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NASA NTRS2017

AOD Distributions and Trends of Major Aerosol Species over a Selection of the World's Most Populated Cities Based on the 1st Version of NASA's MERRA Aerosol Reanalysis

NASA recently extended the Modern-Era Retrospective Analysis for Research and Application (MERRA) with an atmospheric aerosol reanalysis which includes five particulate species: sulfate, organic matter, black carbon, mineral dust and sea salt. The MERRA Aerosol Reanalysis (MERRAero) is an innovative tool to study air quality issues around the world for its global and constant coverage and its distinction of aerosol speciation expressed in the form of aerosol optical depth (AOD). The purpose of this manuscript is to apply MERRAero to the study of urban air pollution at the global scale by analyzing the AOD over a period of 13 years (2003-2015) and over a selection of 200 of the world's most populated cities in order to assess the impacts of urbanization, industrialization, air quality regulations and regional transport which affect urban aerosol load. Environmental regulations and the recent global economic recession have helped to decrease the AOD and sulfate aerosols in most cities in North America, Europe and Japan. Rapid industrialization in China over the last two decades resulted in Chinese cities having the highest AOD values in the world. China has nevertheless recently implemented emission control measures which are showing early signs of success in many cities of Southern China where AOD has decreased substantially over the last 13 years. The AOD over South American cities, which is dominated by carbonaceous aerosols, has also decreased over the last decade due to an increase in commodity prices which slowed deforestation activities in the Amazon rainforest. At the opposite, recent urbanization and industrialization in India and Bangladesh resulted in a strong increase of AOD, sulfate and carbonaceous aerosols in most cities of these two countries. The AOD over most cities in Northern Africa and Western Asia changed little over the last decade. Emissions of natural aerosols, which cities in these two regions tend to be mostly composed of, don't tend to fluctuate significantly on an annual basis.

Urban air pollution↗

DOE OSTI2024

Optical and transport properties of plasma mixtures from ab initio molecular dynamics

Predicting the charged particle transport properties of warm dense matter/hot dense plasma mixtures is a challenge for analytical models. High accuracy ab initio methods are more computationally expensive, but can provide critical insight by explicitly simulating mixtures. In this work, we investigate the transport properties and optical response of warm dense carbon–hydrogen mixtures at varying concentrations under either conserved electronic pressure or mass density at a constant temperature. We compare options for mixing the calculated pure species properties to estimate the results of the mixtures. We find that a combination of the Drude model with the Matthiessen's rule works well for DC electron transport and low-frequency optical response. This breaks down at higher frequencies, where a volumetric mix of pure-species AC conductivities works better.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Coexistence of Soft Modes and Dynamic Ti Disorder in Cubic BaTiO 3 Studied by Inelastic Neutron Scattering

The phonon dispersion relations in cubic BaTiO 3 have been measured along the [100], [110], and [111] directions at T = 453 K using inelastic neutron scattering. The isotropic transverse acoustic (TA) branches indicate that the interatomic force constant between Ba and O atoms in BaTiO 3 is large compared with that between Pb and O atoms in PbTiO 3 . The transverse optical (TO) branches along the [100] and [111] directions soften toward the Brillouin zone center. The TO branch along the [110] direction with [001] polarization is relatively low and flat, indicating the weak interatomic force constant between Ti and O atoms along the Ti–O chain. The intensity of inelastic diffuse scattering along the [100] and [110] directions increases with decreasing temperature down to 453 K. In conclusion, the present results suggest that the soft modes coexist with the dynamic Ti disorder in the Ti–O chain near the phase transition in the cubic phase.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2019

