Exploiting stilbene’s scintillation anisotropy for neutron source localization
Not Available
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
SEARCH · Engineering Papers
Results for “NEUTRON SCIENCE”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
Effect of Water Chemistry on Crack Growth Rates in Neutron Irradiated X-750 and XM-19
The Advanced Test Reactor (ATR) National Science User Facility (NSUF) was used to study the effect of neutron damage on crack growth rates (CGR) under simulated boiling water reactor (BWR) water chemistry conditions using a fast neutron spectrum to accelerate the damage process. Nickel based Alloy X-750 and XM-19 were irradiated in the ATR center flux trap (CFT), with this experiment marking the first civilian project to utilize this position within the reactor. 0.4T-CT specimens were used to study crack growth rates for two sample fluences (~1.9 x 1020 n/cm2 and ~9.5 x 1020 n/cm2, E > 1MeV) in both normal water chemistry (NWC) at 2.5 ppm O2 and hydrogen water chemistry (HWC) at ~80 ppb H2. A decrease in CGR was observed with HWC for both alloys with the average ratio (CGR in NWC/CGR in HWC) being a factor of 281 for the XM-19 samples and a factor of 27.8 for the X-750 samples. Observed CGRs in this study showed little difference compared to non-irradiated samples (the non-irradiated XM-19 was 20% cold worked), suggesting limited sensitivity of these susceptible alloys to irradiation effects. The CGR response to varying environmental electrochemical potential (ECP) and water purity will be presented.
36 MATERIALS SCIENCE↗
Effect of Water Chemistry on Crack Growth Rate in Neutron Irradiated X-750 and XM-19
The Advanced Test Reactor (ATR) National Science User Facility (NSUF) was used to study the effect of neutron damage on crack growth rates (CGR) under simulated boiling water reactor (BWR) water chemistry conditions using a fast neutron spectrum to accelerate the damage process. Nickel based Alloy X-750 and XM-19 were irradiated in the ATR center flux trap (CFT), with this experiment marking the first civilian project to utilize this position within the reactor. 0.4T-CT specimens were used to study crack growth rates for two sample fluences (~1.9 x 1020 n/cm2 and ~9.5 x 1020 n/cm2, E > 1MeV)) in both normal water chemistry (NWC) at 2.5 ppm O2 and hydrogen water chemistry (HWC) at ~80 ppb H2. CGR testing was conducted at a temperature of 288 °C. A decrease in CGR was observed for both alloys with the average ratio (CGR in NWC/CGR in HWC) being a factor of 281 for the XM-19 samples and a factor of 27.8 for the X-750 samples. Observed CGRs in this study showed little difference compared to non-irradiated samples (the non-irradiated XM-19 was 20% cold worked), suggesting limited sensitivity of these susceptible alloys to irradiation effects. Detailed results of CGR response to varying environmental electrochemical potential (ECP) and water purity will be presented in the context of crack growth mitigation in different water chemistries and the change in material behavior relative to non-irradiated samples of the material.
36 MATERIALS SCIENCE↗
Prompt Fission Neutron Spectra of Actinides
No abstract prepared.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Initial Neutronics Investigation of a Liquid-Metal Plasma-Facing Fusion Nuclear Science Facility
Not provided.
Nuclear Science & Technology↗
Method Development for High Temperature In-Situ Neutron Diffraction Measurements of Glass Crystallization on Cooling from Melt
A glass-ceramic borosilicate waste form is being considered for immobilization of waste streams of alkali, alkaline-earth, lanthanide, and transition metals generated by transuranic extraction for reprocessing used nuclear fuel. Waste forms are created by partial crystallization on cooling, primarily of oxyapatite and powellite phases. In-situ neutron diffraction experiments were performed to obtain detailed information about crystallization upon cooling from 1200°C. The combination of high temperatures and reactivity of borosilicate glass with typical containers used in neutron experiments, such as vanadium and niobium, prevented their use here. Thus, methods using sealed thick-walled silica ampoules were developed for the in-situ studies. Unexpectedly, high neutron absorption, low crystal fraction, and high silica container background made quantification difficult for these high temperature measurements. As a follow-up, proof-of-concept measurements were performed on different potential high-temperature container materials, emphasizing crystalline materials so that residual glass in the waste form sample could be more easily analyzed. Room temperature measurements were conducted with a pre-crystallized sample in ‘ideal’ containers stable at low temperatures (i.e., vanadium and thin-wall silica capillaries) and compared to the same measurements in containers stable at high temperatures (i.e, platinum, single crystal sapphire, and thick-walled silica ampoules). Results indicated that Pt is probably the best choice if suitably sealed to prevent contamination from the sample after neutron activation.
