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The Land Ice Representation in the NASA Goddard Seasonal Forecasting System

Models used in seasonal forecasting systems have aimed for a level of sophistication comparable to Earth system models by incorporating complex physical processes, including those relevant to the polar regions. Here, we examine the polar surface climate in version 3 of the NASA Goddard Earth Observing System Sub-seasonal to Seasonal prediction system (GEOS S2S v3). The model is composed of the ⅟₂̊ resolution Jason4.0version of the GEOS AGCM and the MOM5 ocean model at ⅟₄̊ resolution. The GEOSS2S model incorporates interactive aerosols and two-moment cloud microphysics. As compared to version 2, the model incorporates improved radiative transfer and are designed diurnal cycle atmosphere-ocean interface layer. This study aims to understand how the version 3 model compares with version 2, and with contemporary Earth system models.

Richard I Cullather↗

Self-limiting physical and chemical effects in volcanic eruption clouds

One-dimensional aerosol microphysical and photochemical models are used to study the chemistry of stratospheric volcanic clouds. The results indicate that the aerosol microphysical processes of condensation and coagulation produce larger particles as the SO2 injection rate is increased. Larger particles have a smaller optical depth per unit mass and settle out of the stratosphere at a faster rate than smaller ones, restricting the total number of particles in the stratosphere. The microphysical processes moderate the impact of volcanic clouds on the earth's radiation budget and climate, suggesting that volcanic effects may be self limiting. It is noted that the injection of HCl into the stratosphere, which could lead to large ozone changes, is limited by a cold trap effect in which HCl and water vapor condense on ash particles in the rising volcanic plume and fall out as ice.

Pinto, Joseph P.↗

Cloud Microphysics Budget in the Tropical Deep Convective Regime

Cloud microphysics budgets in the tropical deep convective regime are analyzed based on a 2-D cloud resolving simulation. The model is forced by the large-scale vertical velocity and zonal wind and large-scale horizontal advections derived from TOGA COARE for a 20-day period. The role of cloud microphysics is first examined by analyzing mass-weighted mean heat budget and column-integrated moisture budget. Hourly budgets show that local changes of mass-weighted mean temperature and column-integrated moisture are mainly determined by the residuals between vertical thermal advection and latent heat of condensation and between vertical moisture advection and condensation respectively. Thus, atmospheric thermodynamics depends on how cloud microphysical processes are parameterized. Cloud microphysics budgets are then analyzed for raining conditions. For cloud-vapor exchange between cloud system and its embedded environment, rainfall and evaporation of raindrop are compensated by the condensation and deposition of supersaturated vapor. Inside the cloud system, the condensation of supersaturated vapor balances conversion from cloud water to raindrop, snow, and graupel through collection and accretion processes. The deposition of supersaturated vapor balances conversion from cloud ice to snow through conversion and riming processes. The conversion and riming of cloud ice and the accretion of cloud water balance conversion from snow to graupel through accretion process. Finally, the collection of cloud water and the melting of graupel increase raindrop to compensate the loss of raindrop due to rainfall and the evaporation of raindrop.

Li, Xiao-Fan↗

A Study of Heavy Precipitation Events in Taiwan During 10-13 August, 1994: Mesoscale Model Simulations - Part 2

Several heavy precipitation episodes occurred over Taiwan from August 10 to 13, 1994. Precipitation patterns and characteristics are quite different between the precipitation events that occurred from August 10 and I I and from August 12 and 13. In Part I (Chen et al. 2001), the environmental situation and precipitation characteristics are analyzed using the EC/TOGA data, ground-based radar data, surface rainfall patterns, surface wind data, and upper air soundings. In this study (Part II), the Penn State/NCAR Mesoscale Model (MM5) is used to study the precipitation characteristics of these heavy precipitation events. Various physical processes (schemes) developed at NASA Goddard Space Flight Center (i.e., cloud microphysics scheme, radiative transfer model, and land-soil-vegetation surface model) have recently implemented into the MM5. These physical packages are described in the paper, Two way interactive nested grids are used with horizontal resolutions of 45, 15 and 5 km. The model results indicated that Cloud physics, land surface and radiation processes generally do not change the location (horizontal distribution) of heavy precipitation. The Goddard 3-class ice scheme produced more rainfall than the 2-class scheme. The Goddard multi-broad-band radiative transfer model reduced precipitation compared to a one-broad band (emissivity) radiation model. The Goddard land-soil-vegetation surface model also reduce the rainfall compared to a simple surface model in which the surface temperature is computed from a Surface energy budget following the "force-re store" method. However, model runs including all Goddard physical processes enhanced precipitation significantly for both cases. The results from these runs are in better agreement with observations. Despite improved simulations using different physical schemes, there are still some deficiencies in the model simulations. Some potential problems are discussed. Sensitivity tests (removing either terrain or radiative processes) are performed to identify the physical processes that determine the precipitation patterns and characteristics for heavy rainfall events. These sensitivity tests indicated that terrain can play a major role in determining the exact location for both precipitation events. The terrain can also play a major role in determining the intensity of precipitation for both events. However, it has a large impact on one event but a smaller one on the other. The radiative processes are also important for determining, the precipitation patterns for one case but. not the other. The radiative processes can also effect the total rainfall for both cases to different extents.

