency coordination and control for the future power grid with ubiquitous power electronics.

24 POWER TRANSMISSION AND DISTRIBUTION↗

Multiplicity dependence of (multi-)strange hadrons in oxygen-oxygen collisions at $\sqrt{s_{NN}}$ TeV using EPOS4 and AMPT

It is anticipated that the Large Hadron Collider (LHC) will collect data from oxygen-oxygen (O+O) collisions at a center-of-mass energy of $\sqrt{s_{NN}}$ = 7 TeV to explore the effects observed in high multiplicity proton-proton (p+p) and proton-lead (p+pb) collisions that closely related to lead-lead (Pb+Pb) collisions. Furthermore, these effects include azimuthal asymmetries in particle production, as well as variations in the abundances and momentum distributions across different hadron species, which are indicative of collective particle production mechanisms induced by the interactions in the presence of a QGP. The upcoming data on O+O collisions at the LHC are expected to constrain the model parameters and refine our understanding of theoretical models. In this work, the predicted transverse momentum (p T ) spectra, rapidity density distributions (dN/dy), particle yield ratios, and p T -differential ratios of (multi)strange hadrons produced in O+O collisions at $\sqrt{s_{NN}}$ = 7 TeV using AMPT and EPOS4 models are presented. AMPT focuses on preformed hadronic interactions, while EPOS4 incorporates a QGP phase. Stronger radial flow in EPOS4 as compared to AMPT is also observed. AMPT incorporates some flow effects, but the implementation of full hydrodynamic flow in EPOS4 appears to be significantly more effective in reproducing the existing experimental data. Both models predict the final state multiplicity overlap with p+p, p+pb, and Pb+Pb collisions.

Heavy-ion collisions↗

Cyclic loading–unloading impacts on geomechanical stability of multiple salt caverns for underground hydrogen storage

Underground caverns in a salt dome are promising geologic features to store hydrogen because of salt’s extremely low permeability and self-healing behavior. The salt cavern storage community, however, has not fully understood the geomechanical behaviors of salt rock driven by quick operation cycles of injection–production, which may significantly impact the cost-effective storage-recovery performance of multiple caverns. Our field-scale generic model captures the impact of cyclic loading–unloading on the salt creep behavior and deformation under different cycle frequencies, operating pressure, and spatial order of operating cavern(s). This systematic simulation study indicates that the initial operation cycle and arrangement of multiple caverns play a significant role in the creep-driven loss of cavern volumes and cavern deformation. Finally, our future study will develop a new salt constitutive model based on geomechanical tests of site-specific salt rock to probe the cyclic behaviors of salt precisely both beneath and above the dilatancy boundary, including reverse (inverse transient) creep, the Bauschinger effect, and damage-healing mechanism.

08 HYDROGEN↗

Low-stress creep behavior of multiple salt caverns under cyclic operations

Here, the use of multiple salt caverns for large-scale underground hydrogen storage offers a strategic solution to the growing demand for efficient and flexible energy storage, due to the inherent low permeability, high mechanical strength, and self-healing properties of the salt formation. Despite these advantages, the long-term geomechanical response of salt caverns under cyclic injection and withdrawal remains a significant challenge for ensuring operational stability. This mechanistic study highlights the critical role of low-stress creep, also known as pressure solution creep, in governing deformation of salt caverns during cyclic operations. Unlike conventional creep mechanisms that dominate under high-stress conditions, low-stress creep becomes particularly relevant under the moderate stress changes induced by repeated injection and withdrawal, which provides a previously underexplored control on cavern closure. Our three-dimensional computational model integrates the low-stress creep mechanism into the Munson–Dawson creep equation across a spectrum of operational scenarios including variations in cavern pressure cycles, injection-withdrawal frequencies, and caprock mechanical property. The low-stress creep components accelerate the cavern creep closure, which is amplified with shorter cycle frequency and larger pressure difference. Sensitivity analyses capture the complex interactions between multiple caverns and surround formations at the field scale that allows for a quantitative assessment of deformation patterns and closure rates over time and thereby informs the design and operation of sustainable underground hydrogen storage system.