36 MATERIALS SCIENCE↗
Analysis of SPND Material Candidates for Real-Time Neutron Spectrum Monitoring Poster
The future of the nuclear industry will be shaped by advanced reactor designs requiring innovative instrumentation for safe operation. A key area of innovation is the ability to accurately and reliably monitor the neutron energy spectrum during operations, which would also enhance the experimental capabilities of existing research reactors. To address this need, our research focuses on the potential use of Self-Powered Neutron Detectors (SPNDs) for real-time neutron spectrum monitoring. We investigated various candidate materials for SPNDs by evaluating their energy-dependent reaction rates. Promising materials were further modeled using MCNP to determine the free electron production per neutron across the neutron energy spectrum, approximating their energy-dependent signal sensitivity. Our findings identified Samarium (Sm) and Gadolinium (Gd) as top candidates for thermal neutrons, Hafnium (Hf) and Thulium (Tm) for epithermal neutrons, and Tantalum (Ta) for fast neutrons. These materials will undergo future experimental validation to confirm the modeled responses and assess their feasibility for real-time neutron spectrum measurements.
46 - INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AN↗
Neutron Interferometric methods and quantum sensing
Advances in material science and engineering make it possible to access artificial materials or ‘metamaterial’ properties and structures on the length scale comparable to the wavelength of ultracold neutrons ~ 100 nm. Strong neutron scattering effects such as Anderson localization, resonance scattering may be studied in the laboratory according to our recent theoretical studies. UCN interferometry and high-resolution spectroscopy (sub-pico-electronvolt resolution) in neutronic metamaterials are examples of new experimental possibilities that can probe quantum gravitational states of neutrons, and quantum sensing based on ultracold neutrons.
36 MATERIALS SCIENCE↗
Multi-Layered Avalanche Diamond Detector for Fast Neutron Applications
Explore the source record for details and available documents.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Radioactivity Calculator for Research and Test Reactor Neutron-Activated Materials
The Idaho National Laboratory Nuclear Science User Facilities program is proposing to launch a new online expert system that will assist users in planning experiments and writing proposals. The Combined Materials Experimentation Toolkit (CoMET) will include two nuclear calculators. The first of these, the Neutron Damage Calculator, will assist users in selecting reactor positions in order to obtain desired material damage in Damage Per Atom (DPA) and provide the required irradiation time to reach the damage levels. The second, the Radioactivity Calculator, will estimate the post-irradiation radioactivity levels of sample materials, which will inform technical staff of examination facility requirements and any potential scheduling delays. Both of these calculators were designed to simplify the information needed from users in order to properly plan and execute awarded proposals. This paper presents the primary purpose and methodologies implemented by these two calculators.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
Machine learning magnetism classifiers from atomic coordinates
The determination of magnetic structure poses a long-standing challenge in condensed matter physics and materials science. Experimental techniques such as neutron diffraction are resource-limited and require complex structure refinement protocols, while computational approaches such as first-principles density functional theory (DFT) need additional semi-empirical correction, and reliable prediction is still largely limited to collinear magnetism. Here, we present a machine learning model that aims to classify the magnetic structure by inputting atomic coordinates containing transition metal and rare earth elements. By building a Euclidean equivariant neural network that preserves the crystallographic symmetry, the magnetic structure (ferromagnetic, antiferromagnetic, and nonmagnetic) and magnetic propagation vector (zero or non-zero) can be predicted with an average accuracy of 77.8% and 73.6%. In particular, a 91% accuracy is reached when predicting no magnetic ordering even if the structure contains magneticelement(s). Ourworkrepresents onestepforwardtosolvingthegrand challenge of full magnetic structure determination.