Tao, Wei Kuo↗

Microphysical Interpretation of Cirrus Measurements With Lidar

Cirrus measurements obtained with a ground-based polarization Raman lidar at 67.9 N in January 1997 reveal a strong correlation between the particle optical properties, specifically depolarization ratio delta and extinct ion-to-backscatter ratio S, for ambient cloud temperatures above approximately -45 C (delta less than approximately 40%), and an anti-correlation for colder temperatures (delta greater than approximately 40%). Over the length of the measurements (4-7.5 hours) the particle properties vary systematically: Initially, delta approximately equal to 60% and S approximately equal to 10sr are observed. Then, with decreasing delta, S first increases to approximately 27 sr(delta approximately equal to 40%) before decreasing to values around 10 sr again (delta approximately equal to 20%). The particle optical properties distinctly depend on the ambient temperature. For the microphysical analysis of the lidar observations. ray-tracing computations of particle scattering properties and a size-distribution resolving cirrus model with explicit microphysics have been used. The theoretical studies show that the optical properties and their temporal evolution can be interpreted in terms of size, shape, and growth of the cirrus particles: Near the cloud top in the early stage of the cirrus development, light scattering by small hexagonal columns with aspect ratios close to one is dominant. Over time the cloud base height extends to lower altitudes with warmer temperatures, the ice particles grow and get morphologically diverse (the scattering contributions of hexagonal columns and plates are roughly the same for large S and depolarization values of approximately 40%). In the lower ranges of the cirrus clouds, light scattering is predominantly by plate-like or complex ice particles. Mid-latitude cirrus data measured with the same instrument at 53.4 N between 1994 and 1996 follow closely the correlation between delta and S found in the warmer regions of the Arctic cirrus clouds (delta less than approximately 40%). Cirrus clouds with higher depolarization ratios are rarely observed, even for very cold ambient temperatures. Atmospheric parameters other than temperature, e.g., the availability of water vapor, are also important for the growth and the morphology of cirrus particles.

Reichardt, Jens↗

Comparisons of Cloud In-Situ Microphysical Properties of Deep Convective Clouds to Appendix D/P using Data from the HAIC-HIWC and HIWC-RADAR I Flight Campaigns

In-situ cloud data from three international flight campaigns are compared to the Federal Aviation Administration Title 14 Code of Federal Regulations Part 33 Appendix D mixed-phase/glaciated environmental envelope, and the corresponding identical European Aviation Safety Agency CS-25 Appendix P envelope. The appendices consist of a temperature-altitude envelope, a 99th percentile total water content envelope at the 17.4 Nm distance scale, a distance factor for estimation at other distance scales, ice crystal median mass diameter, and recommended liquid water content levels in mixed-phase icing conditions. The data were collected during 54 flights out of one subtropical and two tropical locations, with 472 runs from about 17,000’ to 39,000’ in approximately 115 clouds. The campaigns provide about 29,600 Nm of in situ data in deep convection over four targeted temperature intervals: -10, -30, -40, and -50, all ± 5 C. The dataset is a modern and unique documentation of the ice crystal icing environment, and results described in this article will contribute to regulatory and industry assessment of Appendices D and P.