Late-time observations of the extraordinary Type II supernova iPTF14hls

Aims. We study iPTF14hls, a luminous and extraordinary long-lived Type II supernova, which lately has attracted much attention and disparate interpretation. Methods. We have presented new optical photometry that extends the light curves up to more than three years past discovery. We also obtained optical spectroscopy over this period, and furthermore present additional space-based observations using Swift and HST. Results. After an almost constant luminosity for hundreds of days, the later light curve of iPTF14hls finally fades and then displays a dramatic drop after about 1000 d, but the supernova is still visible at the latest epochs presented. The spectra have finally turned nebular, and our very last optical spectrum likely displays signatures from the deep and dense interior of the explosion. A high-resolution HST image highlights the complex environment of the explosion in this low-luminosity galaxy. Conclusions. We provide a large number of additional late-time observations of iPTF14hls, which are (and will continue to be) used to assess the many different interpretations for this intriguing object. In particular, the very late (+1000 d) steep decline of the optical light curve is difficult to reconcile with the proposed central engine models. The lack of very strong X-ray emission, and the emergence of intermediate-width emission lines including [S II] that we propose originate from dense, processed material in the core of the supernova ejecta, are also key observational tests for both existing and future models.

J. Sollerman↗

DOE OSTI2025

Efficiency droop contributors in InGaN green light emitting diodes

Here, efficiency droop contributors (i.e., inherent Auger–Meitner recombination, polarization-induced effects, thermal effects, and light extraction) in InGaN green light emitting diodes (LEDs) are decoupled and quantified. First, a modified ABC model is developed, and external quantum efficiency measurements are taken under constant and pulsed currents (⁠ EQE Constant and EQE Pulsed ⁠, respectively). The LED internal quantum efficiency with and without thermal effects (⁠ IQE$^{ABC}_{Constant}$ and IQE$^{ABC}_{Pulsed}$⁠, respectively) is extracted using the modified model. Then, using Raman spectroscopy, the LED junction temperature is extracted. Finally, using the optical-electrical model (OEM), the polarization- and temperature-independent LED internal quantum efficiency (⁠ IQE OEM ) is calculated from the modified ABC model and the extracted junction temperature. By comparing external (⁠ EQE Constant ⁠) and the three internal quantum efficiencies (⁠ IQE$^{ABC}_{Constant}$, IQE$^{ABC}_{Pulsed}$⁠, and IQE OEM ), the impacts of inherent Auger–Meitner recombination, polarization-induced effects, thermal effects, and light extraction on the efficiency droop are decoupled and quantified. It is found that inherent Auger–Meitner recombination-induced droop is approximately 49% of the total efficiency droop in commercial green LEDs, while polarization-induced effects contribute about 35%, and thermal droop accounts for nearly 16%. Lastly, these findings suggest, to quash the green gap, it is critical to search for materials and device designs with low inherent Auger–Meitner coefficients and polarization fields, respectively.

42 ENGINEERING↗

NASA NTRS2007

Triboluminescent Materials for Smart Optical Damage Sensors for Space Applications

Triboluminescence is light that is produced by pressure, friction or mechanical shock. New composite materials are constantly being reengi neered in an effort to make lightweight spacecrafts for various NASA missions. For these materials there is interest in monitoring the con dition of the composite in real time to detect any delamination or cr acking due to damage, fatigue or external forces. Methods of periodic inspection of composite structures for mechanical damage such as ult rasonic testing are rather mature. However, there is a need to develop a new technique of damage detection for composites, which could dete ct cracking or delamination from any desired location within a materi al structure in real time. This could provide a valuable tool in the confident use of composite materials for various space applications. Recently, triboluminnescent materials have been proposed as smart sen sors of structural damage. To sense the damage, these materials can b e epoxy bonded or coated in a polymer matrix or embedded in a composi te host structure. When the damage or fracture takes place in the hos t structure, it will lead to the fracture of triboluminescent crystal s resulting in a light emission. This will warn, in real time, that a structural damage has occurred. The triboluminescent emission of the candidate phosphor has to be sufficiently bright, so that the light signal reaching from the point of fracture to the detector through a fiber optic cable is sufficiently strong to be detected. There are a large number of triboluminescent materials, but few satisfy the above criterion. Authors have synthesized a Eu based organic material know n as Europium tetrakis (dibenzoylmethide) triethylammonium .(EuD(sub 4)TEA), one of the bright triboluminescent materials, which is a pote ntial candidate for application as a damage sensor and could be made into a wireless sensor with the addition of microchip, antenna and el ectronics. Preliminary results on the synthesis and characterization of this material shall be presented.