Cyclic operation↗

Modeling multiple scattering transient of an ultrashort laser pulse by spherical particles

The multiple scattering of an ultrashort laser pulse by a turbid dispersive medium (namely a cloud of bubbles in water) is investigated by means of Monte Carlo simulations. The theory of Gouesbet and Gréhan (2000) is used to derive an energetic model of the scattering transient. It is shown that the spreading and extinction of the pulse can be decoupled from the transient of scattering, which allows to describe each phenomenon individually. The transient of scattering is modeled with the Lorenz-Mie Theory and thus is also valid for a relative refractive index lower than one, contrary to the Debye series expansion which does not converge close to the critical angle. This is made possible after the introduction of a new physical object, the Scattering Impulse Response Function (SIRF) which allows to detect the different modes of scattering transient, in time and direction. Here the present approach is more generic, as it enables to simulate clouds of air bubbles in water, which was not possible previously. Two different approaches are proposed within the Monte Carlo framework. The first is a pure Monte Carlo approach where the delay due to the scattering is randomly drawn at each event, while the second is based on the transport of the whole scattering signal. They are both embedded in the Monte Carlo code Scatter3D. Both models produce equivalent trends and are validated against published numerical results. They are then applied to the multiple scattering of ultra short pulse by a cloud of bubble in water in the forward direction. The pulse spread due to the propagation in water is computed for a wide range of traveled distances and pulse durations, and the optimal pulse duration is given to minimize the pulse spread at a given distance. The main result is that the scattered photons exit the turbid medium earlier than the ballistic photons and produce a double peak related to the refraction in the bubble. This demonstrates the possibility to develop new diagnostics to characterize dynamic bubbly flows.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

A time-parallel multiple-shooting method for large-scale quantum optimal control

Quantum optimal control plays a crucial role in quantum computing by providing the interface between compiler and hardware. Solving the optimal control problem is particularly challenging for multi-qubit gates, due to the exponential growth in computational complexity with the system's dimensionality and the deterioration of optimization convergence. To ameliorate the computational complexity of time-integration, this paper introduces a multiple-shooting approach in which the time domain is divided into multiple windows and the intermediate states at window boundaries are treated as additional optimization variables. Further, this enables parallel computation of state evolution across time-windows, significantly accelerating objective function and gradient evaluations. Since the initial state matrix in each window is only guaranteed to be unitary upon convergence of the optimization algorithm, the conventional gate trace infidelity is replaced by a generalized infidelity that is convex for non-unitary state matrices. Continuity of the state across window boundaries is enforced by equality constraints. A quadratic penalty optimization method is used to solve the constrained optimal control problem, and an efficient adjoint technique is employed to calculate the gradients in each iteration. We demonstrate the effectiveness of the proposed method through numerical experiments on quantum Fourier transform gates in systems with 2, 3, and 4 qubits, noting a speedup of 80x for evaluating the gradient in the 4-qubit case, highlighting the method's potential for optimizing control pulses in multi-qubit quantum systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Evaluation of neutron dosimetry capabilities with the MC-15 portable multiplicity counter