Ice Crystal Icing↗

Polarimetric Retrievals of Surface and Cirrus Clouds Properties in the Region Affected by the Deepwater Horizon Oil Spill

In 2010, the Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP) performed several aerial surveys over the region affected by the oil spill caused by the explosion of the Deepwater Horizon offshore platform. The instrument was deployed on the NASA Langley B200 aircraft together with the High Spectral Resolution Lidar (HSRL), which provides information on the distribution of the aerosol layers beneath the aircraft, including an accurate estimate of aerosol optical depth. This work illustrates the merits of polarization measurements in detecting variations of ocean surface properties linked to the presence of an oil slick. In particular, we make use of the degree of linear polarization in the glint region, which is severely affected by variations in the refractive index but insensitive to the waviness of the water surface. Alterations in the surface optical properties are therefore expected to directly affect the polarization response of the RSP channel at 2264 nm, where both molecular and aerosol scattering are negligible and virtually all of the observed signal is generated via Fresnel reflection at the surface. The glint profile at this wavelength is fitted with a model which can optimally estimate refractive index, wind speed and direction, together with aircraft attitude variations affecting the viewing geometry. The retrieved refractive index markedly increases over oil-contaminated waters, while the apparent wind speed is significantly lower than in adjacent uncontaminated areas, suggesting that the slick dampens high-frequency components of the ocean wave spectrum. The constraint on surface reflectance provided by the short-wave infrared channels is a cornerstone of established procedures to retrieve atmospheric aerosol microphysical parameters based on the inversion of the RSP multispectral measurements. This retrieval, which benefits from the ancillary information provided by the HSRL, was in this specific case hampered by prohibitive variability in atmospheric conditions (very inhomogeneous aerosol distribution and cloud cover). Although the results presented for the surface are essentially unaffected, we discuss the results obtained by typing algorithms in sorting the complex mix of aerosol types, and show evidence of oriented ice in cirrus clouds present in the area. In this context, polarization measurements at 1880 nm were used to infer ice habit and cirrus optical depth, which was found in the subvisual/threshold-visible regime, confirming the utility of the aforementioned RSP channel for the remote sensing of even thin cold clouds.