Aggarwal, Mohan D.↗

DOE OSTI2024

Ligand field exciton annihilation in bulk CrCl 3

The layered van der Waals material CrCl 3 exhibits very strongly bound ligand field excitons that control optoelectronic applications and are connected with magnetic ordering by virtue of their d-orbital origin. Time-resolved photoluminescence of these exciton populations at room temperature shows that their relaxation is dominated by exciton–exciton annihilation and that the spontaneous decay lifetime is very long. Furthermore, these observations allow the rough quantification of the exciton annihilation rate constant and contextualization in light of a recent theory of universal scaling behavior of the annihilation process.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1989

U. radio emission from quiescent filaments

Full-disk Very Large Array (VLA) synthesis maps of the quiet Sun indicate that filaments can be seen in emission at 91.6 cm wavelength; they are detected in absorption at shorter microwave wavelengths. The 91.6 cm emission has a brightness temperature of T sub B = 3 x 10(exp 5) K. It is hotter, wider and longer than the underlying filament detected at H alpha wavelengths, but the similarity between the shape, position, elongation and orientation of the radio and optical features suggests their close association. The 91.6 cm emission is attributed to the thermal-bremsstrahlung of a hot transition sheath that envelopes the H alpha filament and acts as an interface between the cool, dense H alpha filament and the hotter, rarefied corona. The transition sheath is seen in emission because of the lower optical depth of the corona at 90 cm wavelength, and the width of this sheet is 10(exp 9) cm. A power law gradient in pressure provides a better match to the observations than a constant pressure model; definitive tests of theoretical models await simultaneous multi-wavelength studies of filaments at different observing angles. When the thermal bremsstrahlung is optically thin, the magnetic field strength in the transition sheath can be inferred from the observed circular polarization. Variable physical parameters of the sheath, such as width, electron density, and electron temperature, can explain controversial reports of the detection of, or the failure to detect, the meter-wavelength counterpart of H alpha filaments.

Lang, Kenneth R.↗

NASA NTRS1978

Photometric study of the X-ray pulsar 4U 1626-67

Results are reported for UBVR photometric observations of the optical candidate for the pulsating X-ray source 4U 1626-67. The data are found to be consistent with a constant V magnitude of approximately 19.00 and marginally consistent with constant B-V and U-B colors, but two averaged measures obtained about 2 hr apart suggest that the B-V and U-B colors are variable and that this variability may be entirely in U and B. Additional evidence for variability of the optical candidate is examined, and it is shown that the optical object is probably variable with a B amplitude of no more than about 0.5 mag and time scales as short as less than the order of 1 min. A power spectrum analysis reveals no significant peaks at or near the X-ray pulse period of 7.68 sec or its harmonics. It is concluded that although the optical data do not provide any additional evidence that 4U 1626-67 is a binary, a short-period binary system with the optical emission strongly dominated by an accretion disk is probably favored.

Grindlay, J. E.↗

NASA NTRS2000

Updating the NASA LEO Orbital Debris Environment Model with Recent Radar and Optical Observations and in Situ Measurements

The Low Earth Orbit (LEO, between 200 and 2000 km altitudes) debris environment has been constantly measured by NASA Johnson Space Center's Liquid Mirror Telescope (LMT) since 1996 (Africano et al. 1999, NASA JSC-28826) and by Haystack and Haystack Auxiliary radars at MIT Lincoln Laboratory since 1990 (Settecerri et al. 1999, NASA JSC-28744). Debris particles as small as 3 mm can be detected by the radars and as small as 3 cm can be measured by LMT. Objects about 10 cm in diameter and greater are tracked and catalogued by the US Space Surveillance Network. Much smaller (down to several micrometers) natural and debris particle populations can be estimated based on in situ measurements, such as Long Duration Exposure Facility, and based on analyses of returned surfaces, such as Hubble Space Telescope solar arrays, European Retrievable Carrier, and Space Shuttles. To increase our understanding of the current LEO debris environment, the Orbital Debris Program Office at NASA JSC has initiated an effort to improve and update the ORDEM96 model (Kessler et al. 1996, NASA TM-104825) utilizing the recently available data. This paper gives an overview of the new NASA orbital debris engineering model, ORDEM2000.