This work proposes a preliminary neutron dose rate estimation method for a neutron multiplicity detector through measurement- and simulation-based analyses. Uncharacterized neutron-emitting sources may be encountered in situations such as nuclear emergency response, safeguards, and treaty verification. These circumstances may present irradiation risk to personnel conducting field assay, search, and characterization measurements. It is therefore of interest to provide a field neutron dosimetry capability with the existing neutron multiplicity counting (NMC) capabilities. To date, no commercially-available neutron detection systems are capable of both accurate NMC and real-time neutron dosimetry. This work will focus on estimating dose rate using input from a single fielded NMC called the MC-15. The energy-dependent neutron detection efficiency response of the MC-15 was quantified in monoenergetic neutron simulations and evaluated in response to two neutron-emitting sources and to a polyethylene-moderated source. The results were compared to existing neutron dosimeters and established the proof of concept for further investigation of the MC-15 for dose estimation. Measurement results were also replicated in simulations; additional simulations were then conducted to expand upon the limited empirical data. The initial empirical results provided a conversion factor appropriate for use when measuring 252 Cf neutrons that is independent of polyethylene shielding presence and thickness. The simulated data sets were then used to evaluate a fit equation allowing estimation of the neutron dose rate for less restricted geometric configurations and dependent only on the distance between the source and the detector. Additionally, the energy dependence of the efficiency response indicates that further empirical evaluations could provide energy-dependent conversion factors for broader neutron dosimetry capabilities with a wider range of neutron-emitting sources.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Modeling the influence of string collective phenomena on the long range rapidity correlations between the transverse momentum and the multiplicities

The long-range rapidity correlations between the multiplicities (n-n) and the transverse momentum and the multiplicity (pT-n) of charge particles are analyzed in the framework of the simple string inspired model with two types of sources. The sources of the first type correspond to the initial strings formed in a hadronic collision. The sources of the second type imitate the appearance of the emitters of a new kind resulting from interaction (fusion) of the initial strings. The model enabled to describe effectively the influence of the string fusion effects on the strength both the n-n and the pT-n correlations. It was found that in the region, where the process of string fusion comes into play, the calculation results predict the non-monotonic behaviour of the n-n and pT-n correlation coefficients with the growth of the mean number of initial strings, i.e. with the increase of the collision centrality. It was shown also that the increase of the event-by-event fluctuation in the number of primary strings leads to the change of the pT-n correlation sign from negative to positive. One can try to search these signatures of string collective phenomena in interactions of various nuclei at different energies varying the class of collision centrality and its width.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Angular width of the Cherenkov radiation with inclusion of multiple scattering

Visible Cherenkov radiation can offer a method of the measurement of the velocity of charged particles. The angular width of the radiation is important since it determines the resolution of the velocity measurement. In this article, the angular width of Cherenkov radiation with inclusion of multiple scattering is calculated through the path-integral method, and the analytical expressions are presented. The condition that multiple scattering processes dominate the angular distribution is obtained.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Stimulated Raman scattering of laser dye mixtures dissolved in multiple scattering media

Stimulated Raman scattering (SRS) of a mixture of rhodamine 6G and pyrromethene 605 laser dyes in vesicular films is studied. It is shown that a peculiar interaction of dyes occurs under conditions of multiple scattering of light from vesicles. This interaction manifests itself as SRS excitation of one of the dyes by random lasing of the other dye, provided that the random lasing spectrum overlaps the Stokes lines of the first dye. In addition, there is energy transfer between molecules of these dyes if their luminescence and absorption spectra overlap. The results obtained confirm that the mechanism of SRS from laser dyes in multiple scattering media is similar to that in coherent-active Raman spectroscopy. These results extend the possibility of determining the vibrational spectrum of dye molecules from their secondary radiation in these media. (nonlinear optical phenomena)

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Spectral multiplicity for powers of weakly mixing automorphisms

We study the behaviour of the maximal spectral multiplicity m(R{sup n}) for the powers of a weakly mixing automorphism R. For some particular infinite sets A we show that there exists a weakly mixing rank-one automorphism R such that m(R{sup n})=n and m(R{sup n+1})=1 for all positive integers n element of A. Moreover, the cardinality cardm(R{sup n}) of the set of spectral multiplicities for the power R{sup n} is shown to satisfy the conditions cardm(R{sup n+1})=1 and cardm(R{sup n})=2{sup m(n)}, m(n){yields}{infinity}, n element of A. We also construct another weakly mixing automorphism R with the following properties: all powers R{sup n} have homogeneous spectra and the set of limit points of the sequence {l_brace}m(R{sup n})/n:n element of N{r_brace} is infinite. Bibliography: 17 titles.

97 MATHEMATICS AND COMPUTING↗