Polarization↗

Chapter 10 - Remote Sensing Measurements of Aerosol Properties

Satellite instruments have proven especially capable at monitoring the quantity of airborne particles in columns of atmosphere, globally. This chapter describes the principles of satellite measurements and retrieval algorithms, and surveys current instruments and their capabilities. We outline the issues associated with retrieval algorithms, such as surface characterization and aerosol proximity to clouds, and the challenges with interpretation of the results. The relationship between measured aerosol properties and climate-relevant aerosol properties simulated in models is outlined, as well as how measurements are used to evaluate models. Most space-based aerosol instruments are passive sensors that measure reflected sunlight at multiple wavelengths, some at multiple viewing angles. A few are active sensors that send out their own laser light and measure the returned signal. Except when clouds are present, the excess amount of light scattered back to space, beyond that expected from the surface and atmospheric gas, is attributed to aerosol. Satellite measurements are used in many ways in aerosol research. They often provide the only method for monitoring hazardous phenomena such as major wildfire and volcanic eruption plumes, especially in remote areas. Stable, long-term, near-global-scale satellite data records make it possible to identify regional and global aerosol trends. Aerosol radiative effects on climate can be quantified on a near-global scale and used to estimate the strength of aerosol–radiation and aerosol–cloud interactions as well as to evaluate climate model simulations of these interactions. Aerosol-type mapping from satellite imagery is helpful for source attribution, model validation, and to constrain particle light-absorption properties that are essential for radiative forcing calculations. The range of aerosol properties retrieved from satellite observations has grown considerably since the first global estimates of aerosol optical depth (τ a) over ocean were made in the late 1970s. Methods for retrieving particle size and light-absorption properties were explored in the 1990s using multispectral, multi-angle observations, and polarization in visible and near-infrared wavelengths. Sensitivity to particle light absorption, primarily from black or brown carbon content, improved with the inclusion of UV channels, and sensitivity to very thin aerosol layers in the upper troposphere and lower stratosphere was advanced with the use of limb-sounding instruments and active sensors. There are limitations to every measurement technique, including satellite aerosol remote sensing. For wide-swath, passive instruments, aerosol retrievals near clouds can present substantial challenges as far as 15 km away due to cloud-scattered light contaminating the signal. In nearly all cases, retrievals over bright snow and ice surfaces are precluded because surface reflectance uncertainties can overwhelm the aerosol signal. Similarly, meteorological cloud is identified and masked out where possible. Data from passive sensors also lack vertical resolution except those that view toward the limb or where multi-angle imagery is acquired over plumes from wildfires, erupting volcanoes, and wind-blown dust. Yet, passive sensors provide vastly more coverage than the active instruments that mitigate these issues. Particle microphysical information is qualitative from all remote sensing techniques, relying on proxies to infer particle composition, hygroscopicity, and the amount of light-absorbing material. Further, particles smaller than about 200 nm diameter cannot be distinguished from atmospheric gas molecules with remote sensing, which hinders studies of cloud condensation nuclei and their effects on clouds. Most satellite instruments dedicated to aerosol observations are in low-Earth, near-polar, sun-synchronous orbits, which means they cross the equator at the same local time each day. Most are set on cycles that repeat approximately every 16 days, which makes it difficult to monitor aerosol evolution locally. Geostationary satellites make it possible to observe changes occurring from minutes to hours over regions up to 8000 km in size, but lack coverage of high latitudes, and often provide more limited constraints on aerosol properties. Ground-truth data are vital for satellite aerosol-retrieval validation. The AErosol RObotic NETwork (AERONET) of sun photometers was created in 1993 and has become an established global network of over 350 instruments for validating satellite measurements. The network, as well as global networks of ground-based lidars, solar flux radiometers and other sun photometers, are widely used for evaluating global satellite retrievals and model simulations. NASA's Earth Observing System (EOS) program beginning in 1999 led to improvements in reliability, spatial resolution, and spectral resolution (and hence, to improved particle size discrimination and light absorption properties). Satellite payloads include advanced broad-swath and multi-angle imagers, along with the first space-based active sensor focused largely on long-term aerosol monitoring. Since about 2002, Europe's SENTINEL and operational meteorological satellite fleets are also providing sustained aerosol observations, with planned continuation until at least 2030. Satellite remote sensing instruments offer valuable data for evaluating aerosol representations in global climate models. They have been used to assess aerosol optical and physical properties, trends and distributions, and are applied increasingly as direct model constraints in data assimilation to create global aerosol reanalysis products. Aerosol optical depth is the most common quantity adopted for routine model evaluation, including multiwavelength data to loosely constrain particle-size distributions. These evaluations of multiple models have revealed general biases in their regional aerosol amounts and seasonal patterns of transport and removal. Although satellite measurements have near-global coverage, substantial errors can be introduced into the model observation comparison unless attention is paid to spatial and temporal collocation, cloud screening, subgrid-scale variability, and measurement uncertainties that vary with retrieval conditions.

aerosol properties↗

Comparisons of Cloud In-Situ Microphysical Properties of Deep Convective Clouds to Appendix D/P, Using Data from the HAIC-HIWC and HIWC RADAR I Flight Campaigns

In-situ cloud data from three international flight campaigns is compared to the new Federal Aviation Administration (FAA) Title 14 Code of Federal Regulations Part 33 Appendix D mixed-phase/glaciated environmental envelope (1), and the corresponding identical European Aviation Safety Agency (EASA) CS-25 Appendix P envelope (2) (hereafter "Appendix D/P"). Appendix D/P consists of a temperature-altitude envelope, a 99th percentile total water content (TWC99) envelope at the 17.4 Nm distance scale, a distance factor to estimate TWC99 values at other distance scales, ice crystal median mass diameter (MMD), and recommended liquid water content (LWC) levels in mixed-phase icing conditions. The dataset is from 45 flight missions in 3 tropical locations, with 472 runs in approximately 115 clouds, providing about 29,600 Nm of in-cloud data in deep convection over four targeted temperature intervals: 10, 30, 40, and 50 +5 C. The measurements span altitueds from about 17,000' to 39,000'. The comparisons will serve as a basis for regulatory and industry assessment of the efficacy of Appendix D/P.