Liou, J.-C.↗

DOE OSTI2023

Giant Magnetic and Optical Anisotropy in Cerium-Substituted M-Type Strontium Hexaferrite Driven by $4f$ Electrons

By performing density-functional calculations, we find a giant magnetocrystalline anisotropy (MCA) constant in abundant element cerium $\mathrm{Ce}$ substituted M-type hexaferrite, in the energetically favorable strontium site, assisted by a quantum confined electron transfer from $\mathrm{Ce}$ to a specific iron $\mathrm{2a}$ site. Remarkably, the calculated electronic structure shows that the electron transfer leads to the formation of $\mathrm{Ce}^{3+}$ and $\mathrm{Fe}^{2+}$ at the $\mathrm{2a}$ site producing an occupied $\mathrm{Ce}$$(4f^1)$ state below the Fermi level that adds a significant contribution to MCA and magnetic moment. A half $\mathrm{Ce}$ substitution forms a metallic state, while a full substitution retains the semiconducting state of the strontium hexaferrite (host). In the latter, the band gap is reduced due to the formation of charge-transferred states in the gap region of the host. The optical absorption coefficient shows an enhanced anisotropy between light polarization in parallel and perpendicular directions. Calculated formation energies, including the analysis of probable competing phases, and elastic constants confirm that both compositions are chemically and mechanically stable. With successful synthesis, the $\mathrm{Ce}$ hexaferrite can be an alternative high-performing critical-element-free permanent magnet material adapted for use in devices such as automotive traction drive motors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1991

Properties of scatterers in the troposphere and lower stratosphere of Uranus based on Voyager imaging data

Scalar and vector radiative transfer and microphysical models are presently constructed from photometrically and geometrically corrected Voyager images of Uranus defining spatially-resolved intensities over a range of phase angles for two latitude bands. The methane ice cloud occupying 1.2-1.3 bar is of 0.7 optical depth at 22.5 deg S, rising to 2.4 at 65 deg S; the volume absorption coefficient of the cloud particles is 50 percent greater at the low latitude than at the high, assuming constant mean cloud particle size. The scattering model also includes photochemically-produced stratospheric hydrocarbon ices in the upper troposphere and stratosphere, as well as an optically thick hydrogen sulfide cloud.

Rages, Kathy↗

NASA NTRS1984

Study of alternate optical and fine guidance sensor designs for the space infrared telescope facility (SIRTF)

A unique optical design was developed that compensates for the coma degraded images caused by field chopping in SIRTF. The conic constants of a Cassegrain telescope were altered to compensate for the coma induced by the secondary mirror tilt. The modulation transfer function is essentially independent of secondary mirror tilt, and diffraction limited image quality is maintained over a several arcminute field during chopping. With an untilted secondary mirror, the coma compensated (CC) design has a smaller field than the unchopped Ritchey-Chretien design; but use of relay optics, such as the inverted Cassegrain design developed for the fine guidance sensor (FGS), can increase the CC telescope's field size. A reactionless secondary mirror chopper mechanism that uses superconducting magnets was studied. The heart producing elements are confined to a reaction plate that is not directly viewed by the IR focal plane. A design was also developed for a low moment of inertia, reticulated HIP beryllium secondary mirror consistent with blank fabrication technology and optical finishing requirements.

Wissinger, A.↗

DOE OSTI2024

Deployment of POLARBEAR-2b

POLARBEAR-2b (PB-2b) is the second receiver in the Simons Array, a cosmic microwave background (CMB) polarization experiment. The Simons Array uses dichroic polarization sensitive lenslet-coupled sinuous antennas and transition-edge sensor (TES) bolometers made of superconducting films. These bolometers are read out with frequency multiplexing electronics. PB-2b contains ~7500 detectors in two bands at 90 and 150 GHz with arcminute resolution. The polarization of these detectors is modulated by a cryogenic continuously rotating half-wave plate. PB-2b was installed on its telescope in 2022 in the Atacama Desert at an altitude of 5.2 km. This paper will detail initial readout commissioning, test of a new loopgain monitoring method, and focusing the optics. Work is ongoing to commission the remaining ambient temperature readout electronics, measure detector time constants, and observe with the cryogenic half-wave plate spinning.