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
Secondary neutron production from thick target deuteron breakup
Thick target deuteron breakup is a variable-energy accelerator-based source of high-energy neutrons, with applications in fundamental and applied nuclear science and engineering. However, the breakup mechanism remains poorly understood, and data on neutron yields from thick target breakup remain relatively scarce. In this work, the double-differential neutron yields from deuteron breakup have been measured on a thick beryllium target at ϵ d = 33 and 40 MeV, using both time-of-flight and activation techniques. We have also introduced a simple hybrid model for the double-differential deuteron breakup cross section, applicable in the ϵ d = 10-100 MeV energy range on light (Z ≤ 6) targets. This model features four empirical parameters that have been fit to reproduce experimental breakup measurements on beryllium targets, using the method of least squares. It was shown that these parameters extrapolate well to higher energies, and to other low-Z target materials. Here, we also include optimization of the parameters that modify the Kalbach systematics for compound and preequilibrium reactions, in order to better reproduce the experimental data for beryllium targets at large angles.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Scintillation Properties of a Cs2LiLa(Br6)90%(Cl6)10%:Ce (CLLBC) Crystal
In investigations of Ce3+-doped Cs2LiLa(Br6)90%(Cl6)10% (CLLBC) elpasolite crystals, the crystals show an excellent neutron and gamma (n/g) radiation response. The results of our studies on the scintillation properties of CLLBC viz. radioluminescence, energy resolution, light yield, decay times, and nonproportionality are discussed. The CLLBC detector can provide energy resolution as good as 4.1% at 662 keV (FWHM), which is better than that of NaI:Tl. Because the crystal contains 6Li, CLLBC can also detect thermal neutrons. In the energy spectra, the full energy thermal neutron peak appears near or above 3 MeV gamma equivalent energy. This high-energy signature for the thermal neutron peak means that very effective pulse height discrimination is possible. Unfortunately, because the core-to-valence luminescence observed in other elpasolites that can be exploited for effective pulse shape discrimination (PSD) is not observed in the CLLBC, other strategies for obtaining the PSD of CLLBC are needed. The n/g discrimination capability of CLLBC detectors may be optimized by tuning the cerium doping content for maximum effect on n/g pulse shape differences. The value of adding a chlorine component to the nominal CLLB crystal is discussed. Because the crystal contains chlorine, its sensitivity to fast neutrons is better than that of Cs2LiLaBr6 (CLLB). Further, an array of three of these CLLBC detectors may be able to perform directional detection in both the neutron and gamma channels simultaneously.
36 MATERIALS SCIENCE↗
Neutron Scattering Cross Sections: (n,n′), (n,n′γ), and (n,γ) Measurements (Final Technical Report)
This technical report discusses the outcomes from a grant to the University of Dallas in collaboration with the University of Kentucky, the United States Naval Academy and Mississippi State University to measure neutron cross sections and to provide educational opportunities in nuclear science for undergraduate and graduate students and postdoctoral scholars.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Characterization of aluminum and boron carbide based additive manufactured material for thermal neutron shielding
Not Available
36 MATERIALS SCIENCE↗
In-Situ Measurement of Crystalline Lattice Strains in Fluoropolymers by Neutron Diffraction
No abstract prepared.
36 MATERIALS SCIENCE↗
Cooperative spin coupling in PrFeO3
A transition from crystal-field to spin wave excitations has been experimentally observed in PrFeO3 using inelastic neutron scattering. Theoretical modeling with density functional theory and the mean field random phase approximation successfully reproduces the experimental observations and allows extraction of the values for the various exchange interactions. The study reveals that the strong coupling between the two magnetic sublattices of Pr and Fe is the fundamental mechanism underlying the low-temperature Pr magnetism. This coupling, analogous to the Dicke cooperative interaction between atoms and photons, polarizes the Pr moments, enhances the Pr-Pr interactions, and contributes to the formation of a quasidoublet, leading to the transition from single-particle to collective excitations within the Pr sublattice. Furthermore, this coupling induces spin reorientation on the Fe sublattice. The manipulation of magnetic moments via spin waves is achievable through the coupling between different magnetic sublattices in a bulk material containing multiple magnetic ions.
Garlea, Vasile [ORNL] (ORCID:0000000253227271)↗