Strapp, J. Walter↗

Lightning Over Central Canada: Skill Assessment for Various Land-Atmosphere Model Configurations and Lightning Indices Over a Boreal Study Area

Current lightning predictions are uncertain because they rely on empirical diagnostic relationships and often use coarse-scale climate scenario simulations in which deep convection is parameterized. Previous studies demonstrated that simulations with convection permitting resolutions improve lightning predictions compared to coarser-grid simulations using convection parameterizations for different geographical locations but not over the boreal zone. In this study, lightning simulations with the NASA Unified-Weather Research and Forecasting (NU-WRF) model are evaluated over a domain including the Great Slave Lake in Canada, for six lightning seasons. The simulations are performed at convection parameterized (9 km) and convection-permitting (3 km) resolution using the Goddard 4ICE and the Thompson microphysics schemes. Four lightning indices are evaluated against observations from the Canadian Lightning Detection Network, in terms of spatiotemporal frequency distribution, spatial pattern, daily climatology, and an event-based overall skill assessment. The Thompson scheme is, regardless of the spatial resolution, superior to the Goddard 4ICE scheme in predicting daily climatology but worse in predicting the spatial patterns of lightning occurrence. Results indicate that lightning estimation benefits from modeling at convection-permitting resolution, in particular for the ice based lightning indices. In contrast, the product of convective available potential energy and precipitation rate proved to be the most robust index that was largely invariant to varying spatial resolution. Finally, this study reveals issues of the models to reproduce the observed spatial pattern of lightning well, which might be related to an insufficient representation of land surface heterogeneity, including peatlands, in the study area.

Jonas Mortelmans↗

Hydrometeor development in cold clouds in FIRE

The microphysical characteristics of cold clouds were examined using aircraft. The clouds investigated ranged in temperature from minus 20 to minus 46 C. Liquid water was detected in these clouds at minus 35 C and may exist at even colder temperatures. Aircraft patterns in the form of Lagrangian spirals were used to interpret particle growth processes. Significant broadening of the particle size spectra is observed with minor changes in the spectra at small sizes. Virtually all of the broadening observed is attributable to ice particle aggregation which occurs at all temperatures. The crystals comprising the aggregates are of comparable size, joined either at tips or edges, and are usually 2 in number at temperatures lower than minus 25 C, increasing to 3 or more at warmer temperatures. The data strongly suggest that sintering is the mechanism through which the crystals aggregate. Aggregation appears to be important in the transfer of water mass from upper to lower levels in clouds.

Heymsfield, Andrew J.↗

Three-dimensional aspects of radiative transfer in remote sensing of precipitation: Application to the 1986 COHMEX storm

Several multifrequency techniques for passive microwave estimation of precipitation based on the absorption and scattering properties of hydrometers have been proposed in the literature. In the present study, plane-parallel limitations are overcome by using a model based on the discrete-ordinates method to solve the radiative transfer equation in three-dimensional rectangular domains. This effectively accounts for the complexity and variety of radiation problems encountered in the atmosphere. This investigation presents result for plane-parallel and three-dimensional radiative transfer for a precipitating system, discusses differences between these results, and suggests possible explanations for these differences. Microphysical properties were obtained from the Colorado State University Regional Atmospehric Modeling System and represent a hailstorm observed during the 1986 Cooperative Huntsville Meteorological Experiment. These properties are used as input to a three-dimensional radiative transfer model in order to simulate satellite observation of the storm. The model output consists of upwelling brightness temperatures at several of the frequencies on the Special Sensor Microwave/Imager. The radiative transfer model accounts for scattering and emission of atmospheric gases and hydrometers in liquid and ice phases. Brightness temperatures obtained from the three-dimensional model of this investigation indicate that horizontal inhomogeneities give rise to brightness temperature fields that can be quite different from fields obtained using plane-parallel radiative transfer theory. These differences are examined for various resolutions of the satellite sensor field of view. In adddition, the issue of boundary conditions for three-dimensional atmospheric radiative transfer is addressed.