47 OTHER INSTRUMENTATION↗

DOE OSTI2021

Sound velocities in shock-compressed soda lime glass: Melting and liquid-state response

Longitudinal sound velocities (and elastic moduli) were determined in soda lime glass (SLG) at peak shock stresses ranging between 40 and 90 GPa. Laser interferometry was used to obtain particle velocity histories and sound velocities by impacting SLG samples on lithium fluoride (LiF) optical windows. In all experiments, the SLG response consists of a sharp jump to a constant state followed by a release wave. The measured longitudinal sound velocities and moduli showed a marked decrease between 52 and 58 GPa, providing experimental evidence for the transformation from an amorphous solid to a liquid in shock-compressed SLG. Furthermore, the stress threshold (~55 GPa) for melting in SLG is considerably lower than the threshold reported in shock-compressed fused silica (~72 GPa), showing the effect of network-modifying cations on the onset of melting. The relative values of sound velocities, shock velocities, and the Hugoniot slopes—between 58 and 90 GPa—are fully consistent with the thermodynamic response of a shock-compressed liquid. Using the experimental results, the Grüneisen parameter (Γ) values were determined for liquid SLG to 90 GPa and then used to provide the Mie-Grüneisen equation of state for liquid SLG.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

ON PROCESS STABILITY IN WAAM-CMT OF ALUMINUM ALLOYS

Wire-arc additive manufacturing (WAAM) has become a cost-efficient metal additive manufacturing process. However, depositing aluminum with WAAM is challenging due to its sensitivity to heat input (linear energy density), which can cause undesirable surface topology waviness if not controlled. Thus, a process window is needed that can produce stable geometry and deposition conditions while minimizing production times. In this study, 5183 aluminum alloy wire is used to deposit 10-layer walls with varying wire feed speeds (WFS) and traverse speeds (TS) (at a constant WFS/TS ratio) and varying interpass temperature (IPT). In-situ process data consisting of optical contact-tip-workpiece-distance (CTWD) and current/voltage measurements are collected to determine process condition stability throughout the build. Part geometry is measured using a 3D scanner and build porosity is characterized via digital X-ray. A process window is identified that produces stable surface topology and process conditions at a minimal production time.

aluminum alloy↗

DOE OSTI2020

Perspective on Some Recent and Future Developments in Casimir Interactions

Here, we present a critical review of recent developments in Casimir physics motivated by discoveries of novel materials. Specifically, topologically nontrivial properties of the graphene family, Chern and topological insulators, and Weyl semimetals have diverse manifestations in the distance dependence, presence of fundamental constants, magnitude, and sign of the Casimir interaction. Limited studies of the role of nonlinear optical properties in the interaction are also reviewed. We show that, since many new materials have greatly enhanced the nonlinear optical response, new efficient pathways for investigation of the characteristic regimes of the Casimir force need to be explored, which are expected to lead to new discoveries. Recent progress in the dynamical Casimir effect is also reviewed and we argue that nonlinear media can open up new directions in this field as well.

36 MATERIALS SCIENCE↗

NASA NTRS1984

Quasars as probes of the intergalactic medium

Spectral energy distributions for 10 high red shift quasars in the wavelength range 1250 to 10,000 A were obtained by IUE. A pronounced steepening is detected shortward of 1200 A, which correlates well with quasar red shift, but poorly with luminosity. The observed slope change is explained by Lyman continuum absorption from the strongest 5% of the Lyman alpha forest lines, identified with the low column density metal containing systems. Reddening may also contribute to the steepening, but a much lower neutral gas to dust ratio than that found in the Galaxy is required. Optically thick Lyman limit discontinuities are seen with zabs zem. These systems are metal containing, constant in comoving density with epoch, and require in L* galaxy to have a cross section of 5 to 10 Holmberg radii.

Green, R. F.↗