Haferman, J. L.↗

Microphysical Properties of Tropical Tropopause Layer Cirrus

Pervasive cirrus clouds in the tropical tropopause layer (TTL) play an important role in determining the composition of stratospheric air through dehydration of tropospheric air entering the stratosphere. This dehydration affects Earth's energy budget and climate, yet uncertainties remain regarding the microphysical processes that govern TTL cirrus. TTL cirrus were sampled with the NASA Global Hawk UAV for over 30 hr in the Western Pacific in 2014 during the Airborne Tropical TRopopause EXperiment. In situ measurements by a Fast Cloud Droplet Probe and Hawkeye probe (combination Fast Cloud Droplet Probe, Two‐Dimensional Stereo optical array probe, and Cloud Particle Imager) provided particle concentrations and sizing between 1‐ and 1,280‐μm diameter and high resolution images for habit identification. We present the variability in ice concentrations, size distributions, and habits as functions of temperature, altitude, and time since convective influence. Observed ice particles were predominantly small and quasi‐spheroidal in shape, with the percentage of quasi‐spheroids increasing with decreasing temperature. In comparison to the large fraction of the population consisting of quasi‐spheroids, faceted habits (columns, plates, rosettes, and budding rosettes) constituted a smaller percentage of the overall population and exhibited the opposite correlation with temperature. The trend of higher percentages of faceted crystals occurring at warmer temperatures may be due to diffusional growth or aggregation as particles descend through cloud, and/or the more rapid diffusional growth rate at warmer temperatures. Sampling was typically well away from deep convection, however, and very few aggregates were observed, so the trend of higher percentages of faceted habits is likely attributable to diffusional growth.

Woods, Sarah↗

Assessment of NASA GISS CMIP5 and Post-CMIP5 Simulated Clouds and TOA Radiation Budgets Using Satellite Observations. Part I: Cloud Fraction and Properties

Although many improvements have been made in phase 5 of the Coupled Model Intercomparison Project (CMIP5), clouds remain a significant source of uncertainty in general circulation models (GCMs) because their structural and optical properties are strongly dependent upon interactions between aerosol/cloud microphysics and dynamics that are unresolved in such models. Recent changes to the planetary boundary layer (PBL) turbulence and moist convection parameterizations in the NASA GISS Model E2 atmospheric GCM(post-CMIP5, hereafter P5) have improved cloud simulations significantly compared to its CMIP5 (hereafter C5) predecessor. A study has been performed to evaluate these changes between the P5 and C5 versions of the GCM, both of which used prescribed sea surface temperatures. P5 and C5 simulated cloud fraction (CF), liquid water path (LWP), ice water path (IWP), cloud water path (CWP), precipitable water vapor (PWV), and relative humidity (RH) have been compared to multiple satellite observations including the Clouds and the Earth's Radiant Energy System-Moderate Resolution Imaging Spectroradiometer (CERES-MODIS, hereafter CM), CloudSat- Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO; hereafter CC), Atmospheric Infrared Sounder (AIRS), and Advanced Microwave Scanning Radiometer for Earth Observing System (AMSR-E). Although some improvements are observed in the P5 simulation on a global scale, large improvements have been found over the southern midlatitudes (SMLs), where correlations increased and both bias and root-mean-square error (RMSE) significantly decreased, in relation to the previous C5 simulation, when compared to observations. Changes to the PBL scheme have resulted in improved total column CFs, particularly over the SMLs where marine boundary layer (MBL) CFs have increased by nearly 20% relative to the previous C5 simulation. Globally, the P5 simulated CWPs are 25 gm22 lower than the previous C5 results. The P5 version of the GCM simulates PWV and RH higher than its C5 counterpart and agrees well with the AMSR-E and AIRS observations. The moister atmospheric conditions simulated by P5 are consistent with the CF comparison and provide a strong support for the increase in MBL clouds over the SMLs. Over the tropics, the P5 version of the GCM simulated total column CFs and CWPs are slightly lower than the previous C5 results, primarily as a result of the shallower tropical boundary layer in P5 relative to C5 in regions outside the marine stratocumulus decks.

General circulation models↗

Exposing and Reducing Biases of Simulating Mixed-Phase Clouds in the Convection-Permitting E3SM Atmosphere Model: Lessons From an Arctic Cold-Air Outbreak

Mixed-phase clouds modulate the water and energy cycles of high-latitude regions, yet their liquid-ice phase partitioning has long been poorly simulated in climate models. Here, simulations of Arctic mixed-phase clouds by the Simple Cloud-Resolving E3SM Atmosphere Model (SCREAM) are assessed against large-eddy simulations, satellite data, and ground-based observations during the Cold-Air Outbreaks in the Marine Boundary Layer Experiment field campaign. SCREAM simulates nearly completely frozen clouds, which is attributed largely to the unreasonably strong Wegener–Bergeron–Findeisen (WBF) process that converts liquid to ice excessively and partly to the early over-abundant ice production at cold temperatures from a temperature-deterministic deposition ice nucleation scheme. Assuming no subgrid variation for the WBF process in the original formulation particularly conflicts with the instantaneous saturation adjustment assumption in the condensation scheme that assumes subgrid variability, leading to exaggerated WBF process rates. A proposed simple physically-based improvement on the treatment of subgrid cloud overlap substantially increases supercooled liquid water content and notably improves cloud-top phase partitioning, aligning better with observations. Improvement of supercooled liquid water content also converges with increasing horizontal resolution. The deposition ice nucleation scheme is found responsible for a falsely-produced ice cloud aloft that is not observed, biasing the simulated cloud radiative effects and top-of-atmosphere radiative fluxes. This study identifies key deficiencies in cloud parameterizations that continue to challenge convection-permitting models.

Geosciences↗

Role of Gravity Waves in Determining Cirrus Cloud Properties

Cirrus clouds are important in the Earth's radiation budget. They typically exhibit variable physical properties within a given cloud system and from system to system. Ambient vertical motion is a key factor in determining the cloud properties in most cases. The obvious exception is convectively generated cirrus (anvils), but even in this case, the subsequent cloud evolution is strongly influenced by the ambient vertical motion field. It is well know that gravity waves are ubiquitous in the atmosphere and occur over a wide range of scales and amplitudes. Moreover, researchers have found that inclusion of statistical account of gravity wave effects can markedly improve the realism of simulations of persisting large-scale cirrus cloud features. Here, we use a 1 -dimensional (z) cirrus cloud model, to systematically examine the effects of gravity waves on cirrus cloud properties. The model includes a detailed representation of cloud microphysical processes (bin microphysics and aerosols) and is run at relatively fine vertical resolution so as to adequately resolve nucleation events, and over an extended time span so as to incorporate the passage of multiple gravity waves. The prescribed gravity waves "propagate" at 15 m s (sup -1), with wavelengths from 5 to 100 km, amplitudes range up to 1 m s (sup -1)'. Despite the fact that the net gravity wave vertical motion forcing is zero, it will be shown that the bulk cloud properties, e.g., vertically-integrated ice water path, can differ quite significantly from simulations without gravity waves and that the effects do depend on the wave characteristics. We conclude that account of gravity wave effects is important if large-scale models are to generate realistic cirrus cloud property climatology (statistics).

OCStarr, David↗

TPSAS-NF1676L-20101-DND

Aerosols influence climate through their direct and indirect effects. The aerosol indirect effect is based on the way they interact with surrounding clouds. During cloud formation and development, aerosols act as cloud nucleation nuclei (CCN) or ice nuclei, which modifies cloud micro-, macro-physical and radiative properties, and hence helps to shape the Earth's radiation budget. Dominant sources of ocean-derived aerosols that may serve as CCN include sea spray and biogenic aerosol. In this study, we used 10-years global observations from the A-Train satellites to show seasonal variations of cloud droplet number concentrations (CDNC), ocean chlorophyll concentrations, aerosol angstrom parameter, and rainfall. Potential cloud-aerosol interactions are further discussed based on seasonal and spatial correlations between microphysics of clouds and aerosols. Emphasis for this study is placed on the southern ocean and tropical Pacific.

Shan Zeng↗

CO2 Snow on Mars and Early Earth: Experimental Constraints

Greenhouse warming due to carbon dioxide atmospheres may be responsible for maintaining the early Earth's surface temperature above freezing and may even have allowed for liquid water on early Mars. However, the high levels of CO2 required for such warming should have also resulted in the formation of CO2 clouds. These clouds, depending on their particle size, could lead to either warming or cooling. The particle size in turn is determined by the nucleation and growth conditions. Here we present laboratory studies of the nucleation and growth of carbon dioxide on water ice under Martian atmospheric conditions. We find that a critical saturation, S = 1.34, is required for nucleation, corresponding to a contact parameter between solid water and solid carbon dioxide of m = 0.95. We also find that after nucleation occurs, growth of CO2 is very rapid and proceeds without a surface kinetic barrier. Because growth would be expected to continue until the CO2 pressure is lowered to its vapor pressure, we expect particles larger than those being currently suggested for the present and past Martian atmospheres. Using this information in a microphysical model described in a companion paper, we find that CO2 clouds are best described as "snow", having a relatively small number of large particles.

Glandorf, David L